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Highly selective and efficient photocatalytic NO removal:Charge carrier kinetics and interface molecular process

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Nano Research 2024年第3期17卷 1003-1026页

作者： Huan Shang Hongbao Jia Pengpeng Li Hao Li Wenbin Zhang Shuangjun Li Qing wang Shuning Xiao Ding wang Guisheng Li Dieqing Zhang School of Materials and Chemistry University of Shanghai for Science and TechnologyShanghai 200093China The Education Ministry Key Lab of Resource Chemistry Joint International Research Laboratory of Resource Chemistry of Ministry of EducationShanghai Key Laboratory of Rare Earth Functional Materialsand Shanghai Frontiers Science Center of Biomimetic CatalysisShanghai Normal UniversityShanghai 200234China School of Environmental Science and Engineering Shanghai Jiao Tong UniversityShanghai 200240China

The widespread nitrogen oxides(NOx,mainly in NO)in the atmosphere have threatened human health and ecological *** dilute NO(ppb)is difficult to efficiently remove via the traditional process due to its characteristics of low concentration,wide range,large total amount,*** can utilize solar energy to purify NO pollutants under mild conditions,but its application is limited due to the low selectivity of nitrate and poor activity of NO *** underlying reason is that the interface mechanism of NO oxidation is not clearly understood,which leads to the inability to accurately regulate the NO oxidation ***,the recent advances in the photocatalytic oxidation of NO are ***,the common strategies to effectively regulate carrier dynamics such as morphology control,facet engineering,defect engineering,plasma coupling,heterojunction and single-atom catalysts are ***,the progress of enhancing the adsorption and activation of reactants such as NO and O_(2) during NO oxidation is described in detail,and the corresponding NO oxidation mechanisms are ***,the challenges and prospects of photocatalytic NO oxidation are presented in term of nanotechnology for air pollution *** review can shed light on the interface mechanism of NO oxidation and provide illuminating information on designing novel catalysts for efficient NOx control.

关键词： nitrogen oxide(NO)oxidation photocatalysis NO/O_(2)activation charge carrier kinetics interfacial mechanism

Millimeter waves in medical applications:status and prospects

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Intelligent Medicine 2024年第1期4卷 16-21页

作者： Honglin wang Lin Lu Pengran Liu Jiayao Zhang Songxiang Liu yi Xie Tongtong Huo Hong Zhou Mingdi Xue ying Fang Jiaming Yang Zhewei Ye Department of Orthopedics Surgery Union HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhanHubei 430022China Departments of Orthopedics Renmin Hospital of Wuhan UniversityWuhanHubei 430060China

Millimeter waves are electromagnetic waves with wavelengths of 1–10 mm,which have characteristics of high frequency and short *** have gradually and widely been used in engineering and medical *** have identified studies related to millimeter waves in the biomedical field and summarized the biological effects of millimeter waves and their current status in medical ***,the shortcomings of existing studies and future developments were analyzed and discussed,with the aim of providing a reference for further research and development of millimeter waves in the medical field.

关键词： Millimeter wave Biological effects Medical applications Vital signs monitoring

Investigations on High-Speed Flash Boiling Atomization of Fuel Based on Numerical Simulations

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Computer Modeling in Engineering & Sciences 2024年第5期139卷 1427-1453页

作者： Wei Zhong Zhenfang Xin Lihua wang Haiping Liu School of Aerospace Engineering and Applied Mechanics Tongji UniversityShanghai200092China Beijing Mechanical Equipment Research Institute Beijing100854China

Flash boiling atomization(FBA)is a promising approach for enhancing spray atomization,which can generate a fine and more evenly distributed spray by increasing the fuel injection temperature or reducing the ambient ***,when the outlet speed of the nozzle exceeds 400 m/s,investigating high-speed flash boiling atomization(HFBA)becomes quite *** difficulty arises fromthe involvement ofmany complex physical processes and the requirement for a very fine mesh in numerical *** this study,an HFBA model for gasoline direct injection(GDI)is *** model incorporates primary and secondary atomization,as well as vaporization and boilingmodels,to describe the development process of the flash boiling *** to lowspeed FBA,these physical processes significantly impact *** this model,the Eulerian description is utilized for modeling the gas,and the Lagrangian description is applied to model the droplets,which effectively captures the movement of the droplets and avoids excessive mesh in the Eulerian *** various conditions,numerical solutions of the Sauter mean diameter(SMD)for GDI show good agreement with experimental data,validating the proposed model’s *** based on this HFBA model investigate the influences of fuel injection temperature and ambient pressure on the atomization *** analyses of the velocity field,temperature field,vapor mass fraction distribution,particle size distribution,and spray penetration length under different superheat degrees reveal that high injection temperature or low ambient pressure significantly affects the formation of small and dispersed droplet *** effect is conducive to the refinement of spray particles and enhances atomization.

关键词： High-speed flash boiling atomization numerical simulations Eulerian description Lagrangian description gasoline direct injection

Unraveling electrolyte solvation architectures for high-performance lithium-ion batteries

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Science China(Technological Sciences) 2024年第3期67卷 958-964页

作者： YANG MengHao SHI Zhe HE ZhiYuan wang Dan School of Materials Science and Engineering Tongji UniversityShanghai 201804China Department of Nuclear Science and Engineering Massachusetts Institute of Technology CambridgeMassachuseis 02139USA School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081China

The design of advanced electrolytes hinges critically on a comprehensive comprehension of lithium-ion migration mechanisms within these electrochemical systems. Fluorination generally improves the stability and reduces the reactivity of organic compounds, making them potentially suitable for use in harsh conditions such as those found in a battery electrolyte. However,the specific properties, such as the solvation power, diffusivity, ion mobility, and so forth, would depend on the exact nature and extent of the fluorination. In this work, we introduce a theoretical framework designed to facilitate the autonomous creation of electrolyte molecular structures and craft methodologies to compute transport coefficients, providing a physical interpretation of fluoride systems. Taking fluorinated-1,2-diethoxyethanes as electrolyte solvents, we present and analyze the relationship between the electronic properties and atomic structures, and further correlate these properties to the transport coefficients, resulting in a good alignment with the experimental diffusion behaviors and Li-solvation structures. The insights derived from this research contribute to the methodological basis for high-throughput evaluation of prospective electrolyte systems, and consequently, propose strategic directions for the improvement of electrochemical cycle characteristics. This comprehensive exploration of the transport mechanisms enhances our understanding, offering avenues for further advancements in the field of lithium-ion battery technology.

关键词： Unraveling electrolyte solvation architectures for high-performance lithium-ion batteries

Monocular Distance Estimated Based on PTZ Camera

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Computers, Materials & Continua 2024年第5期79卷 3417-3433页

作者： Qirui Zhong Xiaogang Cheng Yuxin Song Han wang Bell Honors School Nanjing University of Posts and Telecommunications Nanjing210003China College of Telecommunications and Information Engineering Nanjing University of Posts and TelecommunicationsNanjing210003China College of Automation and College of Artificial Intelligence Nanjing University of Posts and TelecommunicationsNanjing210003China

This paper introduces an intelligent computational approach for extracting salient objects fromimages and estimatingtheir distance information with PTZ (Pan-Tilt-Zoom) cameras. PTZ cameras have found wide applications innumerous public places, serving various purposes such as public securitymanagement, natural disastermonitoring,and crisis alarms, particularly with the rapid development of Artificial Intelligence and global infrastructuralprojects. In this paper, we combine Gauss optical principles with the PTZ camera’s capabilities of horizontal andpitch rotation, as well as optical zoom, to estimate the distance of the *** present a novel monocular objectdistance estimation model based on the Focal Length-Target Pixel Size (FLTPS) relationship, achieving an accuracyrate of over 95% for objects within a 5 km range. The salient object extraction is achieved through a simplifiedconvolution kernel and the utilization of the object’s RGB features, which offer significantly faster computingspeeds compared to Convolutional Neural Networks (CNNs). Additionally, we introduce the dark channel beforethe fog removal algorithm, resulting in a 20 dB increase in image definition, which significantly benefits distanceestimation. Our system offers the advantages of stability and low device load, making it an asset for public securityaffairs and providing a reference point for future developments in surveillance hardware.

关键词： Public security location information PTZ camera image processing

Securing Forwarding Layers from Eavesdropping Attacks Using Proactive Approaches

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Computers, Materials & Continua 2024年第4期79卷 563-580页

作者： Jiajun Yan ying Zhou Anchen Dai Tao wang School of Electronics and Communication Engineering Sun Yat-sen UniversityShenzhen518107China

As an emerging network paradigm,the software-defined network(SDN)finds extensive application in areas such as smart grids,the Internet of Things(IoT),and edge *** forwarding layer in software-defined networks is susceptible to eavesdropping *** hopping is amoving target defense(MTD)technology that is frequently employed to resist eavesdropping *** the traditional route hopping technology,both request and reply packets use the same hopping *** an eavesdropping attacker monitors the nodes along this path,the risk of 100%data leakage becomes *** this paper,we present an effective route hopping approach,called two-day different path(TDP),that turns communication paths into untraceable moving *** technology minimizes the probability of data leakage by transmitting request data and reply data through different ***,a brief introduction to the network model and attack model involved in this paper is ***,the algorithm and processingmethod of the TDP are ***,the paper proposes three differentmetrics tomeasure the effectiveness of the proposed ***,theoretical analysis and simulation results show that the TDP can effectively reduce the percentage of data exposure,decrease eavesdropping attack success probability,and improve the unpredictability of the path.

关键词： Route hopping moving target defense software-defined network two-way different path metrics

Characterizing permeability-porosity relationships of porous rocks using a stress sensitivity model in consideration of elastic-structural deformation and tortuosity sensitivity

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第9期16卷 3437-3451页

作者： Ronghe Xu Liqin wang Xiaoli Zhao Yuze Mao MIIT Key Laboratory of Aerospace Bearing Technology and Equipment Harbin Institute of TechnologyHarbin150001China State Key Laboratory of Robotics and System Harbin Institute of TechnologyHarbin150001China Shanghai Aerospace Control Technology Institute Shanghai201100China

Clarifying the relationship between stress sensitivities of permeability and porosity is of great significance in guiding underground resource *** and more studies focus on how to construct stress sensitivity models to describe the relationship and obtain a comprehensive stress sensitivity of porous ***,the limitations of elastic deformation calculation and incompleteness of considered tortuosity sensitivity lead to the fact that the existing stress sensitivity models are still unsatisfactory in terms of accuracy and ***,a more accurate and generic stress sensitivity model considering elastic-structural deformation of capillary cross-section and tortuosity sensitivity is proposed in this *** elastic deformation is derived from the fractal scaling model and Hooke's *** the effects of elastic-structural deformation on tortuosity sensitivity,an empirical formula is proposed,and the conditions for its applicability are *** predictive performance of the proposed model for the permeability-porosity relationships is validated in several sets of publicly available experimental *** experimental data are from different rocks under different pressure *** mean and standard deviation of relative errors of predicted stress sensitivity with respect to experimental data are 2.63%and 1.91%.Compared with other models,the proposed model has higher accuracy and better predictive generalization *** is also found that the porosity sensitivity exponent a,which can describe permeability-porosity relationships,is 2 when only elastic deformation is considered.a decreases from 2 when structural deformation is also *** addition,a may be greater than 3 due to the increase in tortuosity sensitivity when tortuosity sensitivity is considered even if the rock is not fractured.

关键词： Stress sensitivity model Permeability-porosity relationships Elastic-structural deformation Tortuosity stress sensitivity

YOLO-O2E:A Variant YOLO Model for Anomalous Rail Fastening Detection

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Computers, Materials & Continua 2024年第7期80卷 1143-1161页

作者： Zhuhong Chu Jianxun Zhang Chengdong wang Changhui Yang Department of Computer Science and Engineering Chongqing University of TechnologyChongqing400054China Institute of Flexible Electronics(Future Technologies) Xiamen UniversityXiamen361000China College of Mechanical Engineering Chongqing University of TechnologyChongqing400054China

Rail fasteners are a crucial component of the railway transportation safety *** fasteners,distinguished by their high length-to-width ratio,frequently encounter elevated failure rates,necessitating manual inspection and *** inspection not only consumes time but also poses the risk of potential *** the advancement of deep learning technology in rail fasteners,challenges such as the complex background of rail fasteners and the similarity in their states are *** have proposed an efficient and high-precision rail fastener detection algorithm,named YOLO-O2E(you only look once-O2E).Firstly,we propose the EFOV(Enhanced Field of View)structure,aiming to adjust the effective receptive field size of convolutional kernels to enhance insensitivity to small spatial ***,The OD_MP(ODConv and MP_2)and EMA(EfficientMulti-Scale Attention)modules mentioned in the algorithm can acquire a wider spectrum of contextual information,enhancing the model’s ability to recognize and locate ***,we collected and prepared the GKA dataset,sourced from real train *** testing on the GKA dataset and the publicly available NUE-DET dataset,our method outperforms general-purpose object detection *** the GKA dataset,our model achieved a mAP 0.5 value of 97.6%and a mAP 0.5:0.95 value of 83.9%,demonstrating excellent inference ***-O2E is an algorithm for detecting anomalies in railway fasteners that is applicable in practical industrial settings,addressing the industry gap in rail fastener detection.

关键词： Rail fastening detection deep learning anomalous rail fastening variant YOLO feature reinforcement

Minmax Common Due-Window Assignment Scheduling with Deteriorating Jobs

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Journal of the Operations Research Society of China 2024年第3期12卷 681-693页

作者： Dan-Yang Lv Jing Xue Ji-Bo wang School of Mechatronics Engineering Shenyang Aerospace UniversityShenyang110136LiaoningChina

This paper investigates the common due-window assignment scheduling problem with deteriorating jobs on a single machine in which the processing time of a job is a proportional function of its starting *** goal is to minimize the maximum value of earliness and tardiness penalties,as well as due-window location cost,and size *** on whether the location and size of due-window are known,this paper studies three relevant cases,all of which are solvable in polynomial time.

关键词： Scheduling Single machine Deteriorating jobs Common due-window Earliness Tardiness