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光催化剂纳米粉体的制备技术

粉末冶金技术 2006年第5期24卷 379-383页

作者：倪萌 leung Michael K.H. leung dennis y.c. 香港大学机械工程系

纳米半导体材料作为光催化剂在环境、能源领域具有广阔的应用前景。光催化剂的制备过程对催化剂的晶体结构有重要的影响,从而影响其光催化活性。本文较系统地综述了国内外对光催化剂纳米粉体制备的研究进展,包括固相法、气相法和湿化学... 详细信息

纳米半导体材料作为光催化剂在环境、能源领域具有广阔的应用前景。光催化剂的制备过程对催化剂的晶体结构有重要的影响,从而影响其光催化活性。本文较系统地综述了国内外对光催化剂纳米粉体制备的研究进展,包括固相法、气相法和湿化学法。对比分析了各种制备技术的优缺点,并对今后的研究方向和应用前景进行了分析。

关键词：纳米材料光催化剂制备

Low-cost and efficient Mn/ceO_(2) catalyst for photocatalytic VOcs degradation via scalable colloidal solution combustion synthesis method

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Journal of Materials Science & Technology 2022年第21期116卷 169-179页

作者： yingguang Zhang Muyan Wu yifei Wang Xiaolong Zhao dennis y.c.leung Department of Mechanical Engineering The University of Hong KongPokfulam RoadHong KongChina School of Mechanical Engineering and Automation Harbin Institute of TechnologyShenzhen 518000China

colloidal solution combustion synthesis(cScS)is a simple and easy method for mass-production of crystalline nanomaterials with tunable pore *** this work,mesoporous Mn/ceO_(2) catalysts were fabricated via cScS method coupled with a dip-coating process and used for photocatalytic oxidation(PcO)of *** vacuum ultraviolet(VUV)irradiation,a high toluene removal efficiency of about 92%was achieved with a toluene reaction rate of about 118μmol/g/h in a continuous flow reactor.A possible degradation pathway was proposed based on the analysis of intermediates by Fourier transform infrared photoluminescence spectra(FTIR)and *** temperature-programmed reduction(H_(2)-TPR),Brunauer-Emmett-Teller(BET)surface areas,photoluminescence spectra(PL)spectra and X-ray photoelectron spectroscopy(XPS)were carried out to analyze physical and chemical properties of the *** with Mn_(x)ce_(1-x)O_(2) catalysts synthesized by one step cScS method,Mn/ceO_(2) has a higher photocatalytic activity,which is attributed to the presence of higher contents of ce^(3+),Mn^(2+)and Mn^(3+)*** presence of higher contents of these species plays a key role in the activity enhancement of toluene oxidation and ozone *** method is facile,efficient and scalable,and it may become a promising industrial application technology for catalyst synthesis in the near future.

关键词： Mesoporous ceO_(2) Manganese modification Scalable synthesis Photocatalysis VOcs abatement

Genomics-driven derivatization of the bioactive fungal sesterterpenoid variecolin:creation of an unnatural analogue with improved anticancer properties

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Acta Pharmaceutica Sinica B 2024年第1期14卷 421-432页

作者： Dexiu yan Jemma Arakelyan Teng Wan Ritvik Raina Tsz Ki chan Dohyun Ahn Vladimir Kushnarev Tsz Kiu cheung Ho ching chan Inseo choi Pui yi Ho Feijun Hu yujeong Kim Hill Lam Lau ying Lo Law chi Seng leung chun yin Tong Kai Kap Wong Wing Lam yim Nikolay S.Karnaukhov Richard y.c.Kong Maria V.Babak yudai Matsuda Department of chemistry City University of Hong KongHong Kong SARChina iGEM Team“Variecure” City University of Hong KongHong Kong SARChina Department of Biomedical Engineering City University of Hong KongHong Kong SARChina Moscow clinical Research center Named After A.S.Loginov Moscow 111123Russian Federation

A biosynthetic gene cluster for the bioactive fungal sesterterpenoids variecolin(1)and variecolactone(2)was identified in Aspergillus aculeatus ATcc *** production of 1 and 2 was achieved in Aspergillus oryzae by expressing the sesterterpene synthase VrcA and the cytochrome P450 ***,the replacement of VrcB with homologous P450s from other fungal terpenoid pathways yielded three new variecolin analogues(5-7).Analysis of the compounds’anticancer activity in vitro and in vivo revealed that although 5 and 1 had comparable activities,5 was associated with significantly reduced toxic side effects in cancer-bearing mice,indicating its potentially broader therapeutic *** study describes the first tests of variecolin and its analogues in animals and demonstrates the utility of synthetic biology for creating molecules with improved biological activities.

关键词： Animal studies Anticancer properties Biosynthesis Natural products Sesterterpenoids Synthetic biology Terpene synthases Variecolin

GO-modified flexible polymer nanocomposites fabricated via 3D stereolithography

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Frontiers of chemical Science and Engineering 2019年第4期13卷 736-743页

作者： chi Him Alpha Tsang Adilet Zhakeyev dennis y.c.leung Jin Xuan School of Environmental Sciences and Engineering Sun Yat-Sen UniversityGuangzhou 510006China Department of Mechanical Engineering The University of Hong KongHong KongChina Department of chemical Engineering Loughborough UniversityLoughboroughLE113TUUK

Graphene oxide(GO)induced enhancement of elastomer properties showed a great deal of potential in recent years,but it is still limited by the barrier of the complicated synthesis ***(SLA),used in fabrication of thermosets and very recently in“flexible”polymers with elastomeric properties,presents itself as simple and user-friendly method for integration of GO into *** this work,it was first time demonstrated that GO loadings can be incorporated into commercial flexible photopolymer resins to successfully fabricate GO/elastomer nanocomposites via readily accessible,consumer-oriented SLA *** material properties of the resulting polymer was characterized and *** mechanical strength,stiffness,and the elongation of the resulting polymer decreased with the addition of *** thermal properties were also adversely affected upon the increase in the GO content based on differential scanning calorimetry and thermogravimetric analysis *** was proposed that the GO agglomerates within the 3D printed composites,can result in significant change in both mechanical and thermal properties of the resulting *** study demonstrated the possibility for the development of the GO/elastomer nanocomposites after the optimization of the GO/“Hexible”photoreactive resin formulation for SLA with suitable annealing process of the composite in future.

关键词： graphene oxide polymer flexible 3D printing stereolithography

chemical biology investigation of a triple-action,smart-decomposition antimicrobial booster based-combination therapy against“ESKAPE”pathogens

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Science china chemistry 2024年第9期67卷 3071-3082页

作者： Min Wang Huangsheng Pu yangfan Xu chenxuan Wu yuanxin Gu Qingyun cai Guoxing yin Peng yin chunhui Zhang Wing-leung Wong Muyang Wan yugang Bai Xinxin Feng State Key Laboratory of chem-/Bio-Sensing and chemometrics Hunan Provincial Key Laboratory of Biomacromolecular Chemical Biologyand School of Chemistry and Chemical EngineeringHunan UniversityChangsha 410082China college of Biology Hunan UniversityChangsha 410082China college of Advanced Interdisciplinary Studies&Hunan Provincial Key Laboratory of Novel Nano Optoelectronic Information Materials and Devices National University of Defense TechnologyChangsha 410073China Nanhu Laser Laboratory National University of Defense TechnologyChangsha 410073China Key Laboratory of chemical Biology and Traditional chinese Medicine Research(Ministry of Education) College of Chemistry and Chemical EngineeringHunan Normal UniversityChangsha 410081China State Key Laboratory of chemical Biology and Drug Discovery Department of Applied Biology and Chemical TechnologyThe Hong Kong Polytechnic UniversityHong Kong SAR 999077China Hunan Provincial Key Laboratory of Anti-Resistance Microbial Drugs The Third Hospital of Changsha(The Affiliated Changsha Hospital of Hunan University)Changsha 410015China

The global antibiotic resistance crisis necessitates urgent *** innovative approach involves potentiating antibiotics and non-antibiotic drugs with adjuvants or boosters.A major drawback of these membrane-active boosters is their limited biocompatibility,as they struggle to differentiate between prokaryotic and eukaryotic *** study reports the chemical biology investigation of a dual-action oligoamidine(OA1)booster with a glutathione-triggered decomposition ***1,when combined with other antimicrobial molecules,exhibits a triple-targeting mechanism including cell membrane disruption,DNA targeting,and intracellular enzyme *** multi-targeting mechanism not only enhances the in vitro and in vivo eradication of antibiotic-resistant“ESKAPE”pathogens,but also suppresses the development of bacterial ***,OA1 maintains its activity in bacterial cells by.c.eating an oxidative environment,while it quickly decomposes in mammalian cells due to high glutathione *** mechanistic insights and design principles may provide a feasible approach to develop novel antimicrobial agents and effective anti-resistance combination therapies.

关键词： antimicrobial booster oligoamidine membrane disruption DNA targeting triggered degradation anti-resistance

computational fluid dynamics simulation of the wind flow over an airport terminal building

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Journal of Zhejiang University-Science A(Applied Physics & Engineering) 2010年第6期11卷 389-401页

作者： chun-ho LIU dennis y.c.leung Alex c.S.MAN P.W.cHAN Department of Mechanical Engineering The University of Hong Kong Hong Kong Observatory

Turbulence in the wake generated by wind flow over buildings or obstacles may produce complex flow patterns in downstream *** include the recirculating flow and wind deficit areas behind an airport terminal building and their potential impacts on the aircraft landing on nearby runways.A computational fluid dynamics(cFD) simulation of the wind flow over an airport terminal building was performed in this study of the effect of the building wake on landing *** normal meteorological conditions,the studied airport terminal building causes limited effects on landing aircraft because most of the aircraft have already landed before entering the turbulent wake *** simulating the approach of a tropical cyclone,additional cFD sensitivity tests were performed to study the impacts of building wake under extreme meteorological *** was found that,in a narrow range of prevalent wind directions with wind speeds larger than a certain threshold value,a substantial drop in wind speed(>3.6 m/s) along the glide path of aircraft was observed in the building *** cFD results also showed that under the most critical situation,a drop in wind speed as large as 6.4 m/s occurred right at the touchdown point of landing aircraft on the runway,an effect which may have a significant impact on aircraft *** study indicated that a comprehensive analysis of the potential impacts of building wake on aircraft operations should be carried out for airport terminals and associated buildings in airfields to ensure safe aviation operation under all meteorological conditions and to facilitate implementation of precautionary measures.

关键词： Aviation safety Building aerodynamics computational fluid dynamics (cFD) k-e turbulence model Tropicalcyclone

Solid-state Al-air battery with an ethanol gel electrolyte

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Green Energy & Environment 2023年第4期8卷 1117-1127页

作者： yifei Wang Wending Pan Kee Wah Leong Shijing Luo Xiaolong Zhao dennis y.c.leung School of Mechanical Engineering and Automation Harbin Institute of TechnologyShenzhenChina Department of Mechanical Engineering The University of Hong KongHong KongChina

Hydrogel electrolyte is especially suitable for solid-state Al-air batteries targeted for various portable applications, which may, however, lead to continuous Al corrosion during battery standby. To tackle this issue, an ethanol gel electrolyte is developed for Al-air battery for the first time in this work, by using KOH as solute and polyethylene oxide as gelling agent. The ethanol gel is found to effectively inhibit Al corrosion compared with the water gel counterpart, leading to stable Al storage. When assembled into an Al-air battery, the ethanol gel electrolyte achieves a much improved discharge lifetime and specific capacity, which are 5.3 and 4.1 times of the water gel electrolyte at 0.1 mA cm^(-2), *** studying the gel properties, it is found that a lower ethanol purity.c.n improve the battery power output, but at the price of decreased discharge efficiency. On the contrary, a higher polymer concentration will decrease the power output, but can bring extra benefit to the discharge efficiency. As for the gel thickness, a moderate value of 1 mm is preferred to balance the power output and energy efficiency. Finally, to cater the increasing market of flexible electronics, a flexible Al-air battery is developed by impregnating the ethanol gel into a paper substrate, which can function normally even under serious deformation or damage.

关键词： Al-air battery Gel electrolyte Ethanol gel Al corrosion Polyethylene oxide

Effect of terrain and building structures on the airflow in an airport

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Journal of Zhejiang University-Science A(Applied Physics & Engineering) 2012年第6期13卷 461-468页

作者： dennis y. c. leung W. y. LO W. y. cHOW P. W. cHAN Department of Mechanical Engineering The University of Hong Kong Hong Kong China Hong Kong Observatory Hong Kong China

The aim of this study was to perform computational fluid dynamics (cFD) simulations on the airflows at the Hong Kong International Airport (HKIA). In particular, the effects of hangar buildings and terrain were studied to explore the effects of turbulence on flying aircraft, especially during landing. The cFD simulation showed that significant differences in wind speeds may occur between the north and the south runways on the western part of the HKIA under typhoon conditions with a strong north to northwesterly wind. Simulation also showed that the hanger buildings between the two runways on the western side and the nearby terrain could be causing the observed difference in the wind speeds. The results also indicated that these obstacles could cause significant wind speed variations at the western end of the south runway. This may affect the operation of landing aircraft. The cFD results for a typical typhoon case were analyzed and found to match the wind data recorded by an aircraft landing that day.

关键词： computational fluid dynamics (cFD) Hong Kong International Airport (HKIA) Low-level wind effect Hangars Terrain

Paper-based aqueous Al ion battery with water-in-salt electrolyte

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Green Energy & Environment 2023年第5期8卷 1380-1388页

作者： yifei Wang Wending Pan Kee Wah Leong yingguang Zhang Xiaolong Zhao Shijing Luo dennis y.c.leung School of Mechanical Engineering and Automation Harbin Institute of TechnologyShenzhen518055China Department of Mechanical Engineering The University of Hong KongHong KongChina

Low-cost,flexible and safe battery technology is the key to the widespread usage of wearable electronics,among which the aqueous Al ion battery with water-in-salt electrolyte is a promising *** this work,a flexible aqueous Al ion battery is developed using cellulose paper as *** water-in-salt electrolyte is stored inside the paper,while the electrodes are either printed or attached on the paper surface,leading to a lightweight and thin-film battery ***,this battery.c.n tolerate a charge and discharge rate as high as 4 A g^(-1) without losing its storage *** charge voltage is around 2.2 V,while the discharge plateau of 1.6–1.8 V is among the highest in reported aqueous Al ion batteries,together with a high discharge specific capacity of~140 mAh g^(-1).However,due to the water electrolysis side reaction,the faradaic efficiency.c.n only reach 85%with a cycle life of 250 due to the dry out of *** from using flexible materials and aqueous electrolyte,this paper-based Al ion battery.c.n tolerate various deformations such as bending,rolling and even puncturing without losing its *** two single cells are connected in series,the battery pack can provide a charge voltage of 4.3 V and a discharge plateau as high as 3–3.6 V,which are very.c.ose to commercial Li ion *** a cheap,flexible and safe battery technology may be widely applied in low-cost and large-quantity applications,such as RFID tags,smart packages and wearable biosensors in the future.

关键词： Al ion battery Aqueous electrolyte Water-in-salt Paper battery Flexible battery