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Unraveling atomistic and electronic origins of multiaxial magnetic anisotropy

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Science china(Physics,Mechanics & Astronomy) 2025年第2期68卷 175-182页

作者： Boyu Liu Xueyang Li Junsheng feng Changsong Xu Hongjun Xiang Key Laboratory of Computational Physical Sciences(Ministry of Education) Institute of Computational Physical SciencesState Key Laboratory of Surface Physics and Department of PhysicsFudan UniversityShanghai200433China Shanghai Qi Zhi Institute Shanghai200030China School of Physics and Material Engineering Hefei Normal UniversityHefei230601China

Multiaxial magnetic anisotropy(MA)refers to the phenomenon that multiple axes of the magnetic crystal correspond to different energy *** with the common uniaxial magnetic anisotropy,multiaxial MA facilitates novel forms of applications in ***,by combining the first-principles-based spin Hamiltonian and tight-binding(TB)method,we reveal the microscopic origins,instead of the common phenomenological understanding,of biaxial MA and triaxial *** the example system of NiO,it is found that the multiple minima result from the fourth-order and the sixth-order single ion interactions,while the difference between[110]and[110]directions originates from a second-order bond-dependent anisotropic pair interaction(i.e.,the so-called Gamma interaction).Moreover,through the application of a newly developed general spin dependent TB approach,it is revealed that the triaxial MA arises from the special spin-orbital entangled Hund term,which is different from the orbital-independent Hund term in the usual Slater Koster TB *** work thus not only leads to a thorough understanding of the multiaxial MA in NiO,but also establishes a methodology that can be widely used to explore the microscopic origins of MA in different magnets.

关键词： multiaxial magnetic anisotropy origin of multiaxial magnetic mnisotropy effective spin Hamiltonian tight-binding model antiferromagnetism

Optimizing battery deployment: Aging trajectory prediction enabling homogenous performance grouping

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Journal of Energy Chemistry 2025年第1期100卷 565-577页

作者： Shuquan Wang feng Gao Zhan Ma Hao Tian Yusen Zhang School of Control Science and Engineering Shandong UniversityJinan 250061ShandongChina Key Lab of Power System Intelligent Dispatch and Control of Ministry of Education Shandong UniversityJinan 250061ShandongChina

As battery deployments in electric vehicles and energy storage systems grow, ensuring homogeneous performance across units is crucial. We propose a multi-derivative imaging fusion(MDIF) model, employing advanced imaging and machine learning to predict battery aging trajectories from minimal initial data, thus facilitating effective performance grouping before deployment. Utilizing a derivative strategy and Gramian Angular Difference Field for dimensional enhancement, the MDIF model uncovers subtle predictive features from discharge curve data after only ten cycles. The architecture includes a parallel convolutional neural network with lateral connections to enhance feature integration and *** on a self-developed dataset, the model achieves an average root-mean-square error of 0.047 Ah and an average mean absolute percentage error of 1.60%, demonstrating high precision and *** robustness is further validated through transfer learning on two publicly available datasets, adapting with minimal retraining. This approach significantly reduces the testing cycles required, lowering both time and costs associated with battery testing. By enabling precise battery behavior predictions with limited data, the MDIF model optimizes battery utilization and deployment strategies, enhancing system efficiency and sustainability.

关键词： Lithium-ion battery Battery prognostics Fusion model Convolutional neural network Transfer learning

Precision-Engineered Construction of Proton-Conducting Metal-Organic Frameworks

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Nano-Micro Letters 2025年第4期17卷 230-274页

作者： Liyu Zhu Hongbin Yang Ting Xu feng Shen Chuanling Si State Key Laboratory of Biobased Fiber Manufacturing Technology Tianjin Key Laboratory of Pulp and PaperTianjin University of Science and Technology300457 TianjinPeople’s Republic of China State Key Laboratory of Pulp and Paper Engineering South China University of Technology510640 GuangzhouPeople’s Republic of China Agro-Environmenta Protection Institute Ministry of Agriculture and Rural Affairs300191 TianjinPeople’s Republic of China Robustnique Co.Ltd. Block CPhase IIPioneer ParkLanyuan Road300384 TianjinPeople’s Republic of China

Proton-conducting materials have attracted considerable interest because of their extensive application in energy storage and conversion *** them,metal-organic frameworks(MOFs)present tremendous development potential and possibilities for constructing novel advanced proton conductors due to their special advantages in crystallinity,designability,and *** particular,several special design strategies for the structure of MOFs have opened new doors for the advancement of MOF proton conductors,such as charged network construction,ligand functionalization,metal-center manipulation,defective engineering,guest molecule incorporation,and pore-space *** the implementation of these strategies,proton-conducting MOFs have developed significantly and profoundly within the last ***,in this review,we critically discuss and analyze the fundamental principles,design strategies,and implementation methods targeted at improving the proton conductivity of MOFs through representative ***,the structural features,the proton conduction mechanism and the behavior of MOFs are discussed thoroughly and *** endeavors are also proposed to address the challenges of proton-conducting MOFs in practical *** sincerely expect that this review will bring guidance and inspiration for the design of proton-conducting MOFs and further motivate the research enthusiasm for novel proton-conducting materials.

关键词： MOFs Proton conduction Porous materials Fuel cells

Ferulic acid alleviates long-term avermectin-induced damage to the spleen of carp and restores its inflammatory response and oxidative balance

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Journal of Environmental Sciences 2025年第5期151卷 616-626页

作者： Hanyu Wang Shenye feng Enzhuang Pan Xiaomeng Ji Mengyuan Zhou Shuai Zhang Baoshi Xu Huimiao feng Jilei Yin Zibo Dong Jiangsu Key Laboratory of Marine Bioresources and Environment Co-Innovation Center of Jiangsu Marine Bio-industry TechnologyJiangsu Marine Pharmaceutical Resources Development Engineering Research CenterJiangsu Key Laboratory of Marine Pharmaceutical Compound ScreeningCollege of PharmacyJiangsu Ocean UniversityLianyungang 222005China Department of Traditional chinese Medicine Jiangsu Union Technical Institute Lianyungang Branch institute of Traditional Chinese MedicineLianyungang 222006China

Extensive use of avermectin(AVM)in agriculture can seriously contaminate fish in *** acid(FA)is a strong antioxidant sourced from plants and is widely applied in food and medicine,but its protective function on the immunological damage caused by AVM is still *** this study,carp were chronically exposed to(1/1096 hr LC_(50))AVM for 30 day(s),with a dietary supplement of FA(400 mg/kg)to assess its effects on carp *** experimental groups(n=10)included:control,AVM-exposed(2.404μg/L),FA+AVM co-treated,and FA ***-term AVM exposure altered spleen tissue,reducing serum complement C3(p<0.01)and immunoglobulin M levels(p<0.001),and increasing proinflammatory tnf-α(p<0.001),il-6(p<0.001),il-1β(p<0.001),and inos mRNA levels,whilst down-regulating the anti-inflammatory tgf-β(p<0.05).Additionally,it disrupted the balance of oxidative stress indicators such asMDA(p<0.001),T-AOC,GSH,and CAT,leading to spleen tissue apoptosis(42.4%).However,the addition of FA reversed these conditions,elevated the anti-inflammatory factor,and improved spleen immune function following chronic exposure to AVMin ***,the ability to restore oxidative homeostasis in carp by adjusting the Nrf2/NQO-1 axis protected the health of spleen *** discovery also supports the development of fish feed for aquaculture.

关键词： Avermectin Ferulic acid Oxidative stress Inflammation response

Sky location of massive black hole binaries in the foreground of Galactic white dwarf binaries

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Science china(Physics,Mechanics & Astronomy) 2025年第1期68卷 93-104页

作者： Pan Guo Hong-Bo Jin Cong-feng Qiao Yue-Liang Wu The International Centre for Theoretical Physics Asia-Pacific University of Chinese Academy of SciencesBeijing 100190China Institute for Frontiers in Astronomy and Astrophysics Beijing Normal UniversityBeijing 102206China National Astronomical Observatories Chinese Academy of SciencesBeijing 100101China The School of Physical Sciences University of Chinese Academy of SciencesBeijing 100049China Institute of Theoretical Physics Chinese Academy of SciencesBeijing 100190China

For space-based gravitational wave(GW)detection,the main noise source for massive black hole binaries(MBHBs)is attributed to approximately 107 double white dwarf binaries in the *** a GW source,the amplitude of the detector response,recorded by a space-based gravitational wave detector,exhibits a modulation effect with a year period when observing the source from various orbital *** the adverse conditions mentioned above,where there is a strong foreground noise and annual modulation in the signals,we employed the wavelet transform and the strong-amplitude relevant orbital position search methods,which allows the weak MBHB sources to achieve higher locating *** detail,for two MBHB sources of lower intensity,the precision of luminosity distance,represented by the ratioΔD_(L)/D_(L) at the 95%confidence level,is enhanced by factors of∼*** angular resolutions,denoted byΔΩs,are enhanced by a factor of∼*** improvements increase the number of detectable GW sources,facilitate multi-messenger follow-up observations and provide constraints on the cosmological constant.

关键词： space-based gravitational wave detection gravitational waves massive black hole binaries

Mitochondrial transplantation:a promising strategy for the treatment of retinal degenerative diseases

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Neural Regeneration Research 2025年第12期20卷 3370-3387页

作者： Jing chi Bin Fan Yulin Li Qing Jiao Guang-Yu Li Department of Ophthalmology The Second Norman Bethune Hospital of Jilin UniversityChangchunJilin ProvinceChina

The retina,a crucial neural tissue,is responsible for transforming light signals into visual information,a process that necessitates a significant amount of ***,the primary powerhouses of the cell,play an integral role in retinal physiology by fulfilling the high-energy requirements of photoreceptors and secondary neurons through oxidative *** a healthy state,mitochondria ensure proper visual function by facilitating efficient conversion and transduction of visual ***,in retinal degenerative diseases,mitochondrial dysfunction significantly contributes to disease progression,involving a decline in membrane potential,the occurrence of DNA mutations,increased oxidative stress,and imbalances in quality-control *** abnormalities lead to an inadequate energy supply,the exacerbation of oxidative damage,and the activation of cell death pathways,ultimately resulting in neuronal injury and dysfunction in the *** transplantation has emerged as a promising strategy for addressing these *** procedure aims to restore metabolic activity and function in compromised cells through the introduction of healthy mitochondria,thereby enhancing the cellular energy production capacity and offering new strategies for the treatment of retinal degenerative *** mitochondrial transplantation presents operational and safety challenges that require further investigation,it has demonstrated potential for reviving the vitality of retinal *** review offers a comprehensive examination of the principles and techniques underlying mitochondrial transplantation and its prospects for application in retinal degenerative diseases,while also delving into the associated technical and safety challenges,thereby providing references and insights for future research and treatment.

关键词： age-related macular degeneration Leber’s hereditary optic neuropathy mitochondrial transfer mitochondrial transplantation retinal degenerative diseases

Research on the hazards of gas leakage and explosion in a full-scale residential building

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Defence Technology(防务技术) 2025年第1期43卷 168-181页

作者： Chengjun Yue Li Chen Zhan Li Bin feng Ruizhi Xu Engineering Research Center of Safety and Protection of Explosion&Impact of Ministry of Education Southeast UniversityNanjing 211189China

The gas explosion in residential building has always been a highly concerned *** in homogeneous mixtures have been extensively ***,mixtures are often inhomogeneous in the practical scenarios due to the differences in the densities of methane and *** order to investigate the effects of gas explosions in inhomogeneous mixtures,experimental studies involving gas leakage and explosion are conducted in a full-scale residential building to reproduce the process of gas *** fitting the dimensionless buoyancy as a function of dimensionless height and dimensionless time,a distribution model of gas in large-scale spaces is established,and the mechanism of inhomogeneous distribution of methane is also be ***,the stratified reconstruction method(SRM)is introduced for efficiently setting up inhomogeneous concentration fields in *** simulation results highlight that for the internal overpressure,the distribution of methane has no effect on the first overpressure peak(ΔP1),while it significantly influences the subsequent overpressure peak(ΔP2),and the maximum difference between the overpressure of homogeneous and inhomogeneous distribution is174.3%.Moreover,the initial concentration distribution also has a certain impact on the external overpressure.

关键词： Methane distribution Inhomogeneous mixture Gradient layer Gas explosion Explosive simulation

Seismic design of variable cross-section damped steel support frame for post equipment

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Earthquake Engineering and Engineering Vibration 2025年第1期24卷 155-167页

作者： Yang Zhenyu Ma Yuhong Zhao Guifeng feng Zhiwei Fu Mingyang Earthquake Engineering Research&Test Center Guangzhou UniversityGuangzhou 510405China School of Civil Engineering Guangzhou UniversityGuangzhou 510620China Guangdong Provincial Key Laboratory of Earthquake Engineering and Applied Technology Guangzhou 510405China

High-voltage electrical post equipment is generally installed on steel supports,which amplifies the seismic inputs and degrades the seismic performance of *** study proposed a variable cross-section damped steel support frame(VCDFS)with viscous dampers to reduce seismic responses of both tall and low-rise electrical *** VCDFS contains a trapezoidal damper layer to generate rocking motions,enabling the diagonal viscous dampers to dissipate seismic inputs.A theoretical model of post equipment with VCDFS is established,and an optimal design procedure is *** analysis shows that the remaining static stiffness ratio λ_(k) is the key parameter that determines the effectiveness of the *** VCDFS reduces the average displacement and stress response of a post insulator by 39.4%and 44.6%,respectively,together with a significant decrease in the dynamic amplification ***,it is recommended to use the VCDFS instead of the conventional latticed-steel frame in earthquake zones.

关键词： electrical post equipment steel support frame passive control seismic performance upgrading

Characteristics of catalytic destruction of dichloromethane and ethyl acetate mixture over HxPO4-RuOx/CeO2 catalyst

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Journal of Environmental Sciences 2025年第2期148卷 336-349页

作者： Jiawen Chen Qingjie Meng feng Bi Jingkun Chen Xiaole Weng Zhongbiao Wu Key Laboratory of Environment Remediation and Ecological Health Ministry of EducationCollege of Environmental and Resource SciencesZhejiang UniversityHangzhou 310058China School of Civil&Environmental Engineering and Geography Science Ningbo UniversityNingbo 315211China ZJU-Hangzhou Global Scientific and Technological Innovation Center Hangzhou 311200China Zhejiang Provincial Engineering Research Centre of Industrial Boiler&Furnace Flue Gas Pollution Control Hangzhou 310058China

Catalytic destruction is an ascendant technology for the abatement of volatile organic compounds(VOCs)originating fromsolvent-based industrial *** varied composition tends to influence each VOC’s catalytic behavior in the reaction *** investigated the catalytic destruction of multi-component VOCs including dichloromethane(DCM)and ethyl acetate(EA),as representatives from pharmaceutical waste gases,over co-supported HxPO_(4)-RuOx/CeO_(2) catalyst.A mutual inhibitory effect relating to concentrations because of competitive adsorption was verified in the binary VOCs oxidation and EA posed a more negative effect on DCM oxidation owing to EA’s superior adsorption *** adsorption of EA on acidic sites(HxPO_(4)/CeO_(2))promoted DCM activation on basic sites(O^(2−))and the dominating EA oxidation blocked DCM’s access to oxidation centers(RuOx/CeO_(2)),resulting in boosted monochloromethane yield and increased chlorine deposition for DCM *** impaired redox ability of Ru species owing to chlorine deposition in turn jeopardized deep oxidation of EA and its by-products,leading to increased gaseous by-products such as acetic acid originating fromEA ***,DCM at low concentration slightly promoted EA conversion at low temperatures with or without water,consistent with the enhanced EA adsorption in co-adsorption *** was mainly due to that DCM impeded the shielding effect of hydrolysate deposition from rapid EA hydrolysis depending on the decreased ***,water benefited EA hydrolysis but decreased CO_(2) selectivity while the generated water derived from EA was likely to affect DCM *** work may provide theoretical guidance for the promotion of applied catalysts toward industrial applications.

关键词： Catalytic destruction Multi-component VOCs Mixture effect Interaction mechanism