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Contrasting oxidation states of low-Ti and high-Ti magmas control Ni-Cu sulfide and Fe-Ti oxide mineralization in Emeishan Large Igneous Province

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Geoscience Frontiers 2022年第6期13卷 41-58页

作者： Yonghua Cao christina yan wang Key Laboratory of Metallogenic Prediction of Nonferrous Metals and Geological Environment Monitoring Ministry of EducationSchool of Geosciences and Info-PhysicsCentral South UniversityChangsha 410083China Key Laboratory of Mineralogy and Metallogeny Guangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou 510640China CAS Center for Excellence in Deep Earth Science Guangzhou 510640China Guangdong Provincial Key Laboratory of Mineral Physics and Materials Guangzhou 510640China

Magmatic Ni-Cu-(PGE) sulfide and Fe-Ti oxide deposits in plume-related large igneous provinces(LIPs)are commonly related to low-Ti and high-Ti series magmas, respectively, but the major factors that control such a relationship of metallogenic types and magma compositions are unclear. Magma fOcontrols sulfur status and relative timing of Fe-Ti oxide saturation in mafic magmas, which may help clarify this issue. Taking the Emeishan LIP as a case, we calculated the magma fOof the high-Ti and low-Ti picrites based on the olivine-spinel oxygen barometer, and the partitioning of V in olivine. The obtained fOof the high-Ti series magma(FMQ + 1.1 to FMQ + 2.6) is higher than that of the low-Ti series magma(FMQ-0.5to FMQ + 0.5). The magma fOof the high-Ti and low-Ti picrites containing Fo > 90 olivine reveals that the mantle source of the high-Ti series is likely more oxidized than that of the low-Ti series. The results using the ’lambda REE’ approach show that the high-Ti series may have been derived from relatively oxidized mantle with garnet pyroxenite component. The S contents at sulfide saturation(SCSS) of the two series magmas were calculated based on liquid compositions obtained from the alpha Melts modeling, and the results show that the low-Ti series magma could easily attain the sulfide saturation as it has low fOwith S being dominantly as S. In contrast, the oxidized high-Ti series magma is difficult to attain the sulfide saturation, but could crystallize Fe-Ti oxides at magma MgO content of ~7.0 wt.%. Thus, contrasting magma fOof low-Ti and high-Ti series in plume-related LIPs may play an important role in producing two different styles of metallogeny.

关键词： Emeishan large igneous province Mantle plume High-Ti and low-Ti series magma Magma oxygen fugacity Magmatic Fe-Ti oxide deposits Magmatic Ni-Cu-(PGE)deposits

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The distribution,characteristics and fluid sources of lode gold deposits:An overview

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Science China Earth Sciences 2021年第9期64卷 1463-1480页

作者： christina yan wang Bo WEI Wei TAN Zaicong wang Qingdong ZENG CAS Key Laboratory of Mineralogy and Metallogeny/Guangdong Provincial Key Laboratory of Mineral Physics and Materials Guangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou510640China CAS Center for Excellence in Deep Earth Science Chinese Academy of SciencesGuangzhou510640China State Key Laboratory of Geological Processes and Mineral Resources(GPMR) School of Earth SciencesChina University of GeosciencesWuhan430074China Key Laboratory of Mineral Resources Institute of Geology and GeophysicsChinese Academy of SciencesBeijing100029China Institutions of Earth Science Chinese Academy of SciencesBeijing100029China University of Chinese Academy of Sciences Beijing100029China

Lode gold deposits are among the most economically important types of gold deposits in the ***,they formed mainly in three time intervals,2.8 to 2.5 Ga,2.1 to 1.8 Ga,and 700 Ma to the *** of ore-forming fluids and other components are of critical importance in a better understanding of the genesis and the geodynamic controls of these *** ore-forming fluids were mostly derived from devolatization of sedimentary and/or volcanic sequences during greenschist to amphibolite facies metamorphism associated with orogenic deformation,magmatic hydrothermal fluids have been increasingly shown to be important in many gold deposits in various *** this review paper,we summarize the major features of lode gold deposits,possible sources of ore-forming fluids,and mechanisms of gold *** we acknowledge the critical role of metamorphically derived fluids in the genesis of such deposits worldwide,we emphasize that mantle-or basaltic magma-derived fluids may have been much more important than commonly *** use the Liaodong peninsula of the North China Craton as an example to demonstrate the significance of mantle-derived *** earlier studies and new data,we show that some of the late Mesozoic lode gold deposits in the North China Craton may have formed from magmatic hydrothermal fluids due to the extension and partial melting of the hydrated,metasomatized subcontinental lithosphere mantle,as best exemplified by the Wulong gold deposit.

关键词： Lode gold deposit Ore-forming fluid Metasomatized subcontinental lithosphere mantle Mantle-derived melt/fluid North China Craton

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Textures and mineral compositions of the Xinjie layered intrusion,SW China:Implications for the origin of magnetite and fractionation process of Fe-Ti-rich basaltic magmas

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Geoscience Frontiers 2013年第5期4卷 503-515页

作者： Huan Dong Changming Xing christina yan wang Key Laboratory of Mineralogy and Metallogeny Guangzhou Institute of GeochemistryChinese Academy of Sciences University of Chinese Academy of Sciences

The Xinjie layered intrusion in the Panxi region,SW China,hosts both Fe-Ti oxide and platinum-group element（PGE） sulfide *** intrusion can be divided,from the base upward,into UnitsⅠ,ⅡandⅢ,in terms of mineral ***ⅠandⅡare mainly composed of wehrlite and clino-pyroxenite, whereas UnitⅢis mainly composed of *** sulfide-rich layers mainly occur in Unit I, whereas thick Fe-Ti oxide-rich layers mainly occur in UnitⅢ.An ilmenite-rich layer occurs at the top of UnitⅠ.Fe-Ti oxides include magnetite and *** amounts of cumulus and intercumulus magnetite occur in UnitsⅠandⅡ.Cumulus magnetite grains are commonly euhedral and enclosed within olivine and *** have high Cr2O3 contents ranging from 6.02 to 22.5 wt.%,indicating that they are likely an early crystallized phase from *** magnetite that usually displays ilmenite exsolution occupies the interstices between cumulus olivine crystals and coexists with interstitial clinopyroxene and *** magnetite has Cr2O3 ranging from 1.65 to 6.18 wt.%, lower than cumulus *** intercumulus magnetite may have crystallized from the trapped *** amounts of magnetite in UnitⅢcontains Cr2O3（＆lt;0.28 wt.%） much lower than magnetite in UnitsⅠandⅡ.The magnetite in UnitⅢis proposed to be accumulated from a Fe-Ti-rich *** Fe-Ti-rich melt is estimated to contain 35.9 wt.%of SiO2,26.9 wt.%of FeOt,8.2 wt.%of TiO2,13.2 wt.%of CaO, 8.3 wt.%of MgO,5.5 wt.%of Al2O3 and 1.0 wt.%of *** composition is comparable with the Fe-rich melts in the Skaergaard and Sept Iles *** non-reactive microstructures,granophyre pockets and ilmenite-rich intergrowths,are representative of Si-rich melt and Fe-Ti-rich melt,and are the direct evidence for the existence of an immiscible Fe-Ti-rich melt that formed from an evolved ferro-basaltic magma.

关键词： Geochemistry Fe-Ti oxides Mineral composition The Xinjie layered mafic-ultramafic intrusion Emeishan large igneous province

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Water in coesite: Incorporation mechanism and operation condition,solubility and P-T dependence, and contribution to water transport and coesite preservation

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Geoscience Frontiers 2021年第1期12卷 313-326页

作者： Wei yan yanyao Zhang Yunlu Ma Mingyue He Lifei Zhang Weidong Sun christina yan wang Xi Liu School of Earth and Space Sciences Peking UniversityBeijing100871China Key Laboratory of Orogenic Belts and Crustal Evolution Ministry of Education of ChinaBeijing100871China Department of Geological Sciences Jackson School of GeosciencesThe University of Texas at AustinAustinTX78712USA School of Gemmology China University of Geosciences(Beijing)Beijing100083China Center of Deep Sea Research Institute of OceanographyChinese Academy of SciencesQingdao266071China Key Laboratory of Mineralogy and Metallogeny Guangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou510640China

A series of coesite,coexisting with or without a liquid phase,was synthesized in the nominal system SiO2-H2O at800-1450℃and 5 ***-Raman spectroscopy was used to identity the crystalline phase,electron microprobe and LA-ICP-MS were employed to quantity some major and trace elements,and unpolarized FTIR spectroscopy was applied to probe the different types of hydrogen defects,explore water-incorporation mechanisms and quantify water *** amounts of A1 and B were detected in the *** our results with the results in the literatures,we have found no positive correlation between the Al contents and the"Al"-based hydrogen concentrations,suggesting that previously proposed hydrogen-incorporation mechanism H^++Al^3+■Si^4+does not function in *** contrast,we have confirmed the positive correlation between the B contents and the B-based hydrogen *** hydrogen-incorporation mechanism H^++B3^+■Si^4+readily takes place in coesite at different P-T conditions,and significantly increases the water content at both liquid-saturated and liquid-undersaturated *** the SiO2-H2O system,we have found that type-Ⅰhydrogarnet substitution plays a dictating role in incorporating water into coesite at liquid-saturated condition,type-II hydrogarnet substitution contributes significantly at nearly dry condition,and both operate at conditions in *** water solubility of coesite,as dictated by the type-Ⅰhydrogarnet substitution,positively correlates with both P and T,cH2O=-105(30)+5.2(32)×P+0.112(26)×T,with cH2O in wt ppm,P in GPa and T in℃.Due to its low water solubility and small fraction in subducted slabs,coesite may contribute insignificantly to the vertical water transport in subduction ***,the water solubility of any coesite in exhuming ultra-high pressure metamorphic rocks should be virtually zero as coesite becomes *** an adequately fast waterdiffusion rate,this metastable coesite should be complet

关键词： Coesite preservation FTIR New IR experimental Protocol Anhydrous minerals P-T dependence of water solubility Water-incorporation mechanism

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Detrital zircon U-Pb-He double dating: A method of quantifying long- and short-term exhumation rates in collisional orogens

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Science China Earth Sciences 2014年第11期57卷 2702-2711页

作者： christina yan wang Ian H.CAMPBELL Peter W.REINERS Charlotte M.ALLEN Key Laboratory of Mineralogy and Metallogeny Guangzhou Institute of Geochemistry Chinese Academy of Sciences Research School of Earth Sciences The Australian National UniversityCanberra ACT 0200 Australia Department of Geosciences University of ArizonaTucson AZ 85721 USA

A U-Pb-He double-dating method is applied to detrital zircons with core-rim structure from the Ganges River in order to de- termine average short and long-term exhumation rates for the Himalayas. Long-term rates are calculated from the U/Pb ages of metamorphic rims of the grains that formed during the Himalayan orogeny and their crystallization temperatures, which are calculated from the Ti-in-zircon thermometer. Short-term rates are calculated from （U-Th）/He ages of the grains with appro- priate closure temperatures. The results show that short-term rates for the Himalayas, which range from 0.70 ± 0.09 to 2.67 ± 0.40 km/Myr and average 1.75 ± 0.59 （1δ） km/Myr, are higher and more varied than the long-term rates, which range from 0.84 ±0.16 to 1.85 ± 0.35 km/Myr and average 1.26 ±0.25 （let） km/Myr. The differences between the long-term and short-term rates can be attributed to continuous exhumation of the host rocks in different mechanisms in continental collision orogen. The U/Pb ages of 44.0 ± 3.7 to 18.3 ±0.5 Ma for the zircon rims indicate a protracted episode of -：25 Myr for regional metamorphism of the host rocks at deeper crust, whereas the （U-Th）/He ages of 42.2 ± 1.8 to 1.3 ± 0.2 Ma for the zircon grains represent a protracted period of -40 Myr for exposure of the host rocks to shallower crustal level. In particular, the oldest （U-Th）/He ages of the zircon grains are close to the oldest U/Pb ages for the rims, indicating that some parcels of the rocks that contain zircons were rapidly exhumed from deep to shallow levels in the stage of collisional orogeny. On the other hand, some parcels of the rocks may have been carried upwards by thrust faults in the post-collisional stage. The parcels could be carried upwards by the thrust faults that steepen as they near the surface, or by transient movement faults so that areas of rapid exhu- mation became areas of slow exhumation and visa versa on a time scale of a few Myr in order to maintain the continuous ex- huma

关键词： zircon U-Pb-He double-dating method Himalayas exhumation rate collisional orogen

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Two stages of immiscible liquid separation in the formation of Panzhihua-type Fe-Ti-V oxide deposits,SW China

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Geoscience Frontiers 2013年第5期4卷 481-502页

作者： Mei-Fu Zhou Wei Terry Chen christina yan wang Stephen A.Prevec Patricia Pingping Liu Geoffrey H.Howarth Department of Earth Sciences The University of Hong Kong Key Laboratory of Mineralogy and Metallogeny Guangzhou Institute of GeochemistryChinese Academy of Sciences Department of Geology Rhodes University

Magmatic oxide deposits in the～260 Ma Emeishan Large Igneous Province（ELIP）,SW China and northern Vietnam,are important sources of Fe,Ti and *** giant magmatic Fe-Ti-V oxide deposits, such as the Panzhihua,Hongge,and Baima deposits,are well described in the literature and are hosted in layered mafic-ultramafic intrusions in the Panxi region,the central *** same type of ELIP- related deposits also occur far to the south and include the Anyi deposit,about 130 km south of Panzhihua,and the Mianhuadi deposit in the Red River fault *** Anyi deposit is relatively small but is similarly hosted in a layered mafic *** Mianhuadi deposit has a zircon U-Pb age of～260 Ma and is thus contemporaneous with the *** deposit was variably metamorphosed during the Indosinian orogeny and Red River ***,magnetite of the Mianhuadi deposit contains smaller amounts of Ti and V than that of the other deposits,possibly attributable to the later *** distribution of the oxide ore deposits is not related to the domal structure of the *** major feature of all the oxide deposits in the ELIP is the spatial association of oxide-bearing gabbroic intrusions,syenitic plutons and high-Ti flood ***,we propose that magmas from a mantle plume were emplaced into a shallow magma chamber where they were evolved into a field of liquid immiscibility to form two silicate liquids,one with an extremely Fe-Ti-rich gabbroic composition and the other *** immiscible Fe-Ti-（P） oxide melt may then separate from the mafic magmas to form oxide *** parental magmas from which these deposits formed were likely Fe-Ti-rich picritic in composition and were derived from enriched asthenospheric mantle at a greater depth than the magmas that produced sulfide-bearing intrusions of the ELIP.

关键词： Fe-Ti oxide Gabbroic layered intrusion Immiscible Fe-Ti-(P) rich melt Emeishan Large Igneous Province SW China

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A brief review of ophiolites in China

A brief review of ophiolites in China

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中国科学院地质与地球物理研究所2008学术年会

作者： christina yan wang Paul T.Robinson Department of Geology Northwest University Department of Earth Sciences Dalhousie UniversityHalifaxNSCanada

Ophiolites are widely distributed in western,southwestern and northern China,where they fall into four principal age groups;Neoproterozoic, Early Paleozoic,Late Paleozoic and ***

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我国铂族元素、钴和铬主要矿床类型的分布特征及成矿机制

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科学通报 2020年第33期65卷 3825-3838页

作者：王焰钟宏曹勇华魏博陈晨中国科学院广州地球化学研究所中国科学院矿物学与成矿学重点实验室广州510640 中国科学院地球化学研究所矿床地球化学国家重点实验室贵阳550081 中国科学院大学北京100049

我国赋含铂族元素(platinum-group elements, PGE)、钴(Co)和铬(Cr)资源的主要矿床类型普遍与镁铁-超镁铁质岩有关,岩浆铜镍硫化物矿床提供了几乎全部的PGE储量和约一半的Co储量,蛇绿岩中的豆荚状铬铁矿矿床是Cr的主要来源.我国一直未... 详细信息

我国赋含铂族元素(platinum-group elements, PGE)、钴(Co)和铬(Cr)资源的主要矿床类型普遍与镁铁-超镁铁质岩有关,岩浆铜镍硫化物矿床提供了几乎全部的PGE储量和约一半的Co储量,蛇绿岩中的豆荚状铬铁矿矿床是Cr的主要来源.我国一直未发现与层状岩体有关的大型铂族元素和层状铬铁矿矿床,也缺乏全球Co储量占比很高的沉积层控型铜钴矿和红土型镍钴矿,唯一的大型铬铁矿矿床赋存在西藏罗布莎蛇绿岩中.本文介绍了我国目前已发现的PGE、Co和Cr主要矿床类型及其分布,并总结了近年来一些典型矿床在成矿元素赋存状态和富集机制方面的研究进展.在此基础上,从微-纳米尺度下PGE的赋存状态研究、镁铁-超镁铁质岩及相关矿床中Co的迁移富集机制、赋存状态及资源潜力、以及蛇绿岩豆荚状铬铁矿矿床中Cr迁移-富集机制的精细刻画等三方面提出了今后值得深入探索的问题.

关键词：镁铁-超镁铁质岩铂族元素矿床含钴矿床铬铁矿矿床矿床分布成矿机制

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Volatile and C-H-O isotopic compositions of giant Fe-Ti-V oxide deposits in the Panxi region and their implications for the sources of volatiles and the origin of Fe-Ti oxide ores

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Science China Earth Sciences 2012年第11期55卷 1782-1795页

作者： wang christina yan Key Laboratory of Mineralogy and Metallogeny Guangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou 510640China

The Panzhihua,Hongge,and Baima Fe-Ti-V oxide deposits in the Panzhihua-Xichang(Panxi) region are hosted in large layered mafic-ultramafic *** layered intrusions intrude either the Neoproterozoic Dengying Formation,composed mainly of limestone,or the Paleoproterozoic Hekou Formation,composed of meta-sedimentary-volcanic *** remains unclear if the wall rocks have been involved during the fractionation of magmas and have affected the sequence of crystallization of Fe-Ti *** and their C-H-O isotopic compositions of magnetite,apatite,clinopyroxene,and plagioclase of different types of ores from the three intrusions are analyzed using a technique of stepwise heating mass spectrometer to evaluate the role of wall rocks in the formation of Fe-Ti oxide *** released from magnetite are composed mainly of H 2 O and CO 2,whereas the other minerals are composed mainly of H 2 O,CO 2 and H *** 800-1200°C temperature interval,the average 13 C values of CO 2 of all the minerals from the three intrusions range from 7.7‰ to 13.5‰ and the average 18 O CO 2 values from 19.1‰ to 19.5‰,which are scattered in a mixed field with basalt and the two types of wall rocks as end-members,indicating that CO 2 from the wall rocks may have been involved in the magmas from which the three intrusions *** 400-800 C temperature interval,both 13 C values(13.7‰ to 17.9‰ on the average) and 18 O values(16.2‰ to 19.2‰ on the average) of CO 2 of all the minerals are lower than those for 800-1200 C temperature interval,and much closer to the values of the wall *** H 2 O released at the 400-800 C temperature interval has relatively low D values ranging from 90‰ to 115‰,also indicating the involvement of fluids from the wall *** average bulk contents of volatiles released from magnetite of the Hongge,Baima,and Panzhihua intrusions are 4891,2996,and 1568 mm 3 STP/g,respectively,much higher than those released from other minerals in total,which are 382

关键词： magnetite volatiles C-H-O isotope Fe-Ti-V oxide ore Panxi region

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Carbon‑Based Electrodes for Advanced Zinc‑Air Batteries:Oxygen‑Catalytic Site Regulation and Nanostructure Design

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Electrochemical Energy Reviews 2023年第1期6卷 532-572页

作者： Wenjie Shao Rui yan Mi Zhou Lang Ma christina Roth Tian Ma Sujiao Cao Chong Cheng Bo Yin Shuang Li College of Polymer Science and Engineering State Key Laboratory of Polymer Materials EngineeringSichuan UniversityChengdu 610065SichuanChina College of Biomass Science and Engineering Sichuan UniversityChengdu 610065SichuanChina Department of Ultrasound West China HospitalSichuan UniversityChengdu 610041SichuanChina Electrochemical Process Engineering Engineering SciencesUniversity of BayreuthUniversitätsstr.3095447 BayreuthGermany Med-X Center for Materials Sichuan UniversityChengdu 610065SichuanChina Functional Materials Department of ChemistryTechnische Universität BerlinHardenbergstraße 4010623 BerlinGermany

Zn-air batteries are highly attractive for direct chemical-to-electrical energy conversion and for solving the energy crisis and environmental *** efficient oxygen electrodes has been considered one of the most critical steps in the development of advanced Zn-air batteries because of the sluggish kinetics of the oxygen reduction reaction and the oxygen evolution *** recent years,nanostructured carbon-based electrodes with large surface areas,efficient oxygen-catalytic centers,and hierarchically porous matrices have provided significant opportunities to optimize the performance of the oxygen electrodes in both primary and rechargeable Zn-air *** this review,we provide a comprehensive summary of the reported nanostructured carbon-based electrodes for advanced Zn-air batteries in terms of tailoring the oxygen-catalytic sites and designing carbon *** versatile synthetic strategies,characterization methods,and in-depth understanding of the relationships between the oxygen-catalytic sites/nanostructures and the oxygen electrode performance are systematically ***,we also briefly outline recent progress in engineering flexible and high-power Zn-air ***,a thorough discussion of current primary challenges and future perspectives on the rational design of nanostructured carbon-based oxygen electrodes is given,thus providing inspiration for the future prosperity of fast-kinetic and efficient Zn-air batteries in a broad range of energy fields.

关键词： Zn-air batteries Carbon nanostructures Electrocatalysts Oxygen-catalytic catalysts ORR OER

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