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Low-melting mixture solvents: extension of deep eutectic solvents and ionic liquids for broadening green solvents and green chemistry

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Green chemical Engineering 2024年第4期5卷 409-417页

作者： yu Chen zhiwu yu moe key Laboratory of bioorganic {3. chemistry and chemical biology Department of ChemistryTsinghua University

Green solvents such as water and ionic liquids(ILs) are pillars of the great mansion of green chemistry and green processing. Initially proposed as a new family of ILs,deep eutectic solvents(DESs) have received fast development in the past two decades. In this contribution,DESs are reviewed critically and the concept is extended to lowmelting mixture solvents(Lo MMSs),which cover all kinds of materials including ionic compounds,molecular compounds,and metals. Six classes of Lo MMSs are proposed as the new classification system and examples are given. Finally,several thermodynamic issues concerning Lo MMSs are discussed. Two new concepts,robustness of Lo MMSs and high-entropy Lo MMSs,are proposed.

关键词： Green solvents Deep eutectic solvents Low transition temperature mixture solvents Phase diagram EGaIn

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EXCESS SPECTROSCOPY:A NEW METHOD TO PROBE MOLECULAR INTERACTIONS

EXCESS SPECTROSCOPY:A NEW METHOD TO PROBE MOLECULAR INTERACT...

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40th IUPAC Congress

作者： Qingzhong Li Liming He and zhiwu yu* moe {3. Laboratory of bioorganic phosphorous chemistry and chemical biology Department of chemistry Tsinghua University Beijing 100084 P.R.China

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COMPRESSING BEHAVIOR OF BINARY MIXTURES CONTAINING DIPALMITOYLPHOSPHATIDYLCHOLINE AND STEROLS AT AIR-WATER INTERFACE

COMPRESSING BEHAVIOR OF BINARY MIXTURES CONTAINING DIPALMITO...

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40th IUPAC Congress

作者： yunlan Su Qingzhong Li Lin Chen and zhiwu yu* {3. key Laboratory of bioorganic phosphorous chemistry and chemical biology Department of chemistry Tsinghua University Beijing 100084 P.R.China

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差示扫描微量热法研究蛋白质及其相关体系进展

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科学通报 2016年第28期61卷 3091-3099页

作者：孙海源邓耿周瑜尉志武清华大学化学系生命有机磷化学及化学生物学教育部重点实验室北京100084

蛋白质是一类重要的生物大分子,其结构与性质得到了广泛的研究.差示扫描微量热法(DSC)可以获得蛋白质的热容(C_p)与温度的关系,对我们认识蛋白质的性质有重要的帮助作用.同时,DSC研究蛋白质相关体系新方法也在不断涌现.本文介绍了差示... 详细信息

蛋白质是一类重要的生物大分子,其结构与性质得到了广泛的研究.差示扫描微量热法(DSC)可以获得蛋白质的热容(C_p)与温度的关系,对我们认识蛋白质的性质有重要的帮助作用.同时,DSC研究蛋白质相关体系新方法也在不断涌现.本文介绍了差示扫描微量热法在研究蛋白质解折叠机理、蛋白质稳定性以及复杂蛋白质体系等几个方面的进展.

关键词：差示扫描微量热蛋白质解折叠蛋白质稳定性淀粉样纤维疾病诊断

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What Can Topology Bring to chemistry?

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CCS chemistry 2024年第9期6卷 2084-2109页

作者： Wei Wang Songtao Zhou Xiujun yu Qing-Hui Guo Yanhang Ma Jie Song Liang Zhang Xuzhou Yan Lu Han Qing Liao Xiaopeng Li Wen-Bin Zhang Yiyong Mai Shaodong Zhang Shunai Che Hai-Bo Yang Xuefeng Fu Mei-Xiang Wang School of chemistry and Molecular Engineering East China Normal UniversityShanghai 200062 Hangzhou Institute of Medicine Chinese Academy of SciencesHangzhou 310022Zhejiang College of chemistry and Environmental Engineering Shenzhen UniversityShenzhen 518060Guangdong moe key Laboratory of bioorganic {3. and chemical biology Department of ChemistryTsinghua UniversityBeijing 100084 School of Physical Science and Technology and Shanghai key Laboratory of High-Resolution Electron Microscopy ShanghaiTech UniversityShanghai 201210 School of chemistry and chemical Engineering Frontiers Science Center for Transformative MoleculesState Key Laboratory of Composite MaterialsShanghai Key Laboratory for Molecular Engineering of Chiral DrugsShanghai Jiao Tong UniversityShanghai 200240 School of chemical Science and Engineering Tongji UniversityShanghai 200092 Beijing key Laboratory for Optical Materials and Photonic Devices Department of ChemistryCapital Normal UniversityBeijing 100048 Beijing National Laboratory for Molecular Sciences Key Laboratory of Polymer Chemistry and Physics of Ministry of EducationCenter for Soft Matter Science and EngineeringCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871 Department of chemical Sciences National Natural Science Foundation of ChinaBeijing 10085

The unique mathematical perspectives and principal concepts of topology have not only promoted the development of other branches of mathematics but have also deeply influenced other subjects,particularly physics and *** minireview aims to elucidate the substantial influence of topology on chemistry by critically examining both the contributions of topology to current chemical science and its potential future *** will discuss the topology of molecular structures and assemblies across various scales—from small molecules and mechanically interlocked molecules to polymers,biomacromolecules,and supramolecular *** discussion will include an exploration of cutting-edge techniques for characterizing topological features,underscoring the role of topology as a novel paradigm for the design and synthesis of new molecular ***,a critical analysis of topology’s role in the development of functional materials—such as photonic materials,polymers,biomacromolecules,and chiral materials—will demonstrate its emerging significance as a crucial parameter in unveiling novel properties and *** topology’s formidable potential,it is anticipated to be used increasingly to address pivotal challenges within chemistry and adjacent disciplines.

关键词： chemical topology topological invariants molecular graphs links and knots structureproperty relationship

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