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Enhanced charge separation by incomplete calcination modified co-doped TiO_(2)nanoparticle for isothiazolinone photocatalytic degradation

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Nano Research 2024年第6期17卷 4834-4843页

作者： Zhiren Guo Xiao Zhang Xinyuan li Chang Cui Zilei Zhang Hansheng li Dongxiang Zhang Jinying li Xiyan Xu Jiatao Zhang School of Chemistry and Chemical Engineering Beijing Institute of TechnologyBeijing 102488China Department of Chemistry MSU-BIT UniversityShenzhen 517182Chin

Photocatalytic oxidation techniques are promising for degradation of the highly ecotoxic and refractory isothiazolinone bactericides in relevant industrial ***,low charge separation and directional transport efficiency under solar light radiation restrain their practical ***,we report a nanostructured photocatalyst doped with Gd and B in TiO_(2)with carbon incorporation and defect formation through incomplete *** specific surface area,grain size,and hydrophilicity of TiO_(2)are improved,which is beneficial for the interfacial reaction between the photocatalyst and *** reduction of the bandgap,the broadening of the photo-absorption range,and the retarded electron-hole recombination promote the photocatalytic performance due to the improved oxygen vacancies based on the electron distribution *** difference in partial density of states(ΔPDOS)between the current catalyst and raw TiO_(2)indicates that the co-doping of Gd and B with incomplete calcination changes the electronic hybridization of conduction band and valence band near the Fermi level,and affects the band gap *** improved charge separation and directional transport efficiency and benefited the formation of main active species,including•OH and O_(2)•−,for the pollutant *** rate of photocatalytic removal of benzisothiazolinone(BIT)by the current photocatalyst reaches 1.25 h^(−1),being 4.31 times that of TiO_(2).The current work offers a constructive approach to the design and synthesis of nanostructured photocatalysts for the photocatalytic degradation of refractory organic pollutants.

关键词： TiO_(2)nanoparticle charge separation oxygen vacancies electron distribution modification photocatalytic degradation

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Neighboring optimal guidance using higher-order dynamics approximation with application to orbital injection problem

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Chinese Journal of Aeronautics 2024年第5期37卷 426-440页

作者： Xinglun CHEN Ran ZHANG Huifeng li School of Astronautics Beihang UniversityBeijing 100191China

Neighboring optimal guidance,a method to obtain a suboptimal guidance law by approximately solving the first-order necessary conditions based on a nominal trajectory,is widely used in the aerospace field due to its high computational efficiency and low resource *** more advanced scenarios,the existing methods still have a problem that the guidance accuracy and optimality will seriously degrade when the actual state largely deviates from the nominal *** is mainly caused by the approximate description of the first-order conditions in terms of total flight time and nonlinear *** address this problem,a higher-order neighboring optimal guidance method is ***,a novel total flight time updating strategy,together with a normalized time scale,is presented that transforms the optimal problem with free total flight time into a more tractable optimal problem with fixed total flight ***,using the vector partial derivative method,a higher-order approximation is adopted,instead of the first-order approximation,to accurately describe the nonlinear dynamical and terminal constraints,thus obtaining a polynomially constrained quadratic optimal ***,to numerically solve the polynomially constrained quadratic optimal problem,a Newton-type iterative algorithm based on the orthogonal decomposition is *** the iterative solution within each guidance period,the corrections to control quantities and total flight time are *** proposed method is applied to a launch vehicle orbital injection problem,and simulation results show that it achieves high accuracy of orbital injection and optimality of performance index.

关键词： Optimal control Neighboring optimal guidance Launch vehicles Orbital injection Higher-order approximation

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Four-channel catalytic micro-reactor based on alumina hollow fiber membrane for efficient catalytic oxidation of co

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Chinese Journal of Chemical Engineering 2024年第7期71卷 140-147页

作者： Baichuan Xu Bin Wang Tao li Key Laboratory of Energy Thermal conversion and control of Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 211100China

The traditional automotive catalytic converter using commercial ceramic honeycomb carriers has many problems such as high back pressure,low engine efficiency,and high usage of precious *** study proposes a four-channel catalytic micro-reactor based on alumina hollow fiber membrane,which uses phase inversion method for structural molding and *** to the advantages of its carrier,it can achieve lower ignition temperature under low noble metal *** Pd/CeO_(2) at a loading rate of 2.3%(mass),the result showed that the reaction ignition temperature is even less than 160℃,which is more than 90℃ lower than the data of commercial ceramic substrates under similar catalyst loading and airspeed *** technology in turn significantly reduces the energy consumption of the *** stability tests were conducted under constant conditions for 1000 h,which proved that this catalytic converter has high catalytic efficiency and stability,providing prospects for the design of innovative catalytic converters in the future.

关键词： Catalytic converter Precious metal catalyst Phase inversion method Hollow fiber membrane co oxidation

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Multi-source information fusion:Progress and future

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Chinese Journal of Aeronautics 2024年第7期37卷 24-58页

作者： Xinde li Fir DUNKIN Jean DEZERT School of Automation Southeast UniversityNanjing 210008China Nanjing Center for Applied Mathematics Nanjing 211135China Key Laboratory of Measurement and control of CSE Ministry of EducationNanjing 210096China Southeast University Shenzhen Research Institute Shenzhen 518063China Information Modeling and Processing Department ONERAPalaiseau 92320France

Multi-Source Information Fusion(MSIF),as a comprehensive interdisciplinary field based on modern information technology,has gained significant research value and extensive application prospects in various domains,attracting high attention and interest from scholars,engineering experts,and practitioners *** achieving fruitful results in both theoretical and applied aspects over the past five decades,there remains a lack of comprehensive and systematic review articles that provide an overview of recent development in *** light of this,this paper aims to assist researchers and individuals interested in gaining a quick understanding of the relevant theoretical techniques and development trends in MSIF,which conducts a statistical analysis of academic reports and related application achievements in the field of MSIF over the past two decades,and provides a brief overview of the relevant theories,methodologies,and application domains,as well as key issues and challenges currently ***,an analysis and outlook on the future development directions of MSIF are presented.

关键词： Multi-sensor system Information fusion Artificial intelligence Pattern recognition Human-machine integration

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Understanding Human and Machine Interaction from Decision Perspective: An Empirical Study Based on the Game of Go

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Journal of Systems Science & complexity 2024年第2期37卷 647-667页

作者： ZHAO Ping li Xuerong WANG Shouyang Academy of Mathematics and Systems Science Chinese Academy of SciencesBeijing 100190China School of Mathematical Sciences University of Chinese Academy of SciencesBeijing 100190China

The authors aim to interpret human and AI interactions from the decision *** authors decompose the interaction analysis into the following main components in the context of interactions:Individual behavior patterns,interaction relationships,and comprehensive *** authors interpret intertemporal decisions from a physical perspective and employ cross-discipline concepts and methodologies to extract the behavior characteristics of players in the empirical case *** the individual behavior patterns,the authors find that human players prefer short-term periods to AI in *** interaction relationship analysis reveals a dynamic relationship between possible short-term co-movement and nearly counter-movement in the long *** authors apply principal component analysis to descriptive indicators and discover a regular decision *** main behavior pattern of players in the game of Go is switching between careful and daring *** differences in the decision hierarchies imply a discrepancy of patience between humans and AI.

关键词： coherence analysis decision hierarchy machine behaviour multitaper spectral analysis

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Vision-based survey method for extraordinary loads on buildings

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Frontiers of Structural and Civil Engineering 2024年第6期18卷 815-831页

作者： Yang li Jun CHEN Pengcheng WANG college of Civil Engineering Tongji UniversityShanghai 200092China China United Engineering co.Ltd. Hangzhou 310052China State Key Laboratory of Disaster Reduction in Civil Engineering Tongji UniversityShanghai 200092China Shanghai Key Laboratory of Engineering Structure Safety Shanghai Research Institute of Building Sciences Co.Ltd.Shanghai 200032China

The statistical modeling of extraordinary loads on buildings has been stagnant for decades due to the laborious and error-prone nature of existing survey methods,such as questionnaires and verbal *** study proposes a new vision-based survey method for collecting extraordinary load data by automatically analyzing surveillance *** this purpose,a crowd head tracking framework is developed that integrates crowd head detection and reidentification models based on convolutional neural networks to obtain head trajectories of the crowd in the survey *** crowd head trajectories are then analyzed to extract crowd quantity and velocities,which are the essential factors for extraordinary *** survey areas with frequent crowd movements during temporary events,the equivalent dynamic load factor can be further estimated using crowd velocity to consider dynamic effects.A crowd quantity investigation experiment and a crowd walking experiment are conducted to validate the proposed survey *** experimental results prove that the proposed survey method is effective and accurate in collecting load data and reasonable in considering dynamic effects during extraordinary *** proposed survey method is easy to deploy and has the potential to collect substantial and reliable extraordinary load data for determining design load on buildings.

关键词： load survey extraordinary load live load object detection multiple-object tracking

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Laboratory Evaluation of Performance Recovery of Aged SBS-modified Asphalt Using Regenerants with Different Base Oil components

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China Petroleum Processing & Petrochemical Technology 2024年第2期26卷 98-107页

作者： li Hongzhen li Shengbin Feng Zhuangzhuang Jiang Mengmeng li Ning Dong Fuqiang Shandong Yimeng Traffic Development Group co. Ltd.Zibo 276004China college of Civil and Transportation Engineering Hohai UniversityNanjing 210098China

In this study,the regenerative effects of different regenerants on aged SBS-modified asphalt from different perspectives were investigated,including their conventional properties,viscoelastic behavior,creep-related properties,and *** oils composed of different proportions of aromatic and saturated hydrocarbons as well as the styrene-butadiene-styrene(SBS)restorer were used to prepare the *** results showed that the components of the base oil of the regenerant played a crucial role in determining the characteristics and performance of the recycled SBSmodified *** containing a high proportion of aromatics dissolved the hard segment in the SBS restorer,thereby delaying the effect of a reduction in the regenerants on the performance of the aged asphalts at a high *** containing a high proportion of saturates dissolved the soft segment in the SBS restorer to enhance the lowtemperature performance of the recycled *** addition,the stress sensitivity of the recycled asphalts increased with the fraction of aromatics in the *** the aromatic content of the base oil components of the regenerants increased and their saturate content decreased,the state of dispersion of the SBS phase in the recycled SBS-modified asphalts *** optimal content of aromatics in the base oil of the regenerants should be set in the range of 33%to 47%to ensure the adequate performance of the recycled asphalts and a high efficiency of the SBS restorer.

关键词： aged SBS-modified asphalt regeneration mechanisms base oil rheological properties morphology

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Particles attrition of binary mixtures in the coal-fueled chemical looping system based on fluidized bed

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Particuology 2024年第3期86卷 281-290页

作者： Heyu li Zhe Sun Yan Cao Guangzhou Institute of Energy conversion Chinese Academy of SciencesGuangzhou 510640China University of Chinese Academy of Sciences Bejing 100049China CAS Key Laboratory of Renewable Energy Guangzhou 510640China Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development Guangzhou 510640China college of Chemistry and Chemical Engineering Anhui UniversityHefei230601China

In this work,a reactive air jet attrition device with auto-recording and collection of elutriated fines was *** established insights into the physiochemical interaction and further correlated attrition behaviors between char and oxygen carriers under various operation *** attrition rate increased by over 110% upon the introduced co_(2),which brought in the significant effect of thermo-chemical stress,similarly in effects of the increased char addition ratio and the decreased sizes of char or hematite in different *** the char-hematite co-attrition process,the elutriated carbon loss of char with poor mechanical strength was found to be over 10%,while the reactive iron loss of hematite was found to be 6.3%,and was enriched in elutriated *** reaction-derived thermochemical stress and the collision-derived mechanical stress jointly controls the particle attrition during the cyclic transformation of oxygen carrier particles in coal-fueled chemical looping fluidization,especially sig-nificant in its reduction stage.

关键词： Attrition Binary species Chemical looping Oxygen carrier co_(2)capture

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Improvements in properties of NdFeB magnets obtained via magnetron sputtering and thermal diffusion

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Journal of Rare Earths 2024年第9期42卷 1710-1716,I0003页

作者： Jin Tang Weichao Huang Dan li School of Electronic Engineering Guangxi University of Science and TechnologyLiuzhou545006China China Rare Earth(Guangxi)Jinyuan Rare Earth New Materials co. Ltd.Hezhou542603China China Rare Earth Group co. Ltd.Ganzhou341000China Center of Experimental Teaching for common courses Panzhihua UniversityPanzhihua617000China

The grain boundary diffusion process(GBDP) of Dy and DyAl on sintered NdFeB magnets was conducted via magnetron-sputtering deposition of Dy and DyAl films to enhance coercivity(H_(cj)),The magnetic properties,microstructure and anti-corrosion properties of Dy-surface-alloying NdFeB magnets obtained via magnetron sputtering and thermal diffusion were *** H_(cj) of the Dy_(95)Al_(5)-NdFeB magnet increases by 32.68%,while the remanence declines ***,X-ray diffraction and microstructural analysis confirm the formation of Dy-rich shells,the higher-magnetic-anisotropy field of hard(Nd_(x)Dy_(1-x))2(FeAl)_(14)B magnetic phases and an optimised grain boundary structu re,contributing to the H_(cj)enhancement of the *** elemental distribution and diffusion mechanism of the magnets are also ***,the corrosion resistance of the Dy_(95)Al_(5)-NdFeB magnet is substantially improved by enhancing the electrochemical stability and optimising the distribution and morphology of the intergranular *** findings of this study are of substantial importance in the development of low-heavy rare-earth sintered NdFeB magnets.

关键词： Magnetron sputtering NdFeB Rare earths Microstructure Magnetic property corrosion resistance

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Untethered Micro/Nanorobots for Remote Sensing:Toward Intelligent Platform

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Nano-Micro Letters 2024年第2期16卷 450-483页

作者： Qianqian Wang Shihao Yang li Zhang Jiangsu Key Laboratory for Design and Manufacture of Micro‑Nano Biomedical Instruments School of Mechanical EngineeringSoutheast UniversityNanjing 211189People’s Republic of China Department of Mechanical and Automation Engineering The Chinese University of Hong KongShatinHong Kong 999077People’s Republic of China Chow Yuk Ho Technology Centre for Innovative Medicine The Chinese University of Hong KongShatinHong Kong 999077People’s Republic of China T Stone Robotics Institute The Chinese University of Hong KongShatinHong Kong 999077People’s Republic of China Department of Surgery The Chinese University of Hong KongShatinHong Kong 999077People’s Republic of China

Untethered micro/nanorobots that can wirelessly control their motion and deformation state have gained enormous interest in remote sensing applications due to their unique motion characteristics in various media and diverse *** are developing micro/nanorobots as innovative tools to improve sensing performance and miniaturize sensing systems,enabling in situ detection of substances that traditional sensing methods struggle to *** the past decade of development,significant research progress has been made in designing sensing strategies based on micro/nanorobots,employing various coordinated control and sensing *** review summarizes the latest developments on micro/nanorobots for remote sensing applications by utilizing the self-generated signals of the robots,robot behavior,microrobotic manipulation,and robot-environment *** recent studies and relevant applications in remote sensing,we also discuss the challenges and future perspectives facing micro/nanorobots-based intelligent sensing platforms to achieve sensing in complex environments,translating lab research achievements into widespread real applications.

关键词： Micro/nanorobot Remote sensing Wireless control Self-propulsion Actuation at small scales

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