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Manipulating the Phase Transition Behavior of Dual Temperature-Responsive Block Copolymers by Adjusting Composition and Sequence

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Chinese Journal of Polymer Science 2024年第2期42卷 176-187,I0006页

作者： Zhi Zou xiang Xu Hai-Tao Zhao Jian-Nan cheng Wei-Wei He Li-Fen Zhang zhen-Ping cheng Suzhou key Laboratory of Macromolecular Design and Precision Synthesis Jiangsu Key Laboratory of Advanced Functional Polymer Design and ApplicationState and Local Joint Engineering Laboratory for Novel Functional Polymeric MaterialsCollege of ChemistryChemical Engineering and Materials ScienceSoochow UniversitySuzhou215123China State Key Laboratory of Radiation Medicine and Protection School for Radiological and Interdisciplinary Sciences(RAD-X)and Collaborative Innovation Center of Radiation Medicine of JiangsuSoochow UniversitySuzhou215123China

Temperature-responsive polymers have garnered significant attention due to their ability to respond to external *** this work,dual temperature-responsive block copolymers are synthesized via reversible addition-fragmentation chain transfer polymerization(RAFT)polymerization utilizing zwitterionic monomer methacryloyl ethyl sulfobetaine(SBMA) and N-isopropyl acrylamide(NIPAAm) as *** thermal responsive behaviors can be easily modulated by incorporating additional hydrophobic monomer benzyl acrylate(BN) or hydrophilic monomer acrylic acid(AA),adjusting concentration or pH,or varying the degree of polymerization of the block chain *** cloud points of the copolymers are determined by UV-Vis spectrophotometry,and these copolymers exhibit both controlled upper and lower critical solu bility temperatures(LCST and UCST) in aqueous *** study analyzes and summarizes the influencing factors of dual temperature responsive block copolymers by exploring the effects of various conditions on the phase transition temperature of temperature-sensitive polymers to explore the relationship between their properties and environment and structure to make them more selective in terms of temperature application range and regulation *** is very interesting that the introduction of poly-acrylic acid(PAA) segments in the middle of di-block copolymer PSBMA_(55)-b-PNIPAAm_(80) to form PSBMA_(55)-b-PAA_(x)-b-PNIPAAm_(80) results in a reversal of temperature-responsive behaviors from 'U'(LCST UCST) type,while the copolymer PSBMA_(55)-b-P(NIPAAm_(80)-co-AA_(x)) *** work provides a clue for tuning the phase transition behavior of polymers for manufacture of extreme smart materials.

关键词： Temperature responsive polymers High critical solubility temperature(UCST) Low critical solubility temperature(LCST) Block copolymers

A New Nonlinear Optical Crystal GdCa_(4)O(BO_(3))_(3)

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Chinese Physics Letters 1999年第3期16卷 184-186页

作者： ZHANG Shu-jun cheng zhen-xiang ZHANG Shao-jun ZHANG Ji-guo HAN Jian-ru CHEN Huan-chu National Laboratory of Crystal Materials Shandong UniversityJi’nan 250100

Large size and high quality single crystals GdCa_(4)O(BO_(3))_(3) have been grown from platinum crucible under air atmosphere by the conventional rf-heating Czochralski *** crystal growth conditions,growth habits,and transmission spectra were *** crystal is transparent in the visible and near-infrared region(320-2600nm).It has a good second harmonic generation phase-matching *** phase-matching experiment result is well consistent with the theoretical *** frequency-doubling efficiency is 26.7% in the phase-matching angles θ=45o and ø=45.1o direction.

关键词： Crystal matching doubling

Differentiation and immunosuppressive function of CD19^(+)CD24^(hi)CD27^(+) regulatory B cells are regulated through the miR-29a-3p/NFAT5 pathway

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Hepatobiliary & Pancreatic Diseases International 2024年第5期23卷 472-480页

作者： Jin-Yang Li Tian-Shuo Feng Ji Gao Xin-xiang Yang xiang-cheng Li zhen-Hua Deng Yong-xiang Xia zheng-Shan Wu Hepatobiliary Center the First Affiliated Hospital of Nanjing Medical UniversityNanjing 210029China Key Laboratory of Liver Transplantation Chinese Academy of Medical SciencesNanjing 210029China NHC Key Laboratory of Living Donor Liver Transplantation Nanjing Medical UniversityNanjing 210029China

Background: Regulatory B cells(Bregs) is an indispensable element in inducing immune tolerance after liver transplantation. As one of the microRNAs(miRNAs), mi R-29a-3p also inhibits translation by degrading the target mRNA, and yet the relationship between Bregs and mi R-29a-3p has not yet been fully explored. This study aimed to investigate the impact of miR-29a-3p on the regulation of differentiation and immunosuppressive functions of memory Bregs(m Bregs) and ultimately provide potentially effective therapies in inducing immune tolerance after liver transplantation. Methods: Flow cytometry was employed to determine the levels of Bregs in peripheral blood mononuclear cells. TaqMan low-density array miRNA assays were used to identify the expression of different miRNAs, electroporation transfection was used to induce mi R-29a-3p overexpression and knockdown, and dual luciferase reporter assay was used to verify the target gene of miR-29a-3p. Results: In patients experiencing acute rejection after liver transplantation, the proportions and immunosuppressive function of m Bregs in the circulating blood were significantly impaired. mi R-29a-3p was found to be a regulator of m Bregs differentiation. Inhibition of miR-29a-3p, which targeted nuclear factor of activated T cells 5(NFAT5), resulted in a conspicuous boost in the differentiation and immunosuppressive function of m Bregs. The inhibition of mi R-29a-3p in CD19~+ B cells was capable of raising the expression levels of NFAT5, thereby promoting B cells to differentiate into m Bregs. In addition, the observed enhancement of differentiation and immunosuppressive function of m Bregs upon mi R-29a-3p inhibition was abolished by the knockdown of NFAT5 in B cells. Conclusions: mi R-29a-3p was found to be a crucial regulator for m Bregs differentiation and immunosuppressive function. Silencing mi R-29a-3p could be a potentially effective therapeutic strategy for inducing immune tolerance after liver transplantation.

关键词： Regulatory B cells miR-29a-3p NFAT5 Liver transplantation

Unified Classification and Rejection:A One-versus-all Framework

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Machine Intelligence Research 2024年第5期21卷 870-887页

作者： zhen cheng Xu-Yao Zhang cheng-Lin Liu State Key Laboratory of Multimodal Artificial Intelligence Systems Institute of AutomationChinese Academy of SciencesBeijing100190China School of Artificial Intelligence University of Chinese Academy of SciencesBeijing100049China

Classifying patterns of known classes and rejecting ambiguous and novel(also called as out-of-distribution(OOD))inputs are involved in open world pattern *** neural network models usually excel in closed-set classification while perform poorly in rejecting OOD *** tackle this problem,numerous methods have been designed to perform open set recognition(OSR)or OOD rejection/detection *** methods mostly take post-training score transformation or hybrid models to ensure low scores on OOD inputs while separating known *** this paper,we attempt to build a unified framework for building open set classifiers for both classification and OOD *** formulate the open set recognition of K-known-class as a(K+1)-class classification problem with model trained on known-class samples *** decomposing the K-class problem into K one-versus-all(OVA)binary classification tasks and binding some parameters,we show that combining the scores of OVA classifiers can give(K+1)-class posterior probabilities,which enables classification and OOD rejection in a unified *** maintain the closed-set classification accuracy of the OVA trained classifier,we propose a hybrid training strategy combining OVA loss and multi-class cross-entropy *** implement the OVA framework and hybrid training strategy on the recently proposed convolutional prototype network and prototype classifier on vision transformer(ViT)*** on popular OSR and OOD detection datasets demonstrate that the proposed framework,using a single multi-class classifier,yields competitive performance in closed-set classification,OOD detection,and misclassification *** code is available at https://***/zhen-cheng121/CPN_OVA_unified.

关键词： Open set recognition out-of-distribution detection misclassification detection convolutional prototype network oneversus-all Dempster-Shafer theory of evidence

Astrometric Observations of NEA 1998 HH49 Using the Daocheng 50 cm Telescope

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Research in Astronomy and Astrophysics 2024年第7期24卷 71-78页

作者： Huan Xu xiang-Ming cheng Yi-Gong Zhang Teng-Fei Song zhen-Jun Zhang Qing-Yu Peng Yunnan Observatories Chinese Academy of SciencesKunming 650216China University of Chinese Academy of Sciences Beijing 100049China Key Laboratory of the Structure and Evolution of Celestial Objects Chinese Academy of SciencesKunming 650216China Engineering Laboratory on Applied Astronomical Technology of Yunnan Kunming 650216China School of Information Engineering Kunming UniversityKunming 650214China School of Computer Science and Information Engineering Anyang Institute of TechnologyAnyang 455000China Department of Computer Science Jinan UniversityGuangzhou 510632China Sino-French Joint Laboratory for Astrometry Dynamics and Space ScienceJinan UniversityGuangzhou 510632China

This study details an astrometric observation campaign of the Near-Earth Asteroid 1998 HH49,conducted with the aim of refining our understanding of its physical *** the 50 cm telescope located at the Wumingshan Mountain in Daocheng,Sichuan,images were obtained over four nights,from 2023 October 19 to October *** observations were processed using Astrometrica software,facilitating the precise determination of the asteroid's *** observational results were compared with the ephemerides from three distinct sources to verify accuracy:the Jet Propulsion Laboratory(JPL)Horizons System,the Institut de Mécanique Céleste et de Calcul deséphémérides(IMCCE)Miriade,and the Near-Earth Objects Dynamic Site(NEODyS-2).When compared with the JPL ephemeris,a mean observed-minus-calculated(O-C)result of 0.″07 in the *** and-0.″35 in the *** was ***,the comparison with the IMCCE ephemeris yielded mean O-C results of 0.″08 in the *** and-0.″06 in the *** comparison with the NEODyS-2 ephemeris yielded the mean O-C results of 0.″06 in ***-0.″49 in *** study's findings demonstrate a general consistency between the observed data and the ephemeris predictions,with minor discrepancies observed across the data ***,both the JPL and NEODyS-2 ephemerides show that the residuals in the *** exceed those in the *** disparities may result from atmospheric differential color refraction,ephemeris discrepancies,observational errors,and other ***,it is worth noting that further investigation is required due to the potential influence of additional ***,the Daocheng 50 cm Telescope exhibits the ability to conduct high-precision positional measurements.

关键词： astrometry ephemerides time

Effect of Strontium Ion on the Growth and Second-Harmonic Generation Properties of GdCa_(4)O(BO_(3))_(3) Crystal

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Chinese Physics Letters 2001年第1期18卷 63-64页

作者： ZHANG Shu-Jun cheng zhen-xiang LIU Jun-Hai HAN Jian-Ru WANG Ji-Yang SHAO Zong-Shu CHEN Huan-Chu State Key Laboratory of Crystal Materials Shandong UniversityJi'nan 250100

Large sized and optical quality GdCa_(4)O(BO_(3))_(3)(GdCOB)crystal with calcium partially substituted by strontium(Sr)ions was grown for the first *** x-ray powder diffraction shows that the Sr ion has an effect on the cell parameters of the GdCOB crystal Second-harmonic generation(SHG)experiments were performed on the Sr:GdCOB and GdCOB crystals along the spatial phase-matching *** results show that the cw green laser output power is 1.04 W when the laser diode pump power is 10 W in the Nd:YVO_(4)/Sr:GdCOB intracavity *** the slope efficiency of Nd:YVO_(4) and the fundamental laser in cavity,the intracavity SHG conversion efficiency of the GdCOB crystal is 21%while it is 24%for the Sr:GdCOB crystal,the SHG conversion efficiency is improved by 14%.The effect of the Sr ions on the nonlinearity of the GdCOB crystal is also discussed by using the anion group theory.

关键词： intracavity pump Crystal

Growth and Second-Harmonic-Generation Properties of Tm^(3+), Yb^(3+), Bi^(3+) and Li^(+) Doped GdCa_(4)O(BO_(3))_(3) Crystals

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Chinese Physics Letters 2001年第3期18卷 388-389页

作者： ZHANG Shu-Jun cheng zhen-xiang ZHANG Shao-Jun LIU Jun-Hai HAN Jian-Ru WANG Ji-Yang CHEN Huan-Chu State Key Laboratory of Crystal Materials Shandong UniversityJi’nan 250100

The rare-earth ions(Yb^(3+),Tm^(3+))and Li^(+),Bi^(3+)ions doped GdCa_(4)O(BO_(3))_(3) crystals were grown using the Czochralski pulling *** second-harmonic-generation conversion efficiencies of the GdCOB:Yb and GdCOB:Tm crystals are 31.3%and 33.3%,respectively,while the undoped GdCOB crystal is 27.9%.The conversion efficiencies of Yb^(3+),Tm^(3+)doped GdCOB are improved by 12%and 19%,respectively,compared to that of the undoped *** conversion efficiencies of Li^(+),Bi^(3+)doped GdCOB crystals are 33%and 38.3%,which are improved by 15%and 37%as compared to that of the undoped *** results are discussed using the anion group theory.

关键词： Crystal (3) Harmonic

Preparation and performance evaluation of the slickwater using novel polymeric drag reducing agent with high temperature and shear resistance ability

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Petroleum Science 2024年第2期21卷 1113-1121页

作者： Ming-Wei Zhao zhen-Feng Ma Cai-Li Dai WeiWu Yong-Quan Sun Xu-Guang Song Yun-Long cheng xiang-Yu Wang National Key Laboratory of Deep Oil and Gas China University of Petroleum(East China)Qingdao266580ShandongChina Shandong Key Laboratory of Oilfield Chemistry China University of Petroleum(East China)Qingdao266580ShandongChina Sinopec Shengli Oilfield Dongying257001ShandongChina Department of Chemical and Materials Engineering University of AlbertaEdmontonAB T6G 1H9Canada East China Petroleum Bureau of Sinopec Nanjing210011JiangsuChina

Slickwater fracturing fluids are widely used in the development of unconventional oil and gas resources due to the advantages of low cost,low formation damage and high drag reduction ***,their performance is severely affected at high *** reducing agent is the key to determine the drag reducing performance of *** this work,in order to further improve the temperature resistance of slickwater,a temperature-resistant polymeric drag reducing agent(PDRA)was synthesized and used as the basis for preparing the temperature-resistant *** slickwater system was prepared with the compositions of 0.2 wt%PDRA,0.05 wt%drainage aid nonylphenol polyoxyethylene ether phosphate(NPEP)and 0.5 wt%anti-expansion agent polyepichlorohydrindimethylamine(PDM).The drag reduction ability,rheology properties,temperature and shear resistance ability,and core damage property of slickwater were systematically studied and *** contrast to on-site drag reducing agent(DRA)and HPAM,the temperature-resistant slickwater demonstrates enhanced drag reduction efficacy at 90℃,exhibiting superior temperature and shear resistance ***,the drag reduction retention rate for the slickwater achieved an impressive 90.52%after a 30-min shearing ***,the core damage is only 5.53%.We expect that this study can broaden the application of slickwater in high-temperature reservoirs and provide a theoretical basis for field applications.

关键词： Unconventional resources Polymeric drag reducing agent Slickwater High drag reduction rate Temperature resistance

Continuous Orbit Equivalence of Semigroup Actions

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Acta Mathematica Sinica,English Series 2024年第6期40卷 1581-1598页

作者： xiang Qi QIANG cheng Jun HOU School of Mathematical Science Yangzhou UniversityYangzhou 225002P.R.China

We introduce notions of continuous orbit equivalence and its one-sided version for countable left Ore semigroup actions on compact spaces by surjective local homeomorphisms,and characterize them in terms of the corresponding transformation groupoids and their operator *** particular,we show that two essentially free semigroup actions on totally disconnected compact spaces are continuously orbit equivalent if and only if there is a canonical abelian subalgebra preserving C^(∗)-isomorphism between the associated transformation groupoid C^(∗)-*** also give some examples of orbit equivalence,consider the special case of semigroup actions by homeomorphisms and relate continuous orbit equivalence of semigroup actions to that of the associated group actions.

关键词： Semigroup action continuous one-sided orbit equivalence continuous orbit equivalence groupoid C^(∗)-algebras