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Frontiers of Information Technology & Electronic Engineering 2024年第2期25卷 250-259页

作者： Ying SUN Miaomiao fu Jingyang MAO Guoliang wei Business School University of Shanghai for Science and TechnologyShanghai200093China Shanghai Caoyang Vocational School Shanghai200333China School of Electrical and Electronic Engineering Shanghai Institute of TechnologyShanghai201418China School of Intelligent Emergency Management University of Shanghai for Science and TechnologyShanghai200093China

Cyber-physical systems(CPSs)take on the characteristics of both multiple rates of information collection and processing and the dependency on information *** purpose of this paper is to develop a joint recursive filtering scheme that estimates both unknown inputs and system states for multi-rate CPSs with unknown *** cyberspace,the information transmission between the local joint filter and the sensors is governed by an adaptive event-triggered ***,the desired parameters of joint filters are determined by a set of algebraic matrix equations in a recursive way,and a sufficient condition verifying the boundedness of filtering error covariance is found by resorting to some algebraic operation.A state fusion estimation scheme that uses local state estimation is proposed based on the covariance intersection(CI)based fusion ***,an illustrative example demonstrates the effectiveness of the proposed adaptive event-triggered recursive filtering algorithm.

关键词： Cyber-physical systems Multi-rate Joint recursive filtering Adaptive event-triggered mechanisms Unknown inputs

Photoinduced Dehalocyclization to Access Oxindoles Using Formate as a Reductant

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Chinese Journal of Chemistry 2024年第11期42卷 1203-1208页

作者： wei Ge Jia-Xin Wang Ming-Chen fu Yao fu Hefei National Research Center for Physical Sciences at the Microscale iChEMCAS Key Laboratory of Urban Pollutant ConversionAnhui Province Key Laboratory of Biomass Clean EnergyUniversity of Science and Technology of ChinaHefeiAnhui230026 China Anhui Province Key Laboratory of Value-Added Catalytic Conversion and Reaction Engineering Hefei University of TechnologyHefeiAnhui230009 China

Herein,we report an efficient and practical protocol for the photoinduced dehalocyclization of ortho-halophenylacrylamides with formate by the engagement of a CO_(2) radical anion to access substituted *** method proceeds smoothly under mild conditions and exhibits a wide range of substrate as well as remarkable functional group compatibility.

关键词： Formate CO_(2)Radical ions Oxindole Photocatalysts Cyclization Organohalides

Significantly Enhanced Melt Memory Effect of Metallocene-made Isotactic Polypropylene Containing Talc

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Chinese Journal of Polymer Science 2024年第2期42卷 213-222,I0008页

作者： Hong-Wen Sun fu-Shan Wang Yan Gao fu-Qing wei Jia-Chun Feng State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular ScienceFudan UniversityShanghai200433China Lanzhou Petrochemical Corporation of PetroChina Lanzhou730060China Lanzhou Petrochemical Research Center Petrochemical Research Institute of PetroChinaLanzhou730060China

The melt memory effect is a widely observed phenomenon in semi-crystalline polymers. In practical applications, various additives are usually introduced into polymers, which may affect their melt memory behavior. In this work, the effect of talc on the melt memory effect of metallocene-made isotactic polypropylene(M-PP) was investigated in detail by using the differential scanning calorimetry. The results indicated that the introduction of talc significantly strengthened the melt memory effect of M-PP. Specifically, the upper limit temperature of Domain II increased from 161 ℃ to 174 ℃, resulting in a substantial widening of the temperature range of Domain IIa from 1 ℃ to 14 ℃. Analysis of the crystal orientation of the M-PP containing talc cooled from various Ts suggested that the remarkably enhanced melt memory effect could be ascribed to the stabilization of oriented nuclei facilitated by talc. This stabilizing effect was likely attributable to the prefreezing effect or the sorption interaction between talc and the M-PP chains.

关键词： Metallocene-made isotactic polypropylene Talc Melt memory effect Crystal orientation

Insight into the Role of Isolated Gold Atoms-Ceria Conjunction in Catalyzing the Water-Gas Shift Reaction

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Chinese Journal of Chemistry 2024年第6期42卷 636-644页

作者： Xin-Pu fu Hui-Zhao wei-wei Wang Chun-Jiang Jia Key Laboratory for Colloid and Interface Chemistry Key Laboratory of Special Aggregated MaterialsSchool of Chemistry and Chemical EngineeringShandong UniversityJinanShandong250100 China

As the promising catalysts for the water-gas shift(WGS)reaction,the activity of Au-CeO_(2) composites is susceptible to the aggregation size and electronic state of Au *** reports were extensively focused on the discrepancy between nonmetallic Au and metallic Au nanoparticles,whereas the understanding of the authentic role of the isolated Au atoms was ***,we investigated the catalytic behavior and structural information over two types of Au/CeO_(2) catalysts,in which the predominant conjunctions were isolated Au1-CeO_(2) and Aun-CeO_(2),*** on comprehensive characterizations,particularly by in-situ Raman and in-situ DRIFTS,we found that the isolated Au atoms were responsible for enhancing the reducibility of the CeO_(2) *** CO adsorption ability on the isolated Au sites was significantly inferior to clustered Au atoms,especially at relatively high temperatures(>200°C).As a result,the boosted O vacancy on the isolated Au1-CeO_(2) conjunctions could improve the H2O activation ability for the Au-CeO_(2) catalysts and demonstrate a comparable activity to the clustered Aun-CeO_(2) *** work might deepen understanding of the catalytic function for the isolated Au1 site within Au/CeO_(2) systems while catalyzing the WGS reaction.

关键词： Isolated Au atoms Ceria-based catalysts Water-gas shift reaction Defect Adsorption

Machine learning-assisted efficient design of Cu-based shape memory alloy with specific phase transition temperature

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International Journal of Minerals,Metallurgy and Materials 2024年第4期31卷 773-785页

作者： Mengwei Wu wei Yong Cunqin fu Chunmei Ma Ruiping Liu Department of Materials Science and Engineering China University of Mining&Technology(Beijing)Beijing 100083China Institute for Advanced Materials and Technology University of Science and Technology BeijingBeijing 100083China

The martensitic transformation temperature is the basis for the application of shape memory alloys(SMAs),and the ability to quickly and accurately predict the transformation temperature of SMAs has very important practical *** this work,machine learning(ML)methods were utilized to accelerate the search for shape memory alloys with targeted properties(phase transition temperature).A group of component data was selected to design shape memory alloys using reverse design method from numerous unexplored *** modeling and feature modeling were used to predict the phase transition temperature of the shape memory *** experimental results of the shape memory alloys were obtained to verify the effectiveness of the support vector regression(SVR)*** results show that the machine learning model can obtain target materials more efficiently and pertinently,and realize the accurate and rapid design of shape memory alloys with specific target phase transition *** this basis,the relationship between phase transition temperature and material descriptors is analyzed,and it is proved that the key factors affecting the phase transition temperature of shape memory alloys are based on the strength of the bond energy between *** work provides new ideas for the controllable design and performance optimization of Cu-based shape memory alloys.

关键词： machine learning support vector regression shape memory alloys martensitic transformation temperature

新颖的大环冠醚基对碘苯胺包合物:设计合成、晶体结构及介电性质(英文)

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无机化学学报 2013年第8期29卷 1696-1702页

作者：周琴琴付大伟东南大学化学化工学院有序物质科学研究中心南京210096

合成了新颖的有机一无机杂化超分子化合物，【（4-IA-NH3}·（18-crown．6）12（Cu：C16）（1），4-IA-NH3=对碘苯胺离子，18-crown-6：18-冠-6。并通过红外光谱、粉末衍射、热重分析和单晶结构分析对化合物进行了充分表征。在转子定子... 详细信息

合成了新颖的有机一无机杂化超分子化合物，【（4-IA-NH3}·（18-crown．6）12（Cu：C16）（1），4-IA-NH3=对碘苯胺离子，18-crown-6：18-冠-6。并通过红外光谱、粉末衍射、热重分析和单晶结构分析对化合物进行了充分表征。在转子定子型的超分子化合物1中．[（4-IA-NH3）·（18·crown-6）】-超分子阳离子和（Cu：C16）。一阴离子交错堆积形成包合物结构。变温介电常数测量表明．在130。450K范围内没有相变引起的介电异样。大环醚的热无序运动及由此引起的氢键偶极瞬间变化使得化合物在低频500Hz和高温350K以上具有较高的介电常数并伴随高的介电损耗。

关键词：包合物冠醚大环晶体结构介电

Entropy variances of pure coherent states in the diffusion channel

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CHINESE PHYSICS B 2024年第9期33卷 384-388页

作者： Wu, wei-Feng Fang, Yong fu, Peng Chizhou Univ Sch Mech & Elect Engn Chizhou 247000 Peoples R China Anhui Res Ctr Semicond Ind Gener Technol Chizhou 247000 Peoples R China

Using the operator correspondence of the real and fictious modes in the thermo entangled state representation, we solve the quantum master equation describing the diffusion channel and obtain the Kraus operator-sum representation of its analytical solution. we find that the pure coherent states evolve into the new mixed thermal superposed states in the diffusion channel. Also, we investigate the statistical properties of the initial coherent states and their entropy evolutions in the diffusion channel, and find that the entropy evolutions are only related to the decay time and without the amplitudes of the initial coherent states.

关键词： entangled state representation diffusion channel coherent state entropy evolution 42.50.-p 03.65.-w 05.30.-d OPERATOR-SUM REPRESENTATION

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带升力风扇的垂直起降推进系统建模研究

推进技术 2018年第3期39卷 685-694页

作者：符大伟张海波南京航空航天大学能源与动力学院江苏省航空动力系统重点实验室江苏南京210016

为了填补国内对转升力风扇研究与垂直起降系统建模研究相结合的空缺,分别针对常规与对转升力风扇,建立了垂直起降推进系统的部件级实时数学模型,并进行了性能对比。针对减阻的要求,通过插值将升力风扇进气道的阻力系数选为0.0470;针对... 详细信息

为了填补国内对转升力风扇研究与垂直起降系统建模研究相结合的空缺,分别针对常规与对转升力风扇,建立了垂直起降推进系统的部件级实时数学模型,并进行了性能对比。针对减阻的要求,通过插值将升力风扇进气道的阻力系数选为0.0470;针对升力风扇非设计点特性准确性的要求,采用基元级理论对风扇进行半设计半计算;特别引入中介推力修正系数(κ)用于对转风扇的参数设计,该方法下两升力风扇推力相等,轴功率偏差为0.0265。进一步的动态仿真表明,由于风扇特性的影响,同样工况下非设计点处对转风扇的升力和轴功率更大;并且由于升力风扇与发动机的耦合性,针对不同升力风扇的差异性,发动机会通过调整转速而产生"趋同"的作用效果。

关键词：常规/对转升力风扇基元级理论中介推力修正系数趋同作用

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城市创新系统与风险投资体系互动运作研究

科学学研究 2003年第Z1期21卷 289-295页

作者：隋映辉付大伟山东科技大学科技经济与管理研究所山东青岛266071

城市创新系统与风险投资体系在表面上存在差别的同时本质上有着紧密关联,二者的本质决定了它们通过科技产业这一媒介相互作用、相互联系,形成了动态、开放的互动运作网络,并且这一网络的良性运作对风险投资体系的顺畅运行,对城市创新系... 详细信息

城市创新系统与风险投资体系在表面上存在差别的同时本质上有着紧密关联,二者的本质决定了它们通过科技产业这一媒介相互作用、相互联系,形成了动态、开放的互动运作网络,并且这一网络的良性运作对风险投资体系的顺畅运行,对城市创新系统的持续发展,进而向外延伸对整个国家的产业结构调整、升级都具有重大的战略意义。本文试图通过对此互动网络中城市创新系统与风险投资体系的关系、定位、对接点进行研究,揭示互动运作的实质、运作机理及影响运作绩效的关键因素,为政策的提出进行理论上的探讨。

关键词：城市创新系统风险投资体系互动

Preparation of yttrium oxide coating with enhanced thermal shock resistance on refractories used for titanium alloy melting and casting

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Journal of Iron and Steel Research International 2024年第6期31卷 1411-1422页

作者： Ao Chen Yan Ma Zhou-fu Wang Hao Liu Xi-tang Wang Sen-na Chen Chen-xin Zhang Zi-yi Tang wei-dong fu wei Cheng The State Key Laboratory of Refractories and Metallurgy Wuhan University of Science and TechnologyWuhan 430081HubeiChina Xiangyang Juli High Technology Material Co. Ltd.Xiangyang 441705HubeiChina Xiangyang Public Inspection and Testing Center Xiangyang 441000HubeiChina

In order to enhance the service life of refractories for melting and casting of titanium alloy,preparation of yttrium oxide coatings on the refractories surface is an effective *** improvement of thermal shock stability of the coating is beneficial to its spalling resistance during the high-temperature service,and the available slurry with good performance is the *** effects of the varieties and contents of dispersant(sodium tripolyphosphate,sodium hexametaphosphate,sodium pyrophosphate,citric acid and polycarboxylate ammonium salt)and binder(aluminum dihydrogen phosphate,zirconium acetate and yttria sol)on the stability,rheological and thixotropic properties of yttrium oxide waterbased slurry were investigated,and the effects of slurry composition design on the thermal shock resistance of the coating were *** results showed that the introduction of polycarboxylate ammonium salt as dispersant significantly improved the stability of the slurry,and the varieties of the binders had significant effects on the dispersibility of the *** aluminum dihydrogen phosphate and polycarboxylate ammonium salt were used as binder and dispersant,respectively,the slurry had better stability,suitable rheological and thixotropic *** using aluminum dihydrogen phosphate as binder,the coating had good thermal shock resistance and no obvious cracks were observed for the coating after thermal shock,which was attributed to the yttrium aluminate binding phase generated in the *** effective method was provided for preparing yttrium oxide coatings with enhanced thermal shock resistance applied in the process of titanium alloy melting and casting.

关键词： Yttrium oxide-Slurry Stability Rheological property Thixotropic property-Coating Thermal shock resistance