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Enhanced cycling stability and rate performance of Co-doped and La_(2)O_(3)-coated LiNi_(0.9)Mn_(0.1)O_(2) toward power battery

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Rare Metals 2024年第2期43卷 658-670页

作者： Jia-Qi Peng Yuan-Yuan Wei Dong-Ming Liu Yun Li bin Hu bin huang Jian-Wen Yang Shun-Hua Xiao Ren-Heng Wang Guangxi Key Laboratory of Electrochemical and Magneto-Chemical Functional Materials College of Chemistry and BioengineeringGuilin University of TechnologyGuilin541004China Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province College of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen518060China

Ultra-high nickel layered oxide cathode material with high energy density is the most promising material to improve the electrochemical performance of lithium-ion batteries(LIBs).However,the poor structural stability and severe surface/interface side reactions of the material lead to poor rate performance and cyclic stability,which limits its application in *** this paper,the dual-modification strategy of Co doping and La_(2)O_(3) coating is used to meet the above *** doping can effectively widen layer spacing and reduce Li^(+)/Ni^(2+) mixing,and La_(2)O_(3) coating can effectively eliminate the residual alkali on the surface of active material,inhibit the thickening of cathode electrolyte interphase(CEI)film and reduce surface/interface side ***,the modified material(NM90-CL)with excellent electrochemical properties is achieved through the synergistic enhancement of Co doping and La_(2)O_(3) *** capacity retention rate can reach 77.9%after 200 cycles at 1.0℃ and 75.7%after 200 cycles at 5.0℃.Its reversible capacity can up to 153.5 mAh·g^(–1) at 10.0℃.This dual-modification strategy will provide theoretical guidance and technical support for the synthesis of other high-performance electrode materials.

关键词： High nickel cathode material Co doping La_(2)O_(3) coating Electrochemical performance Electrochemical mechanism

A micro-crosslinked amphoteric hydrophobic association copolymer as high temperature-and salt-resistance fluid loss reducer for water-based drilling fluids

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Petroleum Science 2024年第3期21卷 1980-1991页

作者： Jian Li Yu-Xi Ji Xiao-Xiao Ni Kai-He Lv Xian-bin huang Jin-Sheng Sun School of Petroleum Engineering China University of Petroleum(East China) Key Laboratory of Unconventional Oil & Gas Development China University of Petroleum(East China) Inspection and Testing Center of Huabei Oil Field Company PetroChina Drilling Fluid Research Institute CNPC Engineering Technology R&D Company Limited

During ultradeep oil and gas drilling, fluid loss reducers are highly important for water-based drilling fluids, while preparing high temperature-and salt-resistance fluid loss reducers with excellent rheology and filtration performance remains a challenge. Herein, a micro-crosslinked amphoteric hydrophobic association copolymer(i.e., DADC) was synthesized using N,N-dimethyl acrylamide, diallyl dimethyl ammonium chloride, 2-acrylamido-2-methylpropane sulfonic acid, hydrophobic monomer, and pentaerythritol triallyl ether crosslinker. Due to the synergistic effects of hydrogen bonds, electrostatic interaction, hydrophobic association, and micro-crosslinking, the DADC copolymer exhibited outstanding temperature-and salt-resistance. The rheological experiments have shown that the DADC copolymer had excellent shear dilution performance and a certain degree of salt-responsive viscosity-increasing performance. The DADC copolymer could effectively adsorb on the surface of bentonite particles through electrostatic interaction and hydrogen bonds, which bring more negative charge to the bentonite, thus improving the hydration and dispersion of bentonite particles as well as the colloidal stability of the drilling fluids. Moreover, the drilling fluids constructed based on the DADC copolymer exhibited satisfactory rheological and filtration properties(FLHTHP= 12 m L) after aging at high temperatures(up to200°C) and high salinity(saturated salt) environments. Therefore, this work provided new insights into designing and fabricating high-performance drilling fluid treatment agents, demonstrating good potential applications in deep and ultradeep drilling engineering.

关键词： Fluid loss reducer Temperature- and salt-resistance Hydrophobic association Amphoteric Micro-crosslinking

Nano-frictional mechano-reinforcing porous nanowires scaffolds

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Friction 2024年第5期12卷 968-980页

作者： Licheng HUA Conghu HU Jingkang ZHANG Jin LI Chenjie GU bin huang Guangyong LI Jianke DU Wanlin GUO Smart Materials and Advanced Structures Laboratory School of Mechanical Engineering&MechanicsNingbo UniversityNingbo315211China Key Laboratory for Intelligent Nano Materials and Devices of Ministry of Education Nanjing University of Aeronautics and AstronauticsNanjing210016China Key Laboratory of Impact and Safety Engineering Ministry of EducationSchool of mechanical Engineering and MechanicsNingbo UniversityNingbo315211China Department of Microelectronics and Engineering Ningbo UniversityNingbo315211China

Artificial biomaterials with dynamic mechano-responsive behaviors similar to those of biological tissues have been drawing great *** this study,we report a TiO_(2)-based nanowire(TiO_(2)NWs)scaffolds,which exhibit dynamic mechano-responsive behaviors varying with the number and amplitude of nano-deformation *** is found that the elastic and adhesive forces in the TiO_(2)NWs scaffolds can increase significantly after multiple cycles of *** nanofriction experiments show the triboelectric effect of increasing elastic and adhesive forces during the nano-deformation cycles of TiO_(2)NWs *** properties allow the TiO_(2)NW scaffolds to be designed and applied as intelligent artificial biomaterials to simulate biological tissues in the future.

关键词： TiO_(2)NWs scaffolds nano-deformation mechano-reinforcing triboelectric effect intelligent artificial biomaterials

Dissolved organic matter accelerates microbial degradation of 17 alpha-ethinylestradiol in the presence of iron mineral

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Journal of Environmental Sciences 2024年第5期139卷 364-376页

作者： Huan He Min Shi Xiaoxia Yang Juhong Zhan Yanting Lin Ziwei Guo Zhicheng Liao Chaochao Lai Xiaomin Ren bin huang Xuejun Pan Faculty of Environmental Science and Engineering Kunming University of Science and TechnologyKunming 650500China Yunnan Provincial Key Lab of Soil Carbon Sequestration and Pollution Control Kunming 650500China Research Institute for Environmental Innovation(Suzhou)Tsinghua Suzhou 215163China

Dissolved organic matter(DOM)and iron minerals widely existing in the natural aquatic environment can mediate the migration and transformation of organic ***,the mechanism of interaction between DOM and iron minerals in the microbial degradation of pollutants deserves further *** this study,the mechanism of 17 alphaethinylestradiol(EE2)biodegradation mediated by humic acid(HA)and three kinds of iron minerals(goethite,magnetite,and pyrite)was *** results found that HA and iron minerals significantly accelerated the biodegradation process of EE2,and the highest degradation efficiency of EE2(48%)was observed in the HA-mediated microbial system with pyrite under aerobic ***,it had been demonstrated that hydroxyl radicals(HO·)was the main active substance responsible for the microbial degradation of ***·is primarily generated through the reaction between hydrogen peroxide secreted by microorganisms and Fe(II),with aerobic conditions being more *** presence of iron minerals and HA could change the microbial communities in the EE2 biodegradation *** findings provide new information for exploring the migration and transformation of pollutants by microorganisms in iron-rich environments.

关键词： Dissolved organic matter Iron mineral 17 alpha-ethinylestradiol Biodegradation

Effects of acetylcysteine on micro-inflammation and pulmonary ventilation in chronic obstructive pulmonary disease exacerbation

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World Journal of Clinical Cases 2024年第18期12卷 3482-3490页

作者： Li-Yuan huang bin huang Zheng Lv Xiao-Dan Lu Department of Integration of Traditional Chinese and Western Medicine School of Clinical MedicineChangchun University of Chinese MedicineChangchun 130021Jilin ProvinceChina Department of Infectious Diseases Affiliated People's Hospital of Jiangsu UniversityZhenjiang 212002Jiangsu ProvinceChina Department of Zoology School of Life SciencesChangchun Normal UniversityChangchun 130032Jilin ProvinceChina Precision Medical Center Jilin Province General HospitalChangchun 130021Jilin ProvinceChina

BACKGROUND Acute exacerbation of chronic obstructive pulmonary disease(AECOPD)is a serious complication of chronic obstructive pulmonary disease,often characterized by increased morbidity and *** traditional Chinese medicine,AECOPD is linked to phlegm-heat and blood-stasis,presenting symptoms like thick sputum,fever,and chest *** has been shown that acetylcysteine inhalation in conjunction with conventional therapy significantly reduced inflammatory markers and improved lung function parameters in patients with AECOPD,suggesting that acetylcysteine may be an important adjunctive therapy for patients with phlegm-heat-blood stasis type *** To investigate the effect of acetylcysteine on microinflammation and lung ventilation in patients with phlegm-heat and blood-stasis-type *** One hundred patients with phlegm-heat and blood-stasis-type AECOPD were randomly assigned to two *** treatment group received acetylcysteine inhalation(10%solution,5 mL,twice daily)along with conventional therapy,whereas the control group received only conventional *** treatment duration was 14 *** markers(C-reactive protein,interleukin-6,and tumor necrosis factor-alpha)in the serum and sputum as well as lung function parameters(forced expiratory volume in one second,forced vital capacity,and peak expiratory flow)were assessed pre-and *** inhalation led to significant reductions in inflammatory markers and improvements in lung function parameters compared to those in the control group(P<0.05).This suggests that acetylcysteine could serve as an effective adjunct therapy for patients with phlegm-heat and blood-stasis-type *** Acetylcysteine inhalation significantly reduced inflammatory markers in the serum and sputum and improved lung ventilation function parameters in patients with phlegm-heat and blood-stasis type AECOPD compared with the control *** differences were statistically significant(P

关键词： Acute exacerbation Chronic obstructive pulmonary disease Traditional Chinese medicine Acetylcysteine Phlegm-heat and blood-stasis Lung ventilation function

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圆孔工字型蜂窝梁扭转模态自由振动研究

振动与冲击 2024年第6期43卷 329-335,344页

作者：黄斌张文福南京工程学院建筑工程学院南京211167

从能量等效角度,提出了一种圆孔工字型截面蜂窝梁连续型模型,应用新的薄壁构件扭转理论:板-梁理论,建立了构件扭转模态自由振动能量泛函模型,明确了圆孔工字型截面蜂窝梁名义约束扭转惯性矩(翘曲常数)、自由扭转常数、转动惯量。通过变... 详细信息

从能量等效角度,提出了一种圆孔工字型截面蜂窝梁连续型模型,应用新的薄壁构件扭转理论:板-梁理论,建立了构件扭转模态自由振动能量泛函模型,明确了圆孔工字型截面蜂窝梁名义约束扭转惯性矩(翘曲常数)、自由扭转常数、转动惯量。通过变分运算,获得了平衡微分方程模型。基于扭转模态试函数,推导了圆孔工字型截面蜂窝梁自由振动扭转模态振动圆频率,并与有限元结果对比校验理论模型预测精度。开展了悬臂圆孔工字型蜂窝梁受集中扭矩作用的端部截面转角理论分析与有限元计算,进一步检验了基于板-梁理论建立的蜂窝梁连续模型的适用性。应用板-梁理论对圆孔工字型截面蜂窝梁自由振动扭转的分析过程及推导步骤,为其他开孔类型工字型蜂窝梁扭转模态自由振动研究提供了直接参考。

关键词：圆孔工字型截面蜂窝梁扭转自由振动板-梁理论蜂窝梁连续型模型能量泛函模型

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基于流量分割与填充的网站指纹防御技术

北京理工大学学报 2024年第7期44卷 750-760页

作者：黄斌杜彦辉中国人民公安大学信息网络安全学院北京100038

Tor匿名网络是一种用于保护用户通信隐私的匿名通信系统.网站指纹攻击算法通过分析用户的流量数据来破坏用户通信隐私的匿名性.为防范网站指纹攻击,研究人员提出各种网站指纹防御算法.现阶段,这些防御方法存在着防御开销高、防御性能差... 详细信息

Tor匿名网络是一种用于保护用户通信隐私的匿名通信系统.网站指纹攻击算法通过分析用户的流量数据来破坏用户通信隐私的匿名性.为防范网站指纹攻击,研究人员提出各种网站指纹防御算法.现阶段,这些防御方法存在着防御开销高、防御性能差的问题.为此提出了一种基于流量分割与填充的网站指纹防御算法.该算法由流量分割和数据单元填充这两个模块组成.流量分割模块通过使用随机数量的链路和基于数据单元间隔时间的链路切换策略,将网站流量分割并发送到不同的链路上.数据单元填充模块通过使用Break Burst和Extend Burst两个子模块,分别在传入和传出burst中注入填充数据单元,进一步混淆各个链路上的网站流量模式.在封闭世界场景下,相较于同类算法HyWF,所提算法进一步降低了最优攻击算法RF的精确率18.54%和召回率20.25%;而相较于CoMPS算法,在使用更少链路的情况下,所提算法能够进一步降低RF算法的精确率2.72%和召回率5.23%.实验结果表明,所提算法在防御性能方面优于其他同类算法,并且带来了更低的防御开销.

关键词：网络安全 Tor匿名网络网站指纹防御

Contract Mechanism of Water Environment Regulation for Small and Medium Sized Enterprises Based on Optimal Control Theory

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Journal of Water Resource and Protection 2024年第7期16卷 538-556页

作者： Shuang Zhao Hongbin Gu Lianfang Xue Dongsheng Wang bin huang China Institute of Water Resources and Hydropower Research Beijing China China Renewable Engineering Institute Beijing China School of Environmental Science and Engineering Tianjin University Tianjin China

The small and scattered enterprise pattern in the county economy has formed numerous sporadic pollution sources, hindering the centralized treatment of the water environment, increasing the cost and difficulty of treatment. How enterprises can make reasonable decisions on their water environment behavior based on the external environment and their own factors is of great significance for scientifically and effectively designing water environment regulation mechanisms. Based on optimal control theory, this study investigates the design of contractual mechanisms for water environmental regulation for small and medium-sized enterprises. The enterprise is regarded as an independent economic entity that can adopt optimal control strategies to maximize its own interests. Based on the participation of multiple subjects including the government, enterprises, and the public, an optimal control strategy model for enterprises under contractual water environmental regulation is constructed using optimal control theory, and a method for calculating the amount of unit pollutant penalties is derived. The water pollutant treatment cost data of a paper company is selected to conduct empirical numerical analysis on the model. The results show that the increase in the probability of government regulation and public participation, as well as the decrease in local government protection for enterprises, can achieve the same regulatory effect while reducing the number of administrative penalties per unit. Finally, the implementation process of contractual water environmental regulation for small and medium-sized enterprises is designed.

关键词： Optimal Control Theory Small and Medium-Sized Enterprises Water Environment Regulation Contract Mechanism