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Degradation of Rhodamine b by MnFe-LDH/PMS/O_(3) three-phase catalytic system: performance, mechanism and ecotoxicity studies

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Frontiers of Environmental Science & Engineering 2024年第1期18卷 111-127页

作者： Ying Han Ying Yang Weibao Liu Yilong hou Ce Wang Jiangwei Shang Xiuwen Cheng Key Laboratory of Pollutant Chemistry and Environmental Treatment College of Chemistry and Environmental ScienceYili Normal UniversityYining 835000China Key Laboratory for Environmental Pollution Prediction and Control of Gansu Province College of Earth and Environmental SciencesLanzhou UniversityLanzhou 730000China

This study developed a novel MnFe-LDH/PMS/O3 three-phase catalytic system to degrade the organic dye Rhb, which was used to address the drawbacks of persulfate oxidation and ozonation techniques. The structure, ionic and elemental composition, specific surface area, and magnetic properties of the LDHs were investigated using a variety of physicochemical characterization tools. The results showed that MnFe-LDH had a large specific surface area, a rich crystalline phase composition, and a functional group structure. The Rhb degradation rate of MnFe-LDH/PMS/O3 was 0.34 min−1, which was much higher than that of other comparative systems. Rhb could be completely degraded in 10 min after optimization and had a significant effect on TOC removal. The system was found to be effective over a wide pH range. Common anions were largely unaffected and humic acid acted as an inhibitor. At the same time, the system had generally effective degradation performance for different dyes. Combined with quenching experiments and EPR, it was found that SO4•−, •OH, O_(2)•−, and 1O_(2) all participated in the reaction, and •OH contributed more. The degradation pathway of Rhb was derived by LC-MS, and the T.E.S.T. evaluation found that the toxicity of the intermediate product was significantly reduced. Finally, the stability and availability of LDHs were verified using cycling experiments and metal ion leaching. This work provides a theoretical basis and data support for the synergistic catalysis of PMS/O3 and the deep treatment of dye wastewater.

关键词： Rhodamine b Layered double hydroxides Peroxymonosulfate Ozonation

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Microfluidic-based isolation of circulating tumor cells with high-efficiency and high-purity

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Chinese Chemical Letters 2024年第8期35卷 101-111页

作者： Feng Wu Xuemin Kong Yixuan Liu Shuli Wang Zhong Chen Xu hou Fujian Engineering Research Center for Solid-State Lighting Department of Electronic ScienceSchool of Electronic Science and EngineeringXiamen UniversityXiamen 361005China College of Physics and New Energy Xuzhou University of TechnologyXuzhou 221018China State Key Laboratory of Physical Chemistry of Solid Surfaces College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China College of Physical Science and Technology Xiamen UniversityXiamen 361005China Innovation Laboratory for Sciences and Technologies of Energy Materials of Fujian Province(IKKEM) Xiamen 361102China

The isolation of circulating tumor cells(CTCs)from complex biological samples is of paramount signifi-cance for advancing cancer diagnosis,prognosis,and ***,the low concentration of CTCs and nonspecific adhesion of white blood cells(WbCs)present challenges that hinder the efficiency and purity of captured ***-based strategies utilize precise fluid control at the micron level to incorporate specific micro/nanostructures or recognition molecules,enabling effective CTCs ***,by employing surface modification designs that exhibit exceptional anti-adhesion properties against WbCs,the purity of isolated CTCs can be further *** review offers an in-depth explo-ration of recent advancements,challenges,and opportunities associated with microfluidic-based CTCs iso-lation from biological ***,we will comprehensively introduce the microfluidic-based strate-gies for achieving high-efficiency CTCs isolation,which includes the morphological design of microchan-nels for physical force-based CTCs isolation and the specific modification of microchannel surfaces for affinity-based CTCs ***,a review of recent research advances in microfluidic-based high-purity CTCs isolation is presented,focusing on strategies that decrease the nonspecific adhesion of WbCs through surface micro-/nanostructure construction or chemical and biological ***,we will summarize the article by providing the prospective opportunities and challenges for the future development of microfluidic-based CTCs isolation.

关键词： Microfluidics Isolation Circulating tumor cells High-efficiency High-purity

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Enhanced terahertz vibrational absorption spectroscopy using an integrated high-Q resonator

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Photonics Research 2024年第7期12卷 1542-1547页

作者： ZHIbO hou LIAO CHEN RONGWU LIU CHI ZHANG XIAOJUN WU XINLIANG ZHANG Wuhan National Laboratory for Optoelectronics and School of Optical and Electronic Information Huazhong University of Science and TechnologyWuhan 430074China Optics Valley Laboratory Wuhan 430074China School of Electronic and Information Engineering Beihang UniversityBeijing 100191China

The terahertz(THz) absorption spectrum is a powerful method to identify substances. The improvement focuses on sensitivity and recovery ability. Here, we demonstrate enhanced THz vibrational absorption spectroscopy based on an on-chip THz whispering gallery mode resonator(THz-WGMR). A THz-WGMR with high Q can store energy and enhance the interaction between the THz waves and the target substances to capture the unique absorption fingerprint information. Therefore, it possesses significant sensitivity to identify trace amounts of substances. As a proof of concept, lactose powder and glucose powder are applied to demonstrate the effectiveness of our approach in recovering fingerprint absorption spectroscopy. Compared with a straight waveguide, the high sensitivity of the THz-WGMR is illustrated. The change of the transmissivity caused by the lactose reaches 7.8 d b around 532 GHz for the THz-WGMR, while only 1.4 d b for the straight waveguide, demonstrating the state-ofthe-art sensing performance in fingerprint absorption recovery. We believe the proposed integrated THz-WGMR will promote the THz identification of tiny fingerprint substances.

关键词： resonator waveguide absorption

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Self-supervised recalibration network for person re-identification

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Defence Technology（防务技术） 2024年第1期31卷 163-178页

作者： Shaoqi hou Zhiming Wang Zhihua Dong Ye Li Zhiguo Wang Guangqiang Yin Xinzhong Wang Shenzhen Institute of Information Technology Shenzhen518172China University of Electronic Science and Technology of China Chengdu611731China Kash Institute of Electronics and Information Industry Kashi844099China

The attention mechanism can extract salient features in images,which has been proved to be effective in improving the performance of person re-identification(Re-ID).However,most of the existing attention modules have the following two shortcomings:On the one hand,they mostly use global average pooling to generate context descriptors,without highlighting the guiding role of salient information on descriptor generation,resulting in insufficient ability of the final generated attention mask representation;On the other hand,the design of most attention modules is complicated,which greatly increases the computational cost of the *** solve these problems,this paper proposes an attention module called self-supervised recalibration(SR)block,which introduces both global and local information through adaptive weighted fusion to generate a more refined attention *** particular,a special"Squeeze-Excitation"(SE)unit is designed in the SR block to further process the generated intermediate masks,both for nonlinearizations of the features and for constraint of the resulting computation by controlling the number of ***,we combine the most commonly used Res Net-50 to construct the instantiation model of the SR block,and verify its effectiveness on multiple Re-ID datasets,especially the mean Average Precision(m AP)on the Occluded-Duke dataset exceeds the state-of-the-art(SOTA)algorithm by 4.49%.

关键词： Person re-identification Attention mechanism Global information Local information Adaptive weighted fusion

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Improved forecasting via physics-guided machine learning as exemplified using“21·7”extreme rainfall event in Henan

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Science China Earth Sciences 2024年第5期67卷 1652-1674页

作者： Qi ZHONG Zhicha ZHANG Xiuping YAO Shaoyu hou Shenming FU Yong CAO Linguo JING China Meteorological Administration Training Center Beijing 100081China State Key Laboratory of Severe Weather Chinese Academy of Meteorological SciencesBeijing 100081China Zhejiang Meteorological Observatory Hangzhou 310017China Hebei Provincial Weather Modification Center Shijiazhuang 050020China Institute of Atmospheric Physics Chinese Academy of SciencesBeijing 100029China National Meteorological Center Beijing 100081China School of Computer Science Chengdu University of Information TechnologyChengdu 610225China

As a natural disaster,extreme precipitation is among the most destructive and influential,but predicting its occurrence and evolution accurately is very challenging because of its rarity and *** the example of the“21·7”extreme precipitation event(17–21 July 2021)in Henan Province,this study explores the potential of using physics-guided machine learning to improve the accuracy of forecasting the intensity and location of extreme *** physics-guided ways of embedding physical features,fusing physical model forecasts and revised loss function are used,i.e.,(1)analyzing the anomalous circulation and thermodynamical factors,(2)analyzing the multi-model forecast bias and the associated underlying reasons for it,and(3)using professional forecasting knowledge to design the loss function,and the corresponding results are used as input for machine learning to improve the forecasting *** results indicate that by learning the relationship between anomalous physical features and heavy precipitation,the forecasting of precipitation intensity is improved significantly,but the location is rarely adjusted and more false alarms *** reasons for this are as *** anomalous features used here mainly contain information about large-scale systems and factors which are consistent with the model precipitation deviation;moreover,the samples of extreme precipitation are sparse and so the algorithm used here is ***,by combining“good and different”multi models with machine learning,the advantages of each model are extracted and then the location of the precipitation center in the forecast is improved ***,by combining the appropriate anomalous features with multi-model fusion,an integrated improvement of the forecast of the rainfall intensity and location is ***,this study is a novel exploration to improve the refined forecasting of heavy precipitation with extreme intensity and high variability,

关键词： Extreme precipitation event Refined assessment Anomalous physical features Multi-model fusion Machine learning

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Protein hydrogels for biomedical applications

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biosurface and biotribology 2024年第3期10卷 106-131页

作者： Xinyi Wang Yue hou Xiong Lu Chaoming Xie Yanan Jiang Institute of biomedical Engineering College of MedicineSouthwest Jiaotong UniversityChengduSichuanChina Key Lab of Advanced Technologies of Materials Ministry of EducationSchool of Materials Science and EngineeringSouthwest Jiaotong UniversityChengduSichuanChina Obesity and Metabolism Medicine-Engineering Integration Laboratory Department of General SurgeryThe Third People's Hospital of ChengduThe Affiliated Hospital of Southwest Jiaotong UniversityChengduSichuanChina

Hydrogels,characterised as highly hydrophilic three-dimensional polymer networks,have gained increasing attention due to their unique physicochemical properties,finding applications in various *** polymer hydrogels exhibit higher biocompatibility and biodegradability compared to traditional synthetic polymer ***,being the principal materials of natural polymer hydrogels,bear numerous modifiable functional *** resultant hydrogel possesses responsiveness,adjustable degradability,and underway as an excellent *** common raw materials used to construct protein hydrogels are *** terms of comparing natural polymer hydrogels with traditional synthetic polymer hydrogels,the authors conduct a detailed analysis and comparison,highlighting the advantages of natural polymer hydrogels in terms of biocompatibility and biodegradability,and summarising their *** authors also address the limitations of various protein hydrogels and list existing strengthening cross-linking strategies,proposing new insights to overcome the application limits of protein ***,the applications of protein hydrogels in drug delivery,biosensing,bio-inks and tissue engineering are *** authors conclude by summarising the current challenges faced by protein hydrogels and prospecting its future development.

关键词： biomaterials biomedical application

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Dynamic asymmetric mechanical responsive carbon nanotube fiber for ionic logic gate

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Chinese Chemical Letters 2024年第6期35卷 249-253页

作者： Pei Cao Yilan Wang Lejian Yu Miao Wang Liming Zhao Xu hou State Key Laboratory of Physical Chemistry of Solid Surfaces College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China Innovation Laboratory for Sciences and Technologies of Energy Materials of Fujian Province(IKKEM) Xiamen 361005China The Higher Educational Key Laboratory for biomedical Engineering of Fujian Province Department of BiomaterialsResearch Center of Biomedical Engineering of XiamenCollege of MaterialsXiamen UniversityXiamen 361005China Key Laboratory of Multifunctional Nanomaterials and Smart Systems Advanced Materials DivisionSuzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesSuzhou 215123China Institute of Artificial Intelligence Xiamen UniversityXiamen 361005China Department of Physics Research Institute for Biomimetics and Soft MatterFujian Provincial Key Laboratory for Soft Functional Materials ResearchJiujiang Research InstituteCollege of Physical Science and TechnologyXiamen UniversityXiamen 361005China Engineering Research Center of Electrochemical Technologies of Ministry of Education Xiamen UniversityXiamen 361005China

Inspired by biological ion channels,numerous artificial asymmetric ion channels have been synthesized to facilitate the fabrication of ionic ***,the creation of biomimetic asymmetric ion channels necessitates expensive scientific apparatus and intricate material processing procedures,which constrains its advancement within the realm of ionic *** this study,we have devised dynamic asymmetric ion channels with mechanical responsiveness by combining polymers of varying elastic modulus along the longitudinal axis of carbon nanotube fiber(CNTF).The ion rectification can be modulated via the disparate response of CNTF-based ion channels to mechanical *** have effectively employed these asymmetric ion channels with mechanical sensitivity in the design of a logic gate device,achieving logic operations such as“AND”and“OR”.The conception of these dynamic asymmetric ion channels with mechanical sensitivity offers a straightforward,cost-effective,and versatile approach for generating ion channels,highlighting their potential application in intricate,highly integrated ionic circuits.

关键词： Carbon nanotubes fibers Mechanical response Rectification effect Ionic logic gate

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Complement factor Ⅰ knockdown inhibits colon cancer development by affecting Wnt/β-catenin/c-Myc signaling pathway and glycolysis

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World Journal of Gastrointestinal Oncology 2024年第6期16卷 2646-2662页

作者： Yong-Jun Du Yue Jiang Yan-Mei hou Yong-bo Shi Department of Proctology Hospital of Chengdu University of Traditional Chinese MedicineChengdu 610072Sichuan ProvinceChina School of Clinical Medicine Chengdu University of Traditional Chinese MedicineChengdu 610075Sichuan ProvinceChina Department of Proctology Zigong Hospital of Traditional Chinese MedicineZigong 643000Sichuan ProvinceChina

bACKGROUND Colon cancer(CC)occurrence and progression are considerably influenced by the tumor ***,the exact underlying regulatory mechanisms remain *** To investigate immune infiltration-related differentially expressed genes(DEGs)in CC and specifically explored the role and potential molecular mechanisms of complement factor I(CFI).METHODS Immune infiltration-associated DEGs were screened for CC using *** reverse transcription polymerase chain reaction was used to examine hub DEGs expression in the CC cell *** CFI-knockdown HT29 and HCT116 cell lines were constructed,and the diverse roles of CFI in vitro were assessed using CCK-8,5-ethynyl-2’-deoxyuridine,wound healing,and transwell *** and eosin staining and immunohistochemistry staining were employed to evaluate the influence of CFI on the tumorigenesis of CC xenograft models constructed using bALb/c male nude *** proteins associated with glycolysis and the Wnt pathway were measured using western *** Six key immune infiltration-related DEGs were screened,among which the expression of CFI,complement factor b,lymphoid enhancer binding factor 1,and SRY-related high-mobility-group box 4 was upregulated,whereas that of fatty acid-binding protein 1,and bone morphogenic protein-2 was ***,CFI could be used as a diagnostic biomarker for ***,CFI silencing inhibited CC cell proliferation,migration,invasion,and tumor ***,CFI knockdown downregulated the expression of key glycolysis-related proteins(glucose transporter type 1,hexokinase 2,lactate dehydrogenase A,and pyruvate kinase M2)and the Wnt pathway-related proteins(β-catenin and c-Myc).Further investigation indicated that CFI knockdown inhibited glycolysis in CC by blocking the Wnt/β-catenin/c-Myc *** The findings of the present study demonstrate that CFI plays a crucial role in CC development by influencing g

关键词： Colon cancer Immune infiltration Complement factor I Glycolysis Wnt/β-catenin/c-Myc pathway

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A late Carboniferous transition from subduction to collision:Tectonosedimentary evidence from southern Junggar,NW China

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Geoscience Frontiers 2024年第3期15卷 166-179页

作者： Shuoqin hou Di Li Dengfa He Yu Lu Yu Zhen Hao Yang Dan Fan Key Laboratory of Marine Reservoir Evolution and Hydrocarbon Accumulation Mechanism the Ministry of Educationand School of Energy ResourcesChina University of Geosciences(Beijing)Beijing 100083China

The Carboniferous to Permian tectono-sedimentary evolution of the southern Junggar area brings new insights into understanding the subduction-collision processes in the northern Tianshan *** geophysics,geochemistry,and geochronology approaches,this study investigates the Carboniferous-Permian strata in the southern Junggar *** results have revealed three distinct tectono-stratigraphic evolutionary stages,each marked by a distinctive volcano-sedimentary *** Early Carboniferous strata suggest intense volcanic activities in the southern Junggar *** the Late Carboniferous,the southern Junggar basin was controlled by normal faulting in an extensional setting,receiving sedimentary inputs from the Junggar *** Lower Permian,unconformably overlying the Upper Carboniferous,was shaped by an extensional regime and is comprised by volcano-clastic sequences that received detritus from the Yili-Central Tianshan *** findings indicate that a Late Carboniferous forearc basin developed in the southern Junggar area,and it evolved into a post-collisional rift in the Early *** period marked a dynamic shift from bidirectional subduction(rollback)to the detachment of the North Tianshan oceanic *** propose that the collision between the YiliCentral Tianshan block and the Junggar terrane,along with the closure of the North Tianshan Ocean,likely occurred in the Late Carboniferous(ca.306-303 Ma).

关键词： Tectono-sedimentary evolution Tectonic transition Carboniferous-Permian Junggar basin North Tianshan Ocean

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An in-situ self-etching enabled high-power electrode for aqueous zinc-ion batteries

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Journal of Energy Chemistry 2024年第1期88卷 399-408,I0009页

作者： Shuang hou Dingtao Ma Yanyi Wang Kefeng Ouyang Sicheng Shen Hongwei Mi Lingzhi Zhao Peixin Zhang College of Chemistry and Environmental Engineering Shenzhen UniversityShenzhen 518060GuangdongChina Guangdong Provincial Engineering Technology Research Center for Low Carbon and Advanced Energy Materials School of Semiconductor Science and TechnologySouth China Normal UniversityFoshan 528225GuangdongChina SCNU Qingyuan Institute of Science and Technology Innovation Co. Ltd.Qingyuan 511517GuangdongChina

Sluggish storage kinetics is considered as the main bottleneck of cathode materials for fast-charging aqueous zinc-ion batteries(AZIbs).In this report,we propose a novel in-situ self-etching strategy to unlock the Palm tree-like vanadium oxide/carbon nanofiber membrane(P-VO/C)as a robust freestanding *** investigations including the finite element simulation,in-situ X-ray diffraction,and in-situ electrochemical impedance spectroscopy disclosed it an electrochemically induced phase transformation mechanism from VO to layered Zn_(x)V_(2)O_5·nH_(2)O,as well as superior storage kinetics with ultrahigh pseudocapacitive *** demonstrated,such electrode can remain a specific capacity of 285 mA h g^(-1)after 100 cycles at 1 A g^(-1),144.4 mA h g^(-1)after 1500 cycles at 30 A g^(-1),and even 97 mA h g^(-1)after 3000 cycles at 60 A g^(-1),***,an impressive power density of 78.9 kW kg^(-1)at the super-high current density of 100 A g^(-1)also can be *** design concept of in-situ self-etching free-standing electrode can provide a brand-new insight into extending the pseudocapacitive storage limit,so as to promote the development of high-power energy storage devices including but not limited to AZIbs.

关键词： In-situ self-etching Free-standing electrode Pseudocapacitive storage High-power Zinc-ion batteries

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