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Thin paints for durable and scalable radiative cooling

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Journal of Energy Chemistry 2024年第3期90卷 176-182,I0006页

作者： Shanquan Liu Fei Zhang Xingyu chen Hongjie Yan Wei chen Meijie chen School of Energy Science and Engineering Central South UniversityChangsha 410083HunanChina School of Intelligent Manufacturing Ecosystem Xi'an Jiaotong-Liverpool UniversitySuzhou 215400JiangsuChina

Passive daytime radiative cooling(PDRC) is environment-friendly without energy input by enhancing the coating's solar reflectance(R_(solar)) and thermal emittance(ε_(LWIR)) in the atmosphere's long-wave infrared transmission ***,high R_(solar) is usually achieved by increasing the coating's thickness,which not only increases materials' cost but also impairs heat ***,the desired high R_(solar) is vulnerable to dust pollution in the *** this work,a thin paint was designed by mixing hBN plates,PFOTS,and IPA. R_(solar)=0.963 and ε_(LWIR)=0.927 was achieved at a thickness of 150 μm due to the high backscattering ability of scatters.A high through-plane thermal conductivity(~1.82 W m^(-1) K^(-1)) also can be *** addition,the porous structure coupled with the binder PFOTS resulted in a contact angle of 154°,demonstrating excellent durability under dust *** experiments showed that the thin paint can obtain a 2.3℃ lower temperature for sub-ambient cooling than the reference PDRC coating in the ***,the above-ambient heat dissipation performance can be enhanced by spraying the thin paint on a 3D heat sink,which was 15.7℃ lower than the reference 1D structure,demonstrating excellent performance for durable and scalable PDRC applications.

关键词： Radiative cooling Heat dissipation Solar reflectance Thermal emittance Contact angle

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70万吨/年连续重整装置能耗核算分析

石油石化绿色低碳 2023年第4期8卷 32-37,73页

作者：王奇李林陈爱青中国石化长岭炼化公司湖南岳阳414000

某炼化企业70万吨/年连续重整装置包括预加氢处理、重整反应和后分馏部分,该文利用模拟软件、设计参数核实比对、机泵额定功率核算等综合计算方式,对70万吨/年连续重整装置进行了能源消耗核算,分析得出装置实际的能耗分布和能源消耗情况... 详细信息

某炼化企业70万吨/年连续重整装置包括预加氢处理、重整反应和后分馏部分,该文利用模拟软件、设计参数核实比对、机泵额定功率核算等综合计算方式,对70万吨/年连续重整装置进行了能源消耗核算,分析得出装置实际的能耗分布和能源消耗情况,指出了装置实际能耗与完成情况的偏差,同时提出了节能方向。

关键词：能源消耗核算模拟节能

Evaluation of 3D crustal seismic velocity models in southwest China:Model performance,limitation,and prospects

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Science China Earth Sciences 2024年第2期67卷 604-619页

作者： Xin WANG Ling chen Qi-Fu chen Key Laboratory of Earth and Planetary Physics Institute of Geology and GeophysicsChinese Academy of SciencesBeijing100029China College of Earth and Planetary Sciences University of Chinese Academy of SciencesBeijing100049China State Key Laboratory of Lithospheric Evolution Institute of Geology and GeophysicsChinese Academy of SciencesBeijing100029China

Southwest China is a tectonically and seismically active region,witnessing strong deformation due to the collision between the Indian and Eurasian *** the subsurface velocity structure of this region is thus important in understanding the tectonics and geodynamic processes of continental collision and in mitigating seismic *** studies have provided various 3D seismic velocity models in southwest ***,discrepancies exist among these models,and less effort has been made to quantify the reliability and accuracy of these existing velocity *** this study,we use regional 3D waveform simulation to evaluate the performance of various regional crustal 3D velocity models in reproducing observed *** particularly focus on two recent earthquake sequence in the region,the 2021 Yunnan Yangbi MS_(6.4) earthquake sequence and the 2022 Sichuan Luding MS_(6.8) earthquake *** tested 3D velocity models include the Southwest China Community Velocity model V1.0,the Unified Seismic Tomography Models for Continental China Lithosphere V2.0,the adjoint full waveform tomography model of the crustal and upper mantle beneath Eastern Tibetan Plateau,and the shallow seismic structure model beneath continental *** results show that the tested 3D velocity models generally capture well long-period(<0.2 Hz)waveforms,indicating that the 3D models adequately resolve overall large-scale subsurface ***,the 3D synthetics show discrepancies in higher frequencies(0.05–0.3 Hz)and the performance of the 3D velocity models varies from region to region,suggesting that smaller scale heterogeneities are not well *** shallow velocity structures(<10 km)can improve the waveform fitting,emphasizing the importance of incorporating shallow structures in waveform *** full-waveform tomography model shows a slighter better performance than the other models,especially for the body-waves,highlighting the advantages

关键词： Southwest China Seismic tomography models Shallow Structures Waveform simulation Model evaluation

界面阻燃化玻璃纤维协同聚磷酸铵增强阻燃聚乳酸

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精细化工 2024年第4期41卷 829-839页

作者：阮阳阳陈小随张爱清钱立军中南民族大学化学与材料科学学院湖北武汉430070 北京工商大学中国轻工业先进阻燃剂工程技术研究中心北京100048

采用3-氨丙基三乙氧基硅烷(KH550)对短切玻璃纤维(GF)进行氨基化处理,得到表面富含氨基的GF-KH550,以三乙胺为缚酸剂和催化剂、POCl_(3)和4,4-二氨基二苯甲烷为反应单体,在GF-KH550表面原位聚合,获得超支化聚磷酰胺界面阻燃化玻璃纤维(G... 详细信息

采用3-氨丙基三乙氧基硅烷(KH550)对短切玻璃纤维(GF)进行氨基化处理,得到表面富含氨基的GF-KH550,以三乙胺为缚酸剂和催化剂、POCl_(3)和4,4-二氨基二苯甲烷为反应单体,在GF-KH550表面原位聚合,获得超支化聚磷酰胺界面阻燃化玻璃纤维(GF@HBPN),采用FTIR、XPS、SEM、TGA对其进行了表征。GF-KH550、GF@HBPN单独或与聚磷酸铵(APP)作为阻燃剂用于聚乳酸(PLA)复合材料(GF-KH550/PLA、GF@HBPN/PLA、APP/GF@HBPN/PLA)的制备。对复合材料的热稳定性、力学和阻燃性能进行了测试。结果表明,与PLA相比,GF-KH550/PLA的拉伸强度明显提高,但GF的“烛芯效应”严重恶化了其燃烧性能;GF@HBPN/PLA复合材料的拉伸强度也有提高,且燃烧过程中GF表面形成的界面残炭抑制其“烛芯效应”,改善了其燃烧性能(UL-94V-2),但不足以达到理想阻燃效果。当APP质量分数10%、GF@HBPN质量分数为30%时,制备的复合材料10%APP/30%GF@HBPN/PLA的极限氧指数达到26.8%±0.2%、垂直燃烧等级为UL-94V-0级,且热释放速率峰值、总热释放量和平均有效燃烧热比PLA分别下降了31.39%、23.57%和18.80%,显示出优异的火安全性能。

关键词：超支化聚磷酰胺玻璃纤维聚乳酸阻燃烛芯效应功能材料

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Self-aligned dual-beam superresolution laser direct writing with a polarization-engineered depletion beam

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Photonics Research 2024年第6期12卷 1194-1200页

作者： GUOLIANG chen DEWEI MO JIAN chen QIWEN ZHAN School of Optical-Electrical and Computer Engineering University of Shanghai for Science and TechnologyShanghai 200093China Shanghai Key Laboratory of Modern Optical System University of Shanghai for Science and TechnologyShanghai 200093China Zhangjiang Laboratory Shanghai 201204China

A fiber-based,self-aligned dual-beam laser direct writing system with a polarization-engineered depletion beam is designed,constructed,and *** system employs a vortex fiber to generate a donut-shaped,cylindrically polarized depletion beam while simultaneously allowing the fundamental mode excitation beam to pass *** results in a co-axially self-aligned dual-beam source,enhancing stability and mitigating assembly *** size of the central dark spot of the focused cylindrical vector depletion beam can be easily adjusted using a simple polarization rotation *** a depletion wavelength of 532 nm and an excitation wavelength of800 nm,the dual-beam laser direct writing system has demonstrated a single linewidth of 63 nm and a minimum line spacing of 173 *** optimization of this system may pave the way for practical superresolution photolithography that surpasses the diffraction limit.

关键词： polarization beam depletion

Computing Persistent Homology by Spanning Trees and Critical Simplices

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Research 2024年第2期2023卷 519-527页

作者： Dinghua Shi Zhifeng chen Chuang Ma Guanrong chen Department of Mathematics Cllege of ScienceShanghai UniversityShanghaiChina School of Big Data Fuzhou University of International Studies and TradeFuzhouChina Department of Data Science and Big Data Technology School of InternetAnhui UniversityHefeiChina Department of Electrical Engineering City University of Hong KongHong KongChina

Topological data analysis can extract effective information from higher-dimensional *** mathematical basis is persistent *** persistent homology can calculate topological features at different spatiotemporal scales of the dataset,that is,establishing the integrated taxonomic relation among points,lines,and ***,the simplicial network composed of all-order simplices in a simplicial complex is *** the sequence of nested simplicial subnetworks can be regarded as a discrete Morse function from the simplicial network to real values,a method based on the concept of critical simplices can be developed by searching all-order spanning *** this new method,not only the Morse function values with the theoretical minimum number of critical simplices can be obtained,but also the Betti numbers and composition of all-order cavities in the simplicial network can be calculated ***,this method is used to analyze some examples and compared with other methods,showing its effectiveness and feasibility.

关键词： Morse establishing topological

Photodegradation of xylene isomers:Kinetics,mechanism,secondary pollutant formation potential and health risk evaluation

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Journal of Environmental Sciences 2024年第2期136卷 658-669页

作者： Xiaoyan chen Weikun Zhu Sufen Feng Jiangyao chen Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control Guangdong Technology Research Center for Photocatalytic Technology Integration and Equipment EngineeringInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Guangzhou Key Laboratory of Environmental Catalysis and Pollution Control Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and HealthSchool of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China

Photodegradation technology has been widely applied in the purification of industrial aromatic ***,whether this technology efficiently removes the pollutants to prevent secondary pollution and health risk is still ***,the photodegradation processes of three xylenes were compared under designed reaction atmospheres and light *** lamp showed poor photodegradation ability toward xylenes,no matter in N_(2) or N_(2)+O_(2)system,while much higher photodegradation performance of xylenes were obtained under ultraviolet(UV)and vacuum ultraviolet(VUV)irradiation,especially in N_(2)+O_(2)+VUV system,where 97.9%of m-xylene,99.0%of o-xylene or 87.5%of p-xylene with the initial concentration of 860 mg/m^(3) was removed within 240 *** xylenes underwent three processes of photo-isomerization,photodecomposition and photo-oxidation to produce intermediates of aromatics,alkanes and *** them,the photo-isomerization products showed the highest concentration percentage(e.g.,≥50%in o-xylene system),confirming that photo-isomerization reaction was the dominated photodegradation process of ***,these isomerized products not only contributed about 97%and91%to the formation potential of O3(OFP)and secondary organic aerosols(SOAFP),but also displayed obvious non-carcinogenic risk,although one of photodecomposition product—benzene showed the highest occupational exposure ***,the secondary pollution and health risks of photodegradation products of xylenes were non-ignorable,although the OFP,SOAFP and health risks of the generated products reduced at least 4.5 times in comparison with that of the degraded *** findings are helpful for the appropriate application of this technology in the purification of industrial organic waste gas.

关键词： Isomer aromatics Photodegradation Ozone formation Secondary organic aerosols Health risk

An improved interval model updating method via adaptive Kriging models

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Applied Mathematics and Mechanics(English Edition) 2024年第3期45卷 497-514页

作者： Sha WEI Yifeng chen Hu DING Liqun chen Shanghai Key Laboratory of Mechanics in Energy Engineering Shanghai Frontier Science Center of MechanoinformaticsShanghai Institute of Applied Mathematics and MechanicsSchool of Mechanics and Engineering ScienceShanghai UniversityShanghai 200072China Shanghai Institute of Aircraft Mechanics and Control Shanghai 200092China

Interval model updating(IMU)methods have been widely used in uncertain model updating due to their low requirements for sample ***,the surrogate model in IMU methods mostly adopts the one-time construction *** makes the accuracy of the surrogate model highly dependent on the experience of users and affects the accuracy of IMU ***,an improved IMU method via the adaptive Kriging models is *** method transforms the objective function of the IMU problem into two deterministic global optimization problems about the upper bound and the interval diameter through universal grey *** optimization problems are addressed through the adaptive Kriging models and the particle swarm optimization(PSO)method to quantify the uncertain parameters,and the IMU is *** the construction of these adaptive Kriging models,the sample space is gridded according to sensitivity *** sampling is then performed in key subspaces based on the maximum mean square error(MMSE)*** interval division coefficient and random sampling coefficient are adaptively adjusted without human interference until the model meets accuracy *** effectiveness of the proposed method is demonstrated by a numerical example of a three-degree-of-freedom mass-spring system and an experimental example of a butted cylindrical *** results show that the updated results of the interval model are in good agreement with the experimental results.

关键词： interval model updating(IMU) non-probabilistic uncertainty adaptive Kriging model surrogate model grey number

An ionic liquid-assisted strategy for enhanced anticorrosion of low-energy PEO coatings on magnesium–lithium alloy

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Journal of Magnesium and Alloys 2024年第6期12卷 2380-2396页

作者： You Zhang Chuping chen Haoyue Tian Shuqi Wang chen Wen Fei chen College of New Materials and Chemical Engineering Hydrogen Energy Research CentreBeijing Institute of Petrochemical TechnologyBeijing 102617China Key Laboratory of Advanced Structure-Function Integrated Materials and Green Manufacturing Technology Harbin Institute of TechnologyHarbin 150001China Beijing Spacecrafts China Academy of Space TechnologyBeijing 100190China

A low-energy plasma electrolytic oxidation(LePEO)technique is developed to simultaneously improve energy efficiency and *** liquids(1-butyl-3-methylimidazole tetrafluoroborate(BmimBF_(4)))as sustainable corrosion inhibitors are chosen to investigate the corrosion inhibition behavior of ionic liquid(ILs)during the LePEO process for LA91 magnesium-lithium(Mg-Li)*** show that the ionic liquid BmimBF_(4)participates in the LePEO coating formation process,causing an increment in coating thickness and surface *** low conductivity of the ionic liquid is responsible for the voltage and breakdown voltage increases during the LePEO with IL process(LePEO-IL).After adding BmimBF_(4),corrosion current density decreases from 1.159×10^(−4)A·cm^(−2)to 8.143×10^(−6)A·cm^(−2).The impedance modulus increases to 1.048×10^(4)Ω·cm^(−2)and neutral salt spray remains intact for 24 *** superior corrosion resistance of the LePEO coating assisted by ionic liquid could be mainly attributed to its compact and thick barrier layer and physical absorption of ionic *** ionic liquid-assisted LePEO technique provides a promising approach to reducing energy consumption and improving film performance.

关键词： Magnesium-lithium alloy Plasma electrolytic oxidation Low energy Ionic liquid Corrosion resistance