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Biochar-based composites for removing chlorinated organic pollutants: Applications, mechanisms, and perspectives

Environmental Science and Ecotechnology 2024年第5期21卷 47-61页

作者： Qingqing Song Fanying Kong bing-feng liu Xueting Song Hong-Yu Ren State Key Laboratory of Urban Water Resource and Environment School of EnvironmentHarbin Institute of TechnologyHarbin150090China School of Water Conservancy and Civil Engineering Northeast Agricultural UniversityHarbin150030China

Chlorinated organic pollutants constitute a significant category of persistent organic pollutants due to their widespread presence in the environment,which is primarily attributed to the expansion of agricultural and industrial *** pollutants are characterized by their persistence,potent toxicity,and capability for long-range dispersion,emphasizing the importance of their eradication to mitigate environmental *** conventional methods for removing chlorinated organic pollutants encompass advanced oxidation,catalytic oxidation,and bioremediation,the utilization of biochar has emerged as a prominent green and efficacious method in recent *** we review biochar's role in remediating typical chlorinated organics,including polychlorinated biphenyls(PCBs),triclosan(TCS),trichloroethene(TCE),tetrachloroethylene(PCE),organochlorine pesticides(OCPs),and chlorobenzenes(CBs).We focus on the impact of biochar material properties on the adsorption mechanisms of chlorinated *** review highlights the use of biochar as a sustainable and eco-friendly method for removing chlorinated organic pollutants,especially when combined with biological or chemical *** facilitates electron transfer efficiency between microorganisms,promoting the growth of dechlorinating bacteria and mitigating the toxicity of chlorinated organics through ***,biochar can activate processes such as advanced oxidation or nano zero-valent iron,generating free radicals to decompose chlorinated organic *** observe a broader application of biochar and bioprocesses for treating chlorinated organic pollutants in soil,reducing environmental ***,for water-based pollutants,integrating biochar with chemical methods proved more effective,leading to superior purification *** review contributes to the theoretical and practical application of biochar for removing environmental chlorinated organic pollutants.

关键词： Biochar Chlorinated organic pollutants Polychlorinated biphenyls Triclosan Trichloroethene

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Nitrite-driven anaerobic ethane oxidation

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Environmental Science and Ecotechnology 2024年第5期21卷 361-368页

作者： Cheng-Cheng Dang Yin-Zhu Jin Xin Tan Wen-Bo Nie Yang Lu bing-feng liu De-feng Xing Nan-Qi Ren Guo-Jun Xie State Key Laboratory of Urban Water Resource and Environment School of EnvironmentHarbin Institute of TechnologyHarbin150090China Key Laboratory of the Three Gorges Region's Eco-Environment Ministry of EducationCollege of Environment and EcologyChongqing UniversityChongqing400044China Water Innovation and Smart Environment Laboratory School of Civil and Environmental EngineeringFaculty of EngineeringQueensland University of TechnologyBrisbaneQueensland4001Australia

Ethane,the second most abundant gaseous hydrocarbon in vast anoxic environments,is an overlooked greenhouse *** anaerobic oxidation of ethane can be driven by available electron acceptors such as sulfate and ***,despite nitrite being a more thermodynamically feasible electron acceptor than sulfate or nitrate,little is known about nitrite-driven anaerobic ethane *** this study,a microbial culture capable of nitrite-driven anaerobic ethane oxidation was enriched through the long-term operation of a nitrite-and-ethane-fed *** continuous operation,the nitrite removal rate and the theoretical ethane oxidation rate remained stable at approximately 25.0 mg NO_(2) eN L^(-1) d^(-1) and 11.48 mg C2H6 L^(-1) d^(-1),*** tests demonstrated that ethane is essential for nitrite removal in this microbial *** function analysis revealed that a species affiliated with a novel genus within the family Rhodocyclaceae,designated as'Candidatus Alkanivoras nitrosoreducens',may perform the nitrite-driven anaerobic ethane *** the proposed metabolic model,despite the absence of known genes for ethane conversion to ethyl-succinate and succinate-CoA ligase,'***'encodes a prospective fumarate addition pathway for anaerobic ethane oxidation and a complete denitrification pathway for nitrite reduction to *** findings advance our understanding of nitrite-driven anaerobic ethane oxidation,highlighting the previously overlooked impact of anaerobic ethane oxidation in natural ecosystems.

关键词： Anaerobic ethane oxidation Denitrification Microbial culture Fumarate addition pathway Greenhouse gas

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Effects of Tebufenozide on the Biological Characteristics of Beet Armyworm (Spodoptera exigua Hübner) and Its Resistance Selection

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Agricultural Sciences in China 2008年第10期7卷 1222-1227页

作者： liu Wei-wei MU Wei ZHU bing-yu liu feng Key Laboratory of Pesticide Toxicology ＆ Application Technique College of Plant Protection Shandong Agricultural University Tai＇an271018 P.R.China

In this article, the selection of tebufenozide to beet armyworm （Spodoptera exigua Htibner） was studied by the treatments to alternative generations＇ 3rd-instar larvae with LC50 dose and to continuous generations＇ larvae with LC10 dose; the effects of tebufenozide on the biological characteristics of current and subsequent generations were examined by the treatments to 3rd-instar larvae and egg pods in different concentrations. After treatments with LC50 dose till F11, the toxicity of tebufenozide to beet armyworm had no significant change, whereas the pupation rate, pupal weight, and fecundity were reduced markedly. After treatments with LC10 dose till Fl9, the beet armyworm only developed 3.52-fold resistance, and the main biological characteristics were nearly accordant in each generation. The livability was reduced 72 h later after treatments to 3rd-instar larvae, respectively in 2.5-40 μg mL^-1, and larval duration, pupation rate, and pupal weight changed considerably with the increase in concentrations. The fecundity, larval livability, larval weight and pupal weight of subsequent generations were reduced as the dose increased over 10 μg mL^-1. The hatching rate of egg pods did not differ with that of the controls obviously after treatment in 10-300 μg mL^-1. But the larval livability, larval weight and pupal weight were reduced when eggs were exposed to 50 μg mL^-1 dose or more. The results indicated that tebufenozide had low resistance risk to the current and subsequent generations of beet armyworm even if tebufenozide had significant effects on the biological characteristics of this insect.

关键词： tebufenozide beet armyworm growth and development resistance selection

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Characterization of a Novel Plantain Asr Gene,MpAsr,that is Regulated in Response to Infection of Fusarium oxysporum f. sp. cubense and Abiotic Stresses

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Journal of Integrative Plant Biology 2010年第3期52卷 315-323页

作者： Hai-Yan liu Jin-Ran Dai Dong-Ru feng bing liu Hong-Bin Wang Jin-Fa Wang The State Key Laboratory of Biocontrol and The Key Laborat-ory of Gene Engineering of Ministry of Education School of Life Sciences Sun Yat-sen University Guangzhou 510275 China

Asr （abscisic acid, stress, ripening induced） genes are typically upregulated by a wide range of factors, including drought, cold, salt, abscisic acid （ABA） and injury; in addition to plant responses to developmental and environmental signals. We isolated an Asr gene, MpAsr, from a suppression subtractive hybridization （SSH） cDNA library of cold induced plantain （Musa paradisiaca） leaves. MpAsr expression was upregulated in Fusarium oxysporum f. sp. cubense infected plantain leaves, peels and roots, suggesting that MpAsr plays a role in plantain pathogen response. In addition, a 581-bp putative promoter region of MpAsr was isolated via genome walking and cis-elements involved in abioUc stress and pathogen-related responses were detected in this same region. Furthermore, the MpAsr promoter demonstrated positive activity and inducibility in tobacco under F. oxysporum f. sp. cubense infection and ABA, cold, dehydration and high salt concentration treatments. Interestingly, transgenic Arabidopsis plants overexpressing MpAsr exhibited higher drought tolerance, but showed no significant decreased sensitivity to F. oxysporum f. sp. cubense. These results suggest that MpAsr might be involved in plant responses to both abiotic stress and pathogen attack.

关键词： no english key word

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Highly oriented MXene/polyvinyl alcohol films prepared by scalable layer-by-layer blade coating for efficient electromagnetic interference shielding and infrared stealth

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Nano Research 2024年第6期17卷 5651-5660页

作者： Jingyu Dong Zhaoyang Li Congqi liu bing Zhou Chuntai liu uezhan feng State Key Laboratory of Structural Analysis Optimization and CAE Software for Industrial EquipmentNational Engineering Research Center for Advanced Polymer Processing TechnologyZhengzhou UniversityZhengzhou 450002China Shangqiu Normal University Shangqiu 476000China

Controlling the orientation of two-dimensional MXene within layered films is essential to optimize or tune their mechanical properties and electromagnetic interference shielding(EMI)performance,but achieving the high orientation MXene layers on an industrial scale remains a challenging *** this paper,a scalable layer-by-layer blade coating(LbLBC)method was employed to fabricate highly oriented MXene/polyvinyl alcohol(PVA)*** the LbLBC process,MXene/PVA colloid suffered a strong shearing effect,which induced the ordered alignment of MXene nanosheets along the direction of the blade *** orientation of MXene can be effectively adjusted by changing the scraping gap of LbLBC,achieving a maximum Herman orientation factor f of *** a result,the mechanical properties and EMI performance of the as-prepared MXene/PVA films are in direct proportion to their orientation,with the optimal values of tensile strength of 145.5 MPa,fracture strain of 19.6%,toughness of 17.7 MJ·m^(−3),and EMI shielding effectiveness of 36.7 ***,the inherently low mid-infrared(mid-IR)emissivity of MXene,combined with the densely oriented structure affords the composite films with IR stealth,resulting in a substantial decrease from 150 to 66.1℃in the radiative temperature of a ***,these scalable MXene/PVA films exhibit remarkable potential for integration into the next generation of multifunctional protective camouflage materials.

关键词： MXene nanosheets densely oriented structure layer-by-layer blade coating electromagnetic interference shielding infrared stealth

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Modeling urban scale human mobility through big data analysis and machinelearning

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Building Simulation 2024年第1期17卷 3-21页

作者： Yapan liu bing Dong Department of Mechanical&Aerospace Engineering Syracuse University263 Link HallSyracuseNY 13244USA

In the United States,the buildings sector consumes about 76%of electricity use and 40% of all primary energy use and associated greenhouse gas *** behavior has drawn increasing research interests due to its impacts on the building energy ***,occupant behavior study at urban scale remains a challenge,and very limited studies have been *** an effort to couple big data analysis with human mobility modeling,this study has explored urban scale human mobility utilizing three months Global Positioning System(GPS)data of 93,o00 users at Phoenix Metropolitan *** research extracted stay points from raw data,and identified users'home,work,and other locations by Density-Based Spatial Clustering ***,daily mobility patterns were constructed using different types of *** propose a novel approach to predict urban scale daily human mobility patterns with 12-hour prediction horizon,using Long Short-Term Memory(LSTM)neural network *** shows the developed models achieved around 85%average accuracy and about 86%mean *** developed models can be further applied to analyze urban scale occupant behavior,building energy demand and flexibility,and contributed to urban planning.

关键词： urban human mobility big data analysis urban scale occupant behavior recurrent neural networks

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Quantitative contributions of climate change and human activities to vegetation dynamics in the Zoige Plateau from 2001 to 2020

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Journal of Mountain Science 2024年第9期21卷 3031-3046页

作者： GAO bing liu Enqin YANG Yang YANG Man YAO Yang GUAN Lei feng Yiwen College of Geography and Planning Chengdu University of TechnologyChengdu 610059China Key Laboratory of Smart Earth Beijing 100029China Sichuan Provincial Soil and Water Conservation Ecological Environment Monitoring Station Chengdu 610041China College of Earth and Planetary Sciences Chengdu University of TechnologyChengdu 610059China

Climate change and human activities such as overgrazing and rapid development of tourism simultaneously affected the vegetation of the Zoige ***,the spatiotemporal variations of vegetation and the relative contributions of climate change and human activities to these vegetation dynamics remain ***,clarifying how and why the vegetation on the Zoige Plateau changed can provide a scientific basis for the sustainable development of the ***,we investigate NDVI trends using the Normalized Difference Vegetation Index(NDVI)as an indicator of vegetation greenness and distinguish the relative effects of climate changes and human activities on vegetation changes by utilizing residual trend analysis and the *** find a tendency of vegetation greening from 2001 to 2020,with significant greening accounting for 21.44%of the entire ***,browning area expanded rapidly after *** temperatures are the primary driver of vegetation changes in the Zoige *** variations and human activities were responsible for 65.57%and 34.43%of vegetation greening,and 39.14%and 60.86%of vegetation browning,respectively,with browning concentrated along the Yellow,Black and White *** to 2001-2010,the inhibitory effect of human activity and climate fluctuations on vegetation grew dramatically between 2011 and 2020.

关键词： Vegetation change Climate change Residual trend analysis Geodetector Human activities Zoige plateau

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Gradient honeycomb metastructure with broadband microwave absorption and effective mechanical resistance

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Nano Materials Science 2024年第4期6卷 456-466页

作者： Dongmeng Li Xia Zheng Hao Gu Xiaobo Xuan bing liu Hongquan feng Fuheng Zhang Shanghai Radio Equipment Research Institute

Multifunctional metastructure integrated broadband microwave absorption and effective mechanical resistance has attracted much attention. However, multifunctional performance is limited by the lack of theoretical approaches to integrated design. Herein, a multi-layer impedance gradient honeycomb(MIGH) was designed through theoretical analysis and simulation calculation, and fabricated using 3D printing technique. A theoretical calculation strategy for impedance gradient structure was established based on the electromagnetic parameter equivalent method and the multi-layer finite iterative method. The impedance of MIGH was analyzed by the theoretical calculation strategy to resolve the broadband absorption. Intrinsic loss mechanism of matrix materials and distributions of electric fields, magnetic fields and power loss were analyzed to investigate the absorption mechanism. Experimental results indicated that a 15 mm thick designed metastructure can achieve the absorption more than 88.9% in the frequency range of 2-18 GHz. Moreover, equivalent mechanical parameters of MIGH was calculated by integral method according to the Y-shaped model. Finite Element analysis of stress distributions were carried out to predict the deformation behavior. Mechanical tests demonstrate that MIGH achieved the compression modulus of 22.89 MPa and flexure modulus of 17.05 MPa. The integration of broadband electromagnetic absorption and effective mechanical resistance was achieved by the proposed design principle and fabrication methodology.

关键词： Multifunctional metastructure Broadband microwave absorption Impedance gradient calculation Mechanical characteristics Finite element analysis

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Regulation of solvation structure and the cooperation environment of potassium bonds for wider-temperature adaptive potassium storage

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Rare Metals 2024年第4期43卷 1610-1621页

作者： bing-bing liu Yi-Hui liu You-Bin Zhang Zhen-Guo Qi Guo-Hui Qin State Key Laboratory Base for Eco-Chemical Engineering College of Chemical EngineeringQingdao University of Science and TechnologyQingdao266042China Shandong Synergetic Innovation Center of Ecological and Chemical Engineering Qingdao266042China

Antimony selenide(Sb_(2)Se_(3))is one of the perspective candidates for potassium-ion batteries due to its advanced virtues stem including featured high capacity,fertile reserves and the relative narrow band *** the unique advantages,it is still plagued by the unstable interface compatibility and poor wider-temperature *** optimization of microstructure and the construction of inorganic-organic hybrids with a low desolvation barrier and rapid kinetics behaviors are efficient to address these *** Sb_(2)Se_(3)nanorods enclosed by the S-doped carbon layer(SC),further crosslinked by the poly(N-isopropylacrylamide)(PM)film(PM@Sb_(2)Se_(3)@SC),were artificially fabricated,and it displays the enrichment ion aggregated model as well as contacted ion pair state,the well-tailored cooperation environment of potassium bonds,assuring a homogeneous potassium deposition and an excellent widertemperature *** complicated experimental studies and theoretical calculations authenticate the synergistic effects of geometric conformation and compositional design for the tremendously enhanced potassium ***,the full device over PM@Sb_(2)Se_(3)@SC anode and the potassium Prussian blue cathode manifests impressively durable cycling life and wider-temperature adaptability,verifying the glorious contribution from the finely manipulation in solvation structure and potassium bonds to enhancing the potassium storage behaviors.

关键词： Anode Sb_(2)Se_(3) rods Interface compatibility Inorganic-organic electrode Potassium ion battery

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Glycerol solutions of highly concentrated biomineral counter-ions towards water-responsive mineralization: Demonstration on bacterial cellulose and its application in hard tissue repair

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Nano Research 2024年第3期17卷 2154-2163页

作者： Yunfei Zhao Xiaohao liu Zhi Zhou Chaobo feng Nan Luo Jiajun Yan Shuo Tan Yang Lu feng Chen bing-Qiang Lu Shisheng He Department of Orthopedic Spinal Pain Research InstituteShanghai Tenth People’s HospitalSchool of MedicineTongji UniversityShanghai 200072China Department of Preventive Dentistry Shanghai Ninth People’s HospitalShanghai Jiao Tong University School of MedicineCollege of StomatologyShanghai Jiao Tong UniversityNational Center for StomatologyNational Clinical Research Center for Oral DiseasesShanghai Key Laboratory of StomatologyShanghai Research Institute of StomatologyShanghai 200011China

Mineralization has found widespread use in the fabrication of composite biomaterials for hard tissue *** current mineralization processes are mainly carried out in neutral aqueous solutions of biomineral counter-ions(a pair of cation and anion that form the corresponding minerals at certain conditions),which are stable only at very low *** typically results in inefficient mineralization and weak control over biomineral ***,we find that,in the organic solvent glycerol,a variety of biomineral counter-ions(e.g.,Ca/PO_(4),Ca/CO_(3),Ca/SO_(4),Mg/PO_(4),or Fe/OH)corresponding to distinct biominerals at significantly high concentrations(up to hundreds-fold greater than those of simulated body fluid(SBF))are able to form translucent and stable solutions(mineralizing solution of highly concentrated counter-ions(MSCIs)),and mineralization can be triggered upon them with external solvents(e.g.,water or ethanol).Furthermore,with pristine bacterial cellulose(BC)membrane as a model,we demonstrate an effective and controllable mineralization performance of MSCIs on organic *** approach not only forms the homogeneous biominerals on the BC fibers and in the interspaces,but also provides regulations over mineralization rate,mineral content,phase,and *** resulting mineralized BC membranes(MBCs)exhibit high cytocompatibility and favor the proliferation of rat bone marrow mesenchymal stem cells(rBMSC).Following this,we prepare a mineralized bone suture(MBS)from MBC for non-weight bearing bone fixation,which then is tested on a rabbit median sternotomy *** shows firm fixation of the rabbit sternum without causing discernible toxicity or inflammatory *** study,by extending the mineralization to the organic solution system of highly concentrated counter-ions,develops a promising strategy to design and build targeted mineral-based composites.

关键词： biomineralization organic solvent bacterial cellulose(BC) hard tissue repair

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