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Dielectric nanocomposites with superb high-temperature capacitive performance based on high intrinsic dielectric constant polymer

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Nano Research 2024年第9期17卷 8504-8512页

作者： Ding Ai Yuan Chang Haoliang Liu chenglong Wu Yao Zhou Yuting Han Hao Yu bing Xiao Yonghong cheng Guanglei Wu Zirui Jia State Key Laboratory of Electrical Insulation and Power Equipment School of Electrical EngineeringXi’an Jiaotong UniversityXi’an 710049China Institute of Materials for Energy and Environment State Key Laboratory of Bio-Fibers and Eco-TextilesCollege of Materials Science and EngineeringQingdao UniversityQingdao 266071China

Advancements in power electronics necessitate dielectric polymer films capable of operating at high temperatures and possessing high energy *** significant strides have been achieved by integrating inorganic fillers into high-temperature polymer matrices,the inherently low dielectric constants of these matrices have tempered the magnitude of *** this work,we report an innovative nanocomposite based on sulfonylated polyimide(SPI),distinguished by the incorporation of sulfonyl groups within the SPI backbone and the inclusion of wide bandgap hafnium dioxide(HfO_(2))*** nanocomposite has demonstrated notable enhancements in thermal stability,dielectric properties,and capacitive performance at elevated *** simulations at both molecular and mesoscopic levels have elucidated the mechanisms behind these improvements,which could be attributed to confined segmental motion,an optimized electronic band structure,and a diminished incidence of dielectric breakdown ascribed to the presence of sulfonyl ***,the SPI-HfO_(2)nanocomposite demonstrates a high charge-discharge efficiency of 95.7%at an elevated temperature of 150℃and an applied electric field of 200 MV/***,it achieves a maximum discharged energy density of 2.71 J/cm^(3),signalling its substantial potential for energy storage applications under extreme conditions.

关键词： dielectric polymer nanocomposites high-temperature high dielectric constant sulfonyl groups energy storage performance

Fast fixed-time three-dimensional terminal guidance with non-concave trajectory constraint

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Chinese Journal of Aeronautics 2024年第3期37卷 208-218页

作者： Youmin GONG Yanning GUO Yueyong lyu Dongyu LI Guangfu MA Department of Control Science and Engineering Harbin Institute of TechnologyHarbin 150001China School of Cyber Science and Technology Beihang UniversityBeijing 100191China

Focusing on the non-concave trajectory constraint,a sliding-mode-based nonsingular feedback fast fixed-time three-dimensional terminal guidance of rotor unmanned aerial vehicle landing,planetary landing and spacecraft rendezvous and docking terminal phase with external disturbance is investigated in this ***,a fixed-time observer based on real-time differentiator is developed to compensate for the external disturbance,whose estimation error can converge to zero after a time independent of the initial ***,a sliding surface ensuring fixed-time convergence is *** sliding surface can guarantee that the vehicle achieves a non-concave trajectory,which is better for avoiding collision and maintaining the visibility of the landing site or docking ***,the nonsingular guidance ensuring the fixed-time convergence of the sliding surface is proposed,which is continuous and chatter *** last,three numerical simulations of Mars landing are performed to validate the effectiveness and correctness of the designed scheme.

关键词： Three-dimensional Terminal guidance Non-concave trajectory constraint Fast fixed-time control Sliding mode control

Polymer-encapsulated metal complex catalysts:An emerging and efficient platform for electrochemical CO_(2) reduction

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Journal of Materials Science & Technology 2024年第5期172卷 33-50页

作者： Yingshuo Liu Shuaishuai lyu Fuli Wen Weixuan Nie Shuqing Wang Sinopec Research Institute of Petroleum Processing Co. Ltd.Beijing 100083China School of Engineering Westlake UniversityHangzhou 310024China

Over the past decade,electrocatalytic reduction of CO_(2)has gained substantial ***,hardly any of the previous reviews have focused on the systematic discussion of polymer-molecular catalyst composites as an emerging system for the electrochemical transformation of CO_(2)to value-added *** this review,we first give a brief overview of the general features of solid-state and molecular catalysts,and then advance the discussion to polymer-catalyst composite systems,with particular emphasis on polymer-encapsulated molecular catalysts,where the coordination environment surrounding molecular catalysts can be modified via polymer encapsulation to promote the overall performance of CO_(2)*** elucidation of the possible reaction mechanisms of this emerging electrocat-alytic system along with proposed optimization strategies is also summarized and discussed based on recently published reports,followed by the challenges and prospects of their industrial applications at the end of this *** this review,we hope the audience can gain a comprehensive understanding of the electrocatalytic mechanism of the coordinating polymers and valuable insights into engineering the microenvironment surrounding the metal complexes for potential future research directions.

关键词： Polymer-molecular catalyst composite Polymer encapsulation Coordination environment CO_(2)electrocatalysis Electrocatalytic mechanism

Enhanced Fenton-like process over Cu/L(+)-ascorbic acid co-doping mesoporous silica for toxicity reduction of emerging contaminants

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Frontiers of Environmental Science & Engineering 2024年第4期18卷 49-60页

作者： Yuhang Liu Wenxuan Deng Xiaojun Wu Chun Hu Lai lyu Key Laboratory for Water Quality and Conservation of the Pearl River Delta(Ministry of Education) Institute of Environmental Research at Greater BayGuangzhou UniversityGuangzhou 510006China

Effective removal of emerging contaminants(ECs)to minimize their impacts on human health and the natural environment is a global *** the removal of ECs in water,we fabricated a seaweed spherical microsphere catalyst with Cu cation-πstructures by in situ doping of Cu species and ascorbic acid in mesoporous silica(Cu-C-MSNs)via a hydrothermal *** results indicate that bisphenol A(BPA)is substantially degraded within 5 min under natural conditions,with its biological toxicity considerably ***,industrial wastewater could also be effectively purified by Cu-C-MSNs/H_(2)O_(2) *** presence of metal sites and the complexation of ECs via cation-πinteraction andπ-πstacking on the catalyst surface were directly responsible for the polarization distribution of electrons,thus activating H_(2)O_(2) and dissolved oxygen(DO).The removal of contaminants could be attributed primarily to 1)the activation of H_(2)O_(2) into ^(·)OH to attack the contaminants and 2)self-cleavage because of the transfer of electrons from the contaminants to the *** study provides an innovative solution for the effective treatment of ECs and has positive implications for easing global environmental crises.

关键词： Cation-πstructures Polarization electric field Fenton-like process Contaminants cleavage

Network Evolution Analysis of Vehicle Road-Driving Behavior Strategies and Design of Information Guidance Algorithm

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Journal of Social Computing 2024年第1期5卷 58-87页

作者： Tong lyu Lefeng Shi Weijun He College of Economics and Management China Three Gorges UniversityYichang 443002China National Center for Applied Mathematics in Chongqing Chongqing Normal UniversityChongqing 401331China

By analyzing the influence of time and safety factors on the behavior strategies of vehicles on the road,a network game evolution model between drivers that considers the behavior strategies of the driving vehicle itself and its neighbors is constructed,and the competition relationship between different types of cars is *** influence of the proportion of driving vehicle types on the potential risk of the road is also *** paper presents a guidance algorithm for vehicle dynamic behavior preference *** correctness of the algorithm is verified by an *** shows:The choice of behavior strategies,such as speeding and lane changing,is related to the expected benefits of time,safety,and neighboring vehicle strategies,and the critical value of payable benefits is *** higher the proportion of aggressive vehicles on the road,the greater the potential risk on the *** there is a vehicle in the adjacent lane of the driving vehicle will affect the type of driving *** guidance helps to stabilize the state of vehicles on the road,and the policy transition probability also helps stabilize the form of vehicles cars on the ***,information guidance has a more significant impact on the transition of vehicle ***,the guidance strategy of managers is given when the road is smooth and congested.

关键词： user portrait information guidance network game risk appetite

Investigation of Mode Changing,Pulse Nulling and Subpulse Drifting Properties in the Asymmetric Conal Triple Radio Pulsar B2319+60

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Research in Astronomy and Astrophysics 2022年第11期22卷 147-160页

作者： Jian-Ling Chen Zhi-Gang Wen Hong-Guang Wang Na Wang Rai Yuen Vishal Gajjar Jian-Ping Yuan Zhen Wang Wen-Ming Yan Jin-Peng Wang cheng-bing lyu Hui Wang Xue-Feng Duan Department of Physics and Electronic Engineering Yuncheng UniversityYuncheng 044000China Xinjiang Astronomical Observatory Chinese Academy of SciencesUrumqi 830011China Key Laboratory of Radio Astronomy Chinese Academy of SciencesNanjing 210008China Key Laboratory of Microwave Technology Urumqi 830011China Guizhou Provincial Key Laboratory of Radio Astronomy and Data Processing Guiyang 550001China Center for Astrophysics Guangzhou UniversityGuangzhou 510006China Space Science Laboratory University of CaliforniaBerkeley 94710United States of America School of Physical Science and Technology Xinjiang UniversityUrumqi 830046China

We report on a detailed analysis of the mode changing,nulling and subpulse drifting behavior of the conal triple pulsar B2319+60 at 1.5 GHz observed with the Nanshan 25 m radio *** pulsar’s profile can be interpreted as resulting from a sightline traverse which cuts across an outer cone and tangentially grazes an inner *** 30 per cent of nulls are found to create alternating bunches of nulls and emission in a quasi-periodic manner with an averaged fluctuation rate of about four rotation periods(P_(1)).The presence of two distinct drift modes(A and ABN)plus a phase-stationary non-drift emission mode(B)is confirmed,and each corresponds to a different pulse *** mode A is dominated by a phase modulation in the trailing component with a circulation time of around 7P_(1).In addition to a 3P_(1)phase modulation in the leading component,mode ABN presents an amplitude modulation in the leading and trailing components with a period of around 40P_(1).The emission region and geometry remain constant during mode *** diversity seen in the individual pulse behavior of the pulsar B2319+60 provides a unique window into the emission physics.

关键词： (stars:)pulsars:general (stars:)pulsars:individual(PSR B2319+60) stars:neutron

2D all-organic perovskites refine flexible electronics

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Science China Materials 2024年第7期67卷 2365-2366页

作者： Wei Zhou bing Chen College of Electronic and Optical Engineering and College of Flexible Electronics(Future Technology) Nanjing University of Posts and TelecommunicationsNanjing 210023China

Recent years have witnessed a paradigm shift with the advent of perovskites,a class of materials with a distinct CaTiO_(3)-type crystalline structure that show remarkable promise across a wide array of applications,including photovoltaics,photodetectors,lighting,lasers,and so *** them,the development of two-dimensional(2D)perovskites has garnered significant attention due to their tunable structures(mainly Dion-Jacobson and Ruddlesden-Popper structures)and enhanced stability in comparison with their 3D counterparts[1].Amidst the burgeoning research on perovskites,on the other side,all-organic perovskites stand out as a particularly intriguing subset[2].Unlike traditional perovskites that typically comprise all-inorganic(e.g.,CsPbBr_(3))or organic-inorganic hybrid components(e.g.,(PEA)_(2)PbI_(4)),all-organic perovskites are composed entirely of carbon-or nitrogen-based molecules.

关键词： perovskite inorganic entirely

Review on the recent progress of nearly zero energy building frontiers in China

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Science China(Technological Sciences) 2024年第9期67卷 2620-2636页

作者： lyu YanJie XU Wei ZHANG ShiCong SUN DeYu HOU YueBin China Academy of Building Research Beijing 100013China

Energy efficiency improvement in Chinese construction has progressed rapidly over the past two *** zero energy buildings(NZEBs),as an integrated solution for energy-efficient construction,have gained significant attention during China's 13th Five-Year Plan period,with continuous maturation of the technical *** this study,a research framework built upon the accomplishments of China's National Key Research and Development Program is developed,and an in-depth analysis of the most cutting-edge research is provided by thoroughly reviewing the work conducted *** NZEB in China has been categorized into three stages based on the characteristics of technological development:(1)definition and standards,(2)demonstration and promotion,and(3)cross-domain *** study discerns four noteworthy development trends by examining comprehensive data spanning the last decade from 100 NZEB and zero energy ***,a comprehensive analysis of essential technology advancements in line with these identified trends is *** issues and challenges arising from the increased application of renewable energy in the context of China's carbon peak and carbon neutrality goals have also been ***,based on this analysis,the challenges and corresponding suggestions for future research directions were proposed to help guide future studies exploring emerging trends in the NZEB field.

关键词： nearly zero energy building energy efficiency load flexibility heat pump renewable energy

Transfer learning framework for multi-scale crack type classification with sparse microseismic networks

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International Journal of Mining Science and Technology 2024年第2期34卷 167-178页

作者： Arnold Yuxuan Xie bing QLi Department of Civil and Environmental Engineering Western UniversityLondon N6A 3K7Canada

Rock fracture mechanisms can be inferred from moment tensors(MT)inverted from microseismic ***,MT can only be inverted for events whose waveforms are acquired across a network of *** is limiting for underground mines where the microseismic stations often lack azimuthal ***,there is a need for a method to invert fracture mechanisms using waveforms acquired by a sparse microseismic ***,we present a novel,multi-scale framework to classify whether a rock crack contracts or dilates based on a single *** framework consists of a deep learning model that is initially trained on 2400000+manually labelled field-scale seismic and microseismic waveforms acquired across 692 *** learning is then applied to fine-tune the model on 300000+MT-labelled labscale acoustic emission waveforms from 39 individual experiments instrumented with different sensor layouts,loading,and rock types in *** optimal model achieves over 86%F-score on unseen waveforms at both the lab-and *** model outperforms existing empirical methods in classification of rock fracture mechanisms monitored by a sparse microseismic *** facilitates rapid assessment of,and early warning against,various rock engineering hazard such as induced earthquakes and rock bursts.

关键词： Multi-scale Fracture processes Microseismic Acoustic emission Source mechanism Deep learning