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Reactive molecular dynamics insight into the thermal decomposition mechanism of 2,6-Bis(picrylamino)-3,5-dinitropyridine

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Defence Technology（防务技术） 2024年第3期33卷 134-146页

作者： Jianbo Fu Hui Ren Xinzhou wu Yongjin Chen Mi zhang Yazhi cheng State Key Laboratory of Explosion Science and Technology Beijing Institute of TechnologyBeijing 100081China

2,6-bis(picrylamino)-3,5-dinitropyridine(PYX)has excellent thermostability,which makes its thermal decomposition mechanism receive much *** this paper,the mechanism of PYX thermal decomposition was investigated thoroughly by the ReaxFF-lg force field combined with DFT-B3LYP(6-311++G)*** detailed decomposition mechanism,small-molecule product evolution,and cluster evolution of PYX were mainly *** the initial stage of decomposition,the intramolecular hydrogen transfer reaction and the formation of dimerized clusters are earlier than the denitration *** the progress of the reaction,one side of the bitter amino group is removed from the pyridine ring,and then the pyridine ring is *** final products produced in the thermal decomposition process are CO_(2),H_(2)O,N_(2),and H_(2).Among them,H_(2)O has the earliest generation time,and the reaction rate constant(k_(3))is the *** clusters are formed during the decomposition of PYX,and the formation,aggregation,and decomposition of these clusters are strongly affected by *** low temperatures(2500 K-2750 K),many clusters are *** high temperatures(2750 K-3250 K),the clusters aggregate to form larger *** 3500 K,the large clusters decompose and become *** the late stage of the reaction,H and N in the clusters escaped almost entirely,but more O was trapped in the clusters,which affected the auto-oxidation process of ***'s initial decomposition activation energy(E_(a))was calculated to be 126.58 kJ/*** work contributes to a theoretical understanding of PYX's entire thermal decomposition process.

关键词： PYX Thermal decomposition ReaxFF-lg MD simulations Excellent thermostable explosives

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Experimental study on secondary air mixing along the bed height in a circulating fluidized bed with a multitracer-gas method

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Chinese Journal of Chemical Engineering 2024年第6期70卷 54-62页

作者： Qingyu zhang Leming cheng Kun Li Qixun Kang Qiang Guo Chaogang wu Institute for Thermal Power Engineering State Key Laboratory of Clean Energy UtilizationZhejiang UniversityHangzhou 310027China Dongfang Boiler Group Co.Ltd. Zigong 643001China

A multitracer-gas method was proposed to study the secondary air(SA)mixing along the bed height in a circulating fluidized bed(CFB)using carbon monoxide(CO),oxygen(O_(2)),and carbon dioxide(CO_(2))as tracer *** were carried out on a cold CFB test rig with a cross-section of 0.42 m×0.73 m and a height of 5.50 *** effects of superficial velocity,SA ratio,bed inventory,and particle diameter on the SA mixing were *** results indicate that there are some differences in the measurement results obtained using different tracer gases,wherein the deviation between CO and CO_(2) ranges from 42%to 66%and that between O_(2) and CO_(2) ranges from 45%to 71%in the lower part of the fluidized ***,these differences became less pronounced as the bed height ***,the high solid concentration and fine particle diameter in the CFB may weaken the *** measurement results of different tracer gases show the same trends under the variation of operating *** superficial velocity and SA ratio and decreasing particle diameter result in better mixing of the *** effect of bed inventory on SA mixing is not monotonic.

关键词： Circulating fluidized bed Secondary air injection Gas mixing Multitracer-gas method

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Transcatheter arterial chemoembolization after percutaneous microwave ablation and portal vein embolization for advanced hepatocellular carcinoma

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Hepatobiliary & Pancreatic Diseases International 2023年第2期22卷 213-216页

作者： Jian cheng De-Fei Hong cheng-wu zhang Xiao-Ming Fan Zu-Yan Luo Wei-Feng Yao Li-Ming Jin General Surgery Cancer CenterDepartment of Hepatobiliary&Pancreatic Surgery and Minimally Invasive SurgeryZhejiang Provincial People’s HospitalAffiliated People’s Hospital of Hangzhou Medical CollegeHangzhou 310014China Department of General Surgery Sir Run Run Shaw HospitalZhejiang University School of MedicineHangzhou 310020China

To the Editor: Associating liver partition and portal vein ligation for staged hepatectomy(ALPPS) promotes the future liver remnant(FLR) rapid proliferation in the short term, which in turn provides an opportunity for... 详细信息

关键词： hepatocellular liver microwave

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Is laparoscopic radical cholecystectomy an effective and safe approach for advanced gallbladder cancer?

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Hepatobiliary & Pancreatic Diseases International 2020年第3期19卷 203-204页

作者： Li-Ming Jin Yu-Hua zhang cheng-wu zhang Wei-Ding wu Jia wu Chang-Wei Dou Fang-Qiang Wei Zhi-Fei Wang Zhi-Ming Hu Shu-Sen Zheng Division of Hepatobiliary Pancreatic Surgery First Affiliated HospitalZhejiang University School of MedicineHangzhou 310003China Division of Hepatobiliary and Pancreatic Surgery Zhejiang Provincial People’s HospitalAffiliated People’s Hospital of Hangzhou Medical CollegeHangzhou 310014China Department of Hepatobiliary and Pancreatic Surgery Department of Liver TransplantationShulan(Hangzhou)HospitalZhejiang Shuren University School of MedicineHangzhou 310022China

Although laparoscopy has been widely used in the surgical field and is even considered the first-line to diagnose various diseases,laparoscopic radical cholecystectomy(LRC)for gallbladder cancer(GBC)has always been relatively *** lymphadenectomy,complicated liver resection,specific biological behavior of GBC cells,and chimney and aerosol effects from the pneumoperitoneum are the previously misunderstood areas in laparoscopic surgery[1].Initially,laparoscopic approach was used for intra-abdominal GBC exploration to determine the presence of peritoneal metastasis,intraoperative staging,and palliative *** the advancement of laparoscopic surgery,laparoscopic liver resection,laparoscopic pancreaticoduodenectomy,and laparoscopic radical gastrectomy have been routinely performed in several medical *** et al.[2]recently demonstrated that laparoscopic technique is feasible for ***,the feasibility of LRC depends on the following factors.

关键词： laparoscopic gallbladder routine

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Single-structure 3-axis Lorentz force magnetometer based on an AlN-on-Si MEMS resonator

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Microsystems & Nanoengineering 2024年第3期10卷 75-86页

作者： cheng Tu Xu-heng Ou-Yang Ying-jie wu Xiao-sheng zhang School of Integrated Circuit Science and Engineering University of Electronic Science and Technology of ChinaChengdu 611731China

This work presents a single-structure 3-axis Lorentz force magnetometer(LFM)based on an AlN-on-Si MEMS *** operation of the proposed LFM relies on the flexible manipulation of applied excitation currents in different directions and frequencies,enabling the effective actuation of two mechanical vibration modes in a single device for magnetic field measurements in three ***,the excited out-of-plane drum-like mode at 277 kHz is used for measuring the x-and y-axis magnetic fields,while the in-plane square-extensional mode at 5.4 MHz is used for measuring the z-axis magnetic *** different configurations of applied excitation currents ensure good crossinterference immunity among the three *** to conventional capacitive LFMs,the proposed piezoelectric LFM utilizes strong electromechanical coupling from the AlN layer,which allows it to operate at ambient pressure with a high *** understand and analyze the measured results,a novel equivalent circuit model for the proposed LFM is also reported in this work,which serves to separate the effect of Lorentz force from the unwanted capacitive *** demonstrated 3-axis LFM exhibits measured magnetic responsivities of 1.74 ppm/mT,1.83 ppm/mT and 6.75 ppm/mT in the x-,y-and z-axes,respectively,which are comparable to their capacitive counterparts.

关键词： resonator Lorentz structure

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Dendrimer-induced synthesis of porous organosilica capsules for enzyme encapsulation

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Frontiers of Chemical Science and Engineering 2024年第4期18卷 41-48页

作者： Ziyi Chu Boyu zhang Zhenhua wu Jiaxu zhang Yiran cheng Xueying Wang Jiafu Shi Zhongyi Jiang School of Environmental Science&Engineering Tianjin UniversityTianjin 300072China Collaborative Innovation Center of Chemical Science and Engineering Tianjin 300072China State Key Laboratory of Biochemical Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China Key Laboratory for Green Chemical Technology of Ministry of Education School of Chemical Engineering and TechnologyTianjin UniversityTianjin 300072China

Organic matter-induced mineralization is a green and versatile method for synthesizing hybrid nanostructured materials,where the material properties are mainly influenced by the species of natural biomolecules,linear synthetic polymer,or small molecules,limiting their ***,we adopted dendrimer poly(amidoamine)(PAMAM)as the inducer to synthesize organosilica-PAMAM network(OSPN)capsules for mannose isomerase(MIase)encapsulation based on a hard-templating *** structure of OSPN capsules can be precisely regulated by adjusting the molecular weight and concentration of PAMAM,thereby demonstrating a substantial impact on the kinetic behavior of the MIase@OSPN *** MIase@OSPN system was used for catalytic production of mannose from Dfructose.A mannose yield of 22.24% was obtained,which is higher than that of MIase in organosilica network capsules and similar to that of the free *** overall catalytic efficiency(kcat/Km)of the MIase@OSPN system for the substrate D-fructose was up to 0.556 s^(-1)·mmol^(-1)·***,the MIase@OSPN system showed excellent stability and recyclability,maintaining more than 50% of the yield even after 12 cycles.

关键词： enzyme immobilization enzyme catalysis organosilica networks capsules sugar biosynthesis

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Identification of key genes regulating the synthesis of quercetin derivatives in Rosa roxburghii through integrated transcriptomics and metabolomics

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Journal of Integrative Agriculture 2024年第3期23卷 876-887页

作者： Liyao Su Min wu Tian zhang Yan Zhong Zongming(Max) cheng State Key Laboratory of Crop Genetics and Germplasm Enhancement College of HorticultureNanjing Agricultural UniversityNanjing210095China

Rosa roxburghii fruit is rich in flavonoids, but little is known about their biosynthetic pathways. In this study, we employed transcriptomics and metabolomics to study changes related to the flavonoids at five different stages of R. roxburghii fruit development. Flavonoids and the genes related to their biosynthesis were found to undergo significant changes in abundance across different developmental stages, and numerous quercetin derivatives were identified. We found three gene expression modules that were significantly associated with the abundances of the different flavonoids in R. roxburghii and identified three structural UDP-glycosyltransferase genes directly involved in the synthesis of quercetin derivatives within these modules. In addition, we found that RrBEH4, RrLBD1 and RrPIF8could significantly increase the expression of downstream quercetin derivative biosynthesis genes. Taken together,these results provide new insights into the metabolism of flavonoids and the accumulation of quercetin derivatives in R. roxburghii.

关键词： Rosa roxburghii quercetin derivatives weighted gene co-expression network analysis transcription factor transcriptome metabolome

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Simultaneous transcatheter arterial chemoembolization and portal vein embolization for patients with large hepatocellular carcinoma before major hepatectomy

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World Journal of Gastroenterology 2020年第30期26卷 4489-4500页

作者： cheng-wu zhang Chang-Wei Dou Xin-Long zhang Xi-Qiang Liu Dong-Shen Huang Zhi-Ming Hu Jie Liu Department of Hepatopancreatobiliary Surgery and Minimally Invasive Surgery Zhejiang Provincial People’s HospitalPeople’s Hospital of Hangzhou Medical CollegeHangzhou 310014Zhejiang ProvinceChina Department of General Surgery Aksu Area First HospitalAksu 843000Xinjiang Uygur Autonomous RegionChina

BACKGROUND Sequential transarterial chemoembolization(TACE)and portal vein embolization(PVE)are associated with long time interval that can allow tumor growth and nullify treatments'*** To evaluate the effect of simultaneous TACE and PVE for patients with large hepatocellular carcinoma(HCC)prior to elective major *** Fifty-one patients with large HCC who underwent PVE combined with or without TACE prior to hepatectomy were included in this study,with 13 patients in the simultaneous TACE+PVE group,17 patients in the sequential TACE+PVE group,and 21 patients in the PVE-only *** outcomes of the procedures were compared and *** All patients underwent *** mean interval from embolization to surgery,the kinetic growth rate of the future liver remnant(FLR),the degree of tumor size reduction,and complete tumor necrosis were significantly better in the simultaneous TACE+PVE group than in the other *** the patients in the simultaneous TACE+PVE group had a higher transaminase levels after PVE and TACE,they recovered to comparable levels with the other two groups before *** intraoperative course and the complication and mortality rates were similar among the three *** overall survival and disease-free survival were higher in the simultaneous TACE+PVE group than in the other two *** Simultaneous TACE and PVE is a safe and effective approach to increase FLR volume for patients with large HCC before major hepatectomy.

关键词： Transcatheter arterial chemoembolization Portal vein embolization Major hepatectomy Hepatocellular carcinoma Future liver remnant

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Assessment of natural and anthropogenic impacts on terrestrial water storage in the Loess Plateau based on different types of GRACE/GRACE-FO solutions

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Journal of Mountain Science 2024年第7期21卷 2173-2192页

作者： zhang cheng CHEN Peng ZHU chengchang LU Jierui zhang Yuchen YANG Xinyue wu Mengyan College of Geomatics Xi'an University of Science and TechnologyXi'an 710054China State Key Laboratory of Geodesy and Earth’s Dynamics Innovation Academy for Precision Measurement Science and TechnologyChinese Academy of SciencesWuhan 430077China

Changes in water resource storage are inevitable due to climate change and human activities,thus understanding alterations in water storage within a specific region is imperative for the planning and management of water *** from the Gravity Recovery and Climate Experiment(GRACE)satellite mission are extensively employed to analyze large-scale total terrestrial water storage anomalies(TWSA).In this study,we derived a more reliable TWSA using different types of GRACE gravity models,which served as the basis for evaluating spatial and temporal variations in total terrestrial water storage and its hydrological components(soil moisture and groundwater)across the Loess ***,we analyzed the impact of natural and anthropogenic influences on water storage in the Loess Plateau,categorizing them into primary and secondary influences,utilizing data on climate and human *** findings revealed a declining trend in the overall TWSA of the Loess Plateau,with a rate of decrease at-0.65±0.05 cm/yr from 2003 to 2020(P<0.01).As the direct factors affecting TWSA,soil moisture dominated the change of TWSA before 2009,and groundwater dominated the change of TWSA after ***,there was variability in the changes of TWSA in the Loess *** in-depth studies showed that soil moisture changes in the study area were primarily driven by evapotranspiration and temperature,with precipitation and vegetation cover status playing a secondary *** activities had a secondary effect on soil moisture in some *** change and agricultural development were major factors in altering groundwater storage in the study *** than that,groundwater was influenced by natural factors to a limited *** findings provided valuable insights for local governments to implement proactive water management policies.

关键词： GRACE Terrestrial water storage Human activity Loess Plateau

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Advances in methane emissions from agricultural sources:Part *** and mitigation

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Journal of Environmental Sciences 2024年第6期140卷 279-291页

作者： Xiaokun wu Ying zhang Yinghui Han Yagang zhang Yuhang zhang Xiaodan cheng Pei Zhong Xue Yuan Yuanxun zhang Zhengqiang Li State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources North China Electric Power UniversityBeijing 102206China Hebei Key Laboratory of Physics and Energy Technology North China Electric Power UniversityBaoding 071003China College of Resources and Environment University of Chinese Academy of SciencesBeijing 101408China Interdisciplinary Mathematics Institute University of South CarolinaColumbiaSC 29208United States Aerospace Information Research Institute Chinese Academy of SciencesBeijing 100094China

Methane is one of the major greenhouse gases(GHGs)and agriculture is recognized as its primary *** accounting is a prerequisite for developing effective agriculture mitigation *** this review,methane accounting methods and research status for various agricultural emission source including rice fields,animal enteric fermentation and livestock and poultry manure management were overview,and the influencing factors of each emission source were analyzed and *** the same time,it analyzes the different research efforts involving agricultural methane accounting and makes recommendations based on the actual ***,mitigation strategies based on accounting results and actual situation are *** review aims to provide basic data and reference for agriculture-oriented countries and regions to actively participate in climate action and carry out effective methane emission mitigation.

关键词： Methane emission Agricultural sources Accounting methodology Mitigation Emission influencing factors

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