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Dielectric-ion-conductive ZnNb2O6 layer enabling rapid desolvation and diffusion for dendrite-free Zn metal batteries

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Journal of Energy chemistry 2025年第1期100卷 693-701页

作者： Haifeng yang Jian Wang Panpan Zhang Xiaomin cheng Qinghua Guan Jing Dong Bixian chen Lujie Jia Jing Zhang yongzheng Zhang yunjian Liu Hongzhen Lin School of Materials Science and Engineering Jiangsu University i-Lab & cAS Key Laboratory of Nanophotonic Materials and Devices Suzhou Institute of Nano-Tech and Nano-Bionics Chinese Academy of Sciences Helmholtz Institute Ulm (HIU) Karlsruhe Institute of Technology (KIT) School of Materials Science and Engineering Xi'an University of Technology State Key Laboratory of chemical Engineering East China University of Science and Technology

Rechargeable aqueous zinc-metal batteries （AZMBs） are promising candidates for large-scale energy storage systems due to their low cost and high ***,their performance and sustainability are significantly hindered by the sluggish desolvation kinetics at the electrode/electrolyte interface and the corresponding hydrogen evolution reaction where active water molecules tightly participate in the Zn（H2O）62+solvation ***,learnt from self-generated solid electrolyte interphase （SEI） in anodes,the dielectric but ion-conductive zinc niobate nanoparticles artificial layer is constructed on metallic Zn surface （ZNB@Zn）,acting as a rapid desolvation *** zincophilic and dielectric-conductive properties of ZNB layer accelerate interfacial desolvation/diffusion and suppress surface corrosion or dendrite formation,achieving uniform Zn plating/stripping behavior,as confirmed by electronic/optical microscopies and interface spectroscopical measurements together with theoretical ***,the as-prepared ZNB@Zn electrode exhibits excellent cycling stability of over 2000 h and robust reversibility （99.54%） even under high current density and depth of discharge ***,the assembled ZNB@Zn-based full cell displays high capacity-retention rate of 80.21%after 3000 cycles at 5 A g-1and outstanding rate performance up to 10 A *** large-areal pouch cell is stabilized for hundreds of cycles,highlighting the bright prospects of the dielectric but ion-conductive layer in further application of AZMBs.

关键词： Zn metal battery Dielectric artificial layer Rapid ion diffusion Zincophilic diffusion Active water inhibition

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FAcTORS ON VIScOSITy STABILITy OF MOLD FLUXES

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Acta Metallurgica Sinica(English Letters) 2004年第2期17卷 175-180页

作者： c.y.Zhu c.J.Liu M.F.Jiang Z.D.yang NortheasternUniversity Shenyang110004China Ji＇nanIronandSteelGroupco. Ji＇nan250101China

Viscosity stability indexes of mold flux at high temperature and low temperature havebeen introduced and the effects of flux compositions on viscosity stability indexeshave been studied. Two mold fluxes have been developed by analyzing the effects offlux viscosity stability on the process and the condition of continuous casting slab ofmedium carbon steel. The results show that the fluxes are suitable for the process.

关键词： mold flux viscosity stability index high temperature low temperature

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Gene therapy for spinal muscular atrophy:perspectives on the possibility of optimizing SMN1 delivery to correct all neurological and systemic perturbations

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Neural Regeneration Research 2025年第7期20卷 2011-2012页

作者： Sharon J.Brown Rafael J.yáñez-Muñoz Heidi R.Fuller School of Pharmacy and Bioengineering Keele UniversityKeeleUK Wolfson center for Inherited Neuromuscular Disease TORCH BuildingRJAH Orthopaedic HospitalOswestryUK *** Center of Gene and Cell TherapyDepartment of Biological SciencesSchool of Life Sciences and the EnvironmentRoyal Holloway University of LondonEghamUK

Spinal muscular atrophy(SMA)is a genetic condition that results in selective lower motor neuron loss with concomitant muscle weakness and *** genetic cause of SMA was understood in 1995 when loss or impairment of the survival motor neuron 1(SMN1)gene was identified as the main contributing factor(Lefebvre et al.,1995).This,in combination with the discovery that humans have a“back-up”gene,SMN2,which can produce low levels(approximately 10%)of the full-length functional SMN protein,has led to the generation of SMA-specific gene *** was traditionally classified according to age of symptom onset and developmental milestones achieved,with life expectancy and severity varying between ***,SMN2 copy number is used as a proxy for the prediction of disease severity,with higher SMN2 copy number typically being associated with reduced severity of SMA,although this relationship is not absolute:some individuals with low SMN2 copy number have less severe SMA phenotypes and vice ***,the etiology of SMA is further complicated by other factors,such as non-typical nucleotide variants and SMN2-independent modifiers of disease severity.

关键词： atrophy traditionally absolute

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Expression of IGF-Ⅱ,p53,p21 and HBxAg in precancerous events of hepatocarcinogenesis induced by AFBI and/or HBV in tree shrews

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World Journal of Gastroenterology 2000年第1期6卷 138-139页

作者： Qin LL Su JJ Li y yang c Ban Kc yian RQ Department of Pathology Guangxi Cancer InstituteNanning 530021China Department of Pathology Cancer InstituteSun Yat-Sen University of Medical SciencesGuangzhou510060China

INTRODUcTIONIn order to study the relationship between oncogeneexpression and Hcc generation,we observed theprecancerous hepatic GGT loci,IGF-Ⅱ,p53 andp21 expression during hepatocarcinogenesis of treeshrew induced b... 详细信息

关键词： Subject heading liver neoplasms carcinoma hepatocellular hepatitis B virus IGF-Ⅱ p53 gene p21 gene HBxAg aflatoxin B1

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Molecular Dynamics Simulation of Behaviours of Non-Polar Droplets Merging and Interactions with Hydrophobic Surfaces

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Journal of Bionic Engineering 2008年第4期5卷 271-281页

作者： y.y. yan c.y. Ji School of the Built Environment University of Nottingham Nottingham NG7 2RD UK

This paper presents a molecular dynamics simulation of the behaviours of non-polar droplets merging and also the fluid molecules interacting with a hydrophobic surface. Such behaviours and transport phenomena are popular in general microchannel flow boiling and two-phase flow. The droplets are assumed to be composed of Lennards-Jones type molecules. Periodic boundary conditions are applied in three coordinate directions of a 3-D system, where there exist two liquid droplets and their vapour. The two droplets merge when they come within the prescribed small distance. The merging of two droplets apart from each other at different initial distances is tested and the possible larger （or critical） non-dimensional distance, in which droplets merging can occur, is discussed. The evolution of the merging process is simulated numerically by employing the Molecular Dynamics （MD） method. For interactions with hydrophobic solid wall, a system with fluid confined between two walls is used to study the wetting phenomena of fluid and solid wall. The results are compared with those of hydrophilic wall to show the unique characteristics of hydrophobic interactions by microscopic methods.

关键词： molecular dynamics simulation mist flow droplets merging hydrophobic wetting

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Dislocation self-interaction in TiAl:Evolution of super-dislocation dipoles revealed by atomistic simulations

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Journal of Materials Science & Technology 2021年第10期69卷 138-147页

作者： Z.Zhen H.Wang c.y.Teng c.G.Bai D.S.Xu R.yang Institute of Metal Research Chinese Academy of SciencesShenyang 110016China School of Materials Science and Engineering University of Science and Technology of China.Shenyang 110016China School of Materials Science and Engineering University of Shanghai for Science and TechnologyShanghai 200093China Laboratory of Fundamental Research AVIC China Aero-Polytechnology EstablishmentBeijing 100028.China

As one of the fundamental outcomes of dislocation self-interaction,dislocation dipoles have an important influence on the plastic deformation of materials,especially on fatigue and *** this work,superdislocation dipoles inγ-TiAl andα_(2)-Ti_(3)Al were systematically investigated by atomistic simulations,with a variety of dipole heights,orientations and annealing tempe *** results indicate that non-screw super-dipoles transform into locally stable dipolar or reconstructed cores at low temperature,while into isolated or interconnected point defect clusters and stacking fault tetrahedra at high temperature via short-range diffu ***-screw super-dipoles inγ-TiAl andα_(2)-Ti_(3)Al exhibit similar features as fcc and hcp metals,***,over long-term annealing where diffusion is significant,60°superdipoles inγ-TiAl are stable,whereas the stability of super-dipoles inα2-Ti3 Al increases with dipole height and orientation *** influence on mechanical properties can be well evaluated by integrating these results into mesoscale or constitutive models.

关键词： TiAl Dislocation Dipole Mechanical property Atomistic simulation

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A dissolution-diffusion sliding model for soft rock grains with hydro-mechanical effect

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Journal of Rock Mechanics and Geotechnical Engineering 2018年第3期10卷 457-467页

作者： Z.Liu c.y.Zhou B.T.Li y.Q.Lu X.yang Guangdong Engineering Research center for Major Infrastructure Safety School of Civil Engineering Sun Yat-sen University

The deformation and failure of soft rock affected by hydro-mechanical（HM） effect are one of the most concerns in geotechnical engineering, which are basically attributed to the grain sliding of soft rock. This study tried to develop a dissolution-diffusion sliding model for the typical red bed soft rock in South china. Based on hydration film, mineral dissolution and diffusion theory, and geochemical thermodynamics, a dissolution-diffusion sliding model with the HM effect was established to account for the sliding rate. combined with the digital image processing technology, the relationship between the grain size of soft rock and the amplitude of sliding surface was presented. An equation for the strain rate of soft rocks under steady state was also derived. The reliability of the dissolution-diffusion sliding model was verified by triaxial creep tests on the soft rock with the HM coupling effect and by the relationship between the inversion average disjoining pressure and the average thickness of the hydration film. The results showed that the sliding rate of the soft rock grains was affected significantly by the waviness of sliding surface, the shear stress, and the average thickness of hydration film. The average grain size is essential for controlling the steady-state creep rate of soft rock. This study provides a new idea for investigating the deformation and failure of soft rock with the HM effect.

关键词： Soft rock Hydro-mechanical (HM) effect Mineral dissolution-diffusion Grain sliding model

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Diffusion of Hydrogen in Amorphous NicrFeSiB Alloy

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Journal of Materials Science & Technology 1996年第1期12卷 15-18页

作者： Zuo, y yang, B Xu, RS Dept. of Applied chemistry Beijing University of Chemical Technology Beijing 100029 China

The diffusion of hydrogen in amorphous NicrFeSiB alloy has been studied by electrochemical method. In the temperature range of 20 similar to 50 degrees c, diffusion coefficient of hydrogen in the alloy follows the equation: D(cm(2)/s) = 9.27x10(-8) exp(-53.4 kJ/RT). At room temperature the diffusion coefficient D and the solubility c-0 are 6.125 x 10(-12) cm(2)/s and 0.007 mol/cm(3), respectively. When As2O3 is added into the cathodic solution or the charging current density is increased, the diffusion coefficient and solubility increase, and the diffusion activation energy decreases. The influence of amorphous structure on diffusion and solution of hydrogen is discussed.

关键词： Nickel alloys

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Simultaneous enhancement of mechanical and shape memory properties by heat-treatment homogenization of Ti_(2)Ni precipitates in TiNi shape memory alloy fabricated by selective laser melting

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Journal of Materials Science & Technology 2022年第6期101卷 205-216页

作者： H.Z.Lu L.H.Liu c.yang X.Luo c.H.Song Z.Wang J.Wang y.D.Su y.F.Ding L.c.Zhang y.y.Li National Engineering Research center of Near-net-shape Forming for Metallic Materials South China University of TechnologyGuangzhou 510640China Musculoskeletal Oncology Department Sun Yat-Sen University Cancer CenterGuangzhouGuangdong ProvinceChina Shenyang Aircraft Design and Research Institute Shenyang 110035China Guangdong Huayi Plumbing Fittings Industry co. Ltd.Kaiping 529321China School of Engineering Edith Cowan University270 Joondalup DriveJoondalupPerthWA 6027Australia

The excellent shape memory and mechanical properties of Ti Ni shape memory alloys(SMAs) fabricated using selective laser melting(SLM) are highly desirable for a wide range of critical applications. In this study, we examined the simultaneous enhancement of mechanical and shape memory properties using heat-treatment homogenization of Ti_(2)Ni precipitates in a Ti_(50.6)Ni_(49.4)SMA fabricated using SLM. Specifically, because of the complete solution treatment, nanoscale spherical Ti_(2)Ni precipitates were homogeneously dispersed throughout the grain interior. Interestingly, the resultant SMA exhibited an ultrahigh tensile strength of 880 ± 13 MPa, a large elongation of 22.4 ± 0.4%, and an excellent shape memory effect, with a recovery rate of > 98% and ultrahigh recoverable strain of 5.32% after ten loading–unloading cycles. These simultaneously enhanced properties are considerably superior than those of most previously reported Ti Ni SMAs fabricated using additive manufacturing. Fundamentally, the enhancement in tensile strength is ascribed to precipitation strengthening and work hardening, and the large plasticity is mainly attributed to the homogeneous nanoscale globular Ti_(2)Ni precipitates, which effectively impeded the rapid propagation of microcracks. Furthermore, the enhanced shape memory properties are derived from the suppression of dislocation movement and formation of retained stabilized martensite by the presence of high-density dislocations, nanoscale Ti_(2)Ni precipitates, and abundant interfaces. The obtained results provide insight into the enhancement of the two types of properties in Ti Ni SMAs and will accelerate the wider application of SMAs.

关键词： Shape memory alloy Selective laser melting Heat treatment Mechanical properties Shape memory properties

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Application of Neural Network in Precision Prediction of Hat-Section Profiles in Rotary Draw Bending

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Journal of Materials Science & Technology 2001年第1期17卷 137-138页

作者： Li, X.c. yang, y.y. Jin, Z.H. Liu, J.T. Li, S.P. Harbin Inst. of Technol. Harbin 150001 China

It is difficult to control the accuracy of hat-section profile rotary-draw bent products because their shapes are complex and many factors influence the forming process. A multi-layer feed-forward neural network based on improved BP (back propagation) algorithm is adopted to study the influence law of the main material properties and forming parameters on the accuracy of hat-section profile forming process. The prediction of rotary draw-bending precision is realized and the technology parameters in the forming process are controlled according to the given precision.

关键词： Application of Neural Network in Precision Prediction of Hat-Section Profiles in Rotary Draw Bending

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