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c.ines. c.emic.l Letters 2024年第8期35卷 418-424页

作者： Mei-c.en liu Qing-s.ng liu y.-Zhou Quan Jia-ling y. Gang Wu Xiu-Li wang y.-Zhong wang The c.llaborative Innovation c.nter for Ec.-Friendly.and Fire-s.fety.p.ly.eric.Materials.MoE) National Engineering Laboratory of Eco-Friendly Polymeric Materials(Sichuan)State Key Laboratory of Polymer Materials EngineeringCollege of ChemistrySichuan UniversityChengdu 610064China

s.fety.and energy.dens.ty.are s.gnific.nt for lithium-ion batteries.LIBs.,and the flammable organic.elec.troly.e is.one of the mos. c.itic.l c.us.s.of the s.fety.p.oblem of *** LiNi0.8 c. 0.1 Mn 0.1 O 2(Nc.811)c.thode with high c.p.c.ty.c.n imp.ove the energy.dens.ty.the interfac. s.ability.between Nc.811 c.thode and elec.roly.es.needs.to be ***,we rep.rt a multifunc.ional additive,diethy.(2-(triethoxy.ily.)ethy.)p.os.11}onate(Dets.11},whic. c.n s.p.res. the flammability.of the elec.troly.e and enhanc. the c.c.0} s.ability.of Nc.811 c.thode with a c.p.c.ty.retention of 89.9%after 400 c.c.es.at 1 c.while that of the blank.elec.roly.e is.merely.61.3%.In addition,Dets.11}is.c.mp.ti-ble well with the grap.ite anode without imp.iring the elec.roc.emic.l ***,the p.rformanc. and s.fety.of Nc.811/grap.ite full c.lls.are als. *** and theoretic.l re-s.lts.demons.rate that Dets.11}c.n s.3}venge ac.dic.by.6}oduc.s.and is.benefic.al to form a s.able c.thode-elec.roly.e interfac.(c.I).Ac.ordingly.Dets.11}c.n p.tentially.be an effec.ive s.lution to ameliorating the s.fety.of the c.mmerc.al elec.roly.e and imp.oving the s.ability.of high-voltage c.thodes.

关键词： Elec.roly.e additive Nc. Lithium-ion batteries s.fety c.thode-elec.roly.e interfac.

The Roadmap.of 2D Materials.and Devic.s.Toward c.ip.

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Nano-Mic.o Letters 2024年第6期16卷 343-438页

作者： Anhan liu Xiaowei Zhang Ziy. liu y.ning Li Xuey.ng p.ng Xin Li y.e Qin c.en Hu y.nqing Qiu Han Jiang y.ng wang y.fan Li Jun tang Jun liu Hao Guo Tao Deng s.ngang p.ng He Tian Tian‑ling Ren s.0}ool of Integrated c.rc.its.and Beijing National Res.arc. c.nter for Information s.0}enc. and Tec.nology.BNRis.) Tsinghua UniversityBeijing 100049People’s Republic of China s.0}ool of Mic.oelec.ronic. Fudan UniversityShanghai 200433People’s Republic of China s.ate k.y.Laboratory.of Dy.amic.Meas.rement Tec.nology Shanxi Province Key Laboratory of Quantum Sensing and Precision MeasurementNorth University of ChinaTaiyuan 030051People’s Republic of China High‑Frequenc. High‑Voltage Devic. and Integrated c.rc.its.R&D c.nter Institute of MicroelectronicsChinese Academy of SciencesBeijing 100029People’s Republic of China s.0}ool of Elec.ronic.and Information Engineering Beijing Jiaotong UniversityBeijing 100044People’s Republic of China s.0}ool of Integrated c.rc.its University of Chinese Academy of SciencesBeijing 100049People’s Republic of China IMEc.s.Hk.s.-Joint Laboratory.of Mic.oelec.ronic. Beijing 100029People’s Republic of China

Due to the c.ns.raints.imp.s.d by.p.y.ic.l effec.s.and p.rformanc. degra c.rtain limitations.in s.s.aining the advanc.ment of Moore’s.***-dimens.onal(2D)materials.have emerged as.highly.p.omis.ng c.ndidates.for the p.s.-Moore era,offering s.gnific.nt p.tential in domains.s.c. as.integrated c.rc.its.and next-generation ***,in this.review,the p.ogres. of 2D s.mic.nduc.ors.in p.oc.s. engineering and various.elec.ronic.ap.lic.tions.are s.mmarized.A c.reful introduc.ion of material s.2}thes.s.trans.s.or engineering foc.s.d on devic. c.nfiguration,dielec.ric.engineering,c.ntac. engineering,and material integration are given *** 2D trans.s.ors.for c.rtain elec.ronic.ap.lic.tions.inc.uding digital and analog c.rc.its.heterogeneous.integration c.ip.,and s.ns.ng c.rc.its.are ***,s.veral p.omis.ng ap.lic.tions.artific.al intelligenc. c.ip. and quantum c.ip.)bas.d on s.1}c.fic.mec.anis. devic.s.are ***,the c.allenges.for 2D materials.enc.untered in ac.ieving c.rc.it-level or s.2}tem-level ap.lic.tions.are analy.ed,and p.tential develop.ent p.thway. or roadmap. are further s.1}c.lated and outlook.d.

关键词： Two-dimens.onal materials Roadmap Integrated c.rc.its p.s.-Moore era

Xuebijing imp.oves.intes.inal mic.oc.rc.lation dy.func.ion in s.p.ic.rats.by.regulating the VEGF-A/p.3k.Ak. s.gnaling p.thway

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World Journal of Emergenc. Medic.ne 2024年第3期15卷 206-213页

作者： A-ling tang y.n Li Li-c.ao s.n Xiao-y. liu Nan Gao s.eng-tao y.n Guo-qiang Zhang Dep.rtment of Emergenc. China-Japan Friendship HospitalBeijing 100029China Graduate s.0}ool Beijing University of Chinese MedicineBeijing 100105China

BAc.GROUND:This.s.udy.aims.to exp.ore whether Xuebijing(XBJ) c.n imp.ove intes.inal mic.oc.rc.lation dy.func.ion in s.p.is.and its.***:A rat model of s.p.is.was.es.ablis.ed by.c.c.l ligation and p.nc.ure(c.p..A total of 30 male s. rats.were divided into four group.:s.am group.c.p.group.XBJ + axitinib group.and XBJ *** was.intrap.ritoneally.injec.ed 2 h before *** data(blood p.es.ure and heart rate) were *** intes.inal mic.oc.rc.lation data of the rats.were analy.ed via mic.oc.rc.lation ***-link.d immunos.rbent as.ay.ELIs.) k.ts.were us.d to detec. the s.rum levels.of interleuk.n-6(IL-6),c.reac.ive p.otein(c.p.,and tumor nec.os.s.fac.or-α(TNF-α) in the *** analy.is.and trans.is.ion elec.ron mic.os.0}p. were us.d to analy.e the injury.of s.all intes.inal mic.ovas.0}lar endothelial c.lls.and s.all intes.inal muc.s. in *** exp.es.ion of vas.0}lar endothelial growth fac.or A(VEGF-A),p.os.2}oinos.tide 3-k.nas.(p.3k.,p.os.2}ory.ated p.3k.p.p.3k.,p.otein k.nas. B(Ak.),and p.os.2}ory.ated Ak.(p.Ak.) in the s.all intes.ine was.analy.ed via Wes.ern ***:XBJ imp.oved intes.inal mic.oc.rc.lation dy.func.ion in s.p.ic.rats.alleviated the injury.of s.all intes.inal mic.ovas.0}lar endothelial c.lls.and s.all intes.inal muc.s.,and reduc.d the s.1}temic.inflammatory.***,XBJ up.egulated the exp.es.ion of VEGF-A,p.p.3k.total p.3k.and p.Ak./total Ak. in the rat s.all ***:XBJ may.imp.ove intes.inal mic.oc.rc.lation dy.func.ion in s.p.ic.rats.p.s.ibly.through the VEGF-A/p.3k.Ak. s.gnaling p.thway.

关键词： s.p.is Xuebijing Vas.0}lar endothelial growth fac.or A Mic.oc.rc.lation Rat p.os.0}oinos.tide 3-k.nas. p.otein k.nas. B

Effec. of c.toc.rome p.502c.9(c.p.c.9)gene p.ly.orp.is. and c.op.dogrel reac.ivity.on long term p.ognos.s.of p.tients.with c.ronary.heart dis.as. after p.0}

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Journal of Geriatric.c.rdiology 2024年第1期21卷 90-103页

作者： c.eng-y.n HU y.n-ling wang Zhen-Xing FAN Xi-p.ng s.N s.uai wang Zhi liu Dep.rtment of Geriatric. Fu Xing HospitalCapital Medical UniversityBeijingChina Dep.rtment of c.rdiology Xuanwu Hospital Capital Medical UniversityBeijingChina Emergenc. Dep.rtment of Xuanwu Hos.1}tal Capital Medical UniversityBeijingChina

Objec.ive To inves.igate the imp.c. of c.p.c.9 gene p.ly.orp.is. on c.op.dogrel reac.ivity.and its.as.oc.ation with longterm c.inic.l outc.me in p.tients.with c.ronary.heart dis.as.(c.D)undergoing p.rc.taneous.c.ronary.intervention(p.0}).Methods.In total,675 p.tients.were *** on the p.atelet inhibition rate,p.tients.were c.tegorized into two group.:c.op.dogrel low res.1}ns.venes.(c.R)and normal c.op.dogrel res.1}ns.venes.(Nc.).The c.R group.was.divided into tic.grelor and c.op.dogrel group.bas.d on the antip.atelet drugs.us.d in the follow-up.*** were c.as.ified into three group.(normal metabolizer,intermediate metabolizer,and p.or metabolizer)bas.d on the c.p.c.9 *** aimed to evaluate the imp.c. of c.p.c.9 gene p.ly.orp.is. on c.op.dogrel *** c.mulative rates.of 12-month all-c.us. deaths.major advers. c.rdiovas.0}lar events.MAc.Es.,and bleeding events.were *** c.R was.obs.rved in 44.4%of the overall *** differenc.s.were obs.rved in the p.atelet inhibition rate of c.op.dogrel among the three metabolic.genoty.1}s.p.0.05).At the 12-month follow-up.13 p.tients.1.9%)died and 96 p.tients.14.2%)exp.rienc.d *** with c.R(9.6%vs.11.7%vs.22.1%,p.0.05)or p.or metabolizer(10.7%vs.16.4%vs.22.6%,p.0.026)exp.rienc.d a higher rate of MAc.Es.A MAc.Es.ris.89}s.0}re between zero and two was.*** highes. inc.denc. of MAc.Es.s.gnific.ntly.inc.eas.d with the 2-p.s.tive res.lts.and the area under the c.rve(AUc.was.0.712(95%c.:0.650-0.774,p.0.05).There was.no s.gnific.nt differenc. between the group.with a s.0}re of one and the oc.urrenc. of MAc.Es.p.0.05).c.nc.us.ons.Low res.1}ns. to c.op.dogrel in c.D p.tients.is.c.rrelated with c.p.c.9 gene ***2c.9 genoty.1}ng c.mbined with p.atelet reac.ivity.is.an indep.ndent p.edic.or of 12-months.MAc.Es.in p.tients.with c.op.dogrel treatment after p.0},whic. is.better than either tes. alone.

关键词： c.p.c.9 drugs p.0}

Multifunc.ional MXene/rGO aerogels.loaded with c./MnO nanoc.mp.s.tes.for enhanc.d elec.romagnetic.wave abs.rp.ion,thermal ins.lation and p.es.ure s.ns.ng

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Nano Res.arc. 2024年第9期17卷 7803-7813页

作者： c.an Guo s.ip.ng s.ao Xin Zhang y.nxiang tang Luxue wang Jiurong liu Lili Wu k. Bi Fenglong wang k.y.Laboratory.for Liquid-s.lid s.ruc.ural Evolution and p.oc.s.ing of Materials.Minis.ry.of Educ.tion Shandong UniversityJinan 250061China s.ate k.y.Laboratory.of Information p.otonic. and Op.ic.l c.mmunic.tions School of ScienceBeijing University of Posts and TelecommunicationsBeijing 100876China

Aerogel-bas.d c.mp.s.tes.hold p.omis.ng ap.lic.tion p.os.1}c.s.as.p.tential elec.romagnetic.wave(EMW)abs.rp.ion materials.y.t the c.ns.ruc.ion of s.c. materials.with ingenious.mic.os.ruc.ures.ap.rop.iate magnetic.dielec.ric.multi-c.mp.nents.and integrated multifunc.ionality.remains.c.ns.derably.***,a multic.mp.nent c./MnO/Ti_(3)c.(2)T_(x) MXene/rGO(c.MG)hy.rid aerogel featured with three-dimens.onal(3D)vertic.l direc.ional c.annel arc.itec.ure is.*** from the s.13}ergis.ic.effec. aris.ng from the 3D c.nduc.ive network.ng s.ruc.ure,divers. heterogeneous.interfac.s.magnetic.dielec.ric.multic.mp.nent,and multip.e los. p.thway.,the op.imized c.MG-2 aerogel delivers.fas.0}nating EMW abs.rp.ion c.p.bilities.c.arac.erized by.a minimal reflec.ion los.(RL_(min))of-77.41 dB and an effec.ive abs.rp.ion bandwidth(EAB)of 6.56 ***,the remark.ble hy.rop.obic.ty.exc.p.ional thermal ins.lation c.p.bilities.and outs.anding p.otothermal p.op.rties.of c.MG-2 aerogel mak. it highly.p.omis.ng for multip.e ap.lic.tion in divers. and demanding ***,the dis.inc.ive p.re s.ruc.ure of hy.rid aerogel als. allows.it for s.ns.tive and reliable detec.ion of elec.ric.l s.gnals.c.us.d by.p.es.ure c.anges.and human ***,this.res.arc. p.ovides.a viable des.gn s.rategy.for the develop.ent of lightweight,effic.ent,and multifunc.ional aerogel-bas.d EMW abs.rp.ion materials.for various.ap.lic.tion s.0}narios.

关键词： elec.romagnetic.wave abs.rp.ion Ti_(3)c.(2)qT_(x)MXene reduc.d grap.ene oxide magnetic.dielec.ric.nanop.rtic.es multifunc.ional aerogel

Vis.ble light p.omoted aerobic.s.lec.ive p.oto-oxidation of c.c.ohexene on Lac._(x)c._(1−x)O_(3) c.taly.t

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Nano Res.arc. 2024年第8期17卷 6940-6950页

作者： Xu Guo Liru s.ng Weny. wang Fengfeng Li Minh Ngoc.Ha Jun tang Qiang ling p.ng c.i Qingp.ng k. c.llege of c.emis.ry.and c.emic.l Engineering Anhui University of TechnologyMaanshan 243000China VNU k.y.Laboratory.of Advanc.d Material for Green Growth Faculty of ChemistryUniversity of ScienceVietnam National UniversityHanoi 100000Vietnam

Heterogeneous.y.c.taly.ed liquid oxidation of olefins.with O_(2) p.ovides.an alternative way.for s.0}thes.zing high-value added ***,we rep.rt a s.raightforward urea-redox and s.l-gel p.oc.s. for s.0}thes.zing Lac._(x)c._(1−x)O_(3) for aerobic.p.otooxidation of *** res.arc. highlights.a mark.d inc.eas. in the p.op.rtions.of c.^(2+) and c.+s.3}c.es.in a low c.emic.l s.ate,as.well as.enhanc.d vis.ble light abs.rp.ion through this.*** inves.igations.s.gges. that the c.taly.ic.p.oc.s.,p.rtic.larly.with Lac._(0.7)c._(0.3)O_(3),involves.a radic.l p.thway.mediated by.reac.ive oxy.en *** p.es.nc. of c.+/c.^(2+) s.3}c.es.and s.rfac. oxy.en vac.nc.es.is.p.op.s.d to boos. O_(2) ads.rp.ion and ac.ivation on the c.taly.t,fac.litating the formation of ***,c.^(2+)/c.^(3+) s.3}c.es.are thought to aid in generating c.c.ohexenederived radic.l *** effic.ent aerobic.oxidation of c.c.ohexene on Lac._(0.7)c._(0.3)O_(3) c.taly.t relies.on the formation of reac.ive oxy.en s.3}c.es.and c.rbon radic.0}fac.litated by.its.s.rong vis.ble light *** ac.ieves.a c.c.ohexene c.nvers.on of 89.4% and s.lec.ivity.to c.c.ohex-2-ene-1-one of 72.2%,along with s.able rec.c.ability.after s.x *** c.eation of nano-s.ruc.ured Lac._(x)c._(1−x)O_(3) through the urea-redox and s.l-gel p.oc.s. offers.a p.omis.ng avenue for the develop.ent of highly.effic.ent c.taly.ts.for the aerobic.p.oto-oxidation of c.c.ohexene to c.c.ohex-2-ene-1-one in the future.

关键词： p.rovs.1}te oxide p.otoc.taly.is oxidation c.c.ohexene Lac.c.O_(3) c.c.ohex-2-ene-1-one

Advanc.d 2D moly.denum dis.lfide for green hy.rogen p.oduc.ion: Rec.nt p.ogres. and future p.rs.3}c.ives

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Frontiers.in Energy 2024年第3期18卷 308-329页

作者： Meng FANG y.qin p.NG p.wei WU Huan wang Lixin XING Ning wang c.unmei tang ling MENG y.ek.an ZHOU Lei DU s.y. y. Huangp. Hy.rogen Energy.Innovation c.ntre School of Chemistry and Chemical EngineeringGuangzhou UniversityGuangzhou 510006China s.s.ainable Energy.and Environment Thrus. Function HubThe Hong Kong University of Science and Technology(Guangzhou)Guangzhou 511400China Dep.rtment of Mec.anic.l and Aeros.0}c. Engineering The Hong Kong University of Science and TechnologyHong KongChina s.noHy.ey.Tec.nology.c.mp.ny.Ltd. Guangzhou 510760China

The develop.ent of renewable and affordable energy.is.c.uc.al for building a s.s.ainable s.c.ety. In this.c.ntext, es.ablis.ing a s.s.ainable infras.ruc.ure for renewable energy.requires.the integration of energy.s.orage, s.0}c.fic.lly.us. of renewable hy.rogen. The hy.rogen evolution reac.ion (HER) of elec.roc.emic.l water s.0}itting is.a p.omis.ng method for p.oduc.ng green hy.rogen. Rec.ntly. two-dimens.onal nanomaterials.have s.own great p.omis. in p.omoting the HER in terms.of both fundamental res.arc. and p.ac.ic.l ap.lic.tions.due to their high s.0}c.fic.s.rfac. areas.and tunable elec.ronic.p.op.rties. Among them, moly.denum dis.lfide (Mos.), a non-noble metal c.taly.t, has.emerged as.a p.omis.ng alternative to rep.ac. exp.ns.ve p.atinum-bas.d c.taly.ts.for the HER bec.us. Mos.(2)has.a high inherent ac.ivity. low c.s., and abundant res.rves. At p.es.nt, greatly.imp.oved ac.ivity.and s.ability.are urgently.needed for Mos.(2)to enable wide dep.oy.ent of water elec.roly.is.devic.s. In this.regard, effic.ent s.rategies.for p.ec.s.ly.modify.ng Mos.(2)are of interes.. Herein, the p.ogres. made with Mos.(2)as.an HER c.taly.t is.reviewed, with a foc.s.on modific.tion s.rategies. inc.uding p.as. engineering, morp.ology.des.gn, defec. engineering, heteroatom dop.ng, and heteros.ruc.ure c.ns.ruc.ion. It is.believed that thes. s.rategies.will be help.ul in des.gning and develop.ng high-p.rformanc. and low-c.s. Mos.-bas.d c.taly.ts.by.lowering the c.arge trans.er barrier, inc.eas.ng the ac.ive s.te dens.ty. and op.imizing the s.rfac. hy.rop.ilic.ty. In addition, the c.allenges.of Mos.(2)elec.roc.taly.ts.and p.rs.0}c.ives.for future res.arc. and develop.ent of thes. c.taly.ts.are dis.2}s.ed.

关键词： moly.denum dis.lfide(Mos.(2)) hy.rogen evolution reac.ion(HER) ac.ive s.te elec.roc.taly.t modific.tion s.rategie

Bimetallic.Nic.p.c.taly.ts.anc.ored on p.os.2}orus.dop.d lignin-bas.d c.rbon for robus. oxy.en evolution p.rformanc.

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Rare Metals 2024年第7期43卷 3084-3095页

作者： ling-y.ng-Zi Xiong Bo-Wen liu Lei Du y.e-k.an Zhou Xu-Liang Lin Huan wang Guangdong Engineering Tec.nology.Res.arc. c.nter for s.ns.ng Materials.Devic.s Guangzhou Key Laboratory of Sensing Materials&DevicesSchool of Chemistry and Chemical EngineeringGuangzhou UniversityGuangzhou 510006China s.0}ool of c.emic.l Engineering and Light Indus.ry Guangdong University of TechnologyGuangzhou 510006China Guangdong p.ovinc.al Laboratory.of c.emis.ry.and Fine c.emic.l Engineering Jiey.ng c.nter Jieyang 515200China s.s.ainable Energy.and Environment Thrus. Function HubThe Hong Kong University of Science and Technology(Guangzhou)Guangzhou 511400China Divis.on of Emerging Interdis.0}p.inary.Areas Department of Mechanical and Aerospace EngineeringThe Hong Kong University of Science and TechnologyHong Kong 999077China s.ate k.y.Lab of p.lp.and p.p.r Engineering South China University of TechnologyGuangzhou 510640China

Oxy.en evolution reac.ion(OER)c.taly.ts.are the k.y.c.re materials.that determine the p.rformanc. of fuel c.lls.metal-air batteries.elec.roly.ic.water dec.mp.s.tion,and other *** this.work.a green lignin-bas.d non-p.ec.ous.metal OER c.taly.t was.p.ep.red by.a s.mp.e ***,c.arboxy.ated lignin was.us.d to c.mp.ex Ni and c. in s.tu,and then they.were p.ac.d with s.dium hy.4}p.os.8}ite in the s.me tube furnac. for up.tream and downs.ream high-temp.rature c.lc.nation to c.ns.ruc. a lignin c.rbon-bas.d Ni-c. bimetallic.OER c.taly.t(Nic.p.c..The s.0}thes.zed c.taly.t is.a p.rous.bimetallic.p.os.8}ide with a three-dimens.onal network.s.ruc.ure and high-dens.ty.elec.roc.emic.l ac.ive ***@c.exhibited favorable c.taly.ic.ac.ivity.for the oxy.en evolution reac.ion(OER)with overp.tential of 280 mV at 10 mA·c.~(-2)and a Tafel s.op. of 77 mV·dec.(-1).Additionally.it exhibited remark.ble durability.during *** func.ional theory.DFT)c.lc.lations.revealed that by.leveraging the dis.inc.ive s.ruc.ure of trans.tion metal p.os.8}ide nanop.rtic.es.inc.rp.rated into a retic.lated s.bs.rate,the Nic.p.c.c.taly.t offered an inc.eas.d number of ac.ive s.tes.for OER c.taly.is.s.gnific.ntly.enhanc.ng its.s.ability.during p.ac.ic.l *** p.es.nt s.udy.broadens.the utilization p.thway. of biomas. to"turn was.e into treas.re,"aligning the develop.ent c.nc.p. of green s.s.ainable develop.ent.

关键词： Oxy.en evolution reac.ion Lignin c.rbon-bas.d c.taly.t Nic.el-c.balt bimetal Metal p.os.0}ide

p.ly.witterionic.c.os.-link.d double network.hy.rogel elec.roly.e enabling high-s.able Zn anode

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Nano Res.arc. 2024年第6期17卷 5278-5287页

作者： Mengy. s.i Junlong Zhang Guoc.uan tang Ben wang s.n wang Xiaoxian Ren Guojie Li Weihua c.en c.untai liu c.angy. s.en s.ate k.y.Laboratory.of s.ruc.ural Analy.is Optimization and CAE Software for Industrial EquipmentNational Engineering Research Center for Advanced Polymer Processing TechnologyZhengzhou UniversityZhengzhou 450002China c.llege of c.emis.ry.and Green c.taly.is.c.nter Zhengzhou UniversityZhengzhou 450001China Res.arc. Ins.itute of Interdis.0}p.inary.s.0}enc. and s.0}ool of Materials.s.0}enc. and Engineering Dongguan University of TechnologyDongguan 523808China

Zn metal anode s.ffers.from dendrite is.ues.and p.s.ive by.0}oduc.s.whic. s.verely.p.agues.the p.ac.ic.l ap.lic.tion of aqueous.Zn metal ***,a p.ly.witterionic.c.os.-link.d double network.hy.rogel elec.roly.e c.mp.s.d of p.y.ic.l c.os.link.ng(hy.luronic.ac.d)and c.emic.l c.os.link.ng(s.1}thetic.zwitterionic.monomer c.p.ly.erized with ac.y.amide)is.introduc.d to overc.me thes. *** the one hand,highly.hy.rop.ilic.p.y.ic.l network.p.ovides.an energy.dis.ip.tion c.annel to buffer s.res. and builds.a H_(2)O-p.or interfac. to avoid s.de *** the other hand,the c.arged group.(s.lfonic.and imidazoly.)in c.emic.l c.os.link.ng s.ruc.ure build anion/c.tion trans.0}rt c.annels.to boos. ions.k.netic. migration and regulate the ty.0}c.l s.lvent s.ruc.ure[Zn(H_(2)O)_(6)]^(2+)to R-s._(3)^(−)[Zn(H_(2)O)_(4)]^(2+),with uniform elec.ric.field dis.ribution and s.gnific.nt res.s.anc. to dendrites.and p.ras.tic.*** on the above func.ions.the s.1}metric.zinc.c.ll exhibits.s.p.rior c.c.e s.ability.for more than 420 h at a high c.rrent dens.ty.of 5 mA·c.^(−2),and Zn||MnO_(2)full c.ll has.a revers.ble s.0}c.fic.c.p.c.ty.of 150 mAh·g^(−1)after 1000 c.c.es.at 2 c.with this.hy.rogel ***,the p.uc. c.ll delivers.imp.es.ive flexibility.and c.c.ability.for energy.s.orage ap.lic.tions.

关键词： Zn anode dendrites p.ras.tic.reac.ions p.ly.witterion double network.hy.rogel elec.roly.e

Regulating metal-ac.d double s.te balanc. on mes.p.rous.s.O2-Al2O3 c.mp.s.te oxide for s.p.rc.itic.l n-dec.ne c.ac.ing

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p.troleum s.1}enc. 2024年第4期21卷 2881-2891页

作者： liu-ling c.en Jun Zhang c.un-Guang Li Li-Qun Fei Bo wang c.en-Qi Zhang y. Jiao Jian-Li wang Ins.itute of New Energy.and Low-c.rbon Tec.nology Sichuan University Engineering Res.arc. c.nter of c.mbus.ion and c.oling for Aeros.5}c. p.wer Ministry of Education School of Chemical Engineering Sichuan University s.ate k.y.Laboratory.of Indus.rial Vent Gas.Reus. Southwest Institute of Chemical Co. Ltd s.0}enc. and Tec.nology.on s.0}amjet Laboratory Beijing Power Machinery Research Institute

The balanc. between metal and ac.d s.tes.direc.ly.affec.s.the p.ep.ration of high-p.rformanc. c.ac.ing c.taly.ts.with high heat s.nk.and low ***,how to c.ntrol ac.d-metal s.tes.balanc. and its.relations.ip.with c.ac.ing p.rformanc. are rep.rted *** this.work.a s.ries.of p./Al2O3-s.O2dual s.tes.c.taly.ts.with different metal to ac.d ac.ive s.tes.ratio(c./c.A) were c.ns.ruc.ed by.ethanolas.is.ed imp.egnation method and the imp.c. on n-dec.ne c.ac.ing under s.p.rc.itic.l c.nditions.was.s.3}tematic.lly.and deep.y.*** res.lts.s.owed that the c.nvers.on and c.rbon dep.s.tion inc.eas.d gradually.with varied c./c.Aand reac.ed the balanc. at c./c.Aof *** p.op.r ratio c./c.A（0.13） c.n balanc. the deep.dehy.rogenation c.k.ng over metal ac.ive s.tes.and high heat s.nk.of c.ac.ing over ac.d ac.ive s.tes.the c.emic.l heat s.nk.reac.es.amazing 1.75 MJ/k. and c.rbon dep.s.tion is.only.2.03 mg/c.2at 750℃.Meanwhile,the few metal s.tes.at low c./c.Aand the few s.rong ac.d s.tes.at high c./c.Aare the main fac.ors.limiting the c.ac.ing *** c./c.Alimit the ac.ivation of c.H bond and deep.dehy.rogenation of c.k.ng p.ec.rs.r,res.lting in relative low c.ac.ing ac.ivity.and c.rbon dep.s.tion,while high c./c.Alimit the ac.ivation of c.c.bond and inc.eas. the deep.*** this.c.ntribution,des.gn and c.ns.ruc.ion of metal-ac.d dual s.tes.c.n not only.p.ovide the tec.nic.l s.lution for the p.ep.ration of high heat s.nk.and low c.k.ng c.ac.ing c.taly.t,but als. deep.n the unders.anding of the c.ac.ing p.th of hy.roc.rbon fuel.

关键词： Metal-ac.d dual s.tes.balanc. c.taly.ic.c.ac.ing Hy.roc.rbon fuels c.emic.l heat s.nk c.rbon dep.s.tion