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Enhanced photocatalytic performance of Bi_(2)O_(2)CO_(3)/Bi_(4)O_(5)Br_(2)/reduced graphene oxide Z-schemehe terojunction via a one-pot room-temperature synthesis

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Journal of Environmental Sciences 2024年第4期138卷 418-427页

作者： Xiaoge Wu Lei Yan Rongrong qin Qikai Zhang Wei Yang Xiaozhi wang Yongcai Zhang Min Luo Jianhua Hou College of Environmental Science and Engineering Yangzhou UniversityYangzhouJiangsu 225009China Jiangsu Collaborative Innovation Center for Solid Organic Waste Resource Utilization Nanjing 210095China Beijing Xinfeng Aerospace Equipment Co. Ltd.Beijing 100854China Beijing System Design Institute of Electro-Mechanic Engineering Beijing 100005China College of Chemistry and Chemical Engineering Ningxia UniversityYinchuanNingxia 750021China

Bi_(2)O_(2)CO_(3)(BOC)/Bi_(4)O_5Br_(2)(BOB)/reduced graphene oxide(rGO)Z-scheme heterojunction with promising photocatalytic properties was synthesized via a facile one-pot room-temperature ***-thin nanosheets of BOC and BOB were grown in situ on r *** formed 2D/2D direct Z-scheme heterojunction of BOC/BOB with oxygen vacancies(OVs)effectively leads to lower negative electron reduction potential of BOB as well as higher positive hole oxidation potential of BOC,showing improved reduction/oxidation ***,rGO is an acceptor of the electrons from the conduction band of *** dual roles significantly improve the transfer performance of photo-induced charge carriers and accelerate their *** layered nanosheet structure,rich OVs,high specific surface area,and increased utilization efficiency of visible light,the multiple synergistic effects of BOC/BOB/rGO can achieve effective generation and separation of the electron-holes,thereby generating more·O_(2)^(-)and h^(+).The photocatalytic reduction efficiency of CO_(2)to CO(12.91μmol/(g·hr))is three times higher than that of BOC(4.18μmol/(g·hr)).Moreover,it also achieved almost 100%removal of Rhodamine B and cyanobacterial cells within 2 hours.

关键词： Bi_(2)O_(2)CO_(3) Bi_(4)O_(5)Br_(2) Reduced graphene oxide Z-scheme heterojunction Photocatalysis CO_(2)reduction

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Extrusion-base d 3D-printe d“rolle d-up”composite scaffolds with hierarchical pore structure for bone growth and repair

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Journal of Materials Science & Technology 2024年第4期171卷 222-234页

作者： Yufan Li Li Chen Yijing Stehle Mingyue Lin Chenxin wang Rui Zhang Min Huang Yubao Li qin Zou Research Center for Nano Biomaterials Analytical&Testing CenterSichuan UniversityChengdu 610064China Analytical&Testing Center Sichuan UniversityChengdu 610064China Department of mechanical engineering Union College807 Union St.SchenectadyNY 12308USA Sichuan Institute of Atomic Energy Chengdu 610101China

Three-dimensional(3D)bioprinting,specifically direct ink writing(DIW)capable of printing biologically active substances such as growth factors or drugs under low-temperature conditions,is an emerging di-rection in bone tissue ***,limited by the bio-ink mobility and the poor resolution of this printing technology,the lateral pores of current crisscross-stacked scaffolds printed through DIW tend to clog and are inimical to bone ***,it is critical to develop DIW printed biologi-cal scaffold structure with high mechanical strength,porosity,and biocompatibility ***,patterned polylactic acid(PLA)/polycaprolactone(PCL)/nano-hydroxyapatite(n-HA)based scaffold was printed through DIW technological and rolled-up for properties characterization,cytocompatibility test,and bone repair *** result not only shows that the hexagonal patterned scaffolds are me-chanically strong with porosity,but also demonstrated that the hierarchical pore structure formed during rolled-up has the potential to address the clogging problem and stimulates bone growth and repair.

关键词： Direct ink writing(DIW) Bone repair scaffold,Micro-CT Bio composites

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Hydraulic fracturing behaviors of shale under coupled stress and temperature conditions simulating different burial depths

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International Journal of Mining Science and Technology 2024年第6期34卷 783-797页

作者： qin Zhou Zheming Zhu Wei Liu Huijun Lu Zidong Fan Xiaofang Nie Cunbao Li Jun wang Li Ren MOE Key Laboratory of Deep Earth Science and Engineering College of Architecture and EnvironmentSichuan UniversityChengdu 610065China Downhole Operating Company CNPC Chuanqing Drilling and Exploration Engineering Co.Ltd.Shenzhen 518060China School of Architecture and Civil Engineering Xihua UniversityChengdu 610065China Guangdong Provincial Key Laboratory of Deep Earth Sciences and Geothermal Energy Exploitation and Utilization Shenzhen UniversityShenzhen 518060China

Fracture propagation in shale under in situ conditions is a critical but poorly understood mechanical process in hydraulic fracturing for deep shale gas reservoirs. To address this, hydraulic fracturing experiments were conducted on hollow double-wing crack specimens of the Longmaxi shale under conditions simulating the ground surface(confining pressure σ_(cp)=0, room temperature(Tr)) and at depths of 1600 m(σ_(cp)=40 MPa, Ti=70 ℃) and 3300 m(σ_(cp)=80 MPa, high temperature Ti=110 ℃) in the study *** in situ stress was found to significantly increase fracture toughness through constrained microcracking and particle frictional bridging mechanisms. Increasing the temperature enhances rather than weakens the fracture resistance because it increases the grain debonding length, which dissipates more plastic energy and enlarges grains to close microdefects and generate compressive stress to inhibit microcracking. Interestingly, the fracture toughness anisotropy in the shale was found to be nearly constant across burial depths, despite reported variations with increasing confining pressure. Heated water was not found to be as important as the in situ environment in influencing shale fracture. These findings emphasize the need to test the fracture toughness of deep shales under coupled in situ stress and temperature conditions rather than focusing on either in situ stress or temperature alone.

关键词： Hydraulic fracturing Fracture toughness Shale Anisotropy Deep rock mechanics

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A bi-functional catalyst strategy to selectively regulate sulfur redox kinetics in lithium-sulfur batteries

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Journal of Materials Science & Technology 2024年第6期173卷 54-62页

作者： Yanan Liu Xiaoxiao Huang Honglei Zhang Guangyu qin Xiaoshuang wang Meixiu Song Hongbo Liang Jingzhe Hong Yudong Huang State Key Laboratory of Advanced Welding and Joining Harbin Institute of TechnologyHarbin 150001China MIIT Key Laboratory of Advanced Structural-Functional Integration Materials&Green Manufacturing Technology Harbin Institute of TechnologyHarbin 150001China School of Materials Science and Engineering Harbin Institute of TechnologyHarbin 150001China School of Chemistry and Chemical Engineering Harbin Institute of TechnologyHarbin 150001China

Designing electrochemical catalysts has become a research hotspot due to their accelerating the polysulfide conversion of the sulfur cathode to inhibit the“shuttle effect”in lithium-sulfur ***,it is still a great challenge to design the heterogeneous selective electrochemical catalyst for inhibiting the“shuttle effect”.Herein,nickel cobalt phosphide and cobalt phosphide as the heterogeneous catalyst active sites embedded in the nitrogen-doped hollow carbon nanocages(NiCoP@CoP/NC)are reported,used for multi-step and multi-phase sulfur electrode reaction,and it is found that metal-sulfur d-p hybridization can effectively indicate the intrinsic catalytic activity of metal *** of labor and cooperation of the bi-active NiCoP@CoP as heterogeneous catalysts propel the stepwise polysulfide *** and CoP sites preferentially accelerate the long-chain polysulfide conversion reaction(S_(8)■LiPSs)and the short-chain polysulfide conversion reactions(LiPSs■Li_(2)S),***,the hollow and porous N-doped carbon structure can successfully suppress the volume effect and improve the conductivity of the sulfur *** unique design can obtain an effective inhibition of the shuttle effect and rapid electrode *** a result,Li-S batteries demonstrate a high initial capacity of 1063 mAh g^(-1) and a low-capacity decay of 0.04% per cycle within 1000 *** work provides a feasible idea for the design of host materials in Li-S batteries.

关键词： Shuttle effect d-p hybridization Heterogeneous catalysts Stepwise polysulfide conversion

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Co-Harvest Phase-Change Enthalpy and Isomerization Energy for High-Energy Heat Output by Controlling Crystallization of Alkyl-Grafted Azobenzene Molecules

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Energy & Environmental Materials 2024年第3期7卷 415-424页

作者： Jian Gao Yiyu Feng Wenyu Fang Hui wang Jing Ge Xiaoyu Yang Huitao Yu Mengmeng qin Wei Feng School of Materials Science and Engineering Tianjin UniversityTianjin 300350China Key Laboratory of Materials Processing and Mold Ministry of EducationZhengzhou UniversityZhengzhou 450002China

Photoisomerization-induced phase change are important for co-harvesting the latent heat and isomerization energy of azobenzene *** optimizing heat output and energy delivery at alternating temperatures are challenging because of the differences in crystallizability and *** article reports two series of asymmetrically alkyl-grafted azobenzene(Azo-g),with and without a methyl group,that have an optically triggered phase *** exothermic modes were designed to utilize crystallization enthalpy(△H_(c))and photothermal(isomerization)energy(△H_(p))at different temperatures determined by the ***-g has high heat output(275-303 J g^(-1))by synchronously releasing△H_(c)and△H_(p)over a wide temperature range(-79℃to 25℃).We fabricated a new distributed energy utilization and delivery system to realize a temperature increase of 6.6℃at a temperature of-8℃.The findings offer insight into selective utilization of latent heat and isomerization energy by molecular optimization of crystallization and isomerization processes.

关键词： crystallizability distributed energy utilization system energy density exothermic modes isomerization

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MoS_(2) nanoflowers and PEDOT:PSS nanocomposite enabling wearable dual-mode pressure sensors

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Science China(Technological Sciences) 2024年第6期67卷 1737-1747页

作者： wang FengMing YANG WeiJia MA Ke SHEN GengZhe SU DaoJian LI BaiJun wang ShuangPeng qin BoLong ZHANG Chi XIN Yue CAO XiaoBing HE Xin School of Applied Physics and Materials Wuyi UniversityJiangmen529020China Biomaterials R&D Center Zhuhai Institute of Advanced TechnologyChinese Academy of SciencesZhuhai519003China Joint Key Laboratory of the Ministry of Education Institute of Applied Physics and Materials EngineeringUniversity of MacaoMacao999078China

A versatile sensing platform employing inorganic MoS_(2) nanoflowers and organic poly(3,4-ethylene dioxythiophene):poly(styrene sulfonate)(PEDOT:PSS)has been investigated to develop the resistive and capacitive force-sensitive *** microstructure of the sensing layer heightens the sensitivity and response time of the dual-mode pressure sensors by augmenting electron pathways and inner stress in response to mechanical ***,the capacitive and resistive sensors exhibit sensitivities of 0.37 and 0.12 kPa^(-1),respectively,while demonstrating a remarkable response time of approximately 100 ***,it is noteworthy that the PEDOT:PSS layer exhibits excellent adhesion to polydimethylsiloxane(PDMS)substrates,which contributes to the development of highly robust force-sensitive sensors capable of enduring more than 10000loading/unloading *** combination of MoS_(2)/PEDOT:PSS layers in these dual-mode sensors has shown promising results in detecting human joint movements and subtle physiological ***,the sensors have achieved a remarkable precision rate of 98%in identifying target *** outcomes underscore the significant potential of these sensors for integration into applications such as electronic skin and human-machine interaction.

关键词： MoS_(2)/PEDOT:PSS nanocomposite force-sensitive sensor multi-scaled microstructure physiological signals monitoring object grasping recognition

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HF-VHF NEMS resonators enabled by 2D semiconductor ReSe2

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Science China(Information Sciences) 2024年第10期67卷 393-394页

作者： Jie TANG Ziluo SU Shuang CAI Yalan wang Luming wang Jiaqi WU Jiaze qin Jiankai ZHU Bo XU Juan XIA Zenghui wang Institute of Fundamental and Frontier Sciences University of Electronic Science and Technology of China State Key Lab of Transducer Technology Shanghai Institute of Microsystem and Information TechnologyChinese Academy of Sciences State Key Laboratory of Electronic Thin Films and Integrated Devices University of Electronic Science and Technology of China

Two-dimensional（2D） semiconductors offer a plethora of new opportunities for constructing novel *** them, rhenium diselenide(ReSe2, crystal structure in Figure 1（a）) stands out due to its unique interlayer couplin...

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Reinfection and Risk Factors of SARS-CoV-2 during an Omicron Wave 2022 in Shanghai

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Biomedical and Environmental Sciences 2024年第2期37卷 204-209页

作者： wang Pei qin wang Xiao Hang wang Jian SHI Zhi Wen CHU Dong Mei wang Zhi Fei ZHANG Mu Bai LIU Wei ZHOU Zi Jie XIE Wei Fen Department of Gastroenterology Changzheng HospitalNaval Medical UniversityShanghai 200003China Health examination center Changzheng HospitalNaval Medical UniversityShanghai 200003China

Multiple waves of coronavirus disease 2019(COVID-19) outbreaks have affected numerous countries worldwide. The first case of SARS-CoV-2 reinfection was reported in Hong Kong in August 2020^([1]), leading to increased interest in the effectiveness of natural immunity acquired from primary infection. While data reports vary across countries, all findings indicate that prior SARS-CoV-2 infection provides substantial protection against reinfection^([2]). However, natural immunity from infection with previous non-Omicron or early Omicron sub-lineages offers lower levels of protection against Omicron reinfection, with rates below 60%^([3]) and approximately 75%[4], respectively.

关键词： immunity infection Omi

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Resonance Analysis in a High-Rise Building: Combined Translational and Rotational Measurements

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Journal of Earth Science 2024年第3期35卷 1069-1074页

作者： Linpeng qin Yun wang Chang Chen Yongxiang Wei Chunqi Liao Yi Zhang Chao wang Wentao Wan Quanyang Shao School of Geophysics and Information Technology China University of GeosciencesBeijing 100083China Fujian Earthquake Agency Fuzhou 350003China Institute of Geochemistry Chinese Academy of SciencesGuiyang 550081China

0 INTRODUCTION Resonance frequency is an important indicator for structure health monitoring,which can be exacerbated by various natural forces,such as rainfall,earthquakes,and hurricanes(Wu et al.,2021;Shan et al.,2020;Gentile et al.,2016;Moser and Moaveni,2011).Clinton et al.(2006)found that changes in environmental factors could significantly affect the resonance frequency of the Millikan Library;and that compared with temperature,humidity and strong wind have greater impacts on resonance ***,some studies have confirmed the effects of environmental factors through mathematical statistical analyses,including Xia et al.(2006),Yuen and Kuok(2010),and Guéguen et al.(2017).Other studies(e.g.,Astorga et al.,2018)revealed a building’s self-healing ability,where the building’s resonance frequency drifts due to earthquake events,environmental factors,or random forced vibrations could gradually return to its original level,but the recovery time of frequency drift could be considerably different with respect to different environmental factors.

关键词： humidity rainfall earthquake

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Reversibly Tuning Electrochemiluminescence with Stimulated Emission Route for Single-Cell Imaging

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Research 2024年第3期2023卷 205-215页

作者： Cheng Ma Xiaodan Gou Zejing Xing Min-Xuan wang Wenlei Zhu qin Xu Dechen Jiang Jun-Jie Zhu School of Chemistry and Chemical Engineering Yangzhou University.Yangzhou 225002P.R.China State Key Laboratory of Analytical Chemistry for Life Science State Key Laboratory of Pollution Control and Resource ReuseSchool of Chemistry and Chemical EngineeringSchool of the EnvironmentNanjing UniversityNanjing 210023P.R.China.

Electrochemiluminescence (ECL) has established itself as an excellent transduction technique in biosensing and light-emitting device, while conventional ECL mechanism depending on spontaneous emission of luminophores lacks reversibility and tunable emission characters, limiting the universality of ECL technique in the fields of fundamental research and clinical applications. Here, we report the first observation of stimulated emission route in ECL and thus establish a reversible tuning ECL microscopy for single-cell imaging. This microscopy uses a focused red-shifted beam to transfer spontaneous ECL into stimulated ECL, which enables selective and reversible tuning of ECL emission from homogeneous solution, single particles, and single cells. After excluding other possible competitive routes, the stimulated ECL emission route is confirmed by a dual-objective system in which the suppressed spontaneous ECL is accompanied by the enhanced stimulated ECL. By incorporating a commercial donut-shaped beam, the sharpness of single-cell matrix adhesion is improved 2 to 3 times compared with the counterpart in confocal ECL mode. The successful establishment of this stimulated emission ECL will greatly advance the development of light-emitting device and super-resolution ECL microscopy.

关键词： tuning beam limiting

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