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Edge supercurrent in Josephson junctions based on topological materials

Science china(Physics,Mechanics & Astronomy) 2025年第2期68卷 1-12页

作者： Junjie Qi chui-Zhen chen Juntao Song Jie liu Ke He Qing-Feng Sun X.c.Xie Beijing Academy of Quantum Information Sciences Beijing 100193China School of Physical Science and Technology Soochow UniversitySuzhou 215006China Institute for Advanced Study Soochow UniversitySuzhou 215006China college of Physics and Hebei Advanced Thin Films Laboratory Hebei Normal UniversityShijiazhuang 050024China School of Physics Xi’an Jiaotong UniversityMinistry of Education Key Laboratory for Non-Equilibrium Synthesis and Modulation of Condensed MatterXi’an 710049China State Key Laboratory of Low Dimensional Quantum Physics Department of PhysicsTsinghua UniversityBeijing 100084China Frontier Science center for Quantum Information Beijing 100084China Hefei National Laboratory Hefei 230088China International center for Quantum Materials School of PhysicsPeking UniversityBeijing 100871China Interdisciplinary center for Theoretical Physics and Information Sciences Fudan UniversityShanghai 200433China

The interplay between novel topological states and superconductivity has garnered substantial interest due to its potential for topological quantum *** Josephson effect serves as a useful probe for edge superconductivity in these hybrid topological *** Josephson junctions based on topological materials,supercurrents exhibit unique quantum interference patterns,including the conventional Fraunhofer oscillations,theΦ_(0)-periodic oscillation,and the 2Φ_(0)-periodic oscillation in response to the external magnetic field(Φ_(0)=h/2e is the flux quantum,h the Planck constant,and e the electron charge).These interference patterns stem from varied Andreev reflection mechanisms and the associated current density *** review seeks to comprehensively examine the theoretical and experimental advancements in understanding the quantum interference patterns of edge supercurrents in Josephson junctions based on quantum spin Hall,quantum Hall,and quantum anomalous Hall systems.

关键词： quantum Hall effect quantum spin Hall effect quantum anomalous Hall effect Josephson junction edge supercurrent Andreev reflection

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Anomalous open orbits in Hofstadter spectrum of chern insulator

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Science china(Physics,Mechanics & Astronomy) 2025年第3期Mechanics & Astronomy) .卷 143-148页

作者： Haijiao Ji Peng Zhou Noah F.Q.Yuan Hua Jiang Haiwen liu X.c.Xie center for Advanced Quantum Studies Department of Physics Beijing Normal University Tsung-Dao Lee Institute Shanghai Jiao Tong University Department of Mathematics UC Berkeley Institute for Nanoelectronic Devices and Quantum computing Fudan University International center for Quantum Materials School of Physics Peking University Hefei National Laboratory

The nontrivial band topology of chern insulator can enrich the content of its Hofstadter butterfly spectra, which is closely related to recent experiments in twisted bilayer graphene and cold atom systems. We investigate the Hofstadter spectrum for various models of chern insulators under a rational flux φ0/q, here φ0=h/e and q being an integer. We find the number of splitting subbands is |q-c| with c denoting the chern number of parent band. Importantly, anomalous open-orbital subbands with chern numbers q-1 and-q-1 emerge unexpectedly, which are beyond the parameter window（-q/2, q/2） of the Diophantine equation studied by Thouless-Kohmoto-Nightingale-den Nijs [Phys. Rev. Lett. 49, 405（1982）]. The emergence of anomalous open orbits can be traced by analyzing the evolution of the Hofstadter spectrum, identifying as a new type of topological phase transition. These novel findings not only pinpoint the peculiar Hofstadter spectrum of chern insulator, but also provide routes to study exotic characteristics beyond the Landau level physics.

关键词： Hofstadter spectrum topological phase transition open orbit

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Rational modulation of fluorophosphate cathode by anionic groups to reduce the polarization behavior for fast-charging sodium-ion batteries

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Journal of Energy chemistry 2025年第1期100卷 509-521页

作者： Xinyuan Wang Fan Zhang Xingyu Zhou Qian Wang c.angyu liu Yangyang liu Hui Wang Xiaojie liu Key Laboratory of Synthetic and Natural Functional Molecule of the Ministry of Education College of Chemistry&Materials ScienceNorthwest UniversityXi’an 710127ShaanxiChina

Na_(3)V_(2)(PO_(4))_(2)O_(2)F (VP) is recognized as a promising cathode material for sodium-ion batteries due to its stable structural framework and high specific *** functional theory (DFT) and finite element simulations show that incorporating SO_(4)^(2-)into VP decreases its band gap,lowers the migration energy barrier,and ensures a uniform Na+concentration gradient and stress distribution during charge and discharge ***,the average Na+diffusion coefficient of Na_(3)V_(2)(PO_(4))_(1.95)(SO_(4))_(0.05)O_(2)F(VPS-1) is roughly double that of VP,leading to enhanced rate capability (80 c,75.5 mAh g^(-1)) and cycling stability (111.0 mAh g^(-1)capacity after 1000 cycles at 10 c current density) for ***-1 exhibits outstanding fast-charging capabilities,achieving an 80%state of charge in just 8.1 *** assembled VPS-1//SbSn/NPc full cell demonstrated stable cycling over 200 cycles at a high 5 c current,maintaining an average coulombic efficiency of 95.35%.

关键词： Anionic group modulation Polarization behavior Fast-charging Sodium-ion battery Fluorophosphate cathode

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construction of iron manganese metal-organic framework-derived manganese ferrite/carbon-modified graphene composites toward broadband and efficient electromagnetic dissipation

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International Journal of Minerals,Metallurgy and Materials 2025年第3期32卷 546-555页

作者： Baohua liu Shuai liu Zaigang Luo Ruiwen Shu School of chemical and Blasting Engineering Anhui Province Key Laboratory of Specialty PolymersAnhui University of Science and TechnologyHuainan 232001China Joint National-Local Engineering Research centre for Safe and Precise coal Mining Anhui University of Science and TechnologyHuainan 232001China

The preparation of carbon-based electromagnetic wave(EMW)absorbers possessing thin matching thickness,wide absorption bandwidth,strong absorption intensity,and low filling ratio remains a huge ***-organic frameworks(MOFs)are ideal self-sacrificing templates for the construction of carbon-based EMW *** this work,bimetallic FeMn-MOF-derived MnFe_(2)O_(4)/c/graphene composites were fabricated via a two-step route of solvothermal reaction and the following pyrolysis *** results re-veal the evolution of the microscopic morphology of carbon skeletons from loofah-like to octahedral and then to polyhedron and pomegran-ate after the adjustment of the Fe^(3+)to Mn^(2+)molar ***,at the Fe^(3+)to Mn^(2+)molar ratio of 2:1,the obtained MnFe_(2)O_(4)/c/graphene composite exhibited the highest EMW absorption ***,a minimum reflection loss of-72.7 dB and a max-imum effective absorption bandwidth of 5.1 GHz were achieved at a low filling ratio of 10wt%.In addition,the possible EMW absorp-tion mechanism of MnFe_(2)O_(4)/c/graphene composites was ***,the results of this work will contribute to the construction of broadband and efficient carbon-based EMW absorbers derived from MOFs.

关键词： metal-organic frameworks graphene magnetic composites morphology regulation electromagnetic dissipation

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Exhumation and Preservation of the Yangchuling Porphyry W-Mo Deposit in the Jiangnan Tungsten Ore Belt,South china:Insights from(U-Th)/He and Fission Track Dating

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Journal of Earth Science 2025年第1期36卷 46-56页

作者： Yue Sun Ying Wang Jianzhang Pang Samuel c.Boone Minting Wu chongjian Shao Wei liu Jiangxi Provincial Key Laboratory of Genesis and Prospect for Strategic Minerals School of Earth ScienceEast China University of TechnologyNanchang330013China Institute of Geology china Earthquake Administration Beijing100029China School of Geography Earth and Atmospheric Sciences The University of MelbourneMelbourneVIC3010Australia Department of Earth Sciences The University of AdelaideAdelaideSA5005Australia Jiangxi Duchang JinDing Tungsten cO. Ltd.Jiujiang332611China

The Yangchuling porphyry W-Mo deposit(YPWD),located in the Jiangnan porphyryskarn tungsten ore belt,is one of the most important and large-scale porphyry W-Mo deposits in South *** previous zircon U-Pb and molybdenite Re-Os data suggest that Yangchuling WMo ore bodies formed almost simultaneously with granodiorite and monzogranitic porphyry at~150–144 Ma,their post emplacement history remains poorly understood,making their preservation status at depth *** this paper,new zircon and apatite(U-Th)/He and apatite fission track(ZHe,AHe and AFT,respectively)data of one hornfels and five intrusive rocks from a 1000-meter borehole are ***,together with new inverse thermal history models and previous geochronological data,help elucidate the post-diagenetic exhumation history and preservation status of the Yangchuling porphyry W-Mo *** general,ZHe and AHe ages decrease gradually from the near surface downwards and have relatively little intra-sample variation,ranging from 133 to 73Ma and 67 to 25 Ma,*** four granodiorites yield similar AFT ages that range from 63 to 55 Ma with mean track lengths varying from 12.2±0.7 to 12.6±0.5μ*** history modelling indicates that the Yangchuling ore district experienced slow,monotonic cooling since the ***-depth relationships are interpreted as recording~3.7±0.8 km of cretaceous-recent exhumation in response to regional extension throughout South china thought to have been driven by subduction retreat of the Paleo-Pacific *** of estimated net exhumation and previous metallogenic depth of~4–5 km suggests that W-Mo ore bodies could still exist at depths of up to~1.3±0.8 km relative to Earth surface in the YPWD *** of the YPWD is attributed to the limited amount of regional denudation during the Late cretaceous and cenozoic.

关键词： (U-Th)/He fission track ore preservation thermochronology Yangchuling porphyry W-Mo deposit

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Long-duration aqueous Zn-ion batteries achieved by dual-salt highly-concentrated electrolyte with low water activity

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Journal of Energy chemistry 2025年第2期101卷 778-785页

作者： Lvzhang Jiang Lingbo Yao Gege Wang chang liu Xiaowei chi Yu liu Shanghai Institute of ceramics Chinese Academy of Sciences University of chinese Academy of Sciences

Aqueous Zn-ion batteries have attracted much attention due to their unique high safety and low-cost ***,their practical applications are at a slow pace due to their short cycle life,which fundamentally results from the instability of the positive/negative electrode interface in the traditional dilute aqueous electrolytes with high water *** highly concentrated electrolyte（HcE）has been considered as an effective *** previous studies of single salt-based HcE（SSHcE）,herein,a new dual-salt HcE（15 m Zncl2+10 m NH4NH2SO3DS-HcE） was proposed for the first ***-HcE was proven to simultaneously possess higher conductivity than traditional dilute electrolytes and ultralow water activity of SS-HcE by the regulation of dual high-concentration salts on the solvation structure,which renders the Zn‖Zn symmetric cell the record-long cycling life of 2200 h compared with those with SS-HcE（30 m Zncl2,300 h） and other reported ***,the Zn‖NH4V4O10full cell with DS-HcE demonstrated impressed rate capability within a wide-range current densities from 0.1 to 10 A ***,at the high current density of 5 A g-1,the full cell shows almost100% capacity retention after 4000 cycles,which indicates the promising future of the DS-HcE system for long-duration aqueous Zn-ion batteries.

关键词： Ammonium vanadate Aqueous zinc battery cycling stability Electrolyte

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Functional ternary salt construction enabling an in-situ Li3N/LiF-enriched interface for ultra-stable all-solid-state lithium metal batteries

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Journal of Energy chemistry 2025年第2期101卷 68-75页

作者： Hong-Yan liu Xin-Yu liu Nan Zhang Peng-Fei Wang Zong-Lin liu Jie Shu Ting-Feng Yi School of Materials Science and Engineering Northeastern University Key Laboratory of Dielectric and Electrolyte Functional Material Hebei Province School of Resources and Materials Northeastern University at Qinhuangdao Faculty of Materials Science and chemical Engineering and Key Laboratory of Photoelectric Detection Materials and Devices of Zhejiang Province Ningbo University

Poly（ethylene oxide）-based polymer all-solid-state lithium metal batteries（ASSLBs） have received widespread attention due to their low cost,good process ability,and high energy ***,the growth of Li dendrites within polymer solid-state electrolytes damages the reversibility of Li anodes and still impedes their widespread *** efficient strategy is to construct a superior solid electrolyte ***,a stable interface enriched with Li3N and LiF is in-situ formed between Li anode and a terna ry salt *** terna ry salt electrolyte is innovatively designed by introducing lithium bis（trifluoromethane sulfonyl）imide（LiTFSI）,lithium bis（fluorosulfonyl）imide（LiFSI）,and LiNO3to poly（ethylene oxide） *** characterization indicates that LiNO3and LiFSI contribute to forming a Li3N-LiF-enriched interface and meanwhile LiTFSI ensures excellent ***,among various Li compound components,Li3N has high ionic conductivity,which is beneficial for reducing overpotential,while LiF has high interfacial energy which can enhance nucleation energy and suppress the formation of Li *** experimental results show that ASSLBs coupled with LiFePO4cathode display extremely excellent cycle stability approximately 2200 cycles at 2 c,with a final and corresponding discharge specific capacity of 96.7 mA h g-1. Additionally,a schematic illustration of the working mechanism for the Li3N-LiF interface is proposed.

关键词： All-solid-state lithium metal batteries In-situ SEI Lithium dendrite PEO (LiTFSI) Solid electrolyte

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Engineering nanoparticle structure at synergistic Ru-Na interface for integrated cO_(2)capture and hydrogenation

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Journal of Energy chemistry 2025年第1期100卷 779-791页

作者： Hanzi liu Ling cen Xinlin Xie Lei liu Zhao Sun Zhiqiang Sun Hunan Engineering Research center of clean and Low-carbon Energy Technology School of Energy Science and EngineeringCentral South UniversityChangsha 410083HunanChina

The development of dual functional material for cyclic cO_(2)capture and hydrogenation is of great significance for converting diluted cO_(2)into valuable fuels,but suffers from kinetic limitation and deactivation of adsorbent and ***,we engineered a series of RuNa/γ-Al_(2)O_(3)materials,varying the size of ruthenium from single atoms to clusters/*** coordination environment and structure sensitivity of ruthenium were quantitatively investigated at atomic *** findings reveal that the reduced Ru nanoparticles,approximately 7.1 nm in diameter with a Ru-Ru coordination number of 5.9,exhibit high methane formation activity and selectivity at 340°*** Ru-Na interfacial sites facilitate cO_(2)migration through a deoxygenation pathway,involving carbonate dissociation,carbonyl formation,and ***-situ experiments and theoretical calculations show that stable carbonyl intermediates on metallic Ru nanoparticles facilitate heterolytic c–O scission and c–H bonding,significantly lowering the energy barrier for activating stored cO_(2).

关键词： cO_(2)capture Hydrogenation Ru-Na interface Dual functional material Reaction mechanism

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Evolution and generation mechanism of retained oil in lacustrine shales: A combined ReaxFF-MD and pyrolysis simulation perspective

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Petroleum Science 2025年第1期22卷 29-41页

作者： Biao Sun Xiao-Ping liu Jie liu Tian liu Zu-Xian Hua Wen-Di Peng National Key Laboratory of Petroleum Resources and Engineering China University of Petroleum (Beijing) college of Geosciences China University of Petroleum (Beijing) International Petroleum Exploration and Production corporation SINOPEC

To accurately investigate the evolution characteristics and generation mechanism of retained oil, the study analyzed organic-rich lacustrine shale samples from the Paleogene Kongdian Formation in cangdong Sag, Bohai Bay Basin. This analysis involves Rock-Eval pyrolysis, pyrolysis simulation experiments,Gas chromatograph Mass Spectrometer（Gc-MS）, and reactive molecular dynamics simulations（Reax FF）. The results revealed the retained oil primarily consisted of n-alkanes with carbon numbers ranging from c14to c36. The generation of retained oil occurred through three stages. A slow growth stage of production rate was observed before reaching the peak of oil production in Stage I. Stage II involved a rapid increase in oil retention, with c12-c17and c24-c32serving as the primary components,increasing continuously during the pyrolysis process. The generation process involved the cleavage of weak bonds, including bridging bonds（hydroxyl, oxy, peroxy, imino, amino, and nitro）, ether bonds, and acid amides in the first stage（Ro= 0.50%-0.75%）. The carbon chains in aromatic ring structures with heteroatomic functional groups breaks in the second stage（Ro= 0.75%-1.20%）. In the third stage（Ro= 1.20%-2.50%）, the ring structures underwent ring-opening reactions to synthesize iso-short-chain olefins and radicals, while further breakdown of aliphatic chains occurred. By coupling pyrolysis simulation experiments and molecular simulation technology, the evolution characteristics and bond breaking mechanism of retained oil in three stages were revealed, providing a reference for the formation and evolution mechanism of retained oil.

关键词： Lacustrine shale Retained oiliness evolution Pyrolysis simulation experiments ReaxFF molecular dynamics Hydrocarbon generation evolution

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Boosting cationic and anionic redox activity of Li-rich layered oxide cathodes via Li/Ni disordered regulation

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Journal of Energy chemistry 2025年第1期100卷 533-543页

作者： Zewen liu Zhen Wu Hao Wang Xudong Zhang Yuanzhen chen Yongning liu Shengwu Guo Shenghua chen Yanli Nan Yan liu State Key Laboratory for Mechanical Behavior of Materials Xi’an Jiaotong UniversityXi’an 710049ShaanxiChina School of Materials Science and Engineering Xi’an University of Architecture and TechnologyXi’an 710055ShaanxiChina Hefei Advanced computing center Operation Management corp Ltd Hefei 230088AnhuiChina Network Information center Xi’an Jiaotong UniversityXi’an 710049ShaanxiChina

Lithium-rich layered oxides (LLOs) are increasingly recognized as promising cathode materials for nextgeneration high-energy-density lithium-ion batteries (LIBs).However,they suffer from voltage decay and low initial coulombic efficiency (IcE) due to severe structural degradation caused by irreversible O ***,we introduce a three-in-one strategy of increasing Ni and Mn content,along with Li/Ni disordering and TM–O covalency regulation to boost cationic and anionic redox activity simultaneously and thus enhance the electrochemical activity of *** target material,Li_(1.2)Ni_(0.168)Mn_(0.558)co_(0.074)O_(2)(L1),exhibits an improved IcE of 87.2%and specific capacity of 293.2 mA h g^(-1)and minimal voltage decay of less than 0.53 m V cycle-1over 300 cycles at 1c,compared to Li_(1.2)Ni_(0.13)Mn_(0.54)co_(0.13)O_(2)(Ls)(274.4 mA h g^(-1)for initial capacity,73.8%for IcE and voltage decay of 0.84 mV/cycle over 300 cycles at 1c).Theoretical calculations reveal that the density of states (DOS) area near the Fermi energy level for L1 is larger than that of Ls,indicating higher anionic and cationic redox reactivity than ***,L1 exhibits increased O-vacancy formation energy due to higher Li/Ni disordering of 4.76%(quantified by X-ray diffraction Rietveld refinement) and enhanced TM–O covalency,making lattice O release more difficult and thus improving electrochemical *** increased Li/Ni disordering also leads to more Ni^(2+)presence in the Li layer,which acts as a pillar during Li+de-embedding,improving structural *** research not only presents a viable approach to designing low-co LLOs with enhanced capacity and IcE but also contributes significantly to the fundamental understanding of structural regulation in high-performance LIB cathodes.

关键词： Low-co Li-rich layered oxides Li/Ni disordering TM-O covalency cationic and anionic redox activity

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