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Solar-assisted photocatalytic water splitting using defective UiO-66 solids from modulated synthesis

nano Research 2024年第5期17卷 4134-4150页

作者： Celia M.Rueda-navarro María Cabrero-Antonino Paula Escamilla Valentín díez-Cabanes dong Fan Pedro Atienzar Belén Ferrer Ignacio Vayá Guillaume Maurin Herme G.Baldoví Sergio navalón departamento de Química Universitat Politècnica de ValènciaCamino de Vera s/nValencia 46022Spain Instituto de Ciencia Molecular(ICMOL) Universitat de ValènciaPaterna 46980Spain ICGM Univ.MontpellierCNRSENSCMMontpellier34095France Instituto de Tecnología Química(UPV-CSIC) Universitat Politècnica de ValènciaAvenida de los Naranjos s/nValencia 46022Spain

Metal-organic frameworks(MOFs)are attracting increasing interests as photocatalysts for solar-driven hydrogen production from *** paper reports on a comparative study of using either acetic acid(AA)or trifluoroacetic acid(TFA)as the representative UiO-66 organic modulators for synthesizing visible light responsive UiO-66(Zr)-X(X:nH_(2) or nO_(2))photocatalysts for water *** results show that photocatalytic hydrogen generation from a water/methanol mixture can be improved by varying the nature and amount of the modulator employed to prepare the different UiO-66(Zr)-X(X:nH_(2) or nO_(2))solid ***-66(Zr)-nH_(2) was the most active photocatalyst,followed by UiO-66(Zr)-nO_(2),both prepared with 12 equivalents of AA with respect to the organic *** UiO-66(Zr)-nH_(2) solid was more active than the parent MOF in photocatalytic overall water splitting(OWS)(H_(2) and O_(2) production of 450 and 160μmol·g^(-1),respectively,in 5 h;apparent quantum yield(AQY)at 400 nm of 0.06%)in the absence of methanol and compares favourably with analogous *** on the photocatalytic activity of the most active solids of both series was obtained by means of a series of techniques,including ultraviolet-visible(UV-vis)diffuse reflectance,X-ray photoelectron spectroscopy(XPS),laser flash photolysis(LFP),electron spin resonance(ESR),photoluminescence and photoelectrochemical measurements together with density functional theory(dFT)*** results showed that organic acid modulators can be used to enhance the photocatalytic activity of missing linker UiO-66 defective materials in solar-powered water splitting.

关键词： heterogeneous photocatalysis metal-organic frameworks(MOFs) UiO-66 materials carboxylic acid modulators water splitting solar light

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detailed seismic zoning of the East Kazakhstan region in the Republic of Kazakhstan

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Geodesy and Geodynamics 2024年第2期15卷 156-165页

作者： natalya V.Silacheva n.P.Stepanenko O.K.Kurilova A.d.Kudabayeva A.T.danabayeva Institute of Seismology Ministry of Emergency SituationsAlmaty 050060Kazakhstan

Kazakhstan is currently drafting new construction regulations that comply with the major provisions of the *** regulations are created on the basis of seismic zoning maps of various degrees of detail,developed by our Institute of Seismology using a new methodological approach for *** article is about creating the first normative map of the detailed Seismic Zoning on a probabilistic foundation for the Republic of Kazakhstan’s East Kazakhstan *** carried out the probabilistic assessment of seismic hazard using a methodology consistent with the main provisions of Eurocode 8and updated compared with that used in developing maps of Kazakhstan’s General Seismic Zoning and seismic microzoning of *** most thorough and current data accessible for the area under consideration were combined with contemporary analytical *** have been done to not only the databases being used but also the way seismic sources were shown,including active faults *** a scale of 1:1000000,precise seismic zoning maps of the East Kazakhstan region were created for two probabilities of exceedance:10%and 2%in 50 years in terms of peak ground accelerations and macroseismic *** obtained seismic hazard distribution is generally consistent with the General Seismic Zoning of Kazakhstan’s previous ***,because active faults were included and a thoroughly revised catalog was used,there are more pronounced zones of increased danger along the fault in the western part of the *** the west of the territory,acceleration values also increased due to a more accurate consideration of seismotectonic *** maps are the basis for developing new state building regulations of the Republic of Kazakhstan.

关键词： Probabilistic seismic hazard assessment detailed seismic zoning Peak ground acceleration Microseismical intensity

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A concise review on surface and structural modification of porous zeolite scaffold for enhanced hydrogen storage

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Chinese Journal of Chemical Engineering 2024年第6期70卷 33-53页

作者： B.A.Abdulkadir R.S.R.Mohd Zaki A.T.Abd Wahab S.n.Miskan Anh-Tam nguyen dai-Viet n.Vo H.d.Setiabudi Centre for Research in Advanced Fluid&Processes Universiti Malaysia Pahang Al-Sultan AbdullahLebuh Persiaran Tun Khalil YaakobGambangPahang 26300Malaysia Faculty of Chemical&Process Engineering Technology Universiti Malaysia Pahang Al-Sultan AbdullahLebuh Persiaran Tun Khalil YaakobGambangPahang 26300Malaysia Center of Excellence for Green Energy and Environmental nanomaterials(CE@GrEEn) Nguyen Tat Thanh University300A Nguyen Tat ThanhDistrict 4Ho Chi Minh City 755414Viet Nam

Investigating zeolites as hydrogen storage scaffolds is imperative due to their porous nature and favorable physicochemical ***,the storage capacity of the unmodified zeolites has been rather unsatisfactory(0.224%-1.082%(mass))compared to its modified ***,the contemporary focus on enhancing hydrogen storage capacities has led to significant attention towards the utilization of modified zeolites,with studies exploring surface modifications through physical and chemical treatments,as well as the integration of various active *** enhanced hydrogen storage properties of zeolites are attributed to the presence of aluminosilicates from alkaline and alkaline-earth metals,resulting in increased storage capacity through interactions with the charge density of these ***,there is a great demand to critically review their role such as well-defined topology,pore structure,good thermal stability,and tunable hydrophilicity in enhanced hydrogen *** article aimed to critically review the recent research findings based on modified zeolite performance for enhanced hydrogen *** of the factors affecting the hydrogen storage capacities of zeolites that can affect the rate of reaction and the stability of the adsorbent,like pressure,structure,and morphology were studied,and ***,future perspectives,recommendations,and directions for modified zeolites were discussed.

关键词： Zeolites Hydrogen storage Surface modification Adsorption Active metal

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Localized-states quantum confinement induced by roughness in CdMnte/CdTe heterostructures grown on Si(111) substrates

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Journal of Semiconductors 2024年第9期 34-42页

作者： Leonarde do nascimento Rodrigues Wesley Fiorio lnoch Marcos L.F.Gomes Odilon d.d.Couto Jr. bráulio S.Archanjo Sukarno Olavo Ferreira Physics department Federal University of Vi?osa Instituto de Física Gleb Wataghin Universidade Estadual de Campinas national Institute of Metrology Quality and Technology (Inmetro) Materials Metrology Division (DIMAT)

This work shows that despite a lattice mismatch of almost 20%, CdMnte/CdTe/CdMnte heterostructures grown directly on Si(111) have surprisingly good optical emission properties. The investigated structures were grown by molecular beam epitaxy and characterized by scanning transmission electron microscopy, macro-and micro-photoluminescence. Low temperature macro-photoluminescence experiments indicate three emission bands which depend on the CdTe layer thickness and have different confinement characteristics. Temperature measurements reveal that the lower energy emission band (at 1.48 eV)is associated to defects and bound exciton states, while the main emission at 1.61 eV has a weak 2d character and the higher energy one at 1.71 eV has a well-defined (zero-dimensional, 0d) 0d nature. Micro-photoluminescence measurements show the existence of sharp and strongly circularly polarized (up to 40%) emission lines which can be related to the presence of Mn in the heterostructure. This result opens the possibility of producing photon sources with the typical spin control of the diluted magnetic semiconductors using the low-cost silicon technology.

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Enhancement of coercivity,permeability,and dielectric properties of Co_(0.2)Zn_(0.3)ni_(0.5)Eu_(x)Fe_(2-x)O_(4) ferrites for memory and high frequency devices

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Journal of Rare Earths 2024年第6期42卷 1128-1135,I0005页

作者： I.Sardar M.d.Hossain M.S.Sikder M.n.I.Khan M.R.Rahman Physics discipline Khulna UniversityKhulna9208Bangladesh department of Physics Khulna University of Engineering&TechnologyKhulna9203Bangladesh department ofComputer Science and Engineering Northern University of Business&Technology KhulnaKhulna9100Bangladesh Material Science division Atomic Energy CentreDhaka1000Bangladesh

Spinel cubic ferrites have huge applications in me mory and high frequency *** the improvement of these modern devices,the magnetic coercivity,permeability,and dielectric properties of a ferrite are the important *** article focuses on improving the magnetic coercivity,magnetic permeability,and dielectric properties of Co_(0.2)Zn_(0.3)ni_(0.5)Eu_(x)Fe_(2-x)O_(4) ferrites,where x=0.00,0.06,and *** X-ray diffraction(XRd),Fourier transform infrared spectroscopy(FTIR),field emission scanning electron microscopy(FESEM),energy dispersive X-ray(EdX),vibrating sample magnetometer(VSM),and an impedance analyzer were used to characterize the structural,magnetic,and dielectric properties of the *** XRd patterns indicate the formation of spinel cubic structure of the samples with a secondary peak(EuFeO_(3))for Eu doped *** densities and porosities of the samples follow an inverse trend,where the doped samples’lattice parameters are increased with the increment of rare earth Eu *** FTIR analysis also proves the spinel cubic phase of the *** average grain size of the ferrites is obtained via FESEM images,and it is increased from 121 to 198 *** analysis confirms that doping of the Eu content also changes other hysteresis loop properties of Co_(0.2)Zn_(0.3)ni_(0.5)Eu_(x)Fe_(2-x)O_(4) ***,the coercivity of the Eu doped samples is greater than that of the mother alloy(x=0.00).The EdX study shows that there is no impurity contamination in the *** permeability and dielectric measurements show an improved quality factor of the Eu-doped samples with low magnetic and dielectric *** dependent resistivity and impedance analysis also show the improved *** the observed properties of the samples,all the investigated ferrites might be strong candidates for potential applications in memory devices,magnetic sensors,and high frequency applications.

关键词： Ferrites Raree arths Coercivity Permeability EdX Resistivity

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长寿命UHPFRC组合钢桥面板研究综述

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交通运输工程学报 2024年第1期24卷 68-84页

作者：段兰袁翊竑王春生 brÜHWILER Eugen 长安大学公路学院陕西西安710064 瑞士洛桑联邦理工学院结构维护与安全实验室沃州洛桑CH-1015

从三方面归纳与剖析了超高性能纤维增强水泥基(UHPFRC)复合材料组合钢桥面板的研究进展,包括强韧性组合层选材、界面传力机制与损伤累积机理、设计方法与工程应用;总结了纤维类型、纤维掺量对UHPFRC轴拉性能和抗弯性能的影响规律,确定... 详细信息

从三方面归纳与剖析了超高性能纤维增强水泥基(UHPFRC)复合材料组合钢桥面板的研究进展,包括强韧性组合层选材、界面传力机制与损伤累积机理、设计方法与工程应用;总结了纤维类型、纤维掺量对UHPFRC轴拉性能和抗弯性能的影响规律,确定了支撑组合钢桥面板结构分析的多种本构模型;对比分析了热连接、冷连接和混合连接组合界面设计方式的技术特点,归纳了胶粘界面、冷连接剪力键界面与混合连接界面的传力机理试验与理论研究成果;总结了基于冷连接设计理念的组合钢桥面板在合理构造、设计方法、规范规程与工程实践等方面的研究成果,并探讨了长寿命组合钢桥面板的创新与发展方向。研究结果表明:单一或混杂纤维的掺入综合提升了UHPFRC的应变强化能力、弯曲变形能力、抗断裂能力、裂缝宽度控制能力和抗疲劳性能,轴拉条件下UHPFRC三线型简化本构模型有力支撑了组合钢桥面板的设计计算,弹塑性损伤本构模型可描述不可逆疲劳损伤累积;验证了冷连接组合界面的增韧效果与可靠性,新型剪力键既可以提高组合效应,也能增韧UHPFRC层,混合连接界面具有降低界面局部应力集中、提高整体界面抗剪刚度、改善界面传力、提升施工效率等综合技术优势,内聚界面本构模型可实现冷连接界面损伤累积反演分析,界面损伤预测结果准确可靠;基于冷连接的UHPFRC组合钢桥面板可以有效提高钢桥面板的局部刚度,相关设计方法可支撑标准的编制与工程实践;应进一步提升UHPFRC的性价比和界面连接的高效性和可靠性,以支撑组合钢桥面板的长寿命、强韧性、轻量化、易维护、低能耗设计与建造。

关键词：桥梁工程长寿命 UHPFRC组合钢桥面板冷连接件组合界面设计准则免蒸养

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Environmental changes affect picoplanktonic composition in Antarctic Peninsula ponds

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Advances in Polar Science 2024年第1期35卷 108-122页

作者： Micaela dÍAZ Leonardo LAGOMARSInO Gabriela MATALOnI Marianela BELTRÁn Marcela LIBERTELLI Paulina FERMAnI Laboratorio de Ecología Acuática INTECH-UNSAM-CONICETChascomús 7130Argentina Facultad de Ciencias naturales y de la Salud UNPSJBComodoro Rivadavia 9000Argentina Laboratorio de Biodiversidad Limnología y Biología de la Conservación3IA-UNSAM-CONICETBuenos Aires 1650Argentina departamento de Biología de Predadores Tope Instituto Antártico ArgentinoBuenos Aires 1650Argentina Laboratorio de Microbiología Ambiental IBIOMAR/CESIMAR-CENPAT-CONICETPuerto Madryn 9120Argentina

Antarctic Peninsula is experiencing one of the largest global warming events *** water bodies generated by the melting of snow in summer are numerous,and they might act as sentinels of climate change due to their rapid response and ability to integrate catchment *** in climate can influence the structure of microbial communities which dominate these freshwaters ***,we characterize three ponds at Cierva Point(Antarctic Peninsula)by examining their physico-chemical and morphological characteristics and we explored how different factors modify the structure of the microbial *** studied the abundance and biomass of heterotrophic bacteria,picocyanobacteria and picoeukaryote algae during January and February of two consecutive summers(2017 and 2018).We found that ponds had different limnological characteristics,due to their location,geomorphological features and presence of the surrounding flora and ***-chemical parameters as well as microbial community differed between ponds,months and *** 2017,most ponds were oligo to mesotrophic *** larger accumulated rainfall(as a result of environmental changes on the Antarctic Peninsula)during 2018,particularly in February,causes nutrient runoff into water *** affects those ponds with the highest seabird circulation,such as gentoo penguin,increasing *** a result,picoplanktonic abundances were higher,and the community structure shifts to a largely heterotrophic bacteria dominated *** results suggest that these communities could act as sentinels to environmental changes,anticipating a future with mostly hypertrophic ponds.

关键词： microorganisms freshwater environments climate change Cierva Point

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Measurement of yields and angular distributions ofγ-quanta from the interaction of 14.1 MeV neutrons with oxygen,phosphorus,and sulfur

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Chinese Physics C 2024年第3期48卷 79-92页

作者： d.n.Grozdanov n.A.Fedorov S.B.dabylova Yu.n.Kopatch I.n.Ruskov V.R.Skoy T.Yu.Tretyakova C.Hramco P.I.Kharlamov G.V.Pampushik P.G.Filonchik A.V.Andreev Joint Institute for nuclear Research(JInR) DubnaRussia Institute for nuclear Research and nuclear Energy Bulgarian Academy of SciencesSofiaBulgaria Faculty of Physics Lomonosov Moscow State UniversityMoscowRussia L.n.Gumilyov Eurasian national University AstanaKazakhstan Skobeltsyn Institute of nuclear Physics Moscow State UniversityMoscowRussia Institute of Chemistry of Moldova ChisinauRepublic of Moldova Moscow Institute of Physics and Technology MoscowRussia

A study of the inelastic scattering of neutrons with an energy of 14.1 MeV on the nuclei of oxygen,phosphorus,and sulfur was performed at the TAnGRA facility at JInR(dubna).The experiment aimed to refine existing data and obtain new data on the yields and angular distributions ofγ-quanta emitted by the studied nuclei due to neutron-induced nuclear reactions using the tagged neutron *** types of detector systems were used to registerγ-***γ-ray yields were measured using a high-purity germanium(HPGe)*** angular distributions ofγ-rays were obtained using a system of 18 scintillation detectors based on bismuth germanite Bi_(4)Ge_(3)O_(12)(BGO)located around the *** performed experiments measured the yields of two transitions for the reaction of tagged neutrons with 16O,nine transitions for the reaction with ^(31)P,and nine transitions for the reaction with ^(32)S for the first *** angular anisotropy of theγ-radiation accompanying the inelastic scattering of neutrons with an energy of 14.1 MeV on ^(31)P nuclei was also measured for the first time.

关键词： tagged neutron method yields of gamma-quanta high-resolution gamma-spectrometry neutron-nuclear reactions neutron scattering

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Tilted global solar irradiance in Bahrain:an experimental study

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Clean Energy 2024年第2期8卷 27-34页

作者： n.Vasilikos C.Georgantopoulou H.Alajaimi S.H.Almajed M.Ahmed d.Mathioulakis School of Mechanical Engineering Bahrain PolytechnicIsa TownPO Box 33349Kingdom of Bahrain School of Mechanical Engineering National Technical University of AthensHeroon Polytechniou 7 StZografos 15773AthensGreece

In the present work,tilted global solar irradiance data are presented and analysed,measured for a period of 1 year on the campus of Bahrain Polytechnic,Kingdom of Bahrain,from both a fixed photovoltaic panel and a moving one via a two-axis solar *** fixed panel faces south with an angle of 26°with respect to the horizontal,coinciding with the local geographical *** second panel is moved by two motors,controlled by a global positioning system and suitable software so that the Sun’s rays are perpendicular to the panel surface.A pyranometer is installed on each panel,recording the tilted global solar irradiance,stored by using a data *** analysis of the data obtained shows a 33%solar energy gain on an annual basis for the moving panel(2780 versus 2088 kWh/m^(2) on the fixed panel).More importantly,in June,when the energy demand in Bahrain is elevated due to the increased residential cooling loads,the solar energy received by the moving panel is 54.7%higher compared with that of the fixed *** a percentage basis,the increase in solar energy from the moving panel is profound in the early morning and late evening ***,the reduction in the solar energy received by the fixed panel from May to June does not appear in the moving panel because of the adjustable orientation of the *** the year,the mean daily solar power varies between 0.37 and 0.56 kW/m^(2) for the fixed panel,and 0.45 and 0.70 kW/m^(2) for the moving *** winter,solar energy fluctuations are elevated due to erratic weather conditions that present a peak standard deviation of 28%of the corresponding *** data presented are useful for potential solar investments in Gulf countries.

关键词： tilted solar irradiance renewable energy solar tracking photovoltaic Gulf Cooperation Council Countries

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Characterization of early maturing elite genotypes based on MTSI and MGIdI indexes:an illustration in upland cotton(Gossypium hirsutum L.)

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Journal of Cotton Research 2024年第3期7卷 253-265页

作者： d S RAJ Supritha PATIL Rajesh S. PATIL Bhuvaneshwara R. nAYAK Spurthi n. PAWAR Kasu n. department of Genetics and Plant breeding College of AgricultureUniversity of Agricultural SciencesDharwad 580005India Agricultural Research Station Dharwad 580005India department of Biotechnology College of AgricultureUniversity of Agricultural SciencesDharwad 580005India department of Crop Physiology College of AgricultureUniversity of Agricultural SciencesDharwad 580005India

Background Globally,the cultivation of cotton is constrained by its tendency for extended periods of *** maturity plays a potential role in rainfed-based multiple cropping system especially in the current era of climate *** the current study,a set of 20 diverse Gossypium hirsutum genotypes were evaluated in two crop seasons with three planting densities and assessed for 11 morphological traits related to early *** study aimed to identify genotype(s)that mature rapidly and accomplish well under diverse environmental conditions based on the two robust multivariate techniques called multi-trait stability index(MTSI)and multi-trait genotype-ideotype distance index(MGIdI).Results MTSI analysis revealed that out of the 20 genotypes,three genotypes,viz.,nndC-30,A-2,and S-32 accomplished well in terms of early maturity traits in two ***,three genotypes were selected using MGIdI method for each planting densities with a selection intensity of 15%.The strengths and weaknesses of the genotypes selected based on MGIdI method highlighted that the breeders could focus on developing early-maturing genotypes with specific traits such as days to first flower and boll *** selected genotypes exhibited positive genetic gains for traits related to earliness and a successful harvest during the first and second ***,there were negative gains for traits related to flowering and boll *** The study identified three genotypes exhibiting early maturity and accomplished well under different planting *** multivariate methods(MTSI and MGIdI)serve as novel approaches for selecting desired genotypes in plant breeding programs,especially across various growing *** methods offer exclusive benefits and can easily construe and minimize multicollinearity issues.

关键词： Cotton MTSI MGIdI Genotype environment interaction Early maturity Multi-trait Multi-environment

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