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Synthesis and fluorescence properties of CdSe/CdS nanoparticles in aqueous media

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Science China Chemistry 2010年第5期53卷 1054-1058页

作者： Han, DongMei song, chunfeng Guo, GuangSheng Li, XiaoYu School of Materials Science and Engineering Beijing University of Chemical Technology Beijing 100029 China State Key Laboratory of Chemical Resource Engineering Beijing University of Chemical Technology Beijing 100029 China Key Laboratory for Nanomaterials Ministry of Education Beijing University of Chemical Technology Beijing 100029 China

On the basis of unique structural characteristics of α-cyclodextrin,α-cyclodextrin modified CdSe/CdS nanoparticles have been successfully synthesized in aqueous *** of AFM,TEM,EDS,FTIR,UV-vis absorbance and photoluminescence spectra were used to characterize the morphology,composition and optical characteristics of the synthesized *** results showed that the as-synthesized nanoparticles were elliptical and composed of several small *** average length and diameter were about 20 nm and 15 ***/CdS nanoparticles had single well-crystallized hexagonal *** with a shell of CdS on the surface,α-CD/CdSe-CdS nanoparticles exhibited a red shift in the absorption spectrum,intensity growth in the emission spectrum and a substantial increase in Quantum *** size distribution could be adjusted by precursor ratios in the presence of α-cyclodextrins.

关键词： CdSe/CdS α-cyclodextrins aqueous solution synthesis fluorescence properties

Recent advances in ionic liquids-based hybrid processes for CO_(2) capture and utilization

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Journal of Environmental Sciences 2021年第1期33卷 281-295页

作者： Shaohan Lian chunfeng song Qingling Liu Erhong Duan Hongwei Ren Yutaka Kitamura Tianjin Key Laboratory of Indoor Air Enuironmental Quality Control School of Enuironmental Science and EngineeringTianjin UniversityTianjin 300072China Pollution Prevention Biotechnology Laboratory of Hebei Province School of Environmental Science and EngineeringHebei University of Science and TechnologyshijizhuangHebei 050018China Graduate School of L.ife and Environmental Sciences University of Tsukuba1-1-1TennodaiTsukubalbaraki 305-8572Japan

CO_(2) capture and utilization(CCU)is an effective strategy to mitigate global ***,adsorption and membranes are methods used for CO_(2) separation and capture,and various catalytic pathways have also been developed for CO_(2) *** widely researched and used in industry,these processes are energy-intensive and this challenge needs to be *** realize further optimization,novel materials and processes are continuously being *** generation materials such as ionic liquids(ILs)have shown promising potential for cost-effective CO_(2) capture and *** study reviews the current status of ILs-based solvents,adsorbents,membranes,catalysts and their hybrid processes for CO_(2) capture and *** special properties of ILs are integrated into new materials through hybridization,which significantly improves the performance in the process of CCU.

关键词： CO_(2) Hybrid Ionic liquids Absorption Adsorption Membrane Catalysis

Food processing wastewater purification by microalgae cultivation associated with high value-added compounds production——A review

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Chinese Journal of Chemical Engineering 2019年第12期27卷 2845-2856页

作者： Shuhong Li Shuang Zhao Siliang Yan Yiting Qiu chunfeng song Yang Li Yutaka Kitamura State Key Laboratory of Food Nutrition and Safety Key Laboratory of Food Nutrition and SafetyMinistry of EducationCollege of Food Engineering and BiotechnologyTianjinUniversity of Science&TechnologyTianjin 300457China Tianjin Key Laboratory of Indoor Air Environmental Quality Control School of Environmental Science and EngineeringTianjin University135 Yaguan RoadHaihe Education ParkTianjin 300350China Tianjin Institute of Industrial Biotechnology Chinese Academy of SciencesTianjin 300308China Graduate School of Life and Environmental Sciences University of Tsukuba1-1-1TennodaiTsukubaIbaraki 305-8572Japan

Microalgae have been considered as an efficient microorganism for wastewater treatment with simultaneously bioenergy and high value-added compounds ***,the high energy cost associated with complicated biorefinery(*** cultivation,harvesting,drying,extraction,conversion,and purification)is a critical challenge that inhibits its large-scale *** different nutrition(***,nitrogen and phosphorous)sources,food processing wastewater is a relative safe and suitable one for microalgae cultivation due to its high organic content and low *** this review,the characteristic of different food wastewater is summarized and *** potential routes of value-added products(***,pigment,polysaccharide,and amino acid)production along with wastewater purification are *** existing challenges(*** cost,efficiency and mechanism)of microalgal-based wastewater treatment are also *** prospective of microalgae-based food processing wastewater treatment strategies(such as microalgae-bacteria consortium,poly-generation of bioenergy and value-added products)is *** can be observed that food wastewater treatment by microalgae could be a promising strategy to commercially realize waste source reduce,conversion and reutilization.

关键词： Food wastewater Microalgae Value-added produce Biofuel Polysaccharide Protein

L-3-n-butylphthalide protects against vascular dementia via activation of the Akt kinase pathway

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Neural Regeneration Research 2013年第19期8卷 1733-1742页

作者： Yaping Huai Yanhong Dong Jing Xu Nan Meng chunfeng song Wenbin Li Peiyuan Lv Department of Neurology Hebei Medical University Department of Neurology Hebei General Hospital Electron Microscope Center Hebei Medical University Department of Pathophysiology Hebei Medical University

As a neuroprotective drug for the treatment of ischemic stroke, 3-n-butylphthalide, a celery seed ex- tract, has been approved by the State Food and Drug Administration of China as a clinical therapeutic drug for ischemic stroke patients. L-3-n-butylphthalide possesses significant efficacy in the treatment of acute ischemic stroke. The activated Akt kinase pathway can prevent the death of nerve cells and exhibit neuroprotective effects in the brain after stroke. This study provides the hypothesis that I-3-n- butylphthalide has a certain therapeutic effect on vascular dementia, and its mechanism depends on the activation of the Akt kinase pathway. A vascular dementia mouse model was established by cere- bral repetitive ischemia/reperfusion, and intragastrically administered I-3-n-butylphthalide daily for 28 consecutive days after ischemia/repedusion, or 7 consecutive days before ischemia/reperfusion. The Morris water maze test showed significant impairment of spatial learning and memory at 4 weeks after operation, but intragastric administration of I-3-n-butylphthalide, especially pretreatment with I-3-n- butylphthalide, significantly reversed these changes. Thionine staining and western blot analylsis showed that preventive and therapeutic application of I-3-n-butylphthalide can reduce loss of pyrami- dal neurons in the hippocampal CA1 region and alleviate nerve damage in mice with vascular demen- tia. In addition, phosphorylated Akt expression in hippocampal tissue increased significantly after I-3-n- butylphthalide treatment. Experimental findings demonstrate that I-3-n-butylphthalide has preventive and therapeutic effects on vascular dementia, and its mechanism may be mediated by upregulation of phosphorylated Akt in the hippocampus.

关键词： neural regeneration brain injury ischemia/reperfusion Akt phosphorylated Akt Morris water maze cog-nitive function 3-n-butylphthalide hippocampus learning memory dementia grants-supported paper neuroregeneration

Potential applications of porous organic polymers as adsorbent for the adsorption of volatile organic compounds

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Journal of Environmental Sciences 2021年第7期33卷 184-203页

作者： Shuangchun Lu Qingling Liu Rui Han Miao Guo Jiaqi Shi chunfeng song Na Ji Xuebin Lu Degang Ma Tianjin Key Lab of Indoor Air Environmental Quality Control School of Environmental Science and TechnologyTianjin UniversityTianjin 300350China State Key Laboratory of Engines Tianjin UniversityTianjin 300350China

Volatile organic compounds(VOCs)with high toxicity and carcinogenicity are emitted from kinds of industries,which endanger human health and the *** is a promising method for the treatment of VOCs due to its low cost and high *** recent years,activated carbons,zeolites,and mesoporous materials are widely used to remove VOCs because of their high specific surface area and abundant ***,the hydrophilic nature and low desorption rate of those materials limit their commercial ***,the adsorption capacities of VOCs still need to be *** organic polymers(POPs)with extremely high porosity,structural diversity,and hydrophobic have been considered as one of the most promising candidates for VOCs *** review generalized the superiority of POPs for VOCs adsorption compared to other porous materials and summarized the studies of VOCs adsorption on different types of ***,the mechanism of competitive adsorption between water and VOCs on the POPs was ***,a concise outlook for utilizing POPs for VOCs adsorption was discussed,noting areas in which further work is needed to develop the next-generation POPs for practical applications.

关键词： Porous organic polymers Volatile organic compounds Adsorption superiority Competitive adsorption

Research on critical technology of micro/nano bioparticles manipulation platform based on light-induced dielectrophoresis

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Science China(Technological Sciences) 2009年第10期52卷 2831-2839页

作者： NI ZhongHua YI Hong ZHU ShuCun song chunfeng Jiangsu Key Laboratory for Design and Manufacture of Micro-Nano Biomedical Instruments School of Mechanical EngineeringSoutheast UniversityNanjing 210096China

On the basis of the research on the status and problems of micro/nano bio-particles manipulation using dielectrophoresis, the theoretical basis and the model simulation of micro/nano bio-particles manipu-lation using light-induced dielectrophoresis were discussed. The space distribution of electric field and dielectrophoresis forces in different heights were also obtained. On this basis, the core component of the micro manipulation system, that is, photoconductive layer of the chip, was completed in the mate-rial selection, fabricating process and performance analysis testing. Then the voltage drop of the sus-pension and the effective voltage frequency spectrum were obtained. Finally, by combining the machine vision detection with real-time tracking system, the micro/nano bio-particles manipulation platform based on the light-induced dielectrophoreisis was established, and then the manipulations for micro/nano bio-particles, such as quick collection, transport, separation, were implemented. This provided a basis for rapid, accurate, and low-cost detection of serious diseases based on the micro-fluidic biochip and early diagnosis.

关键词： light-induced dielectrophoresis micro-fluidic biochip dielectric polarization mechanism separation chip

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以微藻固碳减轻碳排放及其强化策略

能源环境保护 2024年第3期38卷 35-42页

作者：王艺陈丹青毛炜炜李鹏程宋春风天津大学环境科学与工程学院天津300350

广泛使用化石燃料导致二氧化碳等温室气体排放量持续攀升,给全球气候变化和生态系统带来了深刻而不可逆的影响,这不仅引发了环境问题,更对地球的气候稳定和生物多样性构成了严重威胁。在众多的碳减排方法中,CCUS技术是实现二氧化碳长期... 详细信息

广泛使用化石燃料导致二氧化碳等温室气体排放量持续攀升,给全球气候变化和生态系统带来了深刻而不可逆的影响,这不仅引发了环境问题,更对地球的气候稳定和生物多样性构成了严重威胁。在众多的碳减排方法中,CCUS技术是实现二氧化碳长期减排的重要手段,其中碳捕集是核心环节,包括从能源利用、工业生产和大气中分离二氧化碳的过程。在这一领域中,着重介绍了微藻固碳技术的重要性和有效性。与此同时进一步指出,通过调节微藻的生长条件,如光照、温度、pH、营养元素和二氧化碳浓度,可以显著提高微藻的固碳能力。目前,通过随机诱变、适应性实验室进化和基因工程等策略,筛选生长速度快、耐受性强、二氧化碳固定效率高、生物量大的微藻品种。这不仅有助于推进碳达峰和碳中和目标,也将为实现能源的清洁、绿色、低碳和高效利用提供坚实的基础,从而支持全面实施可持续发展战略。通过这种方式,微藻固碳技术有望在应对全球变暖和促进环境可持续发展中发挥作用。

关键词：微藻全球变暖碳中和光合作用 CO_(2)减排

MgFe hydrotalcites-derived layered structure iron molybdenum sulfide catalysts for eugenol hydrodeoxygenation to produce phenolic chemicals

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Journal of Energy Chemistry 2018年第2期27卷 600-610页

作者： Xinyong Diao Na Ji Mingyuan Zheng Qingling Liu chunfeng song Yibo Huang Qing Zhang Alazar Alemayehu Luoyun Zhang Changhai Liang Laboratory of Advanced Materials and Catalytic Engineering Dalian University of Technology School of Environmental Science and Engineering Key Laboratory of Biomass-Derived Gas and Oil for Chinese Petrochemical IndustryTianjin University Dalian Institute of Chemical Physics Chinese Academy of Sciences

Hydrodeoxygenation（HDO） is an effective alternative to produce value-added chemicals and liquid fuels by removing oxygen from lignin-derived compounds. Sulfide catalysts have been proved to have good activity for the HDO and particularly high selectivity to phenolic products. Herein, we presented a novel way to prepare the layered structure sulfide catalysts（MgFeMo-S） derived from MgFe hydrotalcites via the intercalation of Mo in consideration of the memory effect of the calcined hydrotalcite. By varying the Mg/Fe mole ratio, a series of MgFeMo-S catalysts were successfully prepared and characterized by nitrogen adsorption/desorption isotherms, X-ray diffraction（XRD）, transmission electron microscopy（TEM）,and inductively coupled plasma optical emission spectrometer（ICP-OES）. The characterization results indicated that the MgFeMo-S catalyst has retained the unique layered structure, which can facilitate uniform dispersion of the MoS2 species on both the surface and interlayer of the catalysts. For the HDO of eugenol, the Mg1Fe2Mo-S catalysts exhibited the best HDO activity among all the catalysts due to its higher active metal contents and larger pore size. The HDO conversion was 99.6% and the yield of phenolics was 63.7%, under 5 MPa initial H2 pressure（measured at RT） at 300 ℃ for 3 h. More importantly,MoS2 species deposited on the interlayer galleries in the MgFeMo-S catalysts resulted in dramatically superior HDO activity to MoS2/Mg1Fe2-S catalyst. Based on the mechanism investigation for eugenol, the HDO reaction route of eugenol under sulfide catalytic system has been proposed for the first time. Further applicability of the catalyst on HDO of more lignin-derived compounds was operated, which showed good HDO activity and selectivity to produce aromatic products.

关键词： MgFe Hydrotalcite Sulfide catalysts Layered structure Hydrodeoxygenation Eugenol

Changes of auditory evoked magnetic fields in patients after acute cerebral infarction using magnetoencephalography

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Neural Regeneration Research 2012年第24期7卷 1906-1913页

作者： Zhanyong Sun chunfeng song Jilin Sun Ling Li Yanhong Dong Jianhua Wang Jie Wu Wenzhu Cui Yujin Wu Peiyuan Lv Department of Neurology Hebei Medical UniversityShijiazhuang 050017Hebei ProvinceChina Institute of Basic Medicine Hebei Medical UniversityShijiazhuang 050017Hebei ProvinceChina Department of Magnetoencephalography Hebei General HospitalShijiazhuang 050051Hebei ProvinceChina Department of Neurology Hebei General HospitalShijiazhuang 050051Hebei ProvinceChina

Auditory evoked magnetic fields were recorded from 15 patients with acute cerebral infarction and 11 healthy volunteers using *** auditory stimuli of 2 kHz pure tone were binaurally presented with an interstimulus interval of 1 *** intensity of stimuli was 90 dB and the stimulus duration was 8 *** results showed that the M100 was the prominent response, peaking approximately 100 ms after stimulus onset in all *** originated from the area close to Heschl’s *** the patient group,the peak latency of M100 responses was significantly prolonged,and the mean strength of equivalent current dipole was significantly smaller in the affected *** three-dimensional inter-hemispheric difference of the M100 positions was increased in the patient *** experimental findings suggested that impairment of cerebral function in patients with acute ischemic stroke can be detected using magnetoencephalography with the higher spatial resolution and temporal *** could provide objective and sensitive indices to estimate auditory cortex function in patients with acute cerebral infarction.

关键词： acute cerebral infarction cerebral ischemia magnetoencephalography auditory evoked magnetic fields equivalent current dipole Heschl’s gyrus brain functional impairment nerve injury regeneration neural regeneration