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View of thermodynamic phase transition of the charged Gauss-bonnet AdS black hole via the shadow

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Chinese physics b 2024年第4期33卷 355-362页

作者：何柯腱郭森罗智李国平 college of physics Chongqing UniversityChongqing 401331China Guangxi Key Laboratory for Relativistic Astrophysics School of Physical Science and TechnologyGuangxi UniversityNanning 530004China School of physics and Astronomy China West Normal UniversityNanchong 637000China

We examine thermodynamic phase transition(PT)of the charged Gauss-bonnet Ad S black hole(bH)by utilizing the shadow *** this system,we rescale the corresponding Gauss-bonnet coefficientαby a factor of 1/(D-4),and ensure thatαis positive to avoid any singularity *** equation derived for the shadow radius indicates that it increases as the event horizon radius increases,making it an independent variable for determining bH *** investigating the PT curve in relation to shadows,we can observe that the shadow radius can be used as an alternative to the event horizon radius in explaining the phenomenon of bH ***,the results indicate that an increase in the parameterαcorresponds to a decrease in the temperature of the *** utilizing the relationship between the temperature and the shadow radius,it is possible to obtain the thermal profile of the Gauss-bonnet AdS *** is evident that there is an N-type variation in temperature for pressures Pby shadow expands while the temperature *** utilization of bH shadows as a probe holds immense significance in gaining a deeper understanding of bH thermodynamic behavior.

关键词： Gauss-bonnet AdS black hole thermodynamic shadow

Advances and challenges in thermal runaway modeling of lithium-ion batteries

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The Innovation 2024年第4期5卷 172-186,171页

作者： Gongquan Wang ping ping Depeng Kong Rongqi Peng Xu He Yue zhang Xinyi Dai Jennifer Wen Center for Offshore Engineering and Safety technology China University of Petroleum(East China)Qingdao 266580China college of Chemical Engineering China University of Petroleum(East China)Qingdao 266580China Centre for Energy Resilience School of Mechanical Engineering SciencesUniversity of SurreyGuildfordSurrey GU27XHUK

The broader application of lithium-ion batteries(LIbs)is constrained by safety concerns arising from thermal runaway(TR).Accurate prediction of TR is essential to comprehend its underlying mechanisms,expedite battery design,and enhance safety protocols,thereby significantly promoting the safer use of *** complex,nonlinear nature of LIb systems presents substantial challenges in TR modeling,stemming from the need to address multiscale simulations,multiphysics coupling,and computing efficiency *** paper provides an extensive review and outlook on TR modeling technologies,focusing on recent advances,current challenges,and potential future *** begin with an overview of the evolutionary processes and underlying mechanisms of TR from multiscale perspectives,laying the foundation for TR *** a comprehensive understanding of TR phenomena and mechanisms,we introduce a multiphysics coupling model framework to encapsulate these *** this framework,we detail four fundamental physics modeling approaches:thermal,electrical,mechanical,and fluid dynamic models,highlighting the primary challenges in developing and integrating these *** address the intrinsic trade-off between computational accuracy and efficiency,we discuss several promising modeling strategies to accelerate TR simulations and explore the role of AI in advancing next-generation TR ***,we discuss challenges related to data availability,model scalability,and safety standards and regulations.

关键词： lithium thermal modeling

Re-usable Cd_(0.9)Zn_(0.1)S-ZnO@C/PVDF piezo-photocatalytic film with exceptional hydrogen evolution capability triggered by the synergetic advantages of piezoelectricity and S-Scheme heterojunction

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Journal of Energy Chemistry 2024年第9期96卷 164-176页

作者： ping Su Dong zhang Minghui Zhu Tengteng Liang Nan Yang Huaihao Zhao Dafeng zhang Junchang Liu Peiqing Cai Xipeng Pu School of Materials science and Engineering Shandong Provincial Key Laboratory of Chemical Energy Science and Novel Cell TechnologyLiaocheng UniversityLiaocheng 252000ShandongChina School of physics science and Information technology Shandong Key Laboratory of Optical Communication Sciencend TechnologyLiaocheng UniversityLiaocheng 252000ShandongChina college of Optical and Electronic technology China Jiliang UniversityHangzhou 310018ZhejiangChina

Piezoelectric materials have advantages of fine-tuning photocatalytic performance through harvesting mechanical energy and open a new avenue in facilitating green catalytic ***,polyvinylidene fluoride(PVDF),a flexible piezoelectric material,was introduced to synthesize a novel Cd_(0.9)Zn_(0.1)S-ZnO@C/PVDF(CZS-ZO@C/PVDF)piezo-photocatalytic film by spin coating and immersion phase conversion *** from the piezoelectricity of PVDF and the internal electric field(IEF)of CZS-ZO@C Step-scheme(S-Scheme)heterojunction,CZS-ZO@C/PVDF was able to induce a hydrogen generation rate of 34.9 mmol g^(−1)h^(−1)activated by ultrasound and visible light(U-L),which is∼17.5 times of Cd_(0.9)Zn_(0.1)S/PVDF(CZS/PVDF)and∼7.4 times of the photocatalysis rate activated by visible light only(L).Piezoelectric measurements and COMSOL simulation illustrated the excellent piezoelectricity of CZS-ZO@C/PVDF film,which exhibits a piezoelectric coefficient(d33)of 9.9 pm V−1 and a piezoelectric potential of 874 mV(under 0.5 MPa).The reaction mechanism for the exceptional piezo-photocatalytic performance was finally disclosed through density functional theory(DFT)calculation and electrochemical *** study enriches the application scope of piezoelectric materials in sustainable energy catalysis and provides a new direction to develop efficient piezoelectric photocatalysts.

关键词： Piezo-photocatalysis Heterojunction Cd_(0.9)Zn_(0.1)S Zno@c PVDF

Ordered bicontinuous Network Structures Regulated by Orientational Interactions in a Rod-Coil block Copolymer

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Chinese Journal of Polymer science 2024年第5期42卷 636-642,I0008页

作者： Xiao-Lin Lyu Shi-Chu Yang An-Qi Xiao ping-ping Hou Wei zhang Hong-bing Pan Zhi-Hao Shen Xing-He Fan Qi-Feng Zhou beijing National Laboratory for Molecular sciences Key Laboratory of Polymer Chemistry and Physics of Ministry of EducationCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing100871China Key Laboratory of Advanced Materials Technologies International(HongKong Macao and Taiwan)Joint Laboratory on Advanced Materials TechnologiesCollege of Materials Science and EngineeringFuzhou UniversityFuzhou350108China

The rich phase behavior of block copolymers(bCPs)has drawn great attention in recent ***,the double diamond(DD)phase is rarely obtained because of the competition between the minimization of interfacial energy and packing ***,a rod-coil bCP containing mesogen-jacketed liquid crystalline polymer is designed to acquire ordered bicontinuous network *** reduction of internal energy originating from the orientational interaction among the rod blocks can compensate for the free energy penalty of packing frustration to stabilize the DD *** resulting bCP can also experience lamellae-to-DD and double gyroid-to-lamellae transitions by changing the annealing *** results make the rod-coil bCP an excellent candidate for the self-assembly of ordered network structures,demonstrating great potential in nanopatterning and metamaterials.

关键词： block copolymer Rod-coil Ordered bicontinuous phase Double diamond Double gyroid

Molecule configurations modulate packing array and charge transfer in cocrystal engineering

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science China Chemistry 2024年第2期67卷 512-516页

作者： Shenglong An Mengyuan Qiao Xin Jin Xuanying Chen Jianhua Su Lifang guo Zhiyun zhang Key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering Feringa Nobel Prize Scientist Joint Research CentreFrontiers Science Center for Materiobiology and Dynamic ChemistryEast China University of Science&TechnologyShanghai200237China

Organic cocrystal as an emerging assembly strategy has received increasing attention in constructing multiple functional materials,through continually screening suitable constituent monomers or changing their stoichiometry ***,the role of molecule configuration in the cocrystal field is rarely explored despite the fascinating potential in regulating the packing *** this study,the N,N′-diphenyl-5,10-dihydrophenazine derivatives(DPPs) with the flexible scaffold and different methyl substitutions are selected as the donors bearing various molecular *** a simple collaborative way,a series of cocrystals based on DPPs and OFN(octafluoronaphthalene) are fabricated,exhibiting two self-adaptive molecular stacking arrays.X-ray crystallographic analysis and theoretical calculation unveil their different π···π interactions and charge transfer characters,leading to the significant emission redshift up to 125 nm compared with individual *** a result,controllable molecule stacking structure,tunable emission,and charge transfer properties can be *** study provides a new perspective to reveal the structure-property relationships at the molecular level by controlling the molecule configuration in cocrystal engineering,contributing to the development of cocrystal theoretical physics and organic functional materials.

关键词： cocrystals molecular configuration self-adaptive packing mode charge transfer

Crystallinity-defect matching relationship of g-C_(3)N_(4): Experimental and theoretical perspectives

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Green Energy & Environment 2024年第4期9卷 623-658页

作者： Yuhan Li Ziteng Ren Zhengjiang He ping Ouyang Youyu Duan Wendong zhang Kangle Lv Fan Dong Engineering Research Center for Waste Oil Recovery technology and Equipment Ministry of EducationChongqing Key Laboratory of Catalysis and New Environmental MaterialsChongqing Technology and Business UniversityChongqing400067China Nanchang Institute of technology Nanchang33044China Key Laboratory of Resources Conversion and Pollution Control of the State Ethnic Affairs Commission College of Resources and Environmental ScienceSouth-Central Minzu UniversityWuhan430074China college of physics and Center of Quantum Materials and Devices Chongqing UniversityChongqing401331China Chongqing Key Laboratory of Green Synthesis and Application Chongqing Normal UniversityChongqing401331China

Good crystallinity can reduce the charge recombination centers caused by defects,whilst structures with strong polycondensation have high charge mobility,leading to more charge transfer to the material surface for *** effort has been put into the preparation of a highly efficient g-C_(3)N_(4) with defects to improve its application potential under the premise in high ***,this review paper emphasizes the importance to balance the defect and crystallinity of g-C_(3)N_(4).In addition,detailed discussion on the relationship between defects and activity of g-C_(3)N_(4) was carried out based on its applications in environmental purification(e.g.,VOCs oxidation,NO_(x) oxidation,H_(2)O_(2) evolution,sterilization,pesticide oxidation)and energy conversion(H_(2) evolution,N_(2) fixation and CO_(2) reduction).Lastly,the challenge in developing more efficient defective g-C_(3)N_(4) photocatalytic materials is summarized.

关键词： Photocatalysis Defect G-C_(3)N_(4) Crystallinity Application

The effects of deformation parameters and cooling rates on the aging behavior of AZ80+0.4%Ce

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Journal of Magnesium and Alloys 2024年第2期12卷 639-658页

作者： Yongbiao Yang Jinxuan guo Cuiying Wang Ting Yan zhang Wenxuan Jiang Zhimin zhang Qiang Wang guojun Li Jun Wang college of Materials science and Engineering North University of ChinaLane 3Xueyuan RoadTaiyuanShanxiChina030051 State Key Laboratory of Advanced Stainless Steel Materials Taiyuan Iron Steel(Group)Co.Ltd.Taiyuan 030003China technology Center Shanxi Taigang Stainless Steel Co.Ltd.Taiyuan 030003China

The extruded AZ80+0.4%Ce magnesium alloy was twisted in the temperature range of 300-380℃by using a Gleeble 3500 thermal simulation test machine with a torsion *** deformed cylindrical specimens were cooled at a cooling rate of 10℃/s or 0.1℃/s,respectively,and aged at 170℃.The microstructure analysis results showed that the grain size decreased with increasing specimen radial position from center(SRPC),and that the strong initial basal texture of the extruded magnesium alloy was *** continuous and discontinuous dynamic recrystallization mechanisms were involved in contributing to the grain refinement for all specimens *** a novel extension twinning induced dynamic recrystallization mechanism was proposed for specimen deformed at 300℃.For the specimens deformed at 300℃and 340℃followed by a slow cooling rate(0.1℃/s),precipitates of various shapes(β-Mg_(17)Al_(12)),with the dominant precipitates being on the grains boundaries,appeared on the surface *** specimen deformed at 380℃,lamellar precipitates(LPS)in the interiors of the grains were *** aging,the LPS still dominated for specimens twisted at 380℃;however,the LPS gradually decreased with decreasing deformation temperatures from 380℃to 300℃.Dynamically precipitatedβ,especially those decorating the grain boundaries,changed the competition pictures for the LPS and precipitates of other shapes after ***,LPS dominated the areas for the center section of the specimens after aging regardless of deformation *** temperature deformation with high SRPC followed by rapid cooling rate increased the micro hardness of the alloy after aging due to refined grain,reduced precipitates size,decreased lamellar spacing as well as strain hardening.

关键词： AZ80+0.4%Ce magnesium alloy Hot torsion Deformation parameters Cooling rate Aging Micro hardness

Influence of network structure on spreading dynamics via tie range

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Chinese physics b 2024年第8期33卷 606-613页

作者：李敏宋玉蓉宋波李汝琦蒋国平张晖 college of Automation and college of Artificial Intelligence Nanjing University of Posts and TelecommunicationsNanjing 210023China School of Modern Posts Nanjing University of Posts and TelecommunicationsNanjing 210023China School of Computer science Nanjing University of Posts and TelecommunicationsNanjing 210023China Full Truck Alliance Co.Ltd. Nanjing 210012China

There are various phenomena of malicious information spreading in the real society, which cause many negative impacts on the society. In order to better control the spreading, it is crucial to reveal the influence of network structure on network spreading. Motifs, as fundamental structures within a network, play a significant role in spreading. Therefore, it is of interest to investigate the influence of the structural characteristics of basic network motifs on spreading *** the edges of the basic network motifs in an undirected network correspond to different tie ranges, two edge removal strategies are proposed, short ties priority removal strategy and long ties priority removal strategy. The tie range represents the second shortest path length between two connected nodes. The study focuses on analyzing how the proposed strategies impact network spreading and network structure, as well as examining the influence of network structure on network spreading. Our findings indicate that the long ties priority removal strategy is most effective in controlling network spreading, especially in terms of spread range and spread velocity. In terms of network structure, the clustering coefficient and the diameter of network also have an effect on the network spreading, and the triangular structure as an important motif structure effectively inhibits the spreading.

关键词： network spreading network motifs tie range edge removal strategy

Unveiling the critical role of TiO_(2)-supported atomically dispersed Cu species for enhanced photofixation of N_(2)to nitrate

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Fundamental Research 2024年第4期4卷 934-940页

作者： Dong Li Yunxuan Zhao Chao Zhou Li-ping zhang Junwang Tang Tierui zhang Key Laboratory of Photochemical Conversion and Optoelectronic Materials Technical Institute of Physics and ChemistryChinese Academy of SciencesBejing 100190China Center of Materials science and Optoelectronics Engineering University of Chinese Academy of SciencesBejing 100049China School of Future technology University of Chinese Academy of SciencesBejing 100049China Department of Chemical Engineering University College LondonLondon WC1E7JEUnited Kingdom

Nitrate products are widely used in manufacturing as crucial raw materials and *** traditional nitrate synthesis process involves high energy consumption and emission,thereby opposing the goals of zero-carbon emission and green ***,a sustainable roadmap for nitrate synthesis that uses green energy input,clean N sources,and direct catalytic processes is urgently required(e.g.,developing a novel photosynthesis system).Here,we synthesized TiO2-supported atomically dispersed Cu species for N_(2)photofixation to nitrate in a flow *** optimized photocatalyst yielded a high nitrate photosynthesis rate of 0.93μmol h-1 and selectivity of~90%,which is superior to most of the values reported thus ***,experimental results and in-situ investigations revealed that the atomically dispersed Cu sites in the as-designed sample significantly enhanced the separation and transfer efficiency of photogenerated carriers,adsorption and activation of reactants,and the formation of chemisorbed O_(x)intermediates,thereby realizing the excellent photofixation of N_(2)to nitrate.

关键词： N_(2) photofixation TiO_(2) Nitrate photosynthesis Cu species NO_(x),intermediates