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Semicrystalline Unfused Polymer Donors with Backbone Halogenation toward Cost-Effective Organic Solar Cells

Chinese journal of Chemistry 2024年第7期42卷 752-759页

作者： Yuxin Kong Shijie ju Hongmei Qin Min Hun jee Simeng Xia jiaqi Ren Chao Gao jianyu yuan Wenyan Su Han Young Woo Yuxiang Li School of Materials Science and Engineering Xi'an University of Science and TechnologyXianShaanxi 710054China Department of Chemistry Korea UniversitySeoul 02841Republic of Korea Xi'an Key Laboratory of Liquid Crystal and Organic Photovoltaic Materials State Key Laboratory of Fluorine&Nitrogen ChemicalsXi'an Modern Chemistry Research InstituteXi'anShaanxi 710065China jiangsu Key Laboratory for Carbon-Based Functional Materials&Devices Institute of Functional Nano&Soft Materials(FUNSOM)Soochow University199 Ren'ai RoadSuzhouJiangsu 215123China

Developing novel unfused building blocks with simple synthesis and low cost is essential to advance and enrich cost-effective poly-mer donors;however,it remains a challenge due to the lack of efficient molecular ***,a class of low-cost and fully unfused polymer donors with precisely regulated backbone planarity via halogenation was designed and synthesized,namely PDTBTBz-2H,PDTBTBz-2F,and *** polymer donors possess a four-step synthesis route with over 80%yield from cheap raw chemicals comparable to existing low-cost polymer donors,such as *** from the planar backbone via in-corporating the F…S non-covalent interactions,PDTBTBz-2F exhibits more robust j-type aggregation in solution and a long-ranged molecular stacking in film relative to PDTBTBz-2H and ***,the systematical study of PDTBTBz-based organic so-lar cells(OSCs)reveals the close relationship between optimized molecular self-assembly and charge separation/transport regarding backbone halogenation when paired with the non-fullerene acceptor(Y6-BO-4F).As a result,the photovoltaic devices based on semicrystalline PDTBTBz-2F achieved a promising power conversion efficiency(PCE)of 12.37%.Our work highlighted the influence of backbone halogenation on the molecular self-assembly properties and a potential unfused backbone motif for further developing cost-effective OSCs.

关键词： Low-cost Polymer donors Backbone halogenation Molecular self-assembly Organic solar cells

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Clinical and genetic heterogeneity of adult polyglucosan body disease caused by GBE1 biallelic mutations in China

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Genes & Diseases 2024年第5期11卷 17-20页

作者： Yikun Chen Yan Shi yuan Gao Yan Hu Linying Zhou jingmei Hong Shirui Gan Xiang Lin Wanjin Chen Guorong Xu jin He Department of Neurology and Institute of Neurology of First Affiliated Hospital Institute of Neuroscienceand Fujian Key Laboratory of Molecular NeurologyFujian Medical UniversityFuzhouFujian 350005China Fujian Key Laboratory of Molecular Neurology Institute of NeuroscienceFujian Medical UniversityFuzhouFujian 350005China Electron Microscopy Lab of Public Technology Service Center Fujian Medical UniversityFuzhouFujian 350005China

Adult polyglucosan body disease(APBD)is a rare and highly heterogeneous glycogen storage disorder due to biallelic variants in GBE1.1 Typical APBD presentations include gait abnormalities with polyneuropathy,leukodystrophy,neurogenic bladder,and mild cognitive *** diagnosis of APBD encompasses a large spectrum of conditions including axonal and demyelinating sensorimotor polyneuropathy,progressive spastic paraparesis,and leukodystrophies.

关键词： GBE bladder diagnosis

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Design and Application of an S-band Fast Radio Bursts Search Pipeline for the Nanshan 26 m Radio Telescope

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Research in Astronomy and Astrophysics 2024年第7期24卷 111-117页

作者： Yan-Ling Liu Mao-Zheng Chen jian Li jian-Ping yuan Rai Yuen Zhi-Yong Liu Hao Yan Wen-Long Du Nan-Nan Zhai Xinjiang Astronomical Observatory Chinese Academy of SciencesUrumqi 830011China Xinjiang Key Laboratory of Microwave Technology Urumqi 830011China University of Chinese Academy of Sciences Beijing 100049China

Fast radio bursts(FRBs)are among the most studied radio transients in astrophysics,but their origin and radiation mechanism are still *** is a challenge to search for FRB events in a huge amount of observational data with high speed and high *** the rapid advancement of the FRB research process,FRB searching has changed from archive data mining to either long-term monitoring of the repeating FRBs or all-sky surveys with specialized ***,establishing a highly efficient and high quality FRB search pipeline is the primary task in FRB *** learning techniques provide new ideas for FRB search *** have detected radio bursts from FRB 20201124A in the L-band observational data of the Nanshan 26 m radio telescope(NSRT-26m)using the constructed deep learning based search pipeline named dispersed dynamic spectra search(DDSS).Afterwards,we further retrained the deep learning model and applied the DDSS framework to S-band *** this paper,we present the FRB observation system and search pipeline using the S-band *** carried out search experiments,and successfully detected the radio bursts from the magnetar SGR j1935+2145and FRB *** experimental results show that the search pipeline can complete the search efficiently and output the search results with high accuracy.

关键词： radio continuum general-methods data analysis-methods observational

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Fusion and one-neutron stripping process for ^(6)Li+^(94)Zr system around the Coulomb Barrier

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Chinese Physics C 2024年第9期48卷 133-141页

作者： Xuedou Su Guangxin Zhang Shipeng Hu Peiwei Wen H.O.Soler Gaolong Zhang Boshuai Cai Cenxi yuan j.L.Ferreira Zhenwei jiao Mingli Wang Xiaoyu Wang Zhen Huang Huanqiao Zhang Chunlei Zhang Xiaoguang Wu Yun Zheng Congbo Li Tianxiao Liand j.Lubian School of Physics Beihang UniversityBeijing 100191China Sino-French Institute of Nuclear Engineering and Technology Sun Yat-sen UniversityZhuhai 519082China Institute for Advanced Study in Nuclear Energy&Safety Shenzhen UniversityShenzhen 518060China Shenzhen Key Laboratory of Research and Manufacture of High Purity Germanium Materials and Fetectors Shenzhen UniversityShenzhen 518060China China Institute of Atomic Energy Beijing 102413China Instituto de Física Universidade Federal FluminenseNiterói 24210-340Rio de JaneiroBrazil State Key Laboratory of Radiation Medicine and Protection School of Radiation Medicine and ProtectionSoochow UniversitySuzhou 215123China The Key Laboratory of Beam Technology and Material Modification of Ministry of Education College of Nuclear Science and TechnologyBeijing Normal UniversityBeijing 100875China

The complete and incomplete fusion cross section as well as one-neutron stripping process of ^(6)Li+^(94)Zr system were measured at the energies around the Coulomb barrier by onlineγ-ray *** addition to a 30%suppression factor when compared with the measured total fusion process,the complete fusion cross section in ^(6)Li+^(94)Zr system was observed to be significantly lower than those in the nearby ^(6)Li+^(90,96)Zr *** new experimental result implies that the coupling with breakup channel in the ^(6)Li-induced fusion processes can be affected by the inner structure of the target,which is still not clear in any available model *** the one-neutron stripping process,the direct production cross sections for each level in 95Zr were extracted and compared with the coupled reaction channel calculation,offering a unique opportunity to examine the single-particle nature of the produced excited *** the fact that an overall overestimation of the production cross section for 954-keV and1618-keV levels was observed in the comparison,further investigation is highly demanded in order to understand the full reaction mechanism for the one-neutron stripping process induced by ^(6)Li.

关键词： weakly bound nuclei complete fusion incomplete fusion transfer reaction

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Community structure and carbon metabolism functions of bacterioplankton in the Guangdong coastal zone

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Marine Life Science & Technology 2024年第3期6卷 547-561页

作者： Ziqi Peng Pandeng Wang Xiaoqing Luo Qiqi Deng Ziwen Yang jiaxue Wu Wendong Xian Weicong Yan Xiaozhen Mou Yang yuan Wenjun Li jialing Li State Key Laboratory of Biocontrol Guangdong Provincial Key Laboratory of Plant Stress BiologySchool of Marine SciencesSchool of EcologySchool of Life SciencesSun Yat-Sen UniversityGuangzhou 510275China Southern Marine Science and Engineering Guangdong Laboratory(Guangzhou) Guangzhou 511458China Department of Biological Sciences Kent State UniversityKentOH 44242USA Marine Microorganism Ecological&Application Lab Marine Science and Technology CollegeZhejiang Ocean UniversityZhoushan 316000China

Coastal ecosystems are an important region for biogeochemical cycling,are a hotspot of anthropogenic disturbance and play a crucial role in global carbon cycling through the metabolic activities of *** can be broadly classified into two lifestyles:free-living(FL)and particle-attached(PA).However,how coastal bacterioplankton the community structure,co-occurrence networks and carbon metabolic functions with different lifestyles are differentiated is still largely *** these processes is necessary to better determine the contributions of coastal bacterioplankton to carbon ***,the characteristics of community structure and carbon metabolism function of bacterioplankton with two lifestyles in the coastal areas of Guangdong Province were investigated using amplicon sequencing,metagenomic,and metatranscriptomic *** results show that the main bacterioplankton responsible for carbon metabolism were the Pseudomonadota,Bacteroidota,and *** microbial community structure,carbon metabolic function,and environmental preferences differ between different *** and PA bacteria exhibited higher carbon fixation and degradation potentials,respectively.A range of environmental factors,such as dissolved oxygen,pH,and temperature,were associated with the community structure and carbon metabolic functions of the *** activities,such as nutrient discharge,may affect the distribution of functional genes and enhance the carbon degradation functions of *** conclusion,this study increased the understanding of the role of microorganisms in regulating carbon export in coastal ecosystems with intense human activity.

关键词： Particle-attached and free-living bacterioplankton Community structure Carbon metabolism Coastal ecosystem

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一种有效的适合F-j方法从背景噪声资料中提取多阶频散曲线的台阵划分方法

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地球物理学报 2024年第2期67卷 492-502页

作者：袁艺陈晓非北京大学地球与空间科学学院北京100871 中国地震局第二监测中心西安710054 广东省地球物理高精度成像技术重点实验室(南方科技大学) 深圳518055 南方科技大学地球与空间科学系深圳518055

近年发展起来的从地震背景噪声提取多阶频散曲线的F-j方法是一种台阵分析方法,对某一特定的研究区域内台阵的划分方式直接影响成像的效果.当研究区域地下结构较简单,且台站间距比较均匀时,可以使用简单的平移式移动阵列法;然而若研究区... 详细信息

近年发展起来的从地震背景噪声提取多阶频散曲线的F-j方法是一种台阵分析方法,对某一特定的研究区域内台阵的划分方式直接影响成像的效果.当研究区域地下结构较简单,且台站间距比较均匀时,可以使用简单的平移式移动阵列法;然而若研究区域地下结构复杂多变,尤其是台站间距疏密不均时,就需要根据具体的地域特征灵活划分台阵.本文介绍了一种适用于地下结构复杂及台站间距不均匀区域的台阵划分方法,具有一定的普适性.我们将其应用于美国阿拉斯加及加拿大西北部,验证了相比于简单的沿经纬度移动阵列,我们的分区方法确实大大提高了结果的分辨率,为后续反演研究区域三维速度结构提供了坚实的保障.

关键词： F-j变换台阵划分方法多阶面波阿拉斯加

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基于张量化微结构表征的筏化镍基单晶高温合金疲劳寿命评估

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力学学报 2024年第7期56卷 2029-2050页

作者：罗诚袁荒清华大学航天航空学院北京100084 清华大学航空发动机研究院北京100084

镍基单晶高温合金的微观组织在长时高温服役下会发生粗化和筏化等微结构演化,导致力学性能衰减,影响航空发动机的服役寿命.文章研究了粗化和筏化镍基单晶DD6合金的低周疲劳行为,通过高温热暴露和预蠕变处理分别制备了粗化和筏化合金,针... 详细信息

镍基单晶高温合金的微观组织在长时高温服役下会发生粗化和筏化等微结构演化,导致力学性能衰减,影响航空发动机的服役寿命.文章研究了粗化和筏化镍基单晶DD6合金的低周疲劳行为,通过高温热暴露和预蠕变处理分别制备了粗化和筏化合金,针对具有不同微结构状态的合金开展了980℃下的等温低周疲劳试验,发现粗化和筏化合金的疲劳寿命相比初态合金显著下降.基于电子扫描显微镜和光学显微镜对试件断口表面进行了微观表征,揭示了筏化组织对低周疲劳损伤机理的影响.裂纹扩展路径受微结构状态影响,相比初态合金,粗化和筏化合金中I型微裂纹会更早发生偏折,沿晶体学面扩展而导致更早的疲劳失效.基于组构张量及其张量分解方案对合金的微结构进行了量化表征,提取了微结构的特征参数,进一步提出了一种新的微结构敏感的等温疲劳寿命预测模型.通过分别关联γ-基体相和γ′-强化相组构张量的独立分量,解耦了粗化和筏化对寿命的影响.在新模型中,γ/γ′微结构形态对低周疲劳的影响得到了较好描述,预测结果的准确性和保守性得到了显著提高.研究结果可为工程中镍基单晶涡轮叶片的强度设计和寿命评估提供理论指导.

关键词：单晶合金张量化表征筏化疲劳寿命评估

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Potentiation of the lateral habenula-ventral tegmental area pathway underlines the susceptibility to depression in mice with chronic pain

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Science China(Life Sciences) 2024年第1期67卷 67-82页

作者： Chun-Kui Zhang Pan Wang yuan-yuan ji jian-Shuai Zhao jun-Xiang Gu Xian-Xia Yan Hong-Wei Fan Ming-Ming Zhang Yu Qiao Xiao-Die Liu Bao-juan Li Ming-Hui Wang Hai-Long Dong Hao-Hong Li Peng-Cheng Huang Yun-Qing Li Wu-Gang Hou jin-Lian Li Tao Chen Department of Anatomy and K.K.Leung Brain Research Centre Fourth Military Medical UniversityXi’an 710032China Beijing Institute of Basic Medical Sciences Beijing 100850China Key Laboratory of Ministry of Public Health for Forensic Science Xi’an Jiaotong UniversityXi’an 710061China Department of Anesthesiology Xijing HospitalFourth Military Medical UniversityXi’an 710032China Department of Neurosurgery the Second Affiliated Hospital of Xian Jiaotong UniversityXi’an 710004China School of Biomedical Engineering Fourth Military Medical UniversityXi’an 710032China Affiliated Mental Health Centre and Hangzhou Seventh People’s Hospital Zhejiang University School of MedicineHangzhou 310013China The MOE Frontier Research Center of Brain&Brain-machine Integration Zhejiang University School of Brain Science and Brain MedicineHangzhou 310058China Department of Neurology The First Affiliated Hospital of Nanchang UniversityNanchang 330006China Department of Anatomy School of MedicineNorthwest UniversityXi’an 710069China

Chronic pain often develops severe mood changes such as ***,how chronic pain leads to depression remains elusive and the mechanisms determining individuals’responses to depression are largely *** we found that depression-like behaviors could only be observed in 67.9%of mice with chronic neuropathic pain,leaving 32.1%of mice with depression *** determined that the spike discharges of the ventral tegmental area(VTA)-projecting lateral habenula(LHb)glutamatergic(Glu)neurons were sequentially increased in sham,resilient and susceptible mice,which consequently inhibited VTA dopaminergic(DA)neurons through a LHbGlu-VTAGABA-VTADA ***,the LHbGlu-VTADA excitatory inputs were dampened via GABAB receptors in a pre-synaptic *** of LHb-VTA pathway largely affected the development of depressive symptoms caused by chronic *** study thus identifies a pivotal role of the LHb-VTA pathway in coupling chronic pain with depression and highlights the activity-dependent contribution of LHbGlu-to-VTADA inhibition in depressive behavioral regulation.

关键词： chronic pain depression lateral habenula ventral tegmental area dopamine susceptibility

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Microglial glutaminase 1 mediates chronic restraint stress-induced depression-like behaviors and synaptic damages

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Signal Transduction and Targeted Therapy 2024年第1期9卷 40-43页

作者： Huili Chen Shengyang Fu Xiangyu Li Meng Shi jiazhen Qian Shu Zhao Ping yuan Lu Ding Xiaohuan Xia jialin C.Zheng Center for Translational Neurodegeneration and Regenerative Therapy Tongji Hospital affiliated to Tongji University School of Medicine200065 ShanghaiChina Department of Cardio-Pulmonary Circulation Shanghai Pulmonary HospitalSchool of MedicineTongji UniversityShanghaiChina Translational Research Institute of Brain and Brain-Like Intelligence Shanghai Fourth People’s Hospital affiliated to Tongji University School of Medicine200434 ShanghaiChina

Dear Editor,Major depressive disorder(MDD)is one of the most common psychiatric illnesses that significantly increase the risk of suicide.1 Stress-triggered dysfunctions of microglia have been identified as a commonly occurred pathological feature of MDD.1–3 Microglial dysfunction contributes to the pathogenesis of MDD via immunoresponses/neuroinflammation-mediated neural damage and pathological synapse loss-mediated neural circuit disruption.1 Although the involvement of microglia in MDD has been widely investigated,the molecular mechanisms underlying microglial dysfunction remain largely ***,we identified glutaminase 1(Gls1)as one key protein that participates in microglial dysfunction.4–6 Gls1 catalyzes the hydrolysis of glutamine to produce glutamate in the brain.4 Besides its well-known role in excitatory neurotoxicity,we found Gls1 up-regulation in microglia in animal models of Alzheimer’s disease and ischemic stroke.4,7 Gls1 activates microglia to overproduce cytokines and release inflammatory extracellular vesicles,therefore leading to neuroinflammation in animal models of Alzheimer’s disease and ischemic stroke.4–6 More importantly,Gls1 has been found to be up-regulated in the brains of MDD patients,and microglial Gls1 deficiency mitigated LPS-induced depression-like behaviors.8 However,LPS exposure is not an appropriate model to mimic MDD phenotypes,leaving the involvement of Gls1 in MDD an undetermined question.

关键词： involvement inflammation media

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Bilateral choroidal ganglioneuroma:a comprehensive analysis of vision decline in a 6-year-old boy

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International journal of Ophthalmology(English edition) 2024年第9期17卷 1755-1759页

作者： Yi-Zhe Cheng Li-Mei Sun Min-Er yuan Lin-Yan Zhang Shu-Ya Ke Xiao-Yan Ding State Key Laboratory of Ophthalmology Zhongshan Ophthalmic CenterSun Yat-sen UniversityGuangdong Provincial Key Laboratory of Ophthalmology and Visual ScienceGuangzhou 510060Guangdong ProvinceChina Guangdong Provincial Clinical Research Center for Ocular Diseases Guangzhou 510060Guangdong ProvinceChina

Dear Editor,We write to present a 6-year-old boy with bilateral choroidal ganglioneuroma(CG)by comprehensive multimodal imaging(MMI)in a duration of 6-year *** our knowledge,this is the first case report with elaborate data to delineate the natural history of visual function and MMI in a boy with rare bilateral CG,confirmed by choroid biopsy.

关键词： comprehensive modal fir

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