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Quantifying structural distortion manipulation for desired perovskite phase:PartⅠ.Paradigm demonstration in tungsten oxides

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Journal of Materiomics 2024年第2期10卷 293-303页

作者： cheng Fang Hong Wang Siqi Shi State Key Laboratory of Green Building Materials China Building Materials AcademyBeijing100024China Beijing Key Laboratory of Solar Energy and Building Energy-saving Glass Materials Processing Technology China Building Materials AcademyBeijing100024China Materials Genome Initiative Center Shanghai Jiao Tong UniversityShanghai200240China School of Materials Science and Engineering Shanghai Jiao Tong UniversityShanghai200240China School of Materials Science and Engineering Shanghai UniversityShanghai200444China Materials Genome Institute Shanghai UniversityShanghai200444China

Slight distortions can cause dramatic changes in the properties of crystalline perovskite materials and their *** to the numerous types of distortions and unclarified distortion-structure relations,a quantitative distortion manipulation for the desired crystalline phase of perovskite materials suitable for various application remains ***,by establishing parameter sets to systematically describe the types,magnitudes and positional relations involved in distortions,we are able to interpret the structural regulations and manipulation strategies in 7 reported crystal *** the con-struction of distortion-phase-property functional curves,we further propose a paradigm to quantify the structural distortion manipulation for desired perovskite *** the example of perovskite-like tungsten oxides,we successfully quantify their volume shrinkage and symmetry increase during *** work verifies that the complicated research and development of perovskite materials can be simplified into a mathematical problem solving process,which will inspire researchers with different backgrounds to participate,especially mathematicians and computer scientists.

关键词： Distortion manipulation Distortion-phase-property function Coordination polyhedron Tungsten oxide Perovskite

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Formation of Superthin Galaxies in IllustrisTNG

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Research in Astronomy and Astrophysics 2024年第7期24卷 235-248页

作者： Jianhong Hu Dandan Xu cheng Li Department of Astronomy Tsinghua UniversityBeijing 100084China

Superthin galaxies are observed to have stellar disks with extremely small minor-to-major axis *** this work,we investigate the formation of superthin galaxies in the TNG100 *** trace the merger history and investigate the evolution of galaxy properties of a selected sample of superthin galaxies and a control sample of galaxies that share the same joint probability distribution in the stellar-mass and color *** making comparisons between the two galaxy samples,we find that present-day superthin galaxies had similar morphologies as the control sample counterparts at higher redshifts,but have developed extended flat“superthin”morphologies since z~*** this latter evolution stage,superthin galaxies undergo an overwhelmingly higher frequency of prograde mergers(with orbit-spin angleθ_(orb)≤40°).Accordingly the spins of their dark matter halos have grown significantly and become noticeably higher than those of their normal disk *** further results in the buildup of their stellar disks at larger distances much beyond the regimes of normal disk *** also discuss the formation scenario of those superthin galaxies that live in larger dark matter halos as satellite galaxies therein.

关键词： Galaxies formation-Galaxies evolution-Galaxies interactions-Galaxies star formation

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Current status of early gastric cancer screening research

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Cancer Biology & Medicine 2024年第3期21卷 218-222页

作者： Can Hu Li Yuan Xiangdong cheng Department of Gastric surgery Zhejiang Cancer HospitalHangzhou Institute of Medicine(HIM)Chinese Academy of SciencesHangzhouZhejiang 310022China Key Laboratory of Prevention Diagnosis and Therapy of Upper Gastrointestinal Cancer of Zhejiang ProvinceHangzhou 310022China Zhejiang Provincial Research Center for Upper Gastrointestinal Tract Cancer Zhejiang Cancer HospitalHangzhou 310022China

Gastric cancer is a predominant threat to the health and well-being of China's residents. Data from the World Health Organization(WHO) in 2020 revealed that gastric cancer in China notably accounted for 44.0% of new c... 详细信息

关键词： cancer Gastric gastric

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基于神经网络PID的无人机自适应变量喷雾系统的设计与试验

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华南农业大学学报 2019年第4期40卷 100-108页

作者：岑振钊岳学军王林惠凌康杰程子耀卢杨华南农业大学电子工程学院

[目的]针对传统植保无人机在定量喷施作业时由于飞行速度的变化造成施药不均匀以及传统控制算法无法满足无人机变量喷雾系统所需的实时性和稳定性等问题,设计一种基于神经网络PID的自适应无人机变量喷雾系统。[方法]采用风压变送器测出... 详细信息

[目的]针对传统植保无人机在定量喷施作业时由于飞行速度的变化造成施药不均匀以及传统控制算法无法满足无人机变量喷雾系统所需的实时性和稳定性等问题,设计一种基于神经网络PID的自适应无人机变量喷雾系统。[方法]采用风压变送器测出无人机的飞行速度,根据速度采用脉宽调制(PWM)方法进行自适应变量喷雾,同步用流量传感器测出实际喷雾流量,融合BP神经网络PID控制算法调节喷雾流量。由MATLAB构建BP神经网络PID控制算法,并与PID、模糊PID和神经元PID对比及分析;田间试验过程中,对比分析无人机定量喷雾与随飞行速度改变的变量喷雾效果,采用水敏纸获取雾滴沉积量分布,分别从整体区域、飞行方向和喷杆方向评价沉积量分布的均匀性。[结果]算法仿真对比试验结果表明,与PID、模糊PID和神经元PID相比,BP神经网络PID阶跃响应上升时间分别少28.57%、84.73%和31.03%,正弦跟踪平均误差分别小63.01%、87.03%和0.58%,方波跟踪平均误差分别小74.00%、79.53%和6.80%,鲁棒性强,无静差,超调量为1.20%;喷雾对比试验结果表明,本系统能够根据飞行速度自适应调节喷雾流量,实际流量与目标流量的平均偏差为8.43%,水敏纸扫描结果表明总体区域雾滴沉积量的变异系数对比定量喷雾平均降低26.25%,喷杆方向平均降低18.79%。[结论]该研究结果可为农业航空变量喷雾技术的应用提供理论基础。

关键词：无人机风压变送器自适应变量喷雾神经网络PID

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Manipulating the Phase Transition Behavior of Dual Temperature-Responsive Block Copolymers by Adjusting Composition and Sequence

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Chinese Journal of Polymer Science 2024年第2期42卷 176-187,I0006页

作者： Zhi Zou Xiang Xu Hai-Tao Zhao Jian-Nan cheng Wei-Wei He Li-Fen Zhang Zhen-Ping cheng Suzhou key Laboratory of Macromolecular Design and Precision Synthesis Jiangsu Key Laboratory of Advanced Functional Polymer Design and ApplicationState and Local Joint Engineering Laboratory for Novel Functional Polymeric MaterialsCollege of ChemistryChemical Engineering and Materials ScienceSoochow UniversitySuzhou215123China State Key Laboratory of Radiation Medicine and Protection School for Radiological and Interdisciplinary Sciences(RAD-X)and Collaborative Innovation Center of Radiation Medicine of JiangsuSoochow UniversitySuzhou215123China

Temperature-responsive polymers have garnered significant attention due to their ability to respond to external *** this work,dual temperature-responsive block copolymers are synthesized via reversible addition-fragmentation chain transfer polymerization(RAFT)polymerization utilizing zwitterionic monomer methacryloyl ethyl sulfobetaine(SBMA) and N-isopropyl acrylamide(NIPAAm) as *** thermal responsive behaviors can be easily modulated by incorporating additional hydrophobic monomer benzyl acrylate(BN) or hydrophilic monomer acrylic acid(AA),adjusting concentration or pH,or varying the degree of polymerization of the block chain *** cloud points of the copolymers are determined by UV-Vis spectrophotometry,and these copolymers exhibit both controlled upper and lower critical solu bility temperatures(LCST and UCST) in aqueous *** study analyzes and summarizes the influencing factors of dual temperature responsive block copolymers by exploring the effects of various conditions on the phase transition temperature of temperature-sensitive polymers to explore the relationship between their properties and environment and structure to make them more selective in terms of temperature application range and regulation *** is very interesting that the introduction of poly-acrylic acid(PAA) segments in the middle of di-block copolymer PSBMA_(55)-b-PNIPAAm_(80) to form PSBMA_(55)-b-PAA_(x)-b-PNIPAAm_(80) results in a reversal of temperature-responsive behaviors from 'U'(LCST UCST) type,while the copolymer PSBMA_(55)-b-P(NIPAAm_(80)-co-AA_(x)) *** work provides a clue for tuning the phase transition behavior of polymers for manufacture of extreme smart materials.

关键词： Temperature responsive polymers High critical solubility temperature(UCST) Low critical solubility temperature(LCST) Block copolymers

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Study on site selection planning of urban electric vehicle charging station

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High Technology Letters 2024年第1期30卷 75-84页

作者：刘娜 cheng Jiaxin DUAN Yukai School of Business Shanghai Dianji UniversityShanghai201306 P.R.China

The large-scale development of electric vehicles(EVs)requires numerous charging stations to serve them,and the charging stations should be reasonably laid out and planned according to the charging demand of electric *** the costs of both operators and users,a site selection model for optimal layout planning of charging stations is constructed,and a queuing theory approach is used to determine the charging pile configuration to meet the charging demand in the planning *** solve the difficulties of particle swarm global optimization search,the improved random drift particle swarm optimization(IRDPSO)and Voronoi diagram are used to jointly solve for the optimal layout of electric *** final arithmetic analysis verifies the feasibility and practicality of the model and algorithm,and the results show that the total social cost is minimized when the charging station is 9,the location of the charging station is close to the center of gravity and the layout is reasonable.

关键词： charging station electric vehicle(EV) improved random drift particle swarm optimization(IRDPSO) optimal planning

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Reconstruction of biomimetic ionic channels within covalent organic frameworks for ultrafast and selective uranyl capture

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Science China Chemistry 2024年第10期67卷 3423-3431页

作者： cheng-Rong Zhang Xiao-Juan Chen cheng-Peng Niu cheng Meng Shun-Mo Yi Xin Liu Jia-Xin Qi Qiu-Xia Luo Ru-Ping Liang Jian-Ding Qiu State Key Laboratory of Nuclear Resources and Environment East China University of TechnologyNanchang 330013China College of Chemistry and Chemical Engineering Nanchang UniversityNanchang 330031China

The efficient extraction of uranium,as the primary component of nuclear energy,holds significant *** inspiration from the charge interaction observed in biological ion channels,we encapsulated negatively charged polystyrene sulfonate(PSS)or sodium polystyrene carboxylate(PVBA)into the nanochannels of amidoxime functionalized covalent organic framework(COF-AO)in-situ to alter the cavity environment of *** synthesized COF-AO-PSS and COF-AO-PVBA are used for ultra-fast and highly selective uranium *** negatively charged PSS/PVBA was confined in the COF-AO channel providing the driving force for uranium transport and blocking other ions,thus creating a highly selective“uranium highway”.Additionally,introducing sulfonate groups or carboxyl groups into COF-AO offers supplementary coordination environments and weak interactions with *** to charge-assisted migration and various interaction mechanisms,both COF-AO-PSS and COF-AO-PVBA exhibit faster adsorption kinetics and higher selectivity compared to COF-AO *** adsorption capacities are 3.8 times and 2.4 times that of COF-AO alone respectively which highlights the necessity for constructing biomimetic ion channels in uranium adsorption *** work presents a bionic adsorbent based on covalent organic frameworks(COFs)for the first time,overcoming environmental and equipment limitations associated with traditional photocatalysis and electrocatalysis methods for uranium capture,opening up new avenues for designing multifunctional materials that mimic biological systems.

关键词： covalent organic frameworks Uranium biomimetic ion-channels adsorption

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A Reliable Iteration Algorithm for One-Bit Compressive Sensing on the Unit Sphere

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Acta Mathematicae Applicatae Sinica 2024年第3期40卷 801-822页

作者： Yan-cheng LU Ning BI An-hua WAN School of Mathematics Sun Yat-sen UniversityGuangzhou 510275China

The one-bit compressed sensing problem is of fundamental importance in many areas,such as wireless communication,statistics,and so ***,the optimization of one-bit problem coustrained on the unit sphere lacks an algorithm with rigorous mathematical proof of convergence and *** this paper,an iteration algorithm is established based on difference-of-convex algorithm for the one-bit compressed sensing problem constrained on the unit sphere,with iterating formula■,where C is the convex cone generated by the one-bit measurements andη_(1)>η_(2)>1/*** new algorithm is proved to converge as long as the initial point is on the unit sphere and accords with the measurements,and the convergence to the global minimum point of the l_(1)norm is discussed.

关键词： one-bit compressed sensing difference of convex algorithm iteration algorithm ■1-minimization

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Recent advances in post-chiroptical manipulation of supramolecular aggregates assembled with molecular modules

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Science China Chemistry 2024年第9期67卷 2842-2863页

作者： Yanling Shen Wanhua Wu Zhipeng Yu cheng Yang Key Laboratory of Green Chemistry&Technology of Ministry of Education College of Chemistry InstitutionSichuan UniversityChengdu 610064China

Recently,various supramolecular assembly systems have been identified where the pre-existing chiral supramolecular structure can be manipulated through environmental adjustments,such as temperature,solvent,and *** changes result in diverse microscopic morphologies during the assembly process and induce chiroptical variations,particularly in circular dichroism(CD)and circularly polarized luminescence(CPL)*** chiroptical properties serve as direct indicators of the chiral supramolecular structure and hold promise for applications in sensing,molecular recognition,asymmetric synthesis,and material *** review focuses on research published in the last five years,highlighting instances where assembled structures aggregated by small organic molecular modules demonstrate in-situ chiroptical changes through external condition *** categorizes and discusses different modes of regulation,aiming to offer insights and guidelines for exploring dynamic changes in assembly processes and designing in-situ adjustable structures of assembly modules.

关键词： supramolecular assemblies post-chiroptical manipulation in-situ structural changes

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Investigation of cracking mechanism of the first tunnel lining during double-arch tunnel construction

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Underground Space 2024年第1期14卷 1-17页

作者： Yi Sui Xiaohui cheng Zuozhou Zhao Weibin Ma Railway Engineering Research Institute China Academy of Railway Sciences Corporation LimitedBeijing 100081China School of Civil Engineering Tsinghua UniversityBeijing 100084China

To solve the engineering problem of the first tunnel lining cracking caused by the second tunnel construction of double-arch highway tunnels,a research method combining distributed optical-fibre monitoring,inversion analysis and numerical simulation that can reflect lining cracking was *** fibres were laid on opposite sides of the steel arches inside the first tunnel *** optical-fibre monitoring was conducted continuously during the second tunnel *** on the fibre-optic strain profile,the lining cracking was deduced and warned in *** mechanical behaviour of the steel arch was investigated by the inversion analysis,which took into consideration the integrated impact of axial force and flexural moment.A two-dimensional(2D)load-structure method–based numerical model was established,considering the influence of different load distributions in each construction *** total strain rotating crack constitutive model was applied to reflect the cracking behaviour of concrete lining in the simulation,and the model was calibrated and verified in the *** analysis between the simulated strain distribution and the distributed optical-fibre monitoring results was carried *** deformation mode and crack distribution of the lining were *** cracking mechanism was ***,the second tunnel construction led to the loading at the top of the middle partition wall and the release of rock pressure in the first *** these load changes,the secondary lining of the first tunnel cracked on the inner side of the top of the middle partition wall owing to tension,and compression-bending failure occurred near the right arch ***,the influence of the parameters on the lining force was analysed,and a construction optimisation scheme was proposed.

关键词： Double-arch tunnel Cracking mechanism Distributed optical-fibre sensing Inversion analysis Total strain rotating crack model Loadstructure method

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