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Promotion effects of alkali metals on iron molybdate catalysts for CO_(2)catalytic hydrogenation

Journal of Energy Chemistry 2023年第10期85卷 291-300,I0009页

作者： Yong Zhou Aliou Sadia Traore Deizi V.Peron Alan J.Barrios Sergei A.Chernyak Massimo Corda Olga V.Safonova Achim Iulian Dugulan Ovidiu Ersen Mirella Virginie Vitaly V.Ordomsky andrei Y.Khodakov University of Lille CNRSCentrale LilleUniversity of ArtoisUMR 8181-UCCS-Unitéde Catalyse et Chimie du SolideLille F-59000France IPCMS UMR 7504 CNRSUniversitéde Strasbourg23 rue du LoessBP 43Cedex 267034 StrasbourgFrance PSI CH-5232 VilligenSwitzerland Fundamental Aspects of Materials and Energy Group Delft University of TechnologyMekelweg 15Delft 2629 JBNetherlands

CO_(2)hydrogenation is an attractive way to store and utilize carbon dioxide generated by industrial processes,as well as to produce valuable chemicals from renewable and abundant *** catalysts are commonly used for the hydrogenation of carbon oxides to ***-molybdenum catalysts have found numerous applications in catalysis,but have been never evaluated in the CO_(2)*** this work,the structural properties of iron-molybdenum catalysts without and with a promoting alkali metal(Li,Na,K,Rb,or Cs)were characterized using X-ray diffraction,hydrogen temperatureprogrammed reduction,CO_(2)temperature-programmed desorption,in-situ^(57)Fe Mossbauer spectroscopy and operando X-ray adsorption *** catalytic performance was evaluated in the CO_(2)*** the reaction conditions,the catalysts undergo the formation of an iron(Ⅱ)molybdate structure,accompanied by a partial reduction of molybdenum and carbidization of *** rate of CO_(2)conversion and product selectivity strongly depend on the promoting alkali metals,and electronegativity was identified as an important factor affecting the catalytic *** CO_(2)conversion rates were observed with the promoters having higher electronegativity,while low electronegativity of alkali metals favors higher light olefin selectivity.

关键词： CO_(2)utilization Iron molybdate catalysts Promotion Alkali metals Light olefins In-situ characterization

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Momentum considerations inside near-zero index materials

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Light(Science & Applications) 2022年第8期11卷 1782-1789页

作者： Michaël Lobet Iñigo Liberal Larissa Vertchenko andrei VLavrinenko Nader Engheta Eric Mazur John A.Paulson School of Engineering and Applied Sciences Harvard University9 Oxford StreetCambridgeMA02138USA Department of Physics and Namur Institute of Structured Materials University of NamurRue de Bruxelles 515000NamurBelgium Electrical and Electronic Engineering Department Universidad Pública de NavarraCampus ArrosadíaPamplona31006Spain Department of Photonics Engineering Technical University of DenmarkØrsteds Plads 345ADK-2800 KgsLyngbyDenmark Department of Electrical and Systems Engineering University of PennsylvaniaPhiladelphiaPA19104USA

Near-zero index (NZI) materials, i.e., materials having a phase refractive index close to zero, are known to enhance or inhibit light-matter interactions. Most theoretical derivations of fundamental radiative processes rely on energetic considerations and detailed balance equations, but not on momentum considerations. Because momentum exchange should also be incorporated into theoretical models, we investigate momentum inside the three categories of NZI materials, i.e., inside epsilon-and-mu-near-zero (EMNZ), epsilon-near-zero (ENZ) and mu-near-zero (MNZ) materials. In the context of Abraham–Minkowski debate in dispersive materials, we show that Minkowski-canonical momentum of light is zero inside all categories of NZI materials while Abraham-kinetic momentum of light is zero in ENZ and MNZ materials but nonzero inside EMNZ materials. We theoretically demonstrate that momentum recoil, transfer momentum from the field to the atom and Doppler shift are inhibited in NZI materials. Fundamental radiative processes inhibition is also explained due to those momentum considerations inside three-dimensional NZI materials. Absence of diffraction pattern in slits experiments is seen as a consequence of zero Minkowski momentum. Lastly, consequence on Heisenberg inequality, microscopy applications and on the canonical momentum as generator of translations are discussed. Those findings are appealing for a better understanding of fundamental light-matter interactions at the nanoscale as well as for lasing applications.

关键词： materials. momentum Minkowski

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Reply to "Discussion 2 on 'Introspection on improper seismic retrofit of Basilica Santa Maria di Collemaggio after 2009 Italian earthquake' by G.P. Cimellaro, A.M. Reinhorn and *** Stefano" by Enzo Cartapati

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Earthquake Engineering and Engineering Vibration 2012年第2期11卷 291-292页

作者： Gian Paolo Cimellaro andrei M. Reinhorn Alessandro De Stefano Department of Structural Geotechnical & Building Engineering (DISEG) Politecnico di Torino Corso Duca degli Abruzzi 24 10129 Turin Italy Department of Civil Structural & Environmental Engineering University at Buffalo the State University of New York 135 Ketter Hall Buffalo NY USA

The authors thank the discusser for the additional information,which is provided related to the historical interventions of the church through the centuries. This information was known to the authors,however they deci... 详细信息

关键词： Reply to A.M Reinhorn and A.De Stefano Introspection on improper seismic retrofit of Basilica Santa Maria di Collemaggio after 2009 Italian earthquake by G.P Discussion 2 on De

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Radial Supershapes for Solid Modeling

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Journal of Computer Science & Technology 2006年第2期21卷 238-243页

作者： Yohan D. Fougerolle andrei Gribok Sebti Foufou Frederic Truchetet Mongi A. Abidi Le2i Lab. UMR CNRS 5158 Universitd de Bourgogne 12 rue de la fonderie 71200 Le Creusot France IRIS Lab. The University of Tennessee Ferris Hall Knoxville 37996 TAT U.S.A.

In the previous work, an efficient method has been proposed to represent solid objects as multiple combinations of globally deformed supershapes. In this paper, this framework is applied with a new supershape implicit function that is based on the notion of radial distance and results are presented on realistic models composed of hundreds of hierarchically globally deformed supershapes. An implicit equation with guaranteed differential properties is obtained by simple combinations of the primitives~ implicit representations using R-function theory. The surface corresponding to the zero-set of the implicit equation is efficiently and directly polygonized using the primitives,parametric forms. Moreover, hierarchical global deformations are considered to increase the range of shapes that can be modeled. The potential of the approach is illustrated by representing complex models composed of several hundreds of primitives inspired from CAD models of mechanical parts.

关键词： implicit surface solid modeling superquadrics supershape

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Paleocene–early Eocene post-subduction magmatism in Sikhote-Alin (Far East Russia): New constraints for the tectonic history of the Izanagi-Pacific ridge and the East Asian continental margin

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Geoscience Frontiers 2021年第4期12卷 71-85页

作者： andrei V.Grebennikov Igor V.Kemkin Alexander I.Khanchuk Far East Geological Institute Far Eastern BranchRussian Academy of Sciencespr.100-letiya Vladivostok 159Vladivostok 690022Russia Institute of Geology of Ore Deposits PetrographyMineralogy and Geochemistry(IGEM)Russian Academy of Sciences35 Staromonetny Per.Moscow 109017Russia

New isotopic,geochemical and geochronological data justify the widespread occurrence of middle Paleocene to early Eocene(60–53 Ma)post-subduction felsic magmatism across the entire Sikhote-Alin territory(southeastern Russia),conform with previous observations in Northeast China,the southern Korean Peninsula,and the Inner Zone of *** igneous activity in East Asia coincided with the reactivation(after tectonic quiescence between~93–60Ma)of left-lateral strike-slip displacements along the Tan-Lu and Central Sikhote-Alin faults and with the post-60 Ma cessation of subduction/accretion recorded in the Shimanto belt of SW *** Sikhote-Alin post-subduction igneous A-type rocks present diverse mineralogical and geochemical features that suggest interactions of the subducting plate with anhydrous mantle upwelling through slab tears in the continental *** middle Paleocene–early Eocene magmatismis not related to subduction but is synchronous with strikeslip tectonics and the termination of accretionary prism development,suggesting a shift in tectonic regime from oceanic plate subduction at a convergent margin to parallel sliding and initiation of a transformcontinental *** new observations are inconsistent with the current tectonic model of 60–50 Ma Izanagi-Pacific ridge subduction beneath East Asian continental margin.

关键词： Post-subduction magmatism Slab tear Sikhote-Alin Paleocene A-type rocks Izanagi-Pacific ridge

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Role of neuronal gap junctions in NMDA receptor-mediated excitotoxicity and ischemic neuronal death

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Neural Regeneration Research 2016年第1期11卷 75-76页

作者： andrei B.Belousov Joseph D.Fontes Department of Molecular and Integrative Physiology University of Kansas Medical Center Department of Biochemistry and Molecular Biology University of Kansas Medical Center

In the mammalian central nervous system（CNS）coupling of neurons by gap junctions and the expression of neuronal gap junction protein,connexin 36（Cx36）rapidly increases（usually during 1–2 hours）following a wide range of neuronal injuries,including ischemia,traumatic brain injury（TBI）,spinal cord injury and epilepsy（reviewed in Belousov and Fontes,2013）.Pharmacological blockade or genetic elimi-nation of Cx36-containing gap junctions dramatically re- duce neuronal death in animal models of ischemia, TBI and epilepsy and prevent NMDA receptor （NMDAR）-mediated excitotoxicity （Belousov and Fontes, 2014）.

关键词： neuronal epilepsy junction connexin traumatic NMDA injuries cortical mammalian minutes

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Deep Forest as a framework for a new class of machine-learning models

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National Science Review 2019年第2期6卷 186-187页

作者： Lev V.Utkin Anna A.Meldo andrei V.Konstantinov Laboratory of Neural Network Technology and Artificial Intelligence Peter the Great St. Petersburg Polytechnic University

A new deep learning framework—the socalled Deep Forest (DF), proposed by Zhi-Hua Zhou and Ji Feng [1,2]—can be regarded as one of the important events of 2017 in machine learning, although it was unjustly unnoticed by a large number of researchers. The DF combines several ensemble-based methods, including Random Forests (RFs) and Stacking, into a structure that is similar to a multi-layer neural network, but each layer in the DF

关键词： Deep Forest as a framework for a new class of machine-learning models

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Development of the Arctic reindeer industry from the perspective of Sino-Russian green biomanufacturing cooperation

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Advances in Polar Science 2022年第4期33卷 326-335页

作者： LUO Ying WANG Jinhui Andrew Alexandrovich LOBANOV Natalia Sergeevna KULESHOVA ZHU Yan Sergei Vasilevich ANDRONOV Lidiya Petrovna LOBANOVA Elena Nikolaevna BOGDANOVA Irina Alexandrovna GRISHECHKINA andrei Ivanovich POPOV South China Business College Guangdong University of Foreign StudiesGuangzhou 510545China Moscow State University Institute of Asian and African StudiesMoscow 125009Russian Federation National Medical Research Center for Rehabilitation and Balneology Ministry of Health of the Russian FederationMoscow 121099Russian Federation Department of Investigation Guangdong Police CollegeGuangzhou 510230China Northern Arctic Federal University Arhangelsk 163000Russian Federation Arctic Research Scientific Centre of Yamalo–Nenets Autonomous Okrug Nadym 629730Russian Federation

Russia’s reindeer population accounts for two thirds of the world’s *** is a strong and resilient population of reindeer on the tundra,and reindeer herders inherit and transmit the unique culture of the *** products have become the subject of innovative developments in the biopharmaceutical and healthcare products industry owing to their unique raw material *** deer antlers and blood are widely used in traditional Chinese medicine,significant quantities of Arctic reindeer products are likely to be sold in *** understanding of the Russian Arctic reindeer industry will help Chinese companies invest in the Russian Arctic,promote Sino-Russian Arctic cooperation on green biomanufacturing,and lead to the development of new products that promote human health.

关键词： reindeer industry Russian Arctic green biomanufacturing Sino-Russian cooperation

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Ischemic colitis and large bowel infarction:A case report

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World Journal of Gastroenterology 2012年第39期18卷 5640-5644页

作者： Eugen Florin Georgescu Doina Carstea Daniela Dumitrescu Ramona Teodorescu andrei Carstea Department of Internal Medicine 1/Gastroenterology Filantropia University Hospital of Craiova200136 CraiovaRomania Department of Cardiology Filantropia University Hospital of Craiova200136 CraiovaRomania Department of Radiology University of Medicine and Pharmacy of Craiova200349 CraiovaRomania

Ischemic bowel disease results from an acute or chronic drop in the blood supply to the bowel and may have various clinical presentations, such as intestinal angina, ischemic colitis or intestinal infarction. Elderly patients with systemic atherosclerosis who are symptomatic for the disease in two or more vascular beds have multiple comorbidities and are particularly at risk. The clinical evolution and outcome of this disease are difficult to predict because of its pleomorphic aspects and the general lack of statistical data. In this paper, we present the case of a patient who was monitored in our unit for six years. For this patient, we encountered iterative changes in the clinical pattern, beginning with chronic "intestinal angina" and finishing with signs of acute mesenteric ischemia after an episode of ischemic colitis. This evolution is particularly rare in clinical practice, and the case is instructive because it raises discussions about the natural history of the condition and the thera-peutic decisions that should be made at every stage of the disease. An important lesson is that ischemic bowel disease should always be considered in patients who have multiple risk factors for atherosclerosis and have experienced recurrent "indistinct" abdominal *** these cases, aggressive investigation and therapeutic decisions must be taken whenever possible. Despite an absence of standardized protocols, angiographic evaluation and revascularization procedures have beneficial outcomes. Current advances in endovascular therapy, such as percutaneous transluminal angioplasty with stenting, should be increasingly used in patients with chronic mesenteric ischemia. Such therapy can avoid the risks that are associated with open repair. However, technical difficulties, especially in severe stenotic lesions, frequently occur.

关键词：大肠杆菌结肠炎缺血病例报告动脉粥样硬化介入治疗临床表现血管成形术

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Nonasthmatic eosinophilic bronchitis in an ulcerative colitis patient-a putative adverse reaction to mesalazine:A case report and review of literature

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World Journal of Clinical Cases 2020年第18期8卷 4162-4168页

作者： andrei Tudor Cernomaz Gabriela Bordeianu Cristina Terinte Cristina Maria Gavrilescu Department of Internal Medicine Grigore T.Popa University of Medicine and PharmacyIasi 700115Romania Department of Biochemistry Grigore T.Popa University of Medicine and PharmacyIasi 700115Romania Department of Pathology Regional Oncology InstituteIasi 700483Romania

BACKGROUND Lung and airway involvement in inflammatory bowel disease are increasingly frequently reported either as an extraintestinal manifestation or as an adverse effect of *** SUMMARY We report a case of a patient with ulcerative colitis controlled under mesalazine treatment who presented with chronic cough and *** computed tomography and bronchoscopy findings supported tracheal involvement in ulcerative colitis;pathology examination demonstrated an unusual eosinophilrich inflammatory pattern,and together with clinical data,a nonasthmatic eosinophilic bronchitis diagnosis was *** recovery was observed within days of mesalazine *** Mesalazine-induced eosinophilic respiratory disorders have been previously reported,generally involving the lung *** the best of our knowledge,this is the first report of mesalamine-induced eosinophilic involvement in the upper airway.

关键词： Mesalamine Ulcerative colitis Hemoptysis Bronchitis Drug-related side effects Case report

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