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Lithium bis(trifluoromethanesulfonyl)imide blended in polyurethane acrylate photocurable solid polymer electrolytes for lithium-ion batteries

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Journal of Energy Chemistry 2021年第11期30卷 485-496,I0011页

作者： cristian mendes-felipe J.C.Barbosa R.Gonsalves D.Miranda C.M.Costa J.L.Vilas-Vilela S.Lanceros-Mendez BCMaterials Basque Center for MaterialsApplications and NanostructuresUPV/EHU Science Park48940 LeioaSpain Macromolecular Chemistry Group(LABQUIMAC) Department of Physical ChemistryFaculty of Science and TechnologyUniversity of the Basque Country(UPV/EHU)Barrio Sarriena s/nE-48940 LeioaSpain Center of Physics University of MinhoCampus of Gualtar4710-057 BragaPortugal Center of Chemistry University of MinhoCampus of Gualtar4710-057 BragaPortugal Ai–School of Technology IPCABarcelosPortugal Ikerbasque Basque Foundation for Science48009 BilbaoSpain

The increased demand of electronic devices promotes the development of advanced and more efficient energy storage devices, such as batteries. Lithium-ion batteries (LIBs) are the most studied battery systems due to their high performance. Among the different battery components, the separator allows the control of lithium ion diffusion between the electrodes. To overcome some drawbacks of liquid electrolytes, including safety and environmental issues, solid polymer electrolytes (SPEs) are being developed. In this work, a UV photocurable polyurethane acrylate (PUA) resin has been blended with lithium bis(trifluoromethanesulfonyl) imide (LiTFSI) up to 30 wt% LiTFSI content to reach a maximum ionic conductivity of 0.0032 mS/cm at room temperature and 0.09 mS/cm at 100 ℃. Those values allowed applying the developed materials as photocurable SPE in Swagelok type Li/C-LiFePO_(4) half-cells, reaching a battery discharge capacity value of 139 mAh.g^(−1) at C/30 rate. Those results, together with the theoretical studies of the discharge capacity at different C-rates and temperatures for batteries with LiTFSI/PUA SPE demonstrate the suitability of the developed photocurable SPE for LIB applications.

关键词： Solid polymer electrolytes Photocuring Polyurethane acrylate LiTFSI Li-ion batteries

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Design of a Socially Inclusive Climate Risk Transfer Mechanism:A Case Study in La Guajira,Colombia

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International Journal of Disaster Risk Science 2024年第4期15卷 565-578页

作者： cristian Camilo Fernández Lopera JoséManuel mendes Eduardo Jorge Barata Centre for Social Studies Institute for Interdisciplinary ResearchUniversity of Coimbra3000-995 CoimbraPortugal Faculty of Economics Centre for Social StudiesUniversity of Coimbra3000-995 CoimbraPortugal Faculty of Economics CeBERUniversity of Coimbra3004-512 CoimbraPortugal

The primary aim of this study was to develop a model of a socially inclusive climate risk insurance(CRI) mechanism based on the differential risk transfer approach. This study focused on the department of La Guajira, Colombia, as a case *** Guajira is the department in Colombia that, due to its critical disaster risk conditions, presents the adequate configuration for implementing a climate risk transfer mechanism. The article starts by analyzing risk conditions by using secondary data. Based on fieldwork, this research explored the perspectives of the most vulnerable sectors in La Guajira Department on the socioeconomic impacts and needs they experience regarding climate-related hazards, their adaptive measures for risk reduction, and their willingness to adopt CRI. This represents the fundamental input for the formulation of the CRI model. Consequently, this research proposed an operational structure as input for future implementations of the model. The results indicate that national and local disaster risk management public policies align with the sectors' needs and priorities. Strengthening sectoral associations can enhance representation in CRI projects. In-kind indemnization is preferred for women entrepreneurs and the indigenous community. The CRI model includes a risk pool through the family compensation fund of La Guajira as a sectoral agglomerator, with contingent credit and traditional/parametric insurance. The methodology developed in this study can be applied in different contexts worldwide as a guidance for informing national and international climate risk finance initiatives.

关键词： Colombia Disaster risk fnancing Disaster risk management La Guajira Climate risk insurance Socioeconomic vulnerability

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