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A coating strategy on titanium implants with enhanced photodynamic therapy and CO-based gas therapy for bacterial killing and inflammation regulation

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Chinese Chemical Letters 2024年第2期35卷 386-395页

作者： Liang Cheng Bingshuai Zhou Manlin Qi Xiaolin sun Shujun Dong Yue sun Biao Dong lin Wang Yingwei Yang Department of Oral Implantology Jilin Provincial Key Laboratory of Sciences and Technology for Stomatology Nanoengineering School and Hospital of StomatologyJilin UniversityChangchun 130021China State Key Laboratory on Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130021China College of Chemistry Jilin UniversityChangchun 130012China

Antimicrobial photodynamic therapy(aPDT)has been considered a noninvasive and effective modality against the bacterial infection of peri‑implantitis,especially the aPDT triggered by near-infrared(NIR)light due to the large penetration depth in ***,the complexity of hypoxia microenvironments and the distance of aPDT sterilization still pose challenges before realizing the aPDT clinical *** to the long lifespan and transmission distance of therapeutic gas molecules,we design a multi-functional gas generator that combines aPDT as well as O_(2) and CO gas release function,which can solve the problem of hypoxia(O_(2))in PDT and the problem of inflammation regulation(CO)in the distal part of peri‑implant inflammation under near-infrared(NIR)*** the composite nanoplatform that spin-coated on the surface of titanium implants,up-conversion nanoparticles(UCNPs)were involved in converting the NIR to visible,which further excites the partially oxidized stannic sulfide(SnS_(2)),realizing the therapeutic gas *** green(ICG)was further integrated to enhance the aPDT performance(Ti-U@SnS_(2)/I).Therefore,reactive oxygen species(ROS),CO,and O_(2) can be controllably administered via a composite nano-platform mediated by a single NIR light(808 nm).This implant surface modification strategy could achieve great self-enhancement antibacterial effectiveness and regulate the lingering questions,such as relieving the anoxic microenvironment and reaching deep infection sites,providing a viable antibiotic-free technique to combat peri‑implantitis.

关键词： Photodynamic therapy Biomaterials Dental implant Reactive oxygen species Carbon monoxide Hybrid nanoplatform

Low-energy-consumption temperature swing system for CO_(2) capture by combining passive radiative cooling and solar heating

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Green Energy & Environment 2024年第3期9卷 507-515页

作者： Ying-Xi Dang Peng Tan Bin Hu Chen Gu Xiao-Qin Liu lin-Bing sun State Key Laboratory of Materials-Oriented Chemical Engineering Jiangsu National Synergetic Innovation Center for Advanced Materials(SICAM)College of Chemical EngineeringNanjing Tech UniversityNanjing211816China

Temperature-swing adsorption(TSA)is an effective technique for CO_(2) capture,but the temperature swing procedure is ***,we report a low-energy-consumption system by combining passive radiative cooling and solar heating for the uptake of CO_(2) on commercial activated carbons(CACs).During adsorption,the adsorbents are coated with a layer of hierarchically porous poly(vinylidene fluoride-co-hexafluoropropene)[P(VdF-HFP)HP],which cools the adsorbents to a low temperature under sunlight through radiative *** desorption,CACs with broad absorption of the solar spectrum are exposed to light irradiation for *** heating and cooling processes are completely driven by solar *** tests under mimicked sunlight using the CACs show that the performance of this system is comparable to that of the traditional ***,under real sunlight irradiation,the adsorption capacity of the CACs can be well maintained after multiple *** present work may inspire the development of new temperature swing procedures with little energy consumption.

关键词： CO_(2)capture Solar heating Passive radiative cooling Temperature swing adsorption

Atomscopic of ripple origins for two-dimensional monolayer transition metal dichalcogenides

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Nano Research 2024年第3期17卷 2136-2144页

作者： Haitao Yu Mingzi sun Xiao Wu Cheuk Hei Chan Bolong Huang Zhong lin Wang CAS Center for Excellence in Nanoscience Beijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijing 100083China School of Nanoscience and Technology University of Chinese Academy of SciencesBeijing 100049China Department of Applied Biology and Chemical Technology The Hong Kong Polytechnic UniversityKowloon 999077Hong KongChina Research Centre for Carbon-Strategic Catalysis The Hong Kong Polytechnic UniversityKowloon 999077Hong KongChina School of Materials Science and Engineering Georgia Institute of TechnologyAtlantaGeorgia 30332USA

During the development of ultrathin two-dimensional(2D)materials,the appearance of ripples has been widely ***,the formation mechanisms and their influences are still rarely investigated,especially their contributions to the electronic structures and optical *** compensate for the knowledge gap,we have carried out comprehensive theoretical studies on the monolayer WSe_(2) with a series of ripple structures from 0 to 12Åin different lattice *** sensitivity of the formation energy,band structures,electronic structures,and optical properties to the ripple structures have been performed systematically for the first *** formation of ripples in Armchair and zigzag simultaneously are more energetically favorable,leading to more flexible optimizations of the optoelectronic *** improved charge-locking effect and extension of absorption ranges indicate the significant role of ripple *** spontaneous formation of ripples is associated with orbital rearrangements and structural *** leads to the unique charge carrier correlate inversion between W-5d and Se-4p orbitals,resulting in the pinning of the Fermi *** work has supplied significant references to understand ultrathin 2D structures and benefit their future developments and applications in high-performance optoelectronic devices.

关键词： two-dimensional(2D)materials ripples strain effect charge carrier correlation inversion optoelectronic properties

Multi-layer network embedding on scc-based network with motif

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Digital Communications and Networks 2024年第3期10卷 546-556页

作者： Lu sun Xiaona Li Mingyue Zhang Liangtian Wan Yun lin Xianpeng Wang Gang Xu Department of Communication Engineering Institute of Information Science TechnologyDalian Maritime UniversityDalian116026China Key Laboratory of Big Data Intelligent Computing Chongqing University of Posts and TelecommunicationsChongqing400065China Key Laboratory for Ubiquitous Network and Service Software of Liaoning Province DUT School of Software Technology&DUT-RU International School of Information Science and EngineeringDalian University of TechnologyDalian 116620China College of Information and Communication Engineering Harbin Engineering UniversityHarbin 150001China School of Information and Communication Engineering Hainan UniversityHaikou 570228China State Key Laboratory of Millimeter Waves School of Information Science and EngineeringSoutheast UniversityNanjing 210096China

Interconnection of all things challenges the traditional communication methods,and Semantic Communication and Computing(SCC)will become new *** is a challenging task to accurately detect,extract,and represent semantic information in the research of SCC-based *** previous research,researchers usually use convolution to extract the feature information of a graph and perform the corresponding task of node ***,the content of semantic information is quite *** graph convolutional neural networks provide an effective solution for node classification tasks,due to their limitations in representing multiple relational patterns and not recognizing and analyzing higher-order local structures,the extracted feature information is subject to varying degrees of ***,this paper extends from a single-layer topology network to a multi-layer heterogeneous topology *** Bidirectional Encoder Representations from Transformers(BERT)training word vector is introduced to extract the semantic features in the network,and the existing graph neural network is improved by combining the higher-order local feature module of the network model representation network.A multi-layer network embedding algorithm on SCC-based networks with motifs is proposed to complete the task of end-to-end node *** verify the effectiveness of the algorithm on a real multi-layer heterogeneous network.

关键词： Semantic communication and computing Multi-layer network Graph neural network Motif

A Deep Neural Collaborative Filtering Based Service Recommendation Method with Multi-Source Data for Smart Cloud-Edge Collaboration Applications

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Tsinghua Science and Technology 2024年第3期29卷 897-910页

作者： Wenmin lin Min Zhu Xinyi Zhou Ruowei Zhang Xiaoran Zhao Shigen Shen Lu sun Alibaba Business School Hangzhou Normal UniversityHangzhou 311121China Blockchain Laboratory of Agricultural Vegetables Weifang University of Science and TechnologyShouguang 262700China School of Computer Science Qufu Normal UniversityRizhao 276827China School of Information Engineering Huzhou UniversityHuzhou 313000China

Service recommendation provides an effective solution to extract valuable information from the huge and ever-increasing volume of big data generated by the large cardinality of user ***,the distributed and rich multi-source big data resources raise challenges to the centralized cloud-based data storage and value mining approaches in terms of economic cost and effective service recommendation *** view of these challenges,we propose a deep neural collaborative filtering based service recommendation method with multi-source data(i.e.,NCF-MS)in this paper,which adopts the cloud-edge collaboration computing paradigm to build recommendation *** specifically,the Stacked Denoising Auto Encoder(SDAE)module is adopted to extract user/service features from auxiliary user profiles and service *** Multiple Layer Perceptron(MLP)module is adopted to integrate the auxiliary user/service features to train the recommendation ***,we evaluate the effectiveness of the NCF-MS method on three public *** experimental results show that our proposed method achieves better performance than existing methods.

关键词： deep neural collaborative filtering multi-source data cloud-edge collaboration application stackeddenoising auto encoder multiple layer perceptron

Acetic acid additive in NaNO_(3)aqueous electrolyte for long-lifespan Mg-air batteries

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Journal of Magnesium and Alloys 2024年第2期12卷 825-839页

作者： Yaqing Zhou Fan sun Gunahua lin Sandrine Zanna Antoine Seyeux Philippe Marcus Jolanta´Swiatowska Chimie ParisTech-CNRS PSL UniversityInstitut de Recherche de Chimie Paris11 rue Pierre et Marie CurieParis 75005France

Mg-air batteries have attracted tremendous attention as a potential next-generation power source for portable electronics and e-transportation due to their remarkable high theoretical volumetric energy density,environmental sustainability,and ***,the fast hydrogen evolution reaction(HER)in NaCl-based aqueous electrolytes impairs the performance of Mg-air batteries and leads to poor specific capacity,low energy density,and low ***,the conventionally used NaCl solute was proposed to be replaced by NaNO_(3)and acetic acid additive as a corrosion inhibitor,therefore an electrolyte engineering for long-life time Mg-air batteries is *** resulting Mg-air batteries based on this optimized electrolyte demonstrate an improved discharge voltage reaching~1.8 V for initial 5 h at a current density of 0.5 mA/cm^(2) and significantly prolonged cells'operational lifetime to over 360 h,in contrast to only~17 h observed in NaCl electrolyte.X-ray photoelectron spectroscopy and time-of-flight secondary ion mass spectrometry were employed to analyse the composition of surface film and scanning electron microscopy combined with transmission electron microscopy to clarify the morphology changes of the surface layer as a function of acetic acid *** thorough studies of chemical composition and morphology of corrosion products have allowed us to elucidate the working mechanism of Mg anode in this optimized electrolyte for Mg-air batteries.

关键词： Acetic acid additive in NaNO_(3)electrolyte Electrolyte engineering Corrosion surface film Surface characterization Hydrogen evolution

Exploring the Predominant Factors Influencing the Oxygen Reduction Performance of PtCo/C Catalysts

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Chemical Research in Chinese Universities 2024年第4期40卷 753-760页

作者： LI Jinrong YU Xianghui sun Qi PENG Yong CAO Shuang HOU chun-Chao XU Qiang College of Chemistry and Chemical Engineering Institute for Sustainable Energy and ResourcesQingdao UniversityQingdao266071P.R.China Leibniz Institute for Catalysis e.V. Albert-Einstein-Strasse 29aRostock18059Germany School of Materials Science and Engineering Ocean University of ChinaQingdao266100P.R.China Shenzhen Key Laboratory of Micro/Nano-Porous Functional Materials(SKLPM) SUSTech-Kyoto University Advanced Energy Materials Joint Innovation Laboratory(SKAEM-JIL)Key University Laboratory of Highly Efficient Utilization of Solar Energy and Sustainable Development of GuangdongDepartment of Chemistry and Department of Materials Science and EngineeringSouthern University of Science and Technology(SUSTech)Shenzhen518055P.R.China

PtCo nanoalloys(NAs)deposited on carbon black are emerging as robust electrocatalysts for addressing the sluggish kinetic issue of oxygen reduction reaction(ORR).However,developing a simple and low-cost method to synthesize PtCo/C with excellent performance is still a great *** this work,a one-pot method was used to successfully obtain the PtCo NAs on commercial carbon supports of acetylene black and Ketjenblack ECP600JD,*** with those grown on Ketjenblack ECP600JD,the PtCo NAs grown on acetylene black exhibited higher electrochemical surface area(ECSA)and mass activity(MA),which may be attributed to the different particle sizes of PtCo NAs,distinct hydrophilicity,electroconductivity and charge distribution between the carbon supports and PtCo *** study provides valuable insights into the optimal design of carbon-supported ORR electrocatalysts with exceptional activity and durability.

关键词： Oxygen reduction reaction PtCo nanoalloy Carbon-supported nanostructure Acetylene black

Coordinated Frequency Control for Isolated Power Systems with High Penetration of DFIG-Based Wind Power

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CSEE Journal of Power and Energy Systems 2024年第4期10卷 1399-1414页

作者： Xin Ding Wei lin Jian Xu Yuanzhang sun Liangzhong Yao Beilin Mao School of Electrical Engineering and Automation Wuhan UniversityWuhan 430072China Department of Electrical Engineering and Computer Science Case Western Reserve UniversityClevelandOH 44106 USA

This paper proposes a coordinated frequency control scheme for emergency frequency regulation of isolated power systems with a high penetration of wind *** proposed frequency control strategy is based on the novel nonlinear regulator theory,which takes advantage of nonlinearity of doubly fed induction generators(DFIGs)and generators to regulate the frequency of the power *** deviations and power imbalances are used to design nonlinear feedback controllers that achieve the reserve power distribution between generators and DFIGs,in various wind speed *** effectiveness and dynamic performance of the proposed nonlinear coordinated frequency control method are validated through simulations in an actual isolated power grid.

关键词： Frequency control isolated power systems nonlinear feedback nonlinear regulator theory wind power

Interconnected microstructure and flexural behavior of Ti_(2)C-Ti composites with superior Young’s modulus

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International Journal of Minerals,Metallurgy and Materials 2024年第9期31卷 2088-2101页

作者： Fengbo sun Rui Zhang Fanchao Meng Shuai Wang Lujun Huang lin Geng School of Materials Science and Engineering Harbin Institute of TechnologyHarbin 150001China Waikato Centre for Advanced Materials and Manufacturing School of EngineeringUniversity of WaikatoHamilton 3240New Zealand State Key Laboratory of Precision Welding&Joining of Materials and Structures Harbin Institute of TechnologyHarbin 150001China

To enhance the Young’s modulus(E)and strength of titanium alloys,we designed titanium matrix composites with intercon-nected microstructure based on the Hashin-Shtrikman *** to the results,the in-situ reaction yielded an interconnected microstructure composed of Ti_(2)C particles when the Ti_(2)C content reached 50vol%.With widths of 10 and 230 nm,the intraparticle Ti lamellae in the prepared composite exhibited a bimodal size distribution due to precipitation and the unreacted Ti phase within the grown Ti_(2)C *** composites with interconnected microstructure attained superior properties,including E of 174.3 GPa and ultimate flexural strength of 1014 *** with that of pure Ti,the E of the composite was increased by 55% due to the high Ti_(2)C content and interconnected *** outstanding strength resulted from the strong interfacial bonding,load-bearing capacity of interconnected Ti_(2)C particles,and bimodal intraparticle Ti lamellae,which minimized the average crack driving *** flexural tests revealed preferential crack initiation along the{001}cleavage plane and grain boundary of Ti_(2)C in the region with the highest tensile *** addition,the propagation can be efficiently inhibited by interparticle Ti grains,which prevented the brittle fracture of the composites.

关键词： titanium matrix composites titanium carbide interface Young’s modulus flexural behavior