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Chinese Chemical Letters 2021年第2期32卷 890-894页

作者： Xietao Yuan amir abdul razzaq Yujie Chen Yuebin Lian Xiaohui Zhao Yang Peng Zhao Deng Soochow Institute for Energy and Materials Innovations College of EnergySoochow UniversitySuzhou 215006China Jiangsu Provincial Key Laboratory for Advanced Carbon Materials and Wearable Energy Technologies Soochow UniversitySuzhou 215006China

Lithium polymer batteries(LPBs) rely on a high ion transport to gain improved cell *** and porous gel polymer electrolytes(GPEs) have attracted much attention due to their excellent properties in electrolyte wettability and ionic *** this work,iron-nickel-cobalt trimetal Prussian blue analogue(PBA) nanocubes are filled into the electro spun polyacrylonitrile(PAN)-based membranes to generate GPE composites with morphological superiority consisting of fine fibers and interconnected *** thus obtained PBA@PAN fibrous membrane showcases good thermal stability,high porosity and electrolyte uptake,as well as a peak io nic conductivity of 2.7 mS/cm with the addition of 10% PBA,Consequently,the assembled lithium iron phosphate(LiFePO_(4)) battery using PBA@PAN-10 as the GPE delivers a high capacity of 152.2 mAh/g at 0.2 C and an ultralow capacity decay of0.09% per cycle in a long-te rm cycle life of 350 cycles at 1 C,endorsing its promising applications in LPBs.

关键词： Prussian blue analogue Gel polymer electrolyte Ionic conductivity Thermal stability Lithium polymer batteries

Cobalt coordination with pyridines in sulfurized polyacrylonitrile cathodes to form conductive pathways and catalytic M-N4S sites for accelerated Li-S kinetics

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Journal of Energy Chemistry 2021年第10期30卷 170-178,I0005页

作者： amir abdul razzaq Ganwen Chen Xiaohui Zhao Xietao Yuan Jiapeng Hu Ziwei Li Yufeng Chen Jiabin Xu Rahim Shah Jun Zhong Yang Peng Zhao Deng Soochow Institute for Energy and Materials Innovations College of EnergySoochow UniversitySuzhou 215006JiangsuChina Key Laboratory of Advanced Carbon Materials and Wearable Energy Technologies of Jiangsu Province Soochow UniversitySuzhou 215006JiangsuChina Institute of Functional Nano and Soft Materials Laboratory(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow UniversitySuzhou 215123JiangsuChina School of Physics University of Electronic Science and Technology of ChinaChengdu 610054SichuanChina

Sulfurized polyacrylonitrile(SPAN)represents a unique class of cathode material for lithium sulfur(Li-S)batteries as it eradicates the polysulfides shuttling issue in carbonate-based ***,due to the essential chemical S-linking and organic nature of SPAN,the active mass percentage and rate capability are two bottleneck issues preventing its ultimate deployment outside of *** the current work,aiming to endow both the charge conductivity and catalytic activity to SPAN for maximizing the redox kinetics of S conversion,a freestanding nanofibrous SPAN cathode embedding conductive CNTs and atomically dispersed Co centers is fabricated via multivariate *** the CNTs enable dramatically enhancing the fiber conductivity and generating mesoscopic porosity for facilitating charge and mass transportation,the cross-linking of SPAN by Co-N_(4) S motifs creates extra charge conduction pathways and further serves as the catalytic active sites for expediting redox S *** a result,an extraordinary Li-SPAN performance is achieved with a high specific capacity up to 1856 mAh g^(-1)@0.2 C,a superb rate capability up to 10 C,and an ultra-long battery life up to 1500 cycles@1 ***,our study here provides insights into the adoption of coordination chemistry to maximize the sulfur utilization by ensuring a more complete redox conversion from SPAN to Li2 S,and vice versa.

关键词： Sulfurized polyacrylonitrile Electrospinning Cobalt Coordination chemistry Lithium sulfur batteries

Forestvoltaics,Floatovoltaics and Building Applied Photovoltaics(BAPV)Potential for a University Campus

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Energy Engineering 2024年第9期121卷 2331-2361页

作者： Rittick Maity Muhammad Khairul Imran bin Ahmad Shuhaimi Kumarasamy Sudhakar amir abdul Razak Faculty of Electrical and Electronics Engineering Technology Universiti Malaysia Pahang Al-Sultan AbdullahPekan26600Malaysia Centre for Research in Advanced Fluid and Processes UniversitiMalaysia Pahang Al-Sultan AbdullahGambang26300Malaysia Faculty of Mechanical and Automotive Engineering Technology Universiti Malaysia Pahang Al-Sultan AbdullahPekan26600Malaysia Centre for Automotive Engineering Universiti Malaysia Pahang Al-Sultan AbdullahPekan26600Malaysia Energy Centre Maulana Azad National Institute of TechnologyBhopal462003India

The United Nations’Sustainable Development Goals(SDGs)highlight the importance of affordable and clean energy *** energy is a perfect example,being both renewable and *** popularity shows no signs of slowing down,with solar photovoltaic(PV)panels being the primary technology for converting sunlight into *** are continuously being made to ensure cost-effectiveness,high-performing cells,extended lifespans,and minimal maintenance *** study focuses on identifying suitable locations for implementing solar PVsystems at theUniversityMalaysia PahangAl Sultanabdullah(UMPSA),Pekan campus including buildings,water bodies,and forest areas.A combined technical and economic analysis is conducted using Helioscope for simulations and the Photovoltaic Geographic Information System(PVGIS)for economic *** simulation examine case studies for PV installations in forested areas,lakes,and *** approach provides comprehensive estimations of solar photovoltaic potential,annual cost savings,electricity costs,and greenhouse gas emission *** on land coverage percentages,Floatovoltaics have a large solar PV capacity of 32.3 Megawatts(MW);forest-based photovoltaics(Forestvoltaics)achieve maximum yearly savings of RM 37,268,550;and Building Applied Photovoltaics(BAPV)have the lowest CO2 emissions and net carbon dioxide reduction compared to other plant *** also clarifies the purpose of using both software tools to achieve a comprehensive understanding of both technical and economic aspects.

关键词： Helioscope solar photovoltaic PV GIS performance land coverage economics

Facile synthesis of hierarchical NiO/NiFe_(2)O_(4) microsphere composite as efficient visible photocatalyst for 2,4-DCP degradation

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Rare Metals 2024年第4期43卷 1580-1588页

作者： Shabana Shaheen Shuai Xu Ji Bian amir Zada Zi-Qing Zhang Yang Qu Li-Qiang Jing Key Laboratory of Functional Inorganic Materials Chemistry(Ministry of Education) International Joint Research Center and Lab for Catalytic TechnologySchool of Chemistry and Materials ScienceHeilongjiang UniversityHarbin150080China Department of Chemistry Abdul Wali Khan UniversityMardan23200Pakistan

It is highly desired to develop efficient photocatalysts with recycling property for practical application to degrade toxic ***,nanosheet-assembled NiFe_(2)O_(4)microspheres with commendable activity are successfully synthesized by a facile solvothermal reaction with NH4F as the modifier,and their photoactivities are further improved by coupling with NiO through an in situ growth *** optimized nickel oxide(NiO)/nickel ferrite(NiFe_(2)O_(4))microsphere composite(5NiO/NFO-4)exhibits a satisfactory photocatalytic activity for 2,4-dichlorophenol(2,4-DCP)degradation under visible-light irradiation,which is attributed to its wide visible-light response,well-designed hierarchical structure and enhanced charge transfer and separation by coupling NiO as a high-level energy platform to accept ***,it is found that the NiO/NiFe_(2)O_(4)microsphere photocatalysts can be easily collected and recycled owing to the distinctive magnetic *** work provides a feasible route to rational design visible-light-driven photocatalysts with high-activity for environmental remediation and purification with good recyclability.

关键词： NiFe_(2)O_(4) microspheres NiO/Fe_(2)O_(4) composite Charge separation Visible-light photocatalysis 2 4-Dichlorophenol degradation

A Hybrid and Lightweight Device-to-Server Authentication Technique for the Internet of Things

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Computers, Materials & Continua 2024年第3期78卷 3805-3823页

作者： Shaha Al-Otaibi Rahim Khan Hashim Ali Aftab Ahmed Khan amir Saeed Jehad Ali Department of Information Systems College of Computer and Information SciencesPrincess Nourah bint Abdulrahman UniversityP.O.Box 84428Riyadh11671Saudi Arabia Department of Computer Science Abdul Wali Khan University MardanMardan23200Pakistan Department of Computer Science and IT UET PeshawarJalozai Campus PeshawarPeshawar24240Pakistan Department of AI Convergence Network Ajou UniversitySuwon16499South Korea

The Internet of Things(IoT)is a smart networking infrastructure of physical devices,i.e.,things,that are embedded with sensors,actuators,software,and other technologies,to connect and share data with the respective server *** IoTs are cornerstones in different application domains,the device’s authenticity,i.e.,of server(s)and ordinary devices,is the most crucial issue and must be resolved on a priority ***,various field-proven methodologies were presented to streamline the verification process of the communicating devices;however,location-aware authentication has not been reported as per our knowledge,which is a crucial metric,especially in scenarios where devices are *** paper presents a lightweight and location-aware device-to-server authentication technique where the device’s membership with the nearest server is subjected to its location information along with other ***,Media Access Control(MAC)address and Advance Encryption Scheme(AES)along with a secret shared key,i.e.,λ_(i) of 128 bits,have been utilized by Trusted Authority(TA)to generate MaskIDs,which are used instead of the original ID,for every device,i.e.,server and member,and are shared in the offline ***,TA shares a list of authentic devices,i.e.,server S_(j) and members C_(i),with every device in the IoT for the onward verification process,which is required to be executed before the initialization of the actual communication ***,every device should be located such that it lies within the coverage area of a server,and this location information is used in the authentication process.A thorough analytical analysis was carried out to check the susceptibility of the proposed and existing authentication approaches against well-known intruder attacks,i.e.,man-in-the-middle,masquerading,device,and server impersonations,etc.,especially in the IoT ***,proposed authentication and existing state-of-the-art approaches have been s

关键词： Internet of things authenticity security location communication

Incidence and predictors of hypocalcemia in end-stage renal disease patients on denosumab therapy: A systematic review and metaanalysis

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World Journal of Meta-Analysis 2024年第3期12卷 68-78页

作者： abdul Hannan Siddiqui Misbah Shaikh Afia Salman Muhammad Ahmed Ali Fahim Fizzah Batool Tahreem Mari Sarah Musani Muneeb Fareed Rooma Rehan Amna Hassni Urooj Nizami Ayesha amir abdul Moeed Salim R Surani Department of Internal Medicine Dow University of Health SciencesKarachi 74200SindhPakistan Department of Medicine&Pharmacology Texas A&M UniversityCollege StationTX 77843United States

BACKGROUND Denosumab inhibits the receptor activator of nuclear factor *** markedly increases bone mineral density and has been proven to reduce the risk of ***,numerous adverse effects,notably hypocalcemia,are prevalent in patients with end-stage renal disease(ESRD).AIM To analyze the incidence and predictors of hypocalcemia caused by denosumab compared to control in patients with *** We conducted this study in accordance with the Preferred Reporting Items for Systematic Reviews and Meta-analyses ***,Scopus,Cochrane Central,and EMBASE were systematically searched from inception through March *** original studies investigating the effects of denosumab on patients with ESRD compared to control were *** primary outcomes of our study were the incidence of mild,severe,and very severe *** outcomes included serum levels of intact parathyroid hormone,calcium,and *** results were pooled and analyzed using a random-effects *** Seven articles comprising 3240 patients were included in our *** treated with denosumab had a significantly increased incidence of mild hypocalcemia[risk ratio(RR):2.79;95%confidence interval(CI):0.99-7.91;P=0.05;I^(2)=37%]and of very severe hypocalcemia(RR:9.58;95%CI:1.58-57.98;P=0.01;I^(2)=49%).However,an increase in the occurrence of severe hypocalcemia was non-significant(RR:4.23;95%CI:0.47-38.34;P=0.20;I^(2)=96%).Alternatively,denosumab showed a significant decrease in serum intact parathyroid hormone[mean difference(MD):-433.20,95%CI:-775.12 to-91.28,I2=98%,P=0.01],while there was a non-significant decrease in phosphate(MD:-0.47,95%CI:-1.35 to 0.41,I^(2)=88%,P=0.30)and calcium levels(MD:-0.33,95%CI:-0.95 to 0.29,I^(2)=94%,P=0.29).CONCLUSION Our study demonstrated that denosumab is significantly associated with mild and very severe hypocalcemia in patients with ESRD making it necessary to detect and prevent this side effect of treatmen

关键词： Denosumab End-stage renal disease Hypocalcemia Parathyroid hormone Dialysis

Insect resistance management in Bacillus thuringiensis cotton by MGPS(multiple genes pyramiding and silencing)

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Journal of Cotton Research 2020年第4期3卷 311-323页

作者： ZAFAR Muhammad Mubashar razzaq abdul FAROOQ Muhammad Awais REHMAN abdul FIRDOUS Hina SHAKEEL amir MO Huijuan REN Maozhi Institute of Cotton Research Chinese Academy of Agricultural SciencesAnyang 455000HenanChina Department of Plant Breeding and Genetics University of Agriculture FaisalabadFaisalabad 38000Pakistan Zhengzhou Research Base State Key Laboratory of Cotton BiologyZhengzhou UniversityZhengzhou 450000China Department of Plant Pathology University of Agriculture FaisalabadFaisalabadPakistan.

The introduction of Bacillus thuringiensis(Bt)cotton has reduced the burden of pests without harming the environment and human ***,the efficacy of Bt cotton has decreased due to field-evolved resistance in insect pests over *** this review,we have discussed various factors that facilitate the evolution of resistance in cotton ***,different strategies like pyramided cotton expressing two or more distinct Bt toxin genes,refuge strategy,releasing of sterile insects,and gene silencing by RNAi are being used to control insect *** cotton has shown resistance against different cotton *** multiple genes pyramiding and silencing(MGPS)approach has been proposed for the management of cotton *** genome information of cotton pests is necessary for the development of MGPS-based *** expression cassettes against various essential genes involved in defense,detoxification,digestion,and development of cotton pests will successfully obtain favorable agronomic characters for crop protection and *** MGPS involves the construction of transformable artificial chromosomes,that can express multiple distinct Bt toxins and RNAi to knockdown various essential target genes to control *** evolution of resistance in cotton pests will be delayed or blocked by the synergistic action of high dose of Bt toxins and RNAi as well as compliance of refuge requirement.

关键词： Bt cotton RNAi Multiple genes pyramiding and silencing(MGPS) Bt resistance

Flow-injection Determination of Cysteine,N-Acetyl Cysteine and Glutathione in Pharmaceuticals via Potassium Ferricyanide-Fe(Ⅲ) Spectrophotometric System

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Chemical Research in Chinese Universities 2010年第6期26卷 893-898页

作者： WASEEM amir YAQOOB Mohammad NABI abdul Department of Chemistry COMSATS Institute of Information Technology Department of Chemistry University of Balochistan

A simple flow injection spectrophotometric method is reported for the determination of cysteine,N-acetyl cysteine and glutathione based on the reduction of Fe（Ⅲ）/ferricyanide,the in situ reduced ions are reacted with unreduced portion of ferricyanide/Fe（Ⅲ） to form soluble Prussian blue,which is monitored at 735 *** calibration graphs are linear in the concentration ranges of（1―100）×10-6 mol/L for cysteine and N-acetyl cysteine,and（1―50）×10-6 mol/L for *** relative standard deviations of 1.8%,2.5% and 1.9% were found for eleven replicate analyses of 5×10-6 mol/L cysteine,N-acetyl cysteine and *** limits of detection（3σ blank） at 5×10-7 mol/L for cysteine,and 3×10-7 mol/L for N-acetyl cysteine and glutathione were *** proposed method allowed 60 injections/*** effects of common substances present in pharmaceuticals and human physiological fluids were *** method was applied to determining cysteine in pharmaceutical formulations with the recoveries in a range of 97% to 106% and the results obtained are agreed well with labeled values.

关键词： Flow injection Spectrophotometry Cysteine Prussian blue Fe(Ⅲ) Ferricyanide Pharmaceutical

Genetic variability for yield and fiber related traits in genetically modified cotton

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Journal of Cotton Research 2021年第3期4卷 219-228页

作者： SAHAR Adeela ZAFAR Muhammad Mubashar razzaq abdul MANAN abdul HAROON Muhammad SAJID Sunaina REHMAN abdul MO Huijuan ASHRAF Muhammad REN Maozhi SHAKEEL amir YUAN Youlu Department of Plant Breeding and Genetics University of AgricultureFaisalabadPakistan Institute of Cotton Research Chinese Academy of Agricultural SciencesAnyang 455000China Institute of Molecular Biology and Biotechnology The University of Lahore-PakistanLahorePakistan National Key Laboratory of Crop Genetic Improvement Huazhong Agricultural UniversityWuhanChina Zhengzhou Research Base State Key Laboratory of Cotton BiologyZhengzhou UniversityZhengzhouChina.

Background:Cotton(Gossypium hirsutum L.)is grown for fiber and oil purposes in tropical and sub-tropical areas of the *** is the 4th largest producer of *** has a significant contribution in the GDP of ***,the present study was performed to assess the genetic variations and genetic diversity of yield and fiber quality traits in cotton and to analyze the associations present among ***:Analysis of variance exhibited significant variation for all studied traits except total number of nodes and the height to node *** phenotypic coefficient of variation was higher than the genotypic coefficient of variation for all studied *** height,monopodial branches,total number of bolls,lint index,seed index,and seed cotton yield displayed high heritabilities in a broad sense with maximum genetic *** analysis revealed that seed cotton yield had a significant positive association with plant height,the nu mber of monopodial branches,the nu mber of sympodia I branches,ginning outturn(GOT),the number of bolls,seed per boll,seed index,uniformity index,the number of sympodial branches,reflectance,and seed index at the genotypic level while a significant positive relationship was observed with plant height,the number of sympodial branches,boll number,and *** height,monopodial branches,GOT,boll weight,seeds per boll,and short fiber index exerted direct positive effects on seed cotton *** first 6 principal component analysis(PCs)out of the total fourteen PCs displayed eigenvalues(>1)and had maximum share to total variability(82.79%).The attributes that had maximum share to total divergence in eluded plant height,uniformity index,the nu mber of sympodial branches,seed per boll,GOT,seed cotton yield,and short fiber ***:The genotype AA-802,IUB-13,FH-159,FH-458,and CIM-595 were genetically diverse for most of the yield and fiber quality traits and could be utilized for the selection of better perform

关键词： Upland cotton Fiber trait Cotton yield Genetic variability Yield components

Flow injection spectrophotometric determination of vitamin E in pharmaceuticals,milk powder and blood serum using potassium ferricyanide-Fe(Ⅲ) detection system

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Chinese Chemical Letters 2010年第6期21卷 712-715页

作者： Saima Jadoon amir Waseem Mohammad Yaqoob abdul Nabi Department of Chemistry University of BalochistanQuettaPakistan

A simple and sensitive flow injection spectrophotometric method is reported for the determination of vitamin E using potassium ferricyanide-Fe(Ⅲ) detection *** the presence of vitamin E,Fe(Ⅲ)/ferricyanide *** in situ reduced ions are then reacted with unreduced portion of ferricyanide/Fe(Ⅲ) to make soluble Prussian blue,which is monitored at absorption wavelength of 735 *** calibration graph was obtained in the concentration range of 0.1-40μg mL^(-1).The relative standard deviations (n=4) were in the range of 1.1-3.6%,with limits of detection(3 s blank) of 0.04μg mL^(-1).The proposed method allowed 12 injections h^(-1).The method is applied to determine vitamin E in pharmaceuticals,infant milk and blood serum samples using hexane extraction with the recoveries in the range of 93±3 to 97.5±4%.The method is validated using certified reference materials SRM 968c for blood serum samples.

关键词： Flow injection Spectrophotometry Vitamin E Prussian blue Fe(III) Ferricyanide Pharmaceuticals Blood serum