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CO_(2)methanation boosted by support-size-dependent strong metal-support interaction and B-O-Ti component

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Green Energy & Environment 2024年第2期9卷 321-332页

作者： Shaoyu yuan Yushan yang Zhangyi Xiong Peijing Guo Sufang Sun Zejiang Li Jianlong Du Yongjun Gao College of Chemistry and Environmental Science Hebei UniversityNo.180Wusidong RoadBaoding071002HebeiChina

Strong metal-support interaction(SMSI)has a great impact on the activity and selectivity of heterogeneous catalysts,which was usually adjusted by changing reduction temperature or processing catalyst in different ***,few researches concentrate on modulating SMSI through regulating the structure of the ***,we show how changing the surface environment of the anatase TiO_(2)(B–TiO_(2))can be used to modulate the *** moderate TiOx overlayer makes the Ni metal highly dispersed on the high specific surface area of support,resulting in a substantially enhanced CO_(2)methanation ***,a novel phenomenon was observed that boron dopants promote the for-mation of the B–O–Ti interface site,enhancing the catalytic performance of CO_(2)*** calculations confirm that the B–O–Ti structure facilitates the activation of CO_(2)and further hydrogenation to methane.

关键词： CO_(2)Methanation B-doped TiO_(2) SMSI Size-dependent

Recovering rare earths,lithium and fluorine from rare earth molten salt electrolytic slag using sub-molten salt method

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Journal of Rare Earths 2024年第9期42卷 1774-1781,I0005页

作者： Delong yang Mingming Yu Yusufujiang Mubula Weiquan yuan Zheyu Huang Bo Lin Guangjun Mei Tingsheng Qiu School of Resources and Environmental Engineering Jiangxi University of Science and TechnologyGanzhou341000China Jiangxi Key Laboratory of Mining Engineering Jiangxi University of Science and TechnologyGanzhou341000China School of Resources and Environmental Engineering Wuhan University of TechnologyWuhan430070China Gannan Institute of Science and Technology Ganzhou341000China

Viewing the problem of high ene rgy consumption in the process of recovering rare earths from rare earth molten salt electrolysis slag,an environmentally friendly and low carbon process by sub-molten salt decomposition was *** thermodynamic analysis of sub-molten salt reaction indicates that the recovery of rare earths from the slag using sub-molten salt medium is thermodynamically *** this process,the rare earth fluoride and lithium in the slag are almost transformed into rare earth hydroxide,sodium fluoride and lithium hydroxide,fluorine and lithium are transferred into the washing solution,and the rare earths in the residues can be leached into solution by acid *** the optimum reaction conditions of reaction temperature 200℃,reaction time 3 h,NaOH initial concentration 80%,NaOH-Slag mass ratio 3:1,the leaching efficiency of rare earths,fluorine and lithium can reach to 99.05%,98.23% and 99.22%.After evaporation,the fluorine and lithium in the washing solution can be obtained in the forms of sodium fluoride and lithium fluoride,the recovery efficiency reach 95.5%and 92.8%,*** RE oxides(99.53%) can be obtained from the leaching solution after precipitation and roasting.

关键词： Rare earth electrolysis slag Sub-molten salt Green extraction Fluorine Lithium Recovery

Evolution of interfacial heat transfer,contact behavior and microstructure during sub-rapid solidification of molten steel with different hydrogen contents

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Journal of Iron and Steel Research International 2024年第1期31卷 215-223页

作者： Cheng Lu Wan-lin Wang Chen-yang Zhu Jie Zeng Xin-yuan Liu Hua-long Li School of Metallurgy and Environment Central South UniversityChangsha410083HunanChina National Center for International Research of Clean Metallurgy Central South UniversityChangsha410083HunanChina Institute of Research of Iron and Steel ShasteelZhangjiagang215625JiangsuChina

Typical Q235 low-carbon steel samples with different hydrogen contents(0.0004,0.0008,and 0.0013 wt.%)were prepared by adjusting the environment humidity and *** effects of hydrogen on interfacial heat transfer,contact behavior,and microstructure evolution were investigated using a novel droplet solidification *** results revealed that when the hydrogen content increases from 0.0004 to 0.0013 wt.%,the maximum heat flux between the molten steel and cooling substrate decreases from 8.01 to 6.19 MW/m^(2),and the total heat removed in the initial 2 s reduces from 10.30 to 8.27 MJ/m^(2).Moreover,the final contact angle between the molten steel and substrate increases from 103.741°to 113.697°,and the number of pores on the droplet bottom surface increases significantly from 21 to 210 with the increase in *** surface roughness of the droplet bottom surface increases from 20.902 to 49.181 *** addition,the average grain size of the droplet increases from 14.778 to 33.548 pm with the increase in the hydrogen *** interfacial contact condition becomes worse due to the escape of hydrogen from the steel matrix during the cooling process,which leads to the reduction in the interfacial heat transfer and the increase in the grain size.

关键词： Strip casting Hydrogen content Interfacial heat transfer behavior Contact behavior Microstructure evolution

Analysis of the influencing factors and clinical related characteristics of pulmonary tuberculosis in patients with type 2 diabetes mellitus

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World Journal of Diabetes 2024年第2期15卷 196-208页

作者： Han Shi yuan yuan Xue Li Yan-Fang Li Ling Fan Xue-Mei yang Department of Infectious Diseases The First Affiliated Hospital of Chengdu Medical CollegeChengdu 610500Sichuan ProvinceChina

BACKGROUND In China,the prevalence of type 2 diabetes mellitus(T2DM)among diabetic patients is estimated to be between 90%-95%.Additionally,China is among the 22 countries burdened by a high number of tuberculosis cases,with approximately 4.5 million individuals affected by active ***,T2DM poses a significant risk factor for the development of tuberculosis,as evidenced by the increased incidence of T2DM coexisting with pulmonary tuberculosis(T2DMPTB),which has risen from 19.3%to 24.1%.It is evident that these two diseases are intricately interconnected and mutually reinforcing in *** To elucidate the clinical features of individuals diagnosed with both T2DM and tuberculosis(T2DM-PTB),as well as to investigate the potential risk factors associated with active tuberculosis in patients with *** T2DM-PTB patients who visited our hospital between January 2020 and January 2023 were selected as the observation group,Simple DM patients presenting to our hospital in the same period were the control group,Controls and case groups were matched 1:2 according to the principle of the same sex,age difference(±3)years and disease duration difference(±5)years,patients were investigated for general demographic characteristics,diabetes-related characteristics,body immune status,lifestyle and behavioral habits,univariate and multivariate analysis of the data using conditional logistic regression,calculate the odds ratio(OR)values and 95%CI of OR *** A total of 315 study subjects were included in this study,including 105 subjects in the observation group and 210 subjects in the control *** of the results of both anthropometric and biochemical measures showed that the constitution index,systolic blood pressure,diastolic blood pressure and lymphocyte count were significantly lower in the case group,while fasting blood glucose and high-density lipoprotein cholesterol levels were significantly higher than those in the control ***

关键词： Type 2 diabetes Pulmonary tuberculosis Blood sugar Infection Risk factors

A Facile Li_(2)TiO_(3) Surface Modification to Improve the Structure Stability and Electrochemical Performance of Full Concentration Gradient Li-Rich Oxides

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Energy & Environmental Materials 2024年第3期7卷 41-48页

作者： Naifang Hu yuan yang Lin Li Yuhan Zhang Zhiwei Hu Lan Zhang Jun Ma Guanglei Cui Qingdao Industrial Energy Storage Research Institute Qingdao Institute of Bioenergy and Bioprocess TechnologyChinese Academy of SciencesQingdao 266101China Institute of Materials Science and Engineering Ocean University of ChinaQingdao 266100China School of Future Technology University of Chinese Academy of SciencesBeijing 100049China Max Planck Institute for Chemical Physics of Solids Nothnitzer Strasse 40Dresden D-01187Germany CAS Key Laboratory of Green Process and Engineering Beijing Key Laboratory of Ionic Liquids Clean ProcessState Key Laboratory of Multiphase Complex SystemsInstitute of Process EngineeringChinese Academy of SciencesBeijing 100190China Shandong Energy Institute Qingdao 266101China

Full concentration gradient lithium-rich layered oxides are catching lots of interest as the next generation cathode for lithium-ion batteries due to their high discharge voltage,reduced voltage decay and enhanced rate performance,whereas the high lithium residues on its surface impairs the structure stability and long-term cycle ***,a facile multifunctional surface modification method is implemented to eliminate surface lithium residues of full concentration gradient lithium-rich layered oxides by a wet chemistry reaction with tetrabutyl titanate and the post-annealing *** realizes not only a stable Li_(2)TiO_(3)coating layer with 3D diffusion channels for fast Li^(+)ions transfer,but also dopes partial Ti^(4+)ions into the sub-surface region of full concentration gradient lithium-rich layered oxides to further strengthen its crystal ***,the modified full concentration gradient lithium-rich layered oxides exhibit improved structure stability,elevated thermal stability with decomposition temperature from 289.57℃to 321.72℃,and enhanced cycle performance(205.1 mAh g^(-1)after 150 cycles)with slowed voltage drop(1.67 mV per cycle).This work proposes a facile and integrated modification method to enhance the comprehensive performance of full concentration gradient lithium-rich layered oxides,which can facilitate its practical application for developing higher energy density lithium-ion batteries.

关键词： full concentration gradient lithium-rich layered oxides structure stability surface modification

Changes in global land surface frozen ground and freeze-thaw processes during 1950-2020 based on ERA5-Land data

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Advances in Climate Change Research 2024年第2期15卷 265-274页

作者： Yong yang Ren-Sheng CHEN Yong-Jian DING Hong-yuan LI Zhang-Wen LIU Qilian Alpine Ecology and Hydrology Research Station Key Laboratory of Ecological Safety and Sustainable Development in Arid LandsNorthwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 73000China State Key Laboratory of Cryospheric Sciences Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 73000China Shandong Provincial Key Laboratory of Water and Soil Conservation and Environmental Protection College of Resources and EnvironmentLinyi UniversityLinyi 276000China

Frozen ground(FG)plays an important role in global and regional climates and environments through changes in land freeze-thaw processes,which have been conducted mainly in different ***,the changes in land surface freeze-thaw processes under climate change on a global scale are still *** on ERA5-Land hourly land skin temperature data,this study evaluated changes in the global FG area,global land surface first freeze date(FFD),last freeze date(LFD)and frost-free period(FFP)from 1950 to *** results show that the current FG areas(1991-2020 mean)in the Northern Hemisphere(NH),Southern Hemisphere(SH),and globe are 68.50×10^(6),9.03×10^(6),and 77.53×10^(6)km^(2),which account for 72.4%,26.8%,and 60.4%of the exposed land(excluding glaciers,ice sheets,and water bodies)in the NH,SH and the globe,respectively;further,relative to 1951-1980,the FG area decreased by 1.9%,8.8%,and 2.8%,*** FG at lower latitudes degrades to intermittently FG,and intermittently FG degrades to non-frozen ground,which caused the global FG boundary to retreat to higher latitudes from 1950 to *** annual FG areas in the NH,SH,and globe all show significant decreasing trends(p<0.05)from 1950 to 2020 at-0.32×10^(6),-0.22×10^(6),and-0.54×10^(6)km^(2)per decade,*** FFP prolongation in the NH is mainly influenced by LFD advance,while in the SH it is mainly controlled by FFD *** prolongation trend of FFP in the NH(1.34 d per decade)is larger than that in the SH(1.15 d per decade).

关键词： Frozen ground Freeze-thaw processes Frost-free period First freeze date Global warming

Effect of electrolyte cation-mediated mechanism on electrocatalytic carbon dioxide reduction

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Chinese Chemical Letters 2024年第7期35卷 139-146页

作者： yuan Dong Mutian Ma Zhenyang Jiao Sheng Han Likun Xiong Zhao Deng yang Peng Soochow Institute of Energy and Material Innovations College of EnergyJiangsu Key Laboratory of Advanced Carbon Materials and Wearable Energy TechnologiesSoochow UniversitySoochow 215006China Jiangsu Key Laboratory of Advanced Negative Carbon Technologies Soochow UniversitySoochow 215123China School of Chemistry and Chemical Engineering Shihezi UniversityShihezi 832003China School of Chemical and Environmental Engineering Shanghai Institute of TechnologyShanghai 201418China

The steep reduction in costs and systematic optimization of renewable electricity has ignited an intensifying interest in harnessing electroreduction of carbon dioxide(CO_(2)RR)for the generation of chemicals and *** focus of research over the past few decades has been on the optimization of the electrode and the electrolyte ***,cation species in the latter have recently been found to dramatically alter the selectivity of CO_(2)RR and even their catalytic activity by multiple orders of *** a result,the selection of cations is a critical factor in designing catalytic interfaces with high selectivity and efficiency for targeted *** decision-making regarding cation selection relies on a comprehensive understanding of prevailing electrolyte effect models that have been used to elucidate observed experimental *** this perspective,we review the hypotheses that explain how electrolyte cations influence CO_(2)RR by mechanisms such as through tuning of the interfacial electric field,buffering of the local pH,stabilization of the key intermediates and regulation of the interfacial *** endeavor is to elucidate the molecular mechanisms underpinning cation effects,thus fostering the evolution of more holistic and universally applicable predictive *** this regard,we highlight the current challenges in this area of research,while also identifying potential avenues for future investigations.

关键词： CO_(2)electrocatalytic reduction Cation effects Catalytic mechanisms Catalytic interfaces Electric double layer

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The Caching and Pricing Strategy for Information-Centric Networking with Advertisers’Participation

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China Communications 2024年第3期21卷 283-295页

作者： Zheng Quan Yan Wenliang Wu Rong Tan Xiaobin yang Jian yuan Liu Xu Zhenghuan Laboratory for Future Networks Department of AutomationUniversity of Science and Technology of ChinaHefei 230026China Institute of Artificial Intelligence Hefei Comprehensive National Science CenterHefei 230088China Institute of Advanced Technology University of Science and Technology of ChinaHefei 230088China Suzhou Nuclear Power Research Institute Suzhou 215004China National Engineering Laboratory for Public Safety Risk Perception and Control by Big Data(NEL-PSRPC) China Academy of Electronics and Information Technology of CETCBeijing 100041China

As users’access to the network has evolved into the acquisition of mass contents instead of IP addresses,the IP network architecture based on end-to-end communication cannot meet users’***,the Information-Centric Networking(ICN)came into *** a technical point of view,ICN is a promising future network *** and customizing a reasonable pricing mechanism plays a positive role in promoting the deployment of *** current research on ICN pricing mechanism is focused on paid ***,we study an ICN pricing model for free content,which uses game theory based on Nash equilibrium to *** this work,advertisers are considered,and an advertiser model is established to describe the economic interaction between advertisers and ICN *** solution can formulate the best pricing strategy for all ICN entities and maximize the benefits of each *** extensive analysis and numerical results show that the proposed pricing framework is significantly better than existing solutions when it comes to free content.

关键词： advertisers cache free content Information-Centric Networking pricing strategy

Association of age at diagnosis of diabetes with subsequent risk of age-related ocular diseases and vision acuity

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World Journal of Diabetes 2024年第4期15卷 697-711页

作者： Si-Ting Ye Xian-Wen Shang Yu Huang Susan Zhu Zhuo-Ting Zhu Xue-Li Zhang Wei Wang Shu-Lin Tang zong-yuan Ge Xiao-Hong yang Ming-Guang He The Second Clinical College Guangzhou University of Chinese MedicineGuangzhou 510120Guangdong ProvinceChina Department of Ultrasound The Second Affiliated Hospital of Guangzhou University of Chinese MedicineGuangzhou 510120Guangdong ProvinceChina Guangdong Eye Institute Department of OphthalmologyGuangdong Provincial People’s HospitalGuangdong Academy of Medical SciencesGuangzhou 510080Guangdong ProvinceChina Guangdong Cardiovascular Institute Guangdong Provincial People's HospitalGuangdong Academy of Medical SciencesGuangzhou 510080Guangdong ProvinceChina Austin Hospital University of MelbourneMelbourne 3084VictoriaAustralia State Key Laboratory of Ophthalmology Zhongshan Ophthalmic CenterSun Yat-sen UniversityGuangzhou 510060Guangdong ProvinceChina Monash e-Research Center Faculty of EngineeringAirdoc ResearchNvidia AI Technology Research CenterMonash UniversityMelbourne 3080VictoriaAustralia Department of Ophthalmic Epidemiology Centre for Eye Research AustraliaMelbourne 3002VictoriaAustralia

BACKGROUND The importance of age on the development of ocular conditions has been reported by numerous *** may have different associations with different stages of ocular conditions,and the duration of diabetes may affect the development of diabetic eye *** there is a dose-response relationship between the age at diagnosis of diabetes and the risk of cardiovascular disease and mortality,whether the age at diagnosis of diabetes is associated with incident ocular conditions remains to be *** is unclear which types of diabetes are more predictive of ocular *** To examine associations between the age of diabetes diagnosis and the incidence of cataract,glaucoma,age-related macular degeneration(AMD),and vision *** Our analysis was using the UK *** cohort included 8709 diabetic participants and 17418 controls for ocular condition analysis,and 6689 diabetic participants and 13378 controls for vision *** diseases were identified using inpatient records until January *** acuity was assessed using a *** During a median follow-up of 11.0 years,3874,665,and 616 new cases of cataract,glaucoma,and AMD,respectively,were identified.A stronger association between diabetes and incident ocular conditions was observed where diabetes was diagnosed at a younger *** with type 2 diabetes(T2D)diagnosed at<45 years[HR(95%CI):2.71(1.49-4.93)],45-49 years[2.57(1.17-5.65)],50-54 years[1.85(1.13-3.04)],or 50-59 years of age[1.53(1.00-2.34)]had a higher risk of AMD independent of glycated haemoglobin.T2D diagnosed<45 years[HR(95%CI):2.18(1.71-2.79)],45-49 years[1.54(1.19-2.01)],50-54 years[1.60(1.31-1.96)],or 55-59 years of age[1.21(1.02-1.43)]was associated with an increased cataract risk.T2D diagnosed<45 years of age only was associated with an increased risk of glaucoma[HR(95%CI):1.76(1.00-3.12)].HRs(95%CIs)for AMD,cataract,and glaucoma associated with type 1 diabetes(T1D)were 4.12(1.99-8.53),

关键词： Diabetes Age at diagnosis Cataract Glaucoma Age-related macular disease Vision acuity