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comparing the temperature sensitivity of organic matter decomposition in oxic and oxygen-deprived soils

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Soil Ecology Letters 2024年第1期6卷 29-32页

作者： Zhenhui jiang Xin Wang Ting Liu Xiaojuan Feng State Key Laboratory of Vegetation and Environmental change Institute of BotanyChinese Academy of SciencesBeiing 100093China University of chinese Academy of Sciences Bejing 100049China State Key Laboratory of Subtropical Silviculture Zhejiang A&F UniversityHangzhou 311300China Henan Key Laboratory of Ecological Environment Protection and Restoration of Yellow River Basin Yellow River Institute of Hydraulic ResearchZhengzhou 450003China

No consistent variation was found in soil respiration Q10 under various O2 *** c quality had a strong effect on Q10 in oxic soils.N limitation had a large impact on Q10 in soils under O2 *** studies on the temperature sensitivity(Q10)of soil organic matter(SOM)decomposition mainly focus on aerobic ***,varia-tions and determinants of Q10 in oxygen(O2)-deprived soils remain *** we incubated three grassland soils under oxic,suboxic,and anoxic conditions subjected to varying temperatures to compare variations in Q10 in relation to changing *** consistent variation was found in Q10 under various O2 *** analysis of edaphic properties demon-strated that substrate carbon quality showed a strong influence on Q10 in oxic soils,whereas nitrogen limitation played a more important role in suboxic and anoxic *** results suggest that substrate carbon quality and nitrogen limitation may play roles of varying importance in determining the temperature sensitivity of SOM decomposition under various O2 conditions.

关键词： oxygen-limited conditions temperature sensitivity soil respiration carbon substrate nitrogen limitation

MDGA2 constrains Glutamatergic Inputs Selectively onto cA1 Pyramidal Neurons to Optimize Neural circuits for Plasticity,Memory,and Social Behavior

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Neuroscience Bulletin 2024年第7期40卷 887-904页

作者： Xuehui Wang Donghui Lin Jie jiang Yuhua Liu Xinyan Dong Jianchen Fan Lifen Gong Weida Shen Linghui Zeng Tonghui Xu Kewen jiang Steven A.connor Yicheng Xie School of Life Sciences Nanchang UniversityNanchang330031China Department of Neurology Children's HospitalZhejiang University School of MedicineNational Clinical Research Center for Child HealthHangzhou 310052China Department of Biology York University4700 Keele StreetTorontoON M3J 1P3Canada Key Laboratory of Novel Targets and Drug Study for Neural Repair of Zhejiang Province School of MedicineHangzhou City UniversityHangzhou 310015China

Synapse organizers are essential for the development,transmission,and plasticity of *** as rare synapse suppressors,the MAM domain containing glycosylphosphatidylinositol anchor(MDGA)proteins contributes to synapse organization by inhibiting the formation of the synaptogenic neuroligin-neurexin complex.A previous analysis of MDGA2 mice lacking a single copy of Mdga2 revealed upregulated glutamatergic synapses and behaviors consistent with ***,MDGA2 is expressed in diverse cell types and is localized to both excitatory and inhibitory *** the network versus cell-specific effects of MDGA2 loss-of-function requires a cell-type and brain region-selective *** address this,we generated mice harboring a conditional knockout of Mdga2 restricted to cA1 pyramidal *** we report that MDGA2 suppresses the density and function of excitatory synapses selectively on pyramidal neurons in the mature *** deletion of Mdga2 in cA1 pyramidal neurons of adult mice upregulated miniature and spontaneous excitatory postsynaptic potentials,vesicular glutamate transporter 1 intensity,and neuronal *** effects were limited to glutamatergic synapses as no changes were detected in miniature and spontaneous inhibitory postsynaptic potential properties or vesicular GABA transporter ***,evoked basal synaptic transmission and AMPAR receptor currents were enhanced at glutamatergic *** a behavioral level,memory appeared to be compromised in Mdga2 cKO mice as both novel object recognition and contextual fear conditioning performance were impaired,consistent with deficits in long-term potentiation in the cA3-cA1 *** affiliation,a behavioral analog of social deficits in autism,was similarly *** results demonstrate that MDGA2 confines the properties of excitatory synapses to cA1 neurons in mature hippocampal circuits,thereby optimizing this network for plasticity,c

关键词： MDGA2 cA1 pyramidal neurons Glutamatergic inputs Synaptic plasticity Memory Social behaviors Autism Synapse organizers

BIG HANKEL OPERATORS ON HARDY SPAcES OF STRONGLY PSEUDOcONVEX DOMAINS

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Acta Mathematica Scientia 2024年第3期44卷 789-809页

作者：陈伯勇江良英 School of Mathematical Sciences Fudan UniversityShanghai200433China Department of Statistics and Mathematics Shanghai Lixin University of Accounting and FinanceShanghai201209China

In this article,we investigate the(big) Hankel operator H_(f) on the Hardy spaces of bounded strongly pseudoconvex domains Ω in c^(n).We observe that H_(f ) is bounded on H~p(Ω)(1

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In this article,we investigate the(big) Hankel operator H_(f) on the Hardy spaces of bounded strongly pseudoconvex domains Ω in c^(n).We observe that H_(f ) is bounded on H~p(Ω)(1 characterizations for Hf on H^(2)(Ω) of other pseudoconvex *** these arguments,Amar's L^(p)-estimations and Berndtsson's L^(2)-estimations for solutions of the ■_(b)-equation play a crucial *** addition,we solve Gleason's problem for Hardy spaces H^(p)(Ω)(1 ≤p≤∞) of bounded strongly pseudoconvex domains.

关键词： Hankel operator Hardy space Bergman space pseudoconvex domain

AB_(2)-type rare earth-based compounds with c-15 structure:Looking for reversible hydrogen storage materials

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Journal of Rare Earths 2024年第5期42卷 803-816,I0001页

作者： Hao Shen Junxian Zhang Valerie Paul-Boncour Ping Li Zhinian Li Yuanfang Wu Lijun jiang National Engineering Research center of Nonferrous Metals Materias and Products for New Energy GRINM Group Co.LtdBeijing00088China Univ Paris Est creteil CNRSICMPEUMR 71822 rue Henri Dunant94320ThiaisFrance Institute for Advanced Materials and Technology University of Science and TechnologyBeijing100083China GRIMAT Engineering Institute co. Ltd.Beijing101407China

AB_(2)-type(A=rare earth,B=transition metal)intermetallic compounds with c15 structure can easily absorb large amount of hydrogen,showing their potential use as hydrogen storage *** crucial problem hindering their application is hydrogen induced amorphization(HIA),which leads to the irreversible hydrogen sorption *** stability of the AB_2 Laves phase compounds,the structural properties,the hydrogenation properties and the controlling factors of HIA are discussed in this *** with other factors,the atomic radii ratio r_A/r_B is the most important one influencing the ***-element substitution is an efficient way to suppress or limit HIA and may enable AB_2 compounds to be suitable for hydrogen storage.

关键词： Rare earth-based AB_2-type compounds Hydrogenation properties Hydrogen induced amorphization Elemental substitution

Single-atom Ni-N_(4) for enhanced electrochemical sensing

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Nano Research 2024年第8期17卷 7658-7664页

作者： Zhuhui Qin Bo Tang Guiru Zhang chongqing Zhu Kun jiang Bowei Zhang Fu-Zhen Xuan Shanghai Key Laboratory of Intelligent Sensing and Detection Technology East China University of Science and TechnologyShanghai 200237China Key Laboratory of Pressure Systems and Safety of Ministry of Education East China University of Science and TechnologyShanghai 200237China School of Mechanical and Power Engineering East China University of Science and TechnologyShanghai 200237China Key Laboratory of Theoretical and computational Photochemistry Ministry of EducationCollege of ChemistryBeijing Normal UniversityBeijing 100875China Interdisciplinary Research center School of Mechanical EngineeringShanghai Jiao Tong UniversityShanghai 200240China

Single-atom catalysts(SAcs)attract widespread attention in heterogeneous catalysis due to their maximum atomic utilization efficiency and unique physical and chemical ***,their applications in chemical sensing keep huge potential but remain ***,a Ni-N_(4)-c SAc was synthesized for the trace detection of dopamine(DA)and uric acid(UA).The Ni-N_(4)-c SAc exhibited superior sensing performance compared to the Ni *** detection range for DA and UA were 0.05–75μM and 5–90μM with detection limits of 0.027 and 0.82μM,*** functional theory(DFT)computations indicate that Ni-N_(4)-c has a lower reaction barrier during electrochemical process,indicating that the atomic Ni sites possess higher intrinsic activity than Ni ***,DA and UA show strong potential dependency on the Ni-N_(4)-c catalyst,indicating its applicability for their concurrent *** work extends the application of SAcs in chemical sensing.

关键词： single-atom catalysts chemical sensing dopamine uric acid

Ten-Minute Synthesis of a New Redox-Active Aqueous Binder for Flame-Retardant Li-S Batteries

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Energy & Environmental Materials 2024年第2期7卷 48-57页

作者： Tianpeng Zhang Borui Li Zihui Song Wanyuan jiang Siyang Liu Runyue Mao Xigao Jian Fangyuan Hu School of Materials Science and Engineering State Key Laboratory of Fine ChemicalsFrontiers Science Center for Smart Materials Oriented Chemical Engineering Technology Innovation Center of High Performance Resin Materials(Liaoning Province)Key Laboratory of Energy Materials and Devices(Liaoning Province)Dalian University of TechnologyDalian 116024China State Key Laboratory of Fine chemicals Frontiers Science Center for Smart Materials Oriented Chemical EngineeringSchool of Chemical Engineering Technology Innovation Center of High Performance Resin Materials(Liaoning Province)Key Laboratory of Energy Materials and Devices(Liaoning Province)Dalian University of TechnologyDalian 116024China

As a critical role in battery systems,polymer binders have been shown to efficiently suppress the lithium polysulfide shuttling and accommodate volume changes in recent ***,preparation processes and safety,as the key criterions for Li-S batteries'practical applications,still attract less ***,an aqueous multifunction binder(named PEI-TIc)is prepared via an easy and fast epoxy-amine ring-opening reaction(10 min),which can not only give the sulfur cathode a stable mechanical property,a strong chemical adsorption and catalytic conversion ability,but also a fire safety *** Li-S batteries based on the PEI-TIc binder display a high discharge capacity(1297.8 mAh g^(-1)),superior rate performance(823.0 mAh g^(-1)at 2 c),and an ultralow capacity decay rate of 0.035%over more than 800 *** under 7.1 mg cm^(-2)S-loaded,the PEI-TIc electrode can also achieve a high areal capacity of 7.2 mA h g^(-1)and excellent cycling stability,confirming its application ***,it is also noted that TG-FTIR test is performed for the first time to explore the flame-retardant mechanism of polymer *** work provides an economically and environmentally friendly binder for the practical application and inspires the exploration of the flame-retardant mechanism of all electrode components.

关键词： 3D cross-linked network environmentally friendly flame retardant Li-S batteries multifunction binder

Molecule aging induced by electron attacking

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Journal of Energy chemistry 2024年第6期93卷 519-525,I0013页

作者： Ping Song Yining Dong Xue Gong Mingbo Ruan Baoxin Ni Xuanhao Mei Kun jiang Weilin Xu State Key Laboratory of Electroanalytical chemistry and Jilin Province Key Laboratory of Low carbon chemical Power Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022JilinChina School of Applied chemistry and Engineering University of Science and Technology of Chin1Hefei 230026AnhuiChina Shanghai Key Laboratory of Molecular catalysis and Innovative Materials Collaborative Innovation Center of Chemistry for Energy MaterialsDepartment of ChemistryFudan UniversityShanghai 200438China

Here we propose a new concept of"molecule aging":with some special treatment,a molecule could be"aged"by losing some unknown tiny particles or pieces from atoms in the molecule,Such"aging"or loss of unknown tiny particles does not change apparently its molecular structure or chemical composition,but some physicochemical properties could be changed *** further confirm such"molecule aging"via a long-term electron attacking to age water(H_(2)O)*** IR spectra show no structural difference between the fresh water and the aged one,while the NMR spectra show that the electron attacking can decrease the size of water *** facts indicate that the electron attacking indeed can"affect"the structure of water molecule slightly but without damaging to its basic molecule *** exploration reveals that the hydrogen evolution reaction(HER)activity of the aged water molecule is lower than the fresh water on the same Pt/c *** density functional theory calculations indicate that the shortened O-H bond in H_(2)O indeed can present lower HER activity,so the observed size decrease of water clusters from NMR probably could be attributed to the shortening of O-H bond in water *** results indicate significantly that the molecule aging can produce materials with new functions for new possible applications.

关键词： Aging of molecules Electron attacking Full width at half maxima Hydrogen evolution reaction

Two-Dimensional Perovskite Single crystals for High-Performance X-ray Imaging and Exploring MeV X-ray Detection

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Energy & Environmental Materials 2024年第1期7卷 139-146页

作者： Xieming Xu Yiheng Wu Yi Zhang Xiaohui Li Fang Wang Xiaoming jiang Shaofan Wu Shuaihua Wang Key Laboratory of Optoelectronic Materials chemistry and Physics Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China University of chinese Academy of Sciences Beijing 100049China Division of Nuclear Technology and Applications Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of china Fuzhou 350108China

Scintillation semiconductors play increasingly important medical diagnosis and industrial inspection ***,two-dimensional(2D)perovskites have been shown to be promising materials for medical X-ray imaging,but they are mostly used in low-energy(≤130 keV)*** detection of MeV X-rays,which ensure thorough penetration of the thick shell walls of containers,trucks,and aircraft,is also highly desired in practical industrial ***,scintillation semiconductors for high-energy X-ray detection are currently ***,This paper reports a 2D(c_(4)H_(9)NH_(3))_(2)PbBr_(4)single crystal with outstanding sensitivity and stability toward X-ray radiation that provides an ultra-wide detectable X-ray range of between 8.20 nGy_(air)s^(-1)(50 keV)and 15.24 mGy_(air)s^(-1)(9 MeV).The(c_(4)H_(9)NH_(3))_(2)PbBr_(4)single-crystal detector with a vertical structure is used for high-performance X-ray imaging,delivering a good spatial resolution of 4.3 Ip mm^(-1)in a plane-scan imaging *** ionic migration in the 2D perovskite enables the vertical device to be operated with hundreds of keV to MeV X-ray radiation at high bias voltages,leading to a sensitivity of 46.90μc Gy_(air)-1 cm^(-2)(-1.16 Vμm^(-1))with 9 MeV X-ray radiation,demonstrating that 2D perovskites have enormous potential for high-energy industrial applications.

关键词： MeV X-ray detection single-crystal X-ray detectors two-dimensional perovskites X-ray imaging

Drilling-based measuring method for the c-φ parameter of rock and its field application

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International Journal of Mining Science and Technology 2024年第1期34卷 65-76页

作者： Bei jiang Fenglin Ma Qi Wang Hongke Gao Dahu Zhai Yusong Deng chuanjie Xu Liangdi Yao State Key Laboratory for Tunnel Engineering China University of Mining and Technology-BeijingBeijing 100083China State Key Laboratory of Explosion Science and Technology Beijing Institute of TechnologyBeijing 100081China Research center of Geotechnical and Structural Engineering Shandong UniversityJinan 250061China

The technology of drilling tests makes it possible to obtain the strength parameter of rock accurately in situ. In this paper, a new rock cutting analysis model that considers the influence of the rock crushing zone(RcZ) is built. The formula for an ultimate cutting force is established based on the limit equilibrium principle. The relationship between digital drilling parameters(DDP) and the c-φ parameter(DDP-cφ formula, where c refers to the cohesion and φ refers to the internal friction angle) is derived, and the response of drilling parameters and cutting ratio to the strength parameters is analyzed. The drillingbased measuring method for the c-φ parameter of rock is constructed. The laboratory verification test is then completed, and the difference in results between the drilling test and the compression test is less than 6%. On this basis, in-situ rock drilling tests in a traffic tunnel and a coal mine roadway are carried out, and the strength parameters of the surrounding rock are effectively tested. The average difference ratio of the results is less than 11%, which verifies the effectiveness of the proposed method for obtaining the strength parameters based on digital drilling. This study provides methodological support for field testing of rock strength parameters.

关键词： Digital drilling Rock crushing zone c-u parameter Measurement method Field application