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Ultrathin organic solvent nanofiltration membrane with polydopamine-HKUST-1 interlayer for organic solvent separation

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Journal of Environmental Sciences 2024年第7期141卷 182-193页

作者： Haike li Xindong li Guozai Ouyang lijinhong Huang Lang li Wenhao li Wanfu Huang Duokun li Ganzhou Key Laboratory of Basin Pollution Simulation and control Jiangxi University of Science and TechnologyGanzhou 341000China Innovation Center for Water Quality Security Technology at Ganjiang River Basin Jiangxi University of Science and TechnologyGanzhou 341000China School of Architecture and Design Jiangxi University of Science and TechnologyGanzhou 341000China WA School of Mines:Minerals Energy and Chemical EngineeringCurtin UniversityWA 6845Australia School of Materials Science and Engineering Tiangong UniversityTianjin 300387China

Polydopamine(PDA)and metal-organic skeleton HKUST-1 were co-deposited on the base membrane of hexamethylenediamine(HDA)-crosslinked polyetherimide(PEI)ultrafiltration membrane as the interlayer,and high-throughput organic solvent nanofiltration membrane(OSN)was prepared by interfacial polymerization and solvent activation *** polyamide(PA)layer surface roughness from 28.4 nm in PA/PEI to 78.3 nm in PA/PDA-HKUST-10.6/PEI membrane,reduced the thickness of the separation layer from 79 to 14 nm,and significantly improved the hydrophilic,thermal and mechanical *** flux of the PA/PDA-HKUST-10.6/PEI membrane in a 0.1 g/L congo Red(CR)ethanol solution at 0.6 MPa test pressure reached 21.8 L/(m^(2)·hr)and the rejection of CR was 92.8%.Solvent adsorption test,N,N-dimethylformamide(DMF)immersion experiment,and long-term operation test in ethanol showed that the membranes had high solvent *** solvent flux test demonstrated that,under the test pressure of 0.6 MPa,the flux of different solvents ranked as follows:methanol(56.9 L/(m^(2)·hr))>DMF(39.6 L/(m^(2)·hr))>ethanol(31.2 L/(m^(2)·hr))>IPA(4.5 L/(m^(2)·hr))>N-hexane(1.9 L/(m^(2)·hr)).The ability of the membranes to retain dyes in IPA/water dyes solution was also *** flux of the membrane was 30.4 L/(m^(2)·hr)and the rejection of CR was 91.6%when the IPA concentration reached 50%.This OSN membrane-making strategy is economical,environment-friendly and efficient,and has a great application prospect in organic solvent separation systems.

关键词： Interfacial polymerization Organic solvent nanofiltration Interlayer Metal-organic frameworks Polydopamine

Diffusionmodels for time-series applications: a survey

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Frontiers of Information Technology & Electronic Engineering 2024年第1期25卷 19-41页

作者： Lequan liN Zhengkun li Ruikun li Xuliang li Junbin GAO Discipline of Business Analytics The University of Sydney Business SchoolCamperdownNSW 2006Australia Postdoctoral Programme of Zhongtai Securities co. Ltd.Jinan 250000China

Diffusion models, a family of generative models based on deep learning, have become increasinglyprominent in cutting-edge machine learning research. With distinguished performance in generating samples thatresemble the observed data, diffusion models are widely used in image, video, and text synthesis nowadays. Inrecent years, the concept of diffusion has been extended to time-series applications, and many powerful models havebeen developed. considering the deficiency of a methodical summary and discourse on these models, we providethis survey as an elementary resource for new researchers in this area and to provide inspiration to motivate futureresearch. For better understanding, we include an introduction about the basics of diffusion models. Except forthis, we primarily focus on diffusion-based methods for time-series forecasting, imputation, and generation, andpresent them, separately, in three individual sections. We also compare different methods for the same applicationand highlight their connections if applicable. Finally, we conclude with the common limitation of diffusion-basedmethods and highlight potential future research directions.

关键词： Diffusion models Time-series forecasting Time-series imputation Denoising diffusion probabilistic models Score-based generative models Stochastic differential equations

Multi-Physics coupled Acoustic-Mechanics Analysis and Synergetic Optimization for a Twin-Fluid Atomization Nozzle

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Chinese Journal of Mechanical Engineering 2024年第3期37卷 204-223页

作者： Wenying li Yanying li Yingjie Lu Jinhuan Xu Bo Chen li Zhang Yanbiao li college of Mechanical Engineering Zhejiang University of TechnologyHangzhou 310023China State Key Laboratory of Fluid Power and Mechatronic Systems Zhejiang UniversityHangzhou 310027China School of Materials Science and Engineering Northwestern Polytechnical UniversityXian 710072China Guizhou Anda Aviation Forging co. Ltd.Anshun 561005China

Fine particulate matter produced during the rapid industrialization over the past decades can cause significant harm to human ***-fluid atomization technology is an effective means of controlling fine particulate matter *** this paper,the influences of the main parameters on the droplet size,effective atomization range and sound pressure level(SPL)of a twin-fluid nozzle(TFN)are investigated,and in order to improve the atomization performance,a multi-objective synergetic optimization algorithm is presented.A multi-physics coupled acousticmechanics model based on the discrete phase model(DPM),large eddy simulation(LES)model,and Ffowcs Williams-Hawkings(FW-H)model is established,and the numerical simulation results of the multi-physics coupled acoustic-mechanics method are verified via experimental *** on the analysis of the multi-physics coupled acoustic-mechanics numerical simulation results,the effects of the water flow on the characteristics of the atomization flow distribution were obtained.A multi-physics coupled acoustic-mechanics numerical simulation result was employed to establish an orthogonal test database,and a multi-objective synergetic optimization algorithm was adopted to optimize the key parameters of the *** optimal parameters are as follows:A gas flow of 0.94 m^(3)/h,water flow of 0.0237 m^(3)/h,orifice diameter of the self-excited vibrating cavity(SVC)of 1.19 mm,SVC orifice depth of 0.53 mm,distance between SVC and the outlet of nozzle of 5.11 mm,and a nozzle outlet diameter of 3.15 *** droplet particle size in the atomization flow field was significantly reduced,the spray distance improved by 71.56%,and the SPL data at each corresponding measurement point decreased by an average of 38.96%.The conclusions of this study offer a references for future TFN research.

关键词： Twin-fluid nozzle BP neural network Multi-objective optimization Multi-physics coupled Acousticmechanics analysis Genetic algorithm

Predicting Turbidite Channel in Deep-Water Canyon Based on Grey Relational Analysis-Support VectorMachineModel:A Case Study of the lingshui Depression in Qiongdongnan Basin,South China Sea

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Energy Engineering 2024年第9期121卷 2435-2447页

作者： Haichen li Jianghai li li li Zhandong li School of Earth and Space Sciences Peking UniversityBeijing100871China Key Laboratory of Orogenic Belts and Crustal Evolution Peking UniversityBeijing100871China Geotechnical Physical and Mechanical Properties Laboratory Langfang Normal UniversityLangfang065000China Heilongjiang Northeast Petroleum University Science Park Development co. Ltd.Daqing163318China college of Petroleum Engineering Northeast Petroleum UniversityDaqing163318China

The turbidite channel of South China Sea has been highly *** by the complex fault and the rapid phase change of lithofacies,predicting the channel through conventional seismic attributes is not accurate *** response to this disadvantage,this study used a method combining grey relational analysis(GRA)and support vectormachine(SVM)and established a set of prediction technical procedures suitable for reservoirs with complex geological *** the case study of the Huangliu Formation in Qiongdongnan Basin,South China Sea,this study first dimensionalized the conventional seismic attributes of Gas Layer Group I and then used the GRA method to obtain the main relational factors.A higher relational degree indicates a higher probability of responding to the attributes of the turbidite *** study then accumulated the optimized attributes with the highest relational factors to obtain a first-order accumulated sequence,which was used as the input training sample of the SVM model,thus successfully constructing the SVM turbidite channel *** results prove that the GRA-SVMmethod has a high drilling coincidence *** the core and logging data and taking full use of the advantages of seismic inversion in predicting the sand boundary of water channels,this study divides the sedimentary microfacies of the Huangliu Formation in the lingshui 17-2 Gas *** comprehensive study has shown that the GRA-SVM method has high accuracy for predicting turbidite channels and can be used as a superior turbidite channel prediction method under complex geological conditions.

关键词： Support vector machine channel Huangliu Formation Qiongdongnan Basin

Humic acid-mediated transport of a typical soil passivation remediation product(chloropyromorphite)in saturated porous media

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Journal of Environmental Sciences 2024年第7期141卷 51-62页

作者： Xinying li Mengjia Zhang Siyuan li Wei Wei School of Environment Jiangsu Engineering Lab of Water and Soil Eco-remediationJiangsu Province Engineering Research Center of Environmental Risk Prevention and Emergency Response TechnologyNanjing Normal UniversityNanjing 210023China Jiangsu Center for collaborative Innovation in Geographical Information Resource Development and Application Nanjing 210023China

conversion of labile Pb species into chloropyromorphite(CPY)using phosphorus-bearing amendments was considered to be an ideal strategy in soil passivation ***,the fate and transport of CPY in the soil are poorly *** study aims to fill the knowledge gap by evaluating the fate and transport of CPY under environmentally relevant conditions of humic acid(HA),pH,electrolyte concentration,and species through the saturated sandy *** showed that bare CPY colloids are basically immobile in sandy porous media while the co-existence of HA made the transport of CPY improved by30%-93.5%.Facilitated transport of CPY was attributed to the increased stability of CPY and the repulsive interaction between CPY particles and sands due to HA *** mobility of CPY was also increased with increasing pH from 5.0 to *** the pH was 9 with a10 mmol/L NaCl background solution,the stronger energy barrier between CPY and sand led to enhanced transport *** divalent Ca^(2+)had a more dramatic effect than monovalent Na^(+)on the aggregation and sedimentation of CPY colloids due to its effectivescreening of the surface charge of CPY and bridging interaction with CPY ***-LandauVerwey-Overbeek theory and attachment efficiency calculation indicated that high energy barriers were responsible for the high mobility of CPY colloids,while the retention of CPY in sands was mainly caused by secondary energy minimum and physically *** findings of this work can help to evaluate the fate of soil passivation remediation products in natural water and soil.

关键词： Chloropyromorphite DLVO theory Stability Saturated porous medium Transport

Malware Evasion Attacks Against IoT and Other Devices: An Empirical Study

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Tsinghua Science and Technology 2024年第1期29卷 127-142页

作者： Yan Xu Deqiang li Qianmu li Shouhuai Xu School of computer Science and Engineering Nanjing University of Science and TechnologyNanjing 210094China School of computer Science Nanjing University of Posts and TelecommunicationsNanjing 210023China Department of computer Science University of Colorado Colorado SpringsColorado SpringsCO 80918USA

The Internet of Things(loT)has grown rapidly due to artificial intelligence driven edge *** enabling many new functions,edge computing devices expand the vulnerability surface and have become the target of malware ***,attackers have used advanced techniques to evade defenses by transforming their malware into functionality-preserving *** systematically analyze such evasion attacks and conduct a large-scale empirical study in this paper to evaluate their impact on *** specifically,we focus on two forms of evasion attacks:obfuscation and adversarial *** the best of our knowledge,this paper is the first to investigate and contrast the two families of evasion attacks *** apply 10 obfuscation attacks and 9 adversarial attacks to 2870 malware *** obtained findings are as follows.(1)commercial Off-The-Shelf(coTS)malware detectors are vulnerable to evasion attacks.(2)Adversarial attacks affect coTS malware detectors slightly more effectively than obfuscated malware examples.(3)code similarity detection approaches can be affected by obfuscated examples and are barely affected by adversarial attacks.(4)These attacks can preserve the functionality of original malware examples.

关键词： Android malware obfuscation adversarial examples

The origins of catalytic selectivity for the electrochemical conversion of carbon dioxide to methanol

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Nano Research 2024年第1期17卷 5-17页

作者： Tian Wang Yating Wang Yuhang li Chunzhong li Key Laboratory for Ultrafine Materials of Ministry of Education Shanghai Engineering Research Center of Hierarchical NanomaterialsFrontiers Science Center for Materiobiology and Dynamic ChemistrySchool of Materials Science and EngineeringEast China University of Science&TechnologyShanghai 200237China School of Chemical Engineering East China University of Science&TechnologyShanghai 200237China

The electrocatalytic conversion of carbon dioxide(co_(2))into useful fuels and chemical feedstocks is an emerging route to alleviate global warming and reduce reliance on fossil ***(CH_(3)OH),as one of the most significant and widely used liquid fuels that can be generated by co_(2)reduction,is essential in the chemical *** this minireview,we unravel the origins of the selective formation of CH_(3)OH via co_(2)reduction,including catalyst composition designs,local structure modulations,and electrolyte/catalyst interface ***,the remaining challenges and perspectives for the co_(2)-to-CH_(3)OH reduction are proposed.

关键词： methanol carbon dioxide(co_(2))reduction reaction electrochemistry electrocatalyst catalyst-electrolyte interface

Dendroclimatological study of Sabina saltuaria and Abies faxoniana in the mixed forests of the Qionglai Mountains,eastern Tibetan Plateau

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Journal of Forestry Research 2024年第1期35卷 72-82页

作者： Teng li Jianfeng Peng Tsun Fung Au Jingru li Jinbao li Yue Zhang School of Geography and Remote Sensing Guangzhou UniversityGuangzhou 510006People’s Republic of China college of Geography and Environmental Science Henan UniversityKaifeng 475004People’s Republic of China Institute for Global Change Biology School for Environment and SustainabilityUniversity of MichiganAnn ArborMIUSA Department of Ecology and Evolutionary Biology University of MichiganAnn ArborMIUSA Department of Geography University of Hong KongHong Kong SARPeople’s Republic of China HKU Shenzhen Institute of Research and Innovation Shenzhen 518057People’s Republic of China

Tree-ring chronologies were developed for Sabina saltuaria and Abies faxoniana in mixed forests in the Qionglai Mountains of the eastern Tibetan ***-growth relationship analysis indicated that the two co-exist-ing species reponded similarly to climate factors,although *** was more sensitive than *** strong-est correlation was between *** chronology and regional mean temperatures from June to *** on this relationship,a regional mean temperature from June to November for the period 1605-2016 was *** explained 37.3%of the temperature variance during th period *** major warm periods and five major cold periods were *** analysis detected significant interannual and multi-decadal *** also revealed the influence of the Atlantic Multi-decadal Oscillation,confirming its importance on climate change on the eastern Tibetan Plateau.

关键词： Tree-ring analysis Mixed forests Dendroclimatology Qionglai Mountains

Screening the optimal co_(x)/CeO_(2)(110)(x=1–6)catalyst for methane activation in coalbed gas

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International Journal of coal Science & Technology 2024年第3期11卷 256-271页

作者： li’nan Huang Danyang li Lei Jiang Zhiqiang li Dong Tian Kongzhai li Engineering Research Center of Metallurgical Energy conservation and Emission Reduction Ministry of EducationKunming University of Science and TechnologyKunming650093China Faculty of Metallurgical and Energy Engineering Kunming University of Science and TechnologyKunming650093China State Key Laboratory of complex Nonferrous Metal Resources Clean Utilization Kunming University of Science and TechnologyKunming650093China

The challenges posed by energy and environmental issues have forced mankind to explore and utilize unconventional energy *** is imperative to convert the abundant coalbed gas(CBG)into high value-added products,i.e.,selective and efficient conversion of methane from *** activation,known as the“holy grail”,poses a challenge to the design and development of *** structural complexity of the active metal on the carrier is of particular *** this work,we have studied the nucleation growth of small co clusters(up to co_(6))on the surface of CeO_(2)(110)using density functional theory,from which a stable loaded co/CeO_(2)(110)structure was selected to investigate the methane activation *** the relatively small size of the selected co clusters,the obtained co_(x)/CeO_(2)(110)exhibits interesting *** optimized co_(5)/CeO_(2)(110)structure was selected as the optimal structure to study the activation mechanism of methane due to its competitive electronic structure,adsorption energy and binding *** energy barriers for the stepwise dissociation of methane to form CH3^(*),CH2^(*),CH^(*),and C^(*)radical fragments are 0.44,0.55,0.31,and 1.20 eV,respectively,indicating that CH^(*)dissociative dehydrogenation is the rate-determining step for the system under investigation *** fundamental study of metal-support interactions based on co growth on the CeO_(2)(110)surface contributes to the understanding of the essence of co/CeO_(2) catalysts with promising catalytic *** provides theoretical guidance for better designing the optimal co/CeO_(2) catalyst for tailored catalytic reactions.

关键词： co cluster growth Ce-based catalysts Methane activation DFT