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Low-temperature NH_(3) abatement via selective oxidation over a supported copper catalyst with high Cu^(+) abundance

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Journal of Environmental Sciences 2024年第9期143卷 12-22页

作者： Zhiming yang Lin Peng Leneng yang Mingli Fu Daiqi Ye Peirong Chen Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution Control National Engineering Laboratory for VOCs Pollution Control Technology and EquipmentSchool of Environment and EnergySouth China University of TechnologyGuangzhou 510006China Guangdong Chengyi Environmental Technology Corp. Shaoguan 512158China

Selective catalytic NH_(3)-to-N_(2) oxidation(NH_(3)-SCO)is highly promising for abating NH_(3) emissions slipped from stationary flue gas after-treatment *** practical application,however,is limited by the non-availability of low-cost catalysts with high activity and N_(2) ***,using defect-rich nitrogen-doped carbon nanotubes(NCNT-AW)as the support,we developed a highly active and durable copper-based NH_(3)-SCO catalyst with a high abundance of cuprous(Cu^(+))*** obtained Cu/NCNT-AW catalyst demonstrated outstanding activity with a T_(50)(*** temperature to reach 50% NH_(3) conversion)of 174℃ in the NH_(3)-SCO reaction,which outperformed not only the Cu catalyst supported on N-free O-functionalized CNTs(OCNTs)or NCNT with less surface defects,but also those most active Cu catalysts in open *** kinetics measurements and temperature-programmed surface reactions using NH_(3)as a probe molecule revealed that the NH_(3)-SCO reaction on Cu/NCNT-AW follows an internal selective catalytic reaction(i-SCR)route involving nitric oxide(NO)as a key *** to mechanistic investigations by X-ray photoelectron spectroscopy,Raman spectroscopy,and X-ray absorption spectroscopy,the superior NH_(3)-SCO performance of Cu/NCNT-AW originated from a synergy of surface defects and ***,surface defects promoted the anchoring of Cu O nanoparticles on N-containing sites and,thereby,enabled efficient electron transfer from N to Cu O,increasing significantly the fraction of SCR-active Cu^(+)sites in the *** study puts forward a new idea for manipulating and utilizing the interplay of defects and N-dopants on carbon surfaces to fabricate Cu^(+)-rich Cu catalysts for efficient abatement of slip NH_(3)emissions via selective oxidation.

关键词： NH_(3)-SCO XANES Localized etching N-doping N_(2) selectivity i-SCR

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Stability and accuracy of central difference method for real-time dynamic substructure testing considering mass participation coefficient

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Earthquake Engineering and Engineering Vibration 2024年第3期23卷 625-636页

作者： Zheng Lichang Xu Guoshan yang Ge Wang Zhen yang Kaibo Zheng Zhenyun School of Civil Engineering Harbin Institute of TechnologyHarbin 150090China Key Lab of Structures Dynamic Behavior and Control Ministry of EducationHarbin Institute of TechnologyHarbin 150090China Key Lab of Intelligent Disaster Mitigation Ministry of Industry and Information TechnologyHarbin 150090China School of Civil Engineering and Architecture Wuhan University of TechnologyWuhan 430070China

For real-time dynamic substructure testing(RTDST),the influence of the inertia force of fluid specimens on the stability and accuracy of the integration algorithms has never been ***,this study proposes to investigate the stability and accuracy of the central difference method(CDM)for RTDST considering the specimen mass participation ***,the theory of the CDM for RTDST is ***,the stability and accuracy of the CDM for RTDST considering the specimen mass participation coefficient are ***,numerical simulations and experimental tests are conducted for verifying the effectiveness of the *** study indicates that the stability of the algorithm is affected by the mass participation coefficient of the specimen,and the stability limit first increases and then decreases as the mass participation coefficient *** most cases,the mass participation coefficient will increase the stability limit of the algorithm,but in specific circumstances,the algorithm may lose its *** stability and accuracy of the CDM considering the mass participation coefficient are verified by numerical simulations and experimental tests on a three-story frame structure with a tuned liquid damper.

关键词： real-time dynamic substructure testing central difference method stability mass participation coefficient tuned liquid damper

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Combined Treatment with Bojungikgi-tang(Buzhong Yiqi Decoction)and Riluzole Attenuates Cell Death in TDP-43-Expressing Cells

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Chinese Journal of Integrative Medicine 2024年第7期30卷 616-622页

作者： Eun Jin yang Department of KM Science Research Korea Institute of Oriental MedicineDaejeonYuseong-gu34054Republic of Korea

Objective To examine the effect of combined treatment with Bojungikgi-tang(BJIGT,Buzhong Yiqi Decoction)and riluzole(RZ)in transactive response DNA-binding protein 43(TDP-43)stress granule(SG)cells,a amyotrophic lateral sclerosis(ALS)cell line using transcriptomic and molecular *** TDP-43 SG cells were pretreated with BJIGT(100µg/mL),RZ(50µmol/L),and combined BJIGT(100µg/mL)/RZ(50µmol/L)for 6 h before treatment with lipopolysaccharide(LPS,200µmol/L).Cell viability assay was performed to elucidate cell toxicity in TDP-43 SC cells using a cell-counting kit-8(CCK8)assay *** expression levels of cell death-related proteins,including Bax,caspase 1,cleaved caspase 3 and DJ1 in TDP-43 SG cells were examined by Western blot *** autophagy-related proteins,including pmTOR/mTOR,LC3b,P62,ATG7 and Bcl-2-associated athanogene 3(Bag3)were investigated using immunofluorescence and immunoblotting *** Cell viability assay and Western blot analysis showed that combined treatment with BJIGT and RZ suppressed LPS-induced cell death and expression of cell death-related proteins,including Bax,caspase 1,and DJ1(P<0.05 or P<0.01).Immunofluorescence and immunoblotting assays showed that combined treatment with BJIGT and RZ reduced LPS-induced formation of TDP-43 aggregates and regulated autophagy-related protein levels,including p62,light chain 3b,Bag3,and ATG7,in TDP-43-expressing cells(P<0.05 or P<0.01).Conclusion The combined treatment of BJIGT and RZ might reduce inflammation and regulate autophagy dysfunction in TDP-43-induced ALS.

关键词： Bojungikgi-tang Buzhong Yiqi Decoction transactive response DNA-binding protein 43 autophagy oxidative stress amyotrophic lateral sclerosis

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Petrogenesis and Tectonic Significance of Shenxianshui Alkaline Granite in Gejiu,Yunnan Province,China

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Acta Geologica Sinica(English Edition) 2024年第2期98卷 368-385页

作者： yang Rong CHEN Yongqing School of Earth Sciences and Resources China University of GeosciencesBeijing 100083China

The Shenxianshui granites in the western Gejiu area were formed in the Late *** ablation inductively coupled plasma mass spectrometry indicates zircon U-Pb ages ranging from 90.67±0.7 to 85.97±0.6 *** intrusive rocks are peraluminous(A/CNK=1.03 to 1.33)and calc-alkaline,showing an affinity towards I-type *** ion lithophilic elements are enriched in K and Rb,while high field strength elements are ***,light rare earth elements are significantly enriched,showing a slight negative Eu anomaly(Eu/Eu^(*)=0.39 to 0.58).Shenxianshui granite has a relatively high initial Sr isotope ratio(^(87)Sr/^(86)Sr)_(i)(0.7098-0.7105),negative ε_(Nd)(t)values(−7.99 to−7.44)and negative ε_(Hf)(t)values(−8.37 to−2.58).Combined with previous studies,these characteristics suggest that the Shenxianshui alkaline granites were formed in a post-collision extensional *** alkaline granitic magma possibly originated from the partial melting of the lower crust during the Mesoproterozoic era and may have contained mantle source *** alkaline granite was formed from mixed magma with a high degree of crystal *** abundance of ore-forming elements indicates that Shenxianshui granite has the potential to mineralize key metals and rare earth elements.

关键词： I-type granite zircon U-Pb geochronology Sr-Nd-Pb isotopes Hf isotope Gejiu

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α-Synuclein pathology from the body to the brain:so many seeds so close to the central soil

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Neural Regeneration Research 2024年第7期19卷 1463-1472页

作者： Yunying yang Zhentao Zhang Department of Neurology Renmin Hospital of Wuhan UniversityWuhanHubei ProvinceChina TaiKang Center for Life and Medical Sciences Wuhan UniversityWuhanHubei ProvinceChina

α-Synuclein is a protein that mainly exists in the presynaptic *** folding and accumulation of α-synuclein are found in several neurodegenerative diseases,including Parkinson’s *** and highly phospho rylated a-synuclein constitutes the main component of Lewy bodies in the brain,the pathological hallmark of Parkinson s *** decades,much attention has been focused on the accumulation of α-synuclein in the brain parenchyma rather than considering Parkinson s disease as a systemic *** evidence demonstrates that,at least in some patients,the initial α-synuclein pathology originates in the peripheral organs and spreads to the *** of α-synuclein preformed fibrils into the gastrointestinal tra ct trigge rs the gutto-brain propagation of α-synuclein ***,whether α-synuclein pathology can occur spontaneously in peripheral organs independent of exogenous α-synuclein preformed fibrils or pathological α-synuclein leakage from the central nervous system remains under *** this review,we aimed to summarize the role of peripheral α-synuclein pathology in the pathogenesis of Parkinson’s *** also discuss the pathways by which α-synuclein pathology spreads from the body to the brain.

关键词： aggregation autonomic nervous system barrier receptors body fluid circulation in situ generation Parkinson’s disease phosphorylation propagation synucleinopathies α-synuclein α-synuclein fibrils

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Transcriptome Analysis of Heterosis in Survival in the Hybrid Progenies of‘Haida No.1’and Orange-Shelled Lines of the Pacific Oyster Crassostrea gigas

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Journal of Ocean University of China 2024年第1期23卷 199-208页

作者： yang Hang LI Qi Key Laboratory of Mariculture Ministry of EducationOcean University of ChinaQingdao 266003China

Heterosis has been exploited to enhance the yield and adaptability in various shellfish species;however,the molecular basis of it remains *** Pacific oyster Crassostrea gigas is one of the most economically important aquaculture species,and its productive traits can be improved by ***,an intraspecific cross between orange shell(O,10th generation)and‘Haida No.1’(H,13th generation)of *** was performed to assess the heterosis of survival *** rates of hybrid family(OH)and inbred families(HH and OO)were compared at larval stage,and eyed-pediveliger larvae of three families were subjected to transcriptome *** analysis results of best-parent heterosis and mid-parent heterosis showed that the hybrid family exhi-bited a high heterosis in survival relative to the parental *** OH-M(OH ***)and OH-P(OH ***)had 425 and 512 dif-ferentially expressed genes(DEGs),*** enrichment analysis of these DEGs revealed that the significantly enrich-ed genes function in virion binding,C-type lectin receptor signaling pathway,cellular defense response and other immune-related pro-cesses,which involves perlucin-like protein,CD209 antigen-like protein,ZNFX1,caspase-3 and acan *** differentially ex-pressed genes in OH-M and OH-P,together with the immune-related processes mentioned above may play an important role in the larval survival of *** addition,three genes(CYP450,fucolectin and perlucin-like)are associated with the orange shell and low survival of maternal oyster *** findings provide support for the application of hybrid with superior survival and will facilitate the understanding of heterosis formation in the Pacific oyster.

关键词： Crassostrea gigas survival rate heterosis transcriptome

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Offline/online attribute-based searchable encryption scheme from ideal lattices for IoT

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Frontiers of Computer Science 2024年第3期18卷 239-241页

作者： yang yang Guoyin ZHANG Sizhao LI Zechao LIU College of Computer Science and Technology Harbin Engineering UniversityHarbin 150001China

1 Introduction The Internet of Things(IoT)has facilitated the development of numerous fields in our ***,some equipment in IoT environment lacks sufficient storage and data processing capabilities[1].A feasible strateg... 详细信息

关键词： IoT encryption scheme

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A multi-scale second-order autoregressive recursive filter approach for the sea ice concentration analysis

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Acta Oceanologica Sinica 2024年第3期43卷 115-126页

作者： Lu yang Xuefeng Zhang School of Marine Science and Technology Tianjin UniversityTianjin 300072China

To effectively extract multi-scale information from observation data and improve computational efficiency,a multi-scale second-order autoregressive recursive filter(MSRF)method is *** second-order autoregressive filter used in this study has been attempted to replace the traditional first-order recursive filter used in spatial multi-scale recursive filter(SMRF)*** experimental results indicate that the MSRF scheme successfully extracts various scale information resolved by ***,compared with the SMRF scheme,the MSRF scheme improves computational accuracy and efficiency to some *** MSRF scheme can not only propagate to a longer distance without the attenuation of innovation,but also reduce the mean absolute deviation between the reconstructed sea ice concentration results and observations reduced by about 3.2%compared to the SMRF *** the other hand,compared with traditional first-order recursive filters using in the SMRF scheme that multiple filters are executed,the MSRF scheme only needs to perform two filter processes in one iteration,greatly improving filtering *** the two-dimensional experiment of sea ice concentration,the calculation time of the MSRF scheme is only 1/7 of that of SMRF *** means that the MSRF scheme can achieve better performance with less computational cost,which is of great significance for further application in real-time ocean or sea ice data assimilation systems in the future.

关键词： second-order auto-regressive filter multi-scale recursive filter sea ice concentration three-dimensional variational data assimilation

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Effect of Skeleton Grain Size on the Saturation of Gas Hydrate in Natural Sediments

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Journal of Ocean University of China 2024年第3期23卷 676-682页

作者： XU Zhenqiang LI yang College of Marine Sciences Ocean University of ChinaQingdao 266100China China Petroleum&Chemical Corporation Beijing 100728China

Natural gas hydrate is prospected as a new and promising,highly clean energy resource that mainly occurs in perma-frost or at continental *** formation is subject to many soil conditions,such as grain size,matrix materials,pore morphology,and *** this study,we propose that grain size is the most decisive parameter that affects the saturation of gas hydrate in sediments based on data from Ocean Drilling Program Leg 164 and Mallik 5L-38,which represent marine sediments and terrestrial sediments,*** study reveals that high gas hydrate saturation generally occurs in coarse-grained sand,regardless of whether sediment formation is homogeneous or inhomogeneous,and the sorting of sediments may affect the hydrate saturation to a certain *** grain size and sorting of sediments may be the most intuitive proxy method for a rough estimation of hydrate *** study is necessary to fully understand the relationship between hydrate morphology and sediment grain size,even though massive hydrates are typically found in fine clayey-rich sediments.

关键词： grain size saturation gas hydrates ODP Leg 164 Mallik 5L-38

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STRONG CONVERGENCE OF JUMP-ADAPTED IMPLICIT MILSTEIN METHOD FOR A CLASS OF NONLINEAR JUMP-DIFFUSION PROBLEMS

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Journal of Computational Mathematics 2024年第1期42卷 248-270页

作者： Xu yang Weidong Zhao School of Mathematics China University of Mining and TechnologyXuzhou 221116China School of Mathematics Shandong UniversityJinan 250100China

In this paper,we study the strong convergence of a jump-adapted implicit Milstein method for a class of jump-diffusion stochastic differential equations with non-globally Lipschitz drift *** with the regular methods,the jump-adapted methods can significantly reduce the complexity of higher order methods,which makes them easily implementable for scenario ***,due to the fact that jump-adapted time discretization is path dependent and the stepsize is not uniform,this makes the numerical analysis of jump-adapted methods much more involved,especially in the non-globally Lipschitz *** provide a rigorous strong convergence analysis of the considered jump-adapted implicit Milstein method by developing some novel analysis techniques and optimal rate with order one is also successfully *** experiments are carried out to verify the theoretical findings.

关键词： Jump-diffusion Jump-adapted implicit Milstein method Poisson jumps Strong convergence rate Non-Lipschitz coefficients

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