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EventLFM:event camera integrated Fourier light field microscopy for ultrafast 3d imaging

Light(Science & Applications) 2024年第7期13卷 1401-1415页

作者： Ruipeng Guo Qianwan Yang Andrew S.Chang Guorong Hu Joseph Greene Christopher v.Gabel Sixian You Lei Tian department of Electrical and Computer Engineering Boston UniversityBostonMA 02215USA department of Physiology and Biophysics Boston UniversityBostonMA 02215USA. Neurophotonics Center Boston UniversityBostonMA 02215USA. Research Laboratory of Electronics(RLE)in the department of Electrical Science and Engineering Massachusetts Institute of TechnologyCambridgeMA 02139USA. department of Biomedical Engineering Boston UniversityBostonMA 02215USA

Ultrafast 3d imaging is indispensable for visualizing complex and dynamic biological *** scanning-based techniques necessitate an inherent trade-off between acquisition speed and space-bandwidth product(SBP).Emerging single-shot 3d wide-field techniques offer a promising alternative but are bottlenecked by the synchronous readout constraints of conventional CMOS systems,thus restricting data throughput to maintain high SBP at limited frame *** address this,we introduce EventLFM,a straightforward and cost-effective system that overcomes these challenges by integrating an event camera with Fourier light field microscopy(LFM),a state-of-theart single-shot 3d wide-field imaging *** event camera operates on a novel asynchronous readout architecture,thereby bypassing the frame rate limitations inherent to conventional CMOS *** further develop a simple and robust event-driven LFM reconstruction algorithm that can reliably reconstruct 3d dynamics from the unique spatiotemporal measurements captured by *** results demonstrate that EventLFM can robustly reconstruct fast-moving and rapidly blinking 3d fluorescent samples at kHz frame ***,we highlight EventLFM’s capability for imaging of blinking neuronal signals in scattering mouse brain tissues and 3d tracking of GFP-labeled neurons in freely moving *** believe that the combined ultrafast speed and large 3d SBP offered by EventLFM may open up new possibilities across many biomedical applications.

关键词： field linking overcome

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Atomic dispersed Hetero‑Pairs for Enhanced Electrocatalytic CO_(2)Reduction

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Nano-Micro Letters 2024年第1期16卷 55-67页

作者： Zhaoyong Jin Meiqi Yang Yilong dong Xingcheng ma Ying Wang Jiandong Wu Jinchang Fan dewen Wang Rongshen Xi Xiao Zhao Tianyi Xu Jingxiang Zhao Lei Zhang david J.Singh Weitao Zheng Xiaoqiang Cui State Key Laboratory of Automotive Simulation and Control School of Materials Science and EngineeringKey Laboratory of Automobile Materials of MOEElectron Microscopy CenterJilin UniversityChangchun 130012People’s Republic of China Key Laboratory of Photonic and Electronic Bandgap materials Ministry of Educationand College of Chemistry and Chemical EngineeringHarbin Normal UniversityHarbin 150025People’s Republic of China College of Chemistry Jilin UniversityChangchun 130012People’s Republic of China department of Physics and Astronomy and department of Chemistry University of MissouriColumbiaMO 65211USA

Electrochemical carbon dioxide reduction reaction(CO_(2)RR)involves a variety of intermediates with highly correlated reaction and ad-desorption energies,hindering optimization of the catalytic *** example,increasing the binding of the*COOH to the active site will generally increase the*CO desorption *** this relationship may be expected to dramatically improve the intrinsic activity of CO_(2)RR,but remains an unsolved ***,we addressed this conundrum by constructing a unique atomic dispersed hetero-pair consisting of Mo-Fe di-atoms anchored on N-doped carbon *** system shows an unprecedented CO_(2)RR intrinsic activity with TOF of 3336 h−1,high selectivity toward CO production,Faradaic efficiency of 95.96%at−0.60 v and excellent *** calculations show that the Mo-Fe diatomic sites increased the*COOH intermediate adsorption energy by bridging adsorption of*COOH *** the same time,d-d orbital coupling in the Mo-Fe di-atom results in electron delocalization and facilitates desorption of*CO ***,the undesirable correlation between these steps is *** work provides a promising approach,specifically the use of di-atoms,for breaking unfavorable relationships based on understanding of the catalytic mechanisms at the atomic scale.

关键词： CO_(2)reduction reaction Atomic dispersed catalyst Hetero-diatomic pair Ad-desorption energy Linear scaling relation

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Global paleobiogeography of Albian—Cenomanian(mid-Cretaceous)marine ostracods

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Journal of Palaeogeography 2024年第2期13卷 212-236页

作者： Bernardo vázquez-García Jorge villegas-martín Gerson Fauth Leonardo Borghi Aristóteles de Moraes Rios Netto Post-Graduate Program in Geology Unisinos UniversitySao LeopoldoRSBrazil Technological Institute of Paleoceanography and Climate Change-Itt Oceaneon Unisinos UniversitySao LeopoldoRSBrazil Laboratory of Sedimentary Geology(Lagesed) Department of GeologyInstitute of GeosciencesUFRJ-Federal Universityof Riode JaneiroBrazil Labmicro Department of GeologyInstitute of GeosciencesUFRJ-Federal University of Rio de JaneiroBrazil

despite their potential for providing important information for paleobiogeography,studies using ostracod assemblages compiled from global datasets have been scarce so *** this study,the paleogeographic implications of the relationship between different ostracod assemblages are analyzed and discussed for the Albian and *** compiled an ostracod dataset at the genus level,with 168 genera for the Albian and 174 for the Cenomanian,to which different multivariate statistical methods of grouping were *** affinity between different ostracod assemblages from different regions allowed for the delineation of 30 operational geographic units(OGUs)for the Albian,and 32 OGUs for the Cenomanian,grouped in three paleobiogeographic units(PBUs;Megatethys,Persia,and Austral)and one sub-unit(PBSU;maghreb associated to the Megatethys).The maghreb PBSU showed minor changes between the Albian and *** relationship among the OGUs grouped in each PBU is related to different factors,such as eustatic sea level events,similar climatic zones,and marine current circulation patterns.A relationship was observed between the Gabon and Nigeria OGUs with the Persia PBU,which suggests a direct east—west connection between them during the *** affinity observed in the Austral PBU between the South American,South African,and Australian regions during the Albian can be explained by their relative geographic isolation due to the Walvis Ridge *** eventual flooding of this barrier led to the relationship observed between the SE Brazilian and Bolivian regions with the Austral ***,the data also suggested that the separation of the Indian subcontinent from the Austral PBU took place during the Cenomanian.

关键词： Operational geographic units Paleobiogeographic units Albian Cenomanian marine ostracods

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A combined computational/experimental study of anode-concerned voltage drop in aqueous primary Mg-air batteries

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Journal of magnesium and Alloys 2024年第5期12卷 1854-1866页

作者： Wen Xu Min deng darya Snihirova Linqian Wang Yulong Wu Sviatlana v.Lamaka Mikhail L.Zheludkevich daniel Hoche Institute of Surface Science Helmholtz-Zentrum Hereon21502 GeesthachtGermany School of materials Science and Engineering Hebei University of Technology300000TianjinChina Institute for materials Science Faculty of EngineeringKiel University24143 KielGermany

The voltage drop appearing at Mg anode-electrolyte interface is a critical issue for the battery power and energy density of aqueous primary Mg-air *** respective voltage loss is typically assigned to the deposits layer forming on the anode surface during *** this work,we experimentally and computationally investigate the critical factors affecting the voltage drop at Mg anode towards a deeper understanding of the contribution of deposit and its growth.A two-dimensional(2d)mathematical model is proposed to compute the voltage drop of Mg-0.15Ca wt.%alloy(Mg-0.15Ca)by means of a semi-empirical formulas and experiments-based modification model,considering the effect of discharge current density,the negative difference effect(NdE)and surface deposits layer *** model is utilized to simulate the discharge potential of the anode at predefined experimental current *** computed voltage drop(half-cell voltage)is in good agreement with the experimental *** applicability of the mathematical model is successfully validated on the second material(namely high-purity Mg).

关键词： Aqueous Mg-air battery voltage drop NdE Charge transfer deposits-related resistances

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Heavy metal pollution of river water and eco-friendly remediation using potent microalgal species

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Water Science and Engineering 2024年第1期17卷 41-50页

作者： Amudham Radha Amal Raj Prabhakaran Mylsamy v.Sivasankar B.Sathish Kumar Kiyoshi Omine T.G.Sunitha Phycological Research Laboratory Research Department of BotanyPachaiyappa's College(Affiliated to University of Madras)Chennai 600030India Research department of Chemistry Pachaiyappa's College(Affiliated to University of Madras)Chennai 600030India department of Botany Sri Vidya Mandir Arts&Science College(Autonomous)KatteriUthangarai 636902India department of Civil Engineering School of Engineering.Nagasaki UniversityNagasaki-Daigaku1-14 Bunkyo-machiNagasaki 8528521Japan

Pollution of rivers is mainly caused by anthropogenic activities such as discharge of effluent from industrial facilities,maintenance of sewage/effluent treatment plants,and dumping of solid waste on river *** study dealt with the pollution issues of the Cooum River in the well-known city of Chennai in South *** samples from 27 locations were collected and analyzed for 12 elements,including Ba,B,and Al,as well as heavy metals such as Pb,Cr,Mn,Fe,Co,Ni,Cu,Zn,and *** samples showed levels of these elements that exceeded World Health Organization *** correlation analysis revealed the inter-dependency among elements,and the contribution of each element based on factor loadings showed its percentage contribution compared to *** samples from six significant locations were chosen for remediation with three algae:Chlorella vulgaris,Scenedesmus dimorphus,and Phormedium *** uptake of pollutants led to the continuous growth of algae during the incubation period of 15 d,effectively removing heavy metals from the river *** increasing levels of algal counts and the chlorophyll a content confirmed the algal growth during the incubation period,followed by a declining stage after the incubation *** scanning electron microscopic images of algae before and after the remediation showed no remarkable modification of morphological *** study showed that the uptake of heavy metals using algae is an effective water pollution remediation measure,making the process practicable in the field on a large scale in the near future.

关键词： Heavy metal Cooum river Phycoremediation Microalgae Factor analysis

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Stroke depression:a concept with clinical applicability

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Stroke & vascular Neurology 2024年第3期9卷 189-193页

作者： Jun Mu Arun v Ravindran Pim Cuijpers Yiqing Shen Wensong Yang Qi Li Xinyu Zhou Peng Xie department of Neurology The First Affiliated Hospital of Chongqing Medical UniversityChongqingChina Campbell Family Mental Health Research Centre Centre for Addiction and Mental HealthDepartment of PsychiatryUniversity of TorontoTorontoOntarioCanada department of Clinical Neuro and Developmental PsychologyAmsterdam Public Health research instituteVrije Universiteit AmsterdamAmsterdamThe Netherlands NHC Key Laboratory of diagnosis and Treatment on Brain Functional diseases The First Affiliated Hospital of Chongqing Medical UniversityChongqingChina department of Psychiatry The First Affiliated Hospital of Chongqing Medical UniversityChongqingChina

Stroke is a common neurological condition and among the leading causes of death and disability *** is both a risk factor for and complication of stroke,and the two conditions may have a complex reciprocal relationship over ***,the secondary effects of depression on stroke are often overlooked,resulting in increased morbidity and *** the previous concept of‘poststroke depression’,stroke and depression were considered as two independent *** often delays the diagnosis and treatment of *** concept‘stroke depression’proposed in this article will emphasise more the necessity of aggressive treatment of depression in the overall management of stroke,thus to reduce the incidence of stroke and in the meantime,improve the prognosis of ***,it will lead us into a new era of acute stroke intervention.

关键词： diagnosis mortality acute

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Recess-free enhancement-mode AlGaN/GaN RF HEMTs on Si substrate

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Journal of Semiconductors 2024年第6期45卷 81-86页

作者： Tiantian Luan Sen Huang Guanjun Jing Jie Fan Haibo Yin Xinguo Gao Sheng Zhang Ke Wei Yankui Li Qimeng Jiang Xinhua Wang Bin Hou Ling Yang Xiaohua ma Xinyu Liu High-Frequency High-voltage device and Integrated Circuits R&d Center Institute of Microelectronics of Chinese Academy of SciencesBe i-jing 100029China School of integrated Circuits University of Chinese Academy of SciencesBeijing 100049China Faculty of integrated Circuits Xidian UniversityXi’an 710071China

Enhancement-mode(E-mode)GaN-on-Si radio-frequency(RF)high-electron-mobility transistors(HEMTs)were fabri-cated on an ultrathin-barrier(UTB)AlGaN(<6 nm)/GaN heterostructure featuring a naturally depleted 2-d electron g... 详细信息

Enhancement-mode(E-mode)GaN-on-Si radio-frequency(RF)high-electron-mobility transistors(HEMTs)were fabri-cated on an ultrathin-barrier(UTB)AlGaN(depleted 2-d electron gas(2dEG)*** fabricated E-mode HEMTs exhibit a relatively high threshold voltage(vTH)of+1.1 v with good uniformity.A maxi-mum current/power gain cut-off frequency(fT/fmaX)of 31.3/99.6 GHz with a power added efficiency(PAE)of 52.47%and an out-put power density(Pout)of 1.0 W/mm at 3.5 GHz were achieved on the fabricated E-mode HEMTs with 1-μm gate and Au-free ohmic contact.

关键词： AlGaN/GaN heterostructure ultrathin-barrier enhancement-mode radio-frequency power added efficiency silicon substrate

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H_(2)mediated mixed culture microbial electrosynthesis for high titer acetate production from CO_(2)

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Environmental Science and Ecotechnology 2024年第3期19卷 125-131页

作者： Yanhong Bian Aaron Leininger Harold d.may Zhiyong Jason Ren department of Civil and Environmental Engineering Princeton University86 Olden StPrincetonNJ08544United States Andlinger Center for Energy and the Environment Princeton University86 Olden St.PrincetonNJ08544United States

Microbial electrosynthesis(MES)converts CO_(2)into value-added products such as volatile fatty acids(vFAs)with minimal energy use,but low production titer has limited scale-up and *** electron transfer via H_(2)on the MES cathode has shown a higher conversion rate than the direct biofilm-based approach,as it is tunable via cathode potential control and accelerates electrosynthesis from CO_(2).Here we report high acetate titers can be achieved via improved in situ H_(2)supply by nickel foam decorated carbon felt cathode in mixed community MES *** concentration of 12.5 g L^(-1)was observed in 14 days with nickel-carbon cathode at a poised potential of-0.89 v(*** hydrogen electrode,SHE),which was much higher than cathodes using stainless steel(5.2 g L^(-1))or carbon felt alone(1.7 g L^(-1))with the same projected surface area.A higher acetate concentration of 16.0 g L^(-1)in the cathode was achieved over long-term operation for 32 days,but crossover was observed in batch operation,as additional acetate(5.8 g L^(-1))was also found in the abiotic anode *** observed the low Faradaic efficiencies in acetate production,attributed to partial H_(2)utilization for *** selective acetate production with high titer demonstrated in this study shows the H_(2)-mediated electron transfer with common cathode materials carries good promise in MES development.

关键词： Microbial electrosynthesis Indirect electron transfer CO_(2)electrolysis vFAs production

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Anomalies in the short-range local environment and atomic diffusion in single crystalline equiatomic CrMnFeCoNi highentropy alloy

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Nano Research 2024年第6期17卷 5336-5348页

作者： Alevtina Smekhova daniel Gaertner Alexei Kuzmin Ana Guilherme Buzanich Goetz Schuck Ivo Zizak Gerhard Wilde Kirill v.Yusenko Sergiy divinski Helmholtz-Zentrum Berlin für materialien und Energie(HZB) D-12489 BerlinGermany Institute of materials Physics University of MünsterD-48149 MünsterGermany Institute of Solid State Physics University of LatviaLV-1063 RigaLatvia Bundesanstalt für materialforschung und–prüfung(BAM) D-12489 BerlinGermany

Multi-edge extended X-ray absorption fine structure(EXAFS)spectroscopy combined with reverse Monte Carlo(RMC)simulations was used to probe the details of element-specific local coordinations and component-dependent structure relaxations in single crystalline equiatomic CrMnFeCoNi high-entropy alloy as a function of the annealing *** representative states,namely a high-temperature state,created by annealing at 1373 K,and a low-temperature state,produced by long-term annealing at 993 K,were compared in *** features identified in atomic configurations of particular principal components indicate variations in the local environment distortions connected to different degrees of compositional disorder at the chosen representative *** detected changes provide new atomistic insights and correlate with the existence of kinks previously observed in the Arrhenius dependencies of component diffusion rates in the CrMnFeCoNi high-entropy alloy.

关键词： high-entropy alloys diffusion short-range order extended X-ray absorption fine structure(EXAFS) reverse Monte Carlo

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Synergistic Co-doping effect of CNTs and PvP in Na_(4)MnCr(PO_(4))3 cathode as a strategy for improving the electrochemical performance of SIBs

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Chinese Chemical Letters 2024年第2期35卷 539-543页

作者： Ruoyu Chen denys S.Butenko Shilin Li Xinyu Zhang Guangshe Li Igor v.Zatovsky Wei Han College of Physics State Key Laboratory of Inorganic Synthesis and Preparative ChemistryInternational Center of Future ScienceJilin UniversityChangchun 130012China Academy for Advanced Interdisciplinary Studies Southern University of Science and TechnologyShenzhen 518055China State Key Laboratory of Inorganic Synthesis and Preparative Chemistry College of ChemistryJilin UniversityChangchun 130012China F.d.Ovcharenko Institute of Biocolloidal Chemistry NAS UkraineKyiv 03142Ukraine

In order to solve the contradiction between the rapidly growing energy demand and the excessive exploitation of fossil fuels,it is urgent to research and develops more environmentally friendly and efficient energy storage ***,the development of high-performance cathode materials to enhance the energy density of SIB is currently one of the most important topics of scientific *** high-voltage and low-cost cathode material for SIBs,a composite of carbon-coated Na_(4)MnCr(PO_(4))_(3)(NASICON-type),polyvinylpyrrolidone(PvP),and modified carbon nanotubes(CNTs)is prepared by sol-gel and freeze-drying *** to the high conductivity of CNTs,the conductivity of the composite is significantly improved,and its initial capacity is increased to 114 mah/g at 0.5 C and 96 mah/g at 5 C(Mn^(2+)/Mn^(4+)conversion for voltage windows 1.4-4.3 v).Moreover,the multi-electrons transfer of Cr^(3+)/Cr^(4+) and Mn^(2+)/Mn^(4+) can provide a high capacity of 165 mah/g at 0.1 C and 102 mah/g at 5 C in the high voltage window of 1.4-4.6 ***,PvP can effectively inhibit the Jahn-Teller effect caused by Mn ion,making the composite have more excellent high-rate performance and *** addition,GITT,EIS and Cv curves were drawn to better reveal the excellent kinetic properties of Na_(4)MnCr(PO_(4))_(3)@C@PvP@CNT cathode,and the mechanism of its performance improvement is deeply studied and ***,the co-doping of CNTs and PvP is a simple way to high conductivity and fast charging of cathode materials for SIBs.

关键词： Sodium-ion batteries Na_(4)MnCr(PO_(4))_(3) Carbon nanotubes Polyvinylpyrrolidone Synergistic effect

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