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Appreciable Enhancement of Photocatalytic Performance for N-doped SrMoO_(4) via the Vapor-thermal Method

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Journal of Wuhan University of Technology(Materials Science) 2024年第1期39卷 24-31页

作者：恽志强戴振翔 ZHU Liwei zheng Ganhong School and Materials Science and Engineering Anhui UniversityHefei 230601China School of Physics and Optoelectronics Engineering Anhui UniversityHefei 230601China

A series of nitrogen-doped SrMoO_(4) with different Sr/N mole ratio (R=0,0.05,0.10,0.15,0.20,0.40,and 0.60) were synthesized using urea as the N source via the vapor-thermal *** photocatalytic degradation ability of all samples was evaluated using methylene blue (MB) as a target *** band gaps of N-doped samples are all higher than that of pristine ones,which is only 3.12 *** specific surface area S_(BET) and pore volume are increased due to the N *** the greater increase of S_(BET),the faster the photodegradation speed of methylene blue on SrMoO_(4).More specifically,the degradation efficiency of MB is improved up to 87%in 100 min.

关键词： SrMoO_(4) photocatalytic property nitrogen element doping

THE GLOBAL EXISTENCE AND UNIQUENESS OF SMOOTH SOLUTIONS TO A FLUID-PARTICLE INTERACTION MODEL IN THE FLOWING REGIME

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Acta Mathematica Scientia 2024年第5期44卷 1877-1885页

作者： Lin zheng Shu WANG College of Mathematics and Statistics North China University of Water Resources and Electric PowerZhengzhou450046China School of Mathematics Statistics and MechanicsBeijing University of TechnologyBeijing100124China

This paper is concerned with the Cauchy problem for a 3D fluid-particle interaction model in the so-called flowing regime inℝ*** the smallness assumption on both the external potential and the initial perturbation of the stationary solution in some Sobolev spaces,the existence and uniqueness of global smooth solutions in H3 of the system are established by using the careful energy method.

关键词： fluid-particle flowing regime global existence

Multiscale engineered hydrogel for solar evaporation with enhanced water transport and purification

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Science China Materials 2024年第8期67卷 2709-2710页

作者： Mingzhan Wang Ronghui Wu Shuang zheng Pritzker School of Molecular Engineering University of ChicagoChicagoIL 60637USA Department of Civil Engineering The University of Hong KongHong Kong 999077China

Solar evaporation is emerging as a powerful solution to alleviate the global water shortage *** a recent work published in Nature Water,Liangti Qu and coworkers[1]report a facile method of preparing a graphene/alginate hydrogel(GAH),which not only possesses nearly total rejections to salts,volatile and non-volatile organic compounds,but also exhibits excellent antifouling properties to bacteria and *** the perspective of chemistry,these impressive properties originate from the systematic engineering of the GAH,ranging from the molecular scale to the macroscopic scale.

关键词： volatile hydrogel preparing

Selective N-Methylation of N-Methylaniline with CO_(2) and H_(2) over Cu/In_(2)O_(3) Catalyst

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Chinese Journal of Chemistry 2024年第3期42卷 276-282页

作者： Huan zheng Bo Qian Lin He State Key Laboratory for Oxo Synthesis and Selective Oxidation Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhouGansu730000 China University of Chinese Academy of Sciences Beijing100049 China

N-Methylation of amines with CO_(2) and H2 is a potential approach for CO_(2) utilization because N-methylated amines can be used as solvents and organic intermediates. In_(2)O_(3)-supported Cu (Cu/In_(2)O_(3)) acts as an effective heterogeneous catalyst for N-methylation reaction of N-methylaniline (MA) with CO_(2) and H_(2),showing higher N,N-dimethylaniline (DMA) selectivity than other supported Cu catalysts. On one hand,the dispersion of Cu can be improved by the defective In_(2)O_(3) support. On the other hand,In_(2)O_(3) support is active in the dissociative adsorption of CO_(2) through C—O bond breaking. In addition,the H_(2) dissociation ability of In_(2)O_(3) can also be enhanced by Cu. The combination of Cu and In_(2)O_(3) is effective in the activation of CO_(2),the adsorption of intermediate N-methylformanilide (MFA),the hydrogenation of MFA to DMA and the prohibition of C—N bond cleavage side reactions,thereby enhancing the reaction rate of MA conversion and the selectivity to DMA.

关键词： N-Methylation CO_(2) Cu/In_(2)O_(3) Supported catalysts Heterogeneous catalysis

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基于Web的财务共享服务平台建设研究

信息与电脑 2023年第13期35卷 147-152页

作者：郑朝亮胡才双广州华商学院广东广州511300 蒙古国研究大学蒙古乌兰巴托11000

随着大智移云时代的到来,财会工作逐渐向平台化和数智化方向发展。财务共享服务平台建设是促进企业数智化转型的重要环节。文章依据企业战略定位,从战略、组织、人才、流程、数据以及技术6个方面阐述基于Web的财务共享服务平台构建、共... 详细信息

随着大智移云时代的到来,财会工作逐渐向平台化和数智化方向发展。财务共享服务平台建设是促进企业数智化转型的重要环节。文章依据企业战略定位,从战略、组织、人才、流程、数据以及技术6个方面阐述基于Web的财务共享服务平台构建、共享服务平台模块功能和建设保障措施,为优化财务共享服务平台管理、促进企业信息化、数智化转型以及高质量发展提供参考。

关键词：财务共享财务管理平台建设

Reliability ensemble averaging reduces surface wind speed projection uncertainties in the 21st century over China

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Advances in Climate Change Research 2024年第2期15卷 222-229页

作者： zheng-Tai ZHANG Chang-Ai XU Key Laboratory for Semi-Arid Climate Change of the Ministry of Education College of Atmospheric SciencesLanzhou UniversityLanzhou 730000China

Accurate prediction of future surface wind speed(SWS)changes is the basis of scientific planning for wind *** studies have projected SWS changes in the 21st century over China on the basis of the multi-model ensemble(MME)of the 6th Coupled Model Intercomparison Project(CMIP6).However,the simulation capability for SWS varies greatly in CMIP6 multi-models,so the MME results still have large *** this study,we used the reliability ensemble averaging(REA)method to assign each model different weights according to their performances in simulating historical SWS changes and project the SWS under different shared socioeconomic pathways(SSPs)in *** results indicate that REA considerably improves the SWS simulation capacity of CMIP6,eliminating the overestimation of SWS by the MME and increasing the simulation capacity of spatial *** spatial correlations with observations increased from 0.56 for the MME to 0.85 for ***,REA could eliminate the overestimation of the SWS by 33%in *** for southeastern China,the SWS generally decreases over China in the near term(2020-2049)and later term(2070-2099),particularly under high-emission *** SWS reduction projected by REA is twice as high as that by the MME in the near term,reaching-4%to-3%.REA predicts a larger area of increased SWS in the later term,which expands from southeastern China to eastern *** study helps to reduce the projected SWS uncertainties.

关键词： Surface wind speed Uncertainty Multi-model ensemble Reliability ensemble averaging CMIP6

Stereochemical editing:Catalytic racemization of secondary alcohols and amines

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Chinese Chemical Letters 2024年第5期35卷 17-31页

作者： Jun Zhang Zhiyao zheng Can Zhu Department of Chemistry Fudan UniversityShanghai 200438China Department of Organic Chemistry Arrhenius LaboratoryStockholm UniversityStockholm 10691Sweden

Chiral alcohols and amines are important structural units widely existing in pharmaceuticals,agrochemicals,and food *** kinetic resolution(DKR)is an efficient strategy to deliver optically active alcohols and amines from their *** the development of DKR method,racemization catalyst plays as a crucial element with the requirement of compatibility with the kinetic resolution(KR)*** this paper,recent advance in the catalytic racemization of secondary alcohols and amines is summarized based on different types of racemizing intermediates,which are redox racemization via ketone/imine intermediates,racemization via radical intermediates,and racemization via carbocation *** racemization of secondary alcohols and amines is also enclosed.

关键词： Racemization Secondary alcohols Amines Kinetic resolution Dynamic kinetic resolution

A Possible γ-Ray Pulsation from PSR J1740-5340B in the Globular Cluster NGC 6397

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Research in Astronomy and Astrophysics 2024年第1期24卷 285-291页

作者： Jiao zheng Pengfei Zhang Li Zhang Department of Astronomy School of Physics and AstronomyKey Laboratory of Astroparticle Physics of Yunnan ProvinceYunnan UniversityKunming 650091China

Recently, a new radio millisecond pulsar(MSP) J1740-5340B, hosted in the globular cluster(GC) NGC 6397,was reported with a 5.78 ms spin period in an eclipsing binary system with a 1.97 days orbital period. Based on a modified radio ephemeris updated by tool tempo2, we analyze the ~15 yr γ-ray data obtained from the Large Area Telescope on board the Fermi Gamma-ray Space Telescope and detect PSR J1740-5340B's γ-ray pulsation at a confidence level of ~4σ with a weighted H-test value of ~26. By performing a phase-resolved analysis, the γ-ray luminosity in on-pulse interval of PSR J1740-5340B is L_(γ)~ 3.8 × 10^(33) erg s^(-1) using NGC 6397's distance of 2.48 kpc. And γ-rays from the on-pulse part of PSR J1740-5340B contribute ~90% of the total observed γ-ray emissions from NGC 6397. No significant γ-ray pulsation of another MSP J1740-5340A in the GC is *** that the previous four cases of MSPs in GCs, more data in γ-ray, X-ray, and radio are encouraged to finally confirm the γ-ray emissions from MSP J1740-5340B, especially starving for a precise ephemeris.

关键词： gamma-rays:galaxies (stars:)pulsars:individual(PSR J1740-5340B) (Galaxy:)globular clusters:individual(NGC 6397)

HetNets Under Decoupled Uplink and Downlink Access with UE Random Discontinuous Transmission: Local Delay and Energy Efficiency

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China Communications 2024年第3期21卷 205-216页

作者： Zhang Yue zheng Fuchun Luo Jingjing School of Electronic and Information Engineering Harbin Institute of Technology(Shenzhen)Shenzhen 518055China

Due to the limited uplink capability in heterogeneousnetworks (HetNets), the decoupled uplinkand downlink access (DUDA) mode has recently beenproposed to improve the uplink performance. In thispaper, the random discontinuous transmission (DTX)at user equipment (UE) is adopted to reduce the interferencecorrelation across different time slots. By utilizingstochastic geometry, we analytically derive themean local delay and energy efficiency (EE) of an uplinkHetNet with UE random DTX scheme under theDUDA mode. These expressions are further approximatedas closed forms under reasonable *** results reveal that under the DUDA mode, there isan optimal EE with respect to mute probability underthe finite local delay constraint. In addition, with thesame finite mean local delay as under the coupled uplinkand downlink access (CUDA) mode, the HetNetsunder the DUDA mode can achieve a higher EE witha lower mute probability.

关键词： decoupled uplink and downlink access(DUDA) heterogeneous networks(HetNets) random discontinuous transmission(DTX) stochastic geometry