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Recent strategies to improve moisture stability in metal halide perovskites materials and devices

Journal of Energy Chemistry 2022年第2期31卷 219-235页

作者： Chenxiao Zhou alexey b.tarasov Eugene A.Goodilin Pengwan Chen Hao Wang Qi Chen School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081China Faculty of Materials Science Lomonosov Moscow State UniversityLenin Hills119991 MoscowRussia Department of Chemistry Lomonosov Moscow State UniversityLenin Hills119991 MoscowRussia State Key Laboratory of Explosion Science and Technology Beijing Institute of TechnologyBeijing 100081China beijing Institute of Technology Chongqing Innovation Center Chongqing 401120China

At present,the stability of the new generation of solar cells based on hybrid perovskites is the bottleneck for their practical *** effects,high temperature,ultraviolet light,humidity and other known or still unknown factors might cause reduction of effectiveness or even irreversible loss of materials properties due to decomposition of functional layers within perovskite solar cells(PSCs).These factors alone have a serious impact on each component of the device,while their combinations lead to much more complicated effects and *** review focuses on the stability of PSCs and the degradation of the device in a humid *** assess the instability factors and deep-seated principles of evolution of the device structure in a humidity environment with the emphasis on the influence on their *** related solutions are reviewed from the perspective of the encapsulation,perovskite active layer,carrier transport layer and *** with the latest research,we believe that the waterproof strategy of PSCs requires either tight encapsulation or thorough modifications in the device ***,it is important to develop feasible strategies to improve the overall device stability over humid according to the target characteristics of various devices.

关键词： Perovskite solar cells Water Stability Composition Encapsulation

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How to stabilize standard perovskite solar cells to withstand operating conditions under an ambient environment for more than 1000 hours using simple and universal encapsulation

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Journal of Energy Chemistry 2023年第3期78卷 246-252,I0008页

作者： Nikolai A.belich Andrey A.Petrov Pavel A.Ivlev Natalia N.Udalova Alla A.Pustovalova Eugene A.Goodilin alexey b.tarasov Laboratory of New Materials for Solar Energetics Faculty of Materials ScienceLomonosov Moscow State University119991 MoscowRussia Department of Chemistry Lomonosov Moscow State University119991 MoscowRussia

We introduce a simple and universal scalable encapsulation strategy for perovskite solar cells based on thermal vacuum evaporation of MgF2or MoO3-xcapping layer followed by sealing the device with glass and UV-curable *** proposed encapsulation method is beneficial to most of the other known encapsulation approaches being fully harmless to perovskite and transporting layers and processible at room *** deposition of the capping layer promotes efficient removal of water,oxygen and organic solvent residuals from the device prior to sealing and could be easily performed using standard equipment for metal electrode *** proposed strategy is transferrable to any lab-scale perovskite solar cell prototypes regardless of their geometry and architecture and results in excellent stability of the devices in ambient air and long operating *** the 1000 hours stability test at ambient air(30%-60% RH),the cells preserved 92.9% of their initial efficiency on average under 1 Sun illumination at constant maximum power point tracking(MPPT,ISOS-L-1) and over 96% under sto rage in the dark(ISOS-D-1),thus evidencing for the high effectiveness of the proposed encapsulation approach.

关键词： Perovskite solar cells Halide perovskites Encapsulation High stability ISOS-L-1

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Evidence for polarization-induced phase transformations and degradation in CH_(3)NH_(3)PbI_(3)

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Nano Research 2023年第7期16卷 9435-9442页

作者： Aleksei Yu.Grishko Maria A.Komkova Ekaterina I.Marchenko Alexandra V.Chumakova alexey b.tarasov Eugene A.Goodilin Andrei A.Eliseev Department of Materials Science MSU-BIT UniversityShenzhen 517182China Department of Chemistry Lomonosov Moscow State UniversityMoscow 119991Russia Department of Materials Science Lomonosov Moscow State UniversityMoscow 119991Russia European Synchrotron Radiation Facility F-38042 GrenobleFrance

In solar cells,hybrid halide perovskites operate under constant bias,thus their stability towards electric field-induced degradation is of key *** we report on evidence of previously unidentified electric field-induced transitions and degradation path of CH_(3)NH_(3)PbI_(3)(MAPbI_(3))using elemental and phase *** films of MAPbI_(3) were deposited onto 1-2μm-pitch interdigitated electrodes and subjected to direct current(DC)-*** MAPbI_(3) layer polarized withbution to methylammonium-rich MAPbI_(3)-y(ybI3(xboth methylammonium and iodine provokes degradation of MAPbI_(3).Using nanofocus grazing-incidence wide-angle X-ray scattering(GIWAXS),we unambiguously showed that the bias voltage induces the transformation ofβ-MAPbI_(3) to metastableδ-MAPbI_(3) polymorph via alignment of polar organic cation with the electric *** transformation is partially reversible upon field ***,once formed,δ-MAPbI_(3) disrupts the morphology of pristine film and undergoes decomposition toβ-MAPbI_(3)(β-MAPI)and PbI_(2).With the aforementioned compositional and phase changes,only MA-rich part serves as the charge separation layer,while the I-rich excitation is blocked with the PbI_(2) barrier serving as holes trapping *** observations reveal the intermediate steps in electric-field-driven degradation of halide perovskites and show the role of polar cations in the process,which is instructive for further material design with higher stability metrics.

关键词： halide perovskites stability degradation electric field ionic conductivity stoichiometry

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Modified biot Elastic Coefficients in Poroelastic Solid

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Journal of Earth Science 2024年第4期35卷 1397-1401页

作者： Chun Yang Yun Wang alexey Stovas Liheng Wang School of Geophysics and Information Technology China University of GeosciencesBeijing100083China Department of Geoscience and Petroleum Norwegian University of Science and TechnologyTrondheim 7031Norway Key Laboratory of Shale Gas and Geoengineering Institute of Geology and GeophysicsChinese Academy of SciencesBeijing 100029China

0 INTRODUCTION Sedimentary rocks predominantly consist of porous solids saturated with fluids,the kinematic and dynamic characteristics of which are described through poroelasticity theory(biot,1956a,b,1941).The wave propagation in fluid-saturated po-rous rocks obtains extensive attention owing to its relevance in diverse fields,such as ocean acoustics,exploration geophysics,and soil dynamics(Yang et al.,2023a;Xie et al.,2022).

关键词： saturated Elastic a,b

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Gradient-induced long-range optical pulling force based on photonic band gap

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Light(Science & Applications) 2024年第5期13卷 865-874页

作者： Wenlong Lu alexey V.Krasavin Sheng Lan Anatoly V.Zayats Qiaofeng Dai Guangdong basic Research Center of Excellence for Structure and Fundamental Interactions of Matter Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and DevicesSchool of Information and Optoelectronic Science and EngineeringSouth China Normal UniversityGuangzhou 510006China Department of Physics and London Centre for Nanotechnology King’s College LondonLondon WC2R 2LSUK

Optical pulling provides a new degree of freedom in optical *** is generally believed that long-range optical pulling forces cannot be generated by the gradient of the incident ***,we theoretically propose and numerically demonstrate the realization of a long-range optical pulling force stemming from a self-induced gradient field in the manipulated *** analogy to potential barriers in quantum tunnelling,we use a photonic band gap design in order to obtain the intensity gradients inside a manipulated object placed in a photonic crystal waveguide,thereby achieving a pulling *** the usual scattering-type optical pulling forces,the proposed gradient-field approach does not require precise elimination of the reflection from the manipulated *** particular,the Einstein-Laub formalism is applied to design this unconventional gradient *** magnitude of the force can be enhanced by a factor of up to 50 at the optical resonance of the manipulated object in the waveguide,making it insensitive to *** developed approach helps to break the limitation of scattering forces to obtain longrange optical pulling for manipulation and sorting of nanoparticles and other *** developed principle of using the band gap to obtain a pulling force may also be applied to other types of waves,such as acoustic or water waves,which are important for numerous applications.

关键词： optical waveguide scattering

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Atherosclerosis originating from childhood:Specific features

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Journal of biomedical Research 2024年第3期38卷 233-240页

作者： Anastasia V.Poznyak alexey A.Yakovlev MikhailА.Popov Elena b.Zhigmitova Vasily N.Sukhorukov Alexander N.Orekhov Institute for Atherosclerosis Research Moscow 121609Russia Federal Research and Clinical Center of Intensive Care Medicine and Rehabilitology Moscow 109240Russia Department of Cardiac Surgery Moscow Regional Research and Clinical InstituteMoscow 129110Russia Laboratory of Angiopathology Institute of General Pathology and PathophysiologyMoscow 125315Russia

Atherosclerosis is extremely ***,it is considered a disease of older people,who most often experience problems with the heart and blood *** much attention from the scientific community has been paid to studying the association between aging and atherosclerosis,as well as its consequences,there is evidence that atherosclerosis occurs at an early *** may form both during intrauterine development and in *** plays an important role in childhood atherosclerosis,along with previous infectious diseases and excess weight of both the child and the *** the present review,we examined the development of atherosclerosis and the prerequisites in childhood.

关键词： atherosclerosis childhood pediatrics cardiovascular disease

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A high-power electromagnetic source for disabling improvised explosive devices

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High Voltage 2024年第2期9卷 403-409页

作者： Laurent Ariztia Njomza Ibrahimi alexey Zhabin Antoine Silvestre de Ferron Marc Rivaletto Edson Martinod Valérie bertrand bucur Novac Laurent Pécastaing Universite de Pau et des Pays de l’Adour E2S UPPASIAMEPauFrance XLIM UMR CNRS BriveLimogesFrance CISTEME LimogesFrance Wolfson School of Mechanical Electrical and Manufacturing EngineeringLoughborough UniversityLoughboroughLeicestershireUK

Ultra-wideband(UWb)microwave sources driven by specialised pulsed power generators have experienced a considerable development in the last decade due to their wide domain of new applications such as defence or counter-terrorism *** authors present the main findings of a research dedicated to the development of a pulsed power-driven electromagnetic field source for disabling improvised explosive devices(IED).The pulsed power generator driving the source is a 13-stage compact Marx producing voltage pulses reaching an amplitude of 0.5 MV,with a pulse repetition frequency(PRF)of up to 100 *** generator is coupled to a bipolar pulse forming line,providing bipolar pulses with a dV/dt of around 1.6 MV/*** pulsed power system feeds an array composed of 16 Koshelev-type UWb antennas through an impedance matching *** resulting electromagnetic source is capable to produce pulsed electric fields(PEFs)having a figure-of-merit(FOM)of 1 ***,practical experiments were carried out to study the effects of the PEFs on *** targets used in the present study are M2b type flashbulbs,known to have the same susceptibility as the US army M6 *** configurations of wires(shielded,twisted,etc)with different lengths were used in connecting items inside these *** tests were performed by placing the flashbulbs at different distances to determine the essential parameters(i.e.,amplitude,duration,and frequency range)of the PEFs required to trigger *** overview of the experimental campaign and the main findings are also presented followed by conclusions.

关键词： power bipolar source

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Artificial enhancement of sturgeon stock in freshwater reservoirs:A case study on sterlet Acipenser ruthenus of the Kama reservoir

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Aquaculture and Fisheries 2024年第2期9卷 287-294页

作者： Pavel b.Mikheev Semyon N.Kazarinov Alla G.Melnikova Stanislav V.Ponosov Nikolai G.Petrenko Andrei I.Nikiforov alexey Yu Puzik Olga N.Elchenkova Perm State National Research University Perm614990Russia Khabarovsk branch of the Federal State budget Scientific Institution“Russian Federal Research Institute of Fisheries and Oceanography”“KhabarovskNIRO” Khabarovsk680038Russia Perm branch of the Federal State budget Scientific Institution“Russian Federal Research Institute of Fisheries and Oceanography”“PermNIRO” Perm614991Russia Federal State budget Scientific Institution“Russian Federal Research Institute of Fisheries and Oceanography”“VNIRO” Moscow117454Russia Moscow State Institute of International Relations(University)of the Ministry for Foreign Affairs of Russia“MGIMO” Moscow117454Russia Department of State Control Supervision and Protection of Aquatic Biological Resources for Perm KraiMiddle-Volga Regional Office of the Federal Fishery AgencyPerm614990Russia

The paper presents the results of the sterlet sturgeon Acipenser ruthenus reintroduction into the Kama Reservoir(Perm Krai,Russia)by sterlet fry from hatcheries into the reservoir since *** effectiveness of hatchery releases was evaluated by monitoring gillnet sampling *** results showed that the species was reported throughout entire Kama Reservoir,which contrasts with 1988-1994 data,when the species was registered only at the upper part of the reservoir near the Kama River *** highest number and biomass values of catch per unit effort(CPUE)of the sterlet were found in submerged river channels-the deepest habitats with flow conditions which are close to the ecological requirements of the *** distribution of the sterlet within the channel biotopes of the reservoir is defined by reduced *** biggest individuals and the widest size range of the sterlet were typical for the upper area of the reservoir and Chusovskoy bay,which have the greatest *** smallest sizes were typical for fish from catches near the dam of the reservoir,which is consistent with the published data on the distribution of sterlet in reservoir *** presented results may indicate the artificial formation of the sterlet stock in the Kama Reservoir maintained by hatchery *** revealed distribution of the sterlet in the reservoir determines the direction of further research on natural reproduction and thus formation of an artificially formed ***,future studies are required to assess the possibility of hybridization of the sterlet of artificial origin with natural populations of the species,since the low genetic diversity of the sterlet released into the Kama Reservoir which can lead to irreversible loss of genetic individuality of the natural stocks of the species in the catchment of upper course of the Kama River.

关键词： Sterlet Acipenser ruthenus Kama reservoir Hatchery releases CPUE Artificial stock formation

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The effect of long-term application of nitrogen-rich fertilizers on soil resistome:A study of conventional and organic cropping systems

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Soil Ecology Letters 2024年第3期6卷 135-150页

作者： alexey S.Vasilchenko Evgenii O.burlakov Darya V.Poshvina Denis S.Gruzdev Sergey V.Kravchenko Aleksandr V.Iashnikov Ning Ling Anastasia V.Vasilchenko Laboratory of Antimicrobial Resistance Institute of Environmental and Agricultural Biology(X-BIO)Tyumen State UniversityTyumenRussia Research Institute of Mathematics Physics and Computer ScienceDerzhavin Tambov State UniversityTambovRussia International Integrated Research Laboratory for Climate Change Land Use and BiodiversityInstitute of Environmental and Agricultural Biology(X-BIO)Tyumen State UniversityTyumenRussia Scibear OU Tartu Mnt 67/1-13bKesklinna Linnaosa10115 TallinnEstonia Center for Grassland Microbiome State Key Laboratory of Grassland Agro-EcosystemsCollege of Pastoral Agriculture Science and TechnologyLanzhou UniversityLanzhou 730000China

Metagenomic studies of various soil environments have previously revealed the widespread distribution of antibiotic resistance genes(ARGs)around the *** this study,we applied shotgun metagenomics to investigate differences in microbial communities and resistomes in Chernozem soils that have been under long-term organic and conventional cropping *** organic cropping system was seeded with Triticum spelta without any *** conventional cropping system was seeded with Tríticum durum Desf and used mineral fertilizer(NPK),that resulted in an increased amount of total and available carbon and nitrogen in *** all samples,we identified a total of 21 ARG classes,among which the dominant were vancomycin,tetracycline and *** of soil microbial communities revealed differences between the studied fields in the relative abundances of 14 and 53 genera in topsoil and subsoil,*** analysis showed significant correlations(positive and negative)among 18 genera and 6 ARGs,as well as between these ARGs and some chemical properties of *** analysis of metagenome-assembled genomes revealed that Nitrospirota,Thermoproteota,Actinobacteriota and binatota phyla of archaea and bacteria serve as hosts for glycopeptide and fluoroquinolone/tetracycline ***,the data obtained enrich knowledge about the consequences of human agricultural activities in terms of soil microbiome modification and highlight the role of nitrogen cycling taxa,including uncultivated genera,in the formation of soil resistome.

关键词： soil microbiome inorganic fertilizer nitrogen cycle uncultured bacteria chemolithotrophs binatia

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Expanded Porphyrin Exhibiting Off-Centered Out-of-Plane Coordination to Dysprosium

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CCS Chemistry 2024年第7期6卷 1731-1738页

作者： Dmitry I.Nazarov Jorge Labella alexey V.Kuzmin Maxim A.Faraonov Evgenii N.Ivanov Salavat S.Khasanov Tomas Torres Mikhail K.Islyaikin Dmitri V.Konarev Federal Research Center of Problems of Chemical Physics and Medicinal Chemistry RAS 142432 Chernogolovka Department of Organic Chemistry Universidad Autonoma de Madrid28049 Madrid Institute of Solid-State Physics RAS 142432 Chernogolovka Research Institute of Macroheterocycles Ivanovo State University of Chemistry and Technology15300 Ivanovo G.A.Krestov Institute of Solution Chemistry of the Russian Academy of Sciences 153045 Ivanovo Institute for Advanced Research in Chemical Sciences Universidad Autonoma de Madrid28049 Madrid IMDEA-Nanociencia 28049 Madrid

The complexation of high-spin lanthanides to porphyrinoids is a powerful strategy for the development of advanced molecular *** this context,the use of expanded porphyrinoids remains elusive since their coordination chemistry is challenging to ***,taking inspiration from on-surface chemistry,we explored the coordination of Dy^(3+)to a six-membered porphyrinoid,namely,the hemihexaphyrazine ***,we observed the selective formation of a mono-nuclear off-centered,out-of-plane H_(2)Hhp-Dy^(3+)complex when performing the complexation under reductive *** this reaction,the oxidation state of the macrocycle did not *** X-ray diffraction analysis,we found that the coordination number of Dy in this complex was *** macrocycle cocrystallized with decamethylcobaltocene(Cp_(2)^(*)Co)molecules,giving rise to a wellordered solid-state packing,governed byπ-π*** a result of this organization,a small magnetic coupling between the neighboring molecules was *** in all,this work provides key insights into the coordination of magnetically active metals with expanded porphyrinoids,thus motivating the development of advanced spintronic devices.

关键词： porphyrins dysprosium macrocycle coordination chemistry magnetism

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