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A simple path to ambient temperature ionic H^(-)superconductors

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Science China Chemistry 2024年第1期67卷 321-322页

作者： Bingru liu Shiyuan liu Jianglan Shui School of Materials Science and Engineering Beihang UniversityBeijing 100191China

Hydride ion(H^(-))has high polarizability(α_(H^(-))=10.17A^(3))and high redox potential(H^(-)/H_(2):-2.3 V),and therefore is an attractive energy carrier[1,2].The H^(-)superconductors play a crucial role in the devel... 详细信息

关键词： attractive ambient superconductors

A combinatorial synthesis method for identification of orally bioavailable cyclic peptide

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Science China Chemistry 2024年第8期67卷 2429-2430页

作者： Zhenzhen liu Li liu Bo Tang College of Chemistry Chemical Engineering and Materials ScienceKey Laboratory of Molecular and Nano ProbesMinistry of EducationCollaborative Innovation Center of Functionalized Probes for Chemical Imaging in Universities of ShandongInstitutes of Biomedical SciencesShandong Normal UniversityJinan 250014China Laoshan Laboratory Qingdao 266237China

Cyclic peptides are a type of polypeptide with macrocyclic structure formed by canonical and non-canonical amino *** to their rigid conformation and large surface area,cyclic peptides typically exhibit high binding affinity and specificity with target proteins,particularly those considered undruggable by traditional small molecule drugs,such as protein-protein interactions[1].Additionally,they are convenient to be chemical modified to improve the pharmacological or pharmacokinetic properties.

关键词： properties. canonical synthesis

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Multi-granularity sequence generation for hierarchical image classification

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Computational Visual Media 2024年第2期10卷 243-260页

作者： Xinda liu Lili Wang State Key Laboratory of Virtual Reality Technology and Systems Beihang UniversityBeijing 100191China Peng Cheng Laboratory Shengzhen 518000China

Hierarchical multi-granularity image classification is a challenging task that aims to tag each given image with multiple granularity labels *** methods tend to overlook that different image regions contribute differently to label prediction at different granularities,and also insufficiently consider relationships between the hierarchical multi-granularity *** introduce a sequence-to-sequence mechanism to overcome these two problems and propose a multi-granularity sequence generation(MGSG)approach for the hierarchical multi-granularity image classification ***,we introduce a transformer architecture to encode the image into visual representation ***,we traverse the taxonomic tree and organize the multi-granularity labels into sequences,and vectorize them and add positional *** proposed multi-granularity sequence generation method builds a decoder that takes visual representation sequences and semantic label embedding as inputs,and outputs the predicted multi-granularity label *** decoder models dependencies and correlations between multi-granularity labels through a masked multi-head self-attention mechanism,and relates visual information to the semantic label information through a crossmodality attention *** this way,the proposed method preserves the relationships between labels at different granularity levels and takes into account the influence of different image regions on labels with different *** on six public benchmarks qualitatively and quantitatively demonstrate the advantages of the proposed *** project is available at https://***/liuxindazz/mgs.

关键词： hierarchical multi-granularity classification vision and text transformer sequence generation fine-grained image recognition cross-modality attenti

Global adaptive output-feedback tracking with prescribed performance for uncertain nonlinear systems

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Science China(Information Sciences) 2024年第5期67卷 150-164页

作者： Yuan WANG Yungang liu School of Control Science and Engineering Shandong University

At present, one typical control strategy for guaranteeing transient and steady-state performance is funnel control and prescribed performance control. The strategy features completely discarding the system nonlinearities, even if they are completely known and available. Such an intrinsic feature requires the controller to produce a larger control effect to eliminate the negative impact caused by the high nonlinearities, leading to a conservative controller. In this paper, we fully take advantage of known information on nonlinearities in control design, instead of completely discarding it as done in funnel control. Particularly, we leverage adaptive techniques(i.e., high-gain dynamic compensation) to deal with unknown system nonlinearities. Meanwhile, we integrate the tools of output feedback, tracking control, and the performance *** such, an adaptive output-feedback scheme is developed for global tracking with spatiotemporal performance specifications: arbitrarily given tracking accuracy and accuracy-ensured time. A simulation example supports the developed approach.

关键词： uncertain nonlinear systems output feedback prescribed performance unknown control direction dynamic high gain global tracking

Reconfigurable optical neural networks with Plug-and-Play metasurfaces

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Opto-Electronic Advances 2024年第7期7卷 1-3页

作者： Yongmin liu Yuxiao Li Department of Mechanical and Industrial Engineering Northeastern UniversityBostonMassachusetts 02115USA Department of Electrical and Computer Engineering Northeastern UniversityBostonMassachusetts 02115USA

In a very recent study,*** Huang and co-workers proposed and demonstrated reconfigurable optical neural networks based on cascaded *** fixing one metasurface and switching the other pluggable metasurfaces,the neural networks,which operate at near-infrared wavelengths,can perform distinct recognition tasks for handwritten digits and fashion *** innovative device opens up an avenue for all-optical,high-speed,low-power,and multifunctional artificial intelligence systems.

关键词： surfaces networks neural

Self-Aligning Multi-Modal Transformer for Oropharyngeal Swab Point Localization

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Tsinghua Science and Technology 2024年第4期29卷 1082-1091页

作者： Tianyu liu Fuchun Sun Department of Computer Science and Technology Tsinghua UniversityBeijing 100083China

The oropharyngeal swabbing is a pre-diagnostic procedure used to test various respiratory diseases, including COVID and Influenza A (H1N1). To improve the testing efficiency of testing, a real-time, accurate, and robust sampling point localization algorithm is needed for robots. However, current solutions rely heavily on visual input, which is not reliable enough for large-scale deployment. The transformer has significantly improved the performance of image-related tasks and challenged the dominance of traditional convolutional neural networks (CNNs) in the image field. Inspired by its success, we propose a novel self-aligning multi-modal transformer (SAMMT) to dynamically attend to different parts of unaligned feature maps, preventing information loss caused by perspective disparity and simplifying overall implementation. Unlike preexisting multi-modal transformers, our attention mechanism works in image space instead of embedding space, rendering the need for the sensor registration process obsolete. To facilitate the multi-modal task, we collected and annotate an oropharynx localization/segmentation dataset by trained medical personnel. This dataset is open-sourced and can be used for future multi-modal research. Our experiments show that our model improves the performance of the localization task by 4.2% compared to the pure visual model, and reduces the pixel-wise error rate of the segmentation task by 16.7% compared to the CNN baseline.

关键词： segmentation localization transformer multi-modal perception robotic perception

Approaching Ultimate Synthesis Reaction Rate of Ni-Rich Layered Cathodes for Lithium-Ion Batteries

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Nano-Micro Letters 2024年第10期16卷 392-402页

作者： Zhedong liu Jingchao Zhang Jiawei Luo Zhaoxin Guo Haoran Jiang Zekun Li Yuhang liu zijing Song Rui liu Wei-Di liu Wenbin Hu Yanan Chen School of Materials Science and Engineering Tianjin UniversityTianjin 300072People's Republic of China School of Materials Science and Engineering Shandong University of Science and TechnologyQingdao 266590People's Republic of China Australian Institute of Bioengineering and Nanotechnology The University of QueenslandSt LuciaQLD 4072Australia

Nickel-rich layered oxide LiNi_(x)Co_(y)MnzO_(2)(NCM,x+y+z=1)is the most promising cathode material for high-energy lithium-ion ***,conventional synthesis methods are limited by the slow heating rate,sluggish reaction dynamics,high energy consumption,and long reaction *** overcome these chal-lenges,we first employed a high-temperature shock(HTS)strategy for fast synthesis of the NCM,and the approaching ultimate reaction rate of solid phase transition is deeply investigated for the first *** the HTS process,ultrafast average reaction rate of phase transition from Ni_(0.6)Co_(0.2)Mn_(0.2)(OH)_(2) to Li-containing oxides is 66.7(%s^(-1)),that is,taking only 1.5 *** ultrahigh heating rate leads to fast reaction kinetics,which induces the rapid phase transition of NCM *** HTS-synthesized nickel-rich layered oxides perform good cycling performances(94%for NCM523,94%for NCM622,and 80%for NCM811 after 200 cycles at 4.3 V).These findings might also assist to pave the way for preparing effectively Ni-rich layered oxides for lithium-ion batteries.

关键词： Nickel-rich layered oxides High-temperature shock Solid reaction kinetics Phase transition Reaction rate

Antibody-modified integrated microfluidic terahertz biosensor for detection of breast cancer biomarkers

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Optoelectronics Letters 2024年第4期20卷 249-256页

作者： liu Jianjun School of Intelligent Engineering Shaoguan UniversityShaoguan 512005China

Breast cancer is the most common malignant tumor in women,which seriously threatens the physical and mental health of women *** existing detection methods have problems,such as large sample consumption,time-consuming sample preparation,expensive equipment,and low *** order to solve these problems,this paper proposes a method for quickly detecting breast cancer using surface-functionalized terahertz metamaterial *** use of PIK3CA-modified sensors enhances the detection sensitivity and specificity of *** on the red shift of the sensor absorption peak caused by exosomes,breast cancer patients can be distinguished from healthy *** study demonstrates that exosome detection is effective for the repeatable and non-invasive diagnosis of breast cancer *** terahertz metamaterial biosensor designed in this paper has high specificity,repeatability,and sensitivity,and has great potential for application in the development of modern diagnostic instruments.

关键词： specificity diagnosis modified

Achieving Negatively Charged Pt Single Atoms on Amorphous Ni(OH)_(2)Nanosheets with Promoted Hydrogen Absorption in Hydrogen Evolution

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Nano-Micro Letters 2024年第10期16卷 213-224页

作者： Yue liu Gui liu Xiangyu Chen Chuang Xue Mingke Sun Yifei liu Jianxin Kang Xiujuan Sun Lin Guo School of Chemistry Beijing Advanced Innovation Center for Biomedical EngineeringKey Laboratory of Bio-inspired Smart Interfacial Science and TechnologyBeihang UniversityBeijing 100191People's Republic of China School of Chemistry Key Laboratory of Environmentally Friendly Chemistry and Applications of Ministry of EducationXiangtan UniversityXiangtan 411105HunanPeople'Republic of China

Single-atom(SA)catalysts with nearly 100%atom utilization have been widely employed in electrolysis for decades,due to the outperforming catalytic activity and ***,most of the reported SA catalysts are fixed through the strong bonding between the dispersed single metallic atoms with nonmetallic atoms of the substrates,which greatly limits the controllable regulation of electrocatalytic activity of SA *** this work,Pt-Ni bonded Pt SA catalyst with adjustable electronic states was successfully constructed through a controllable electrochemical reduction on the coordination unsaturated amorphous Ni(OH)_(2)nanosheet *** on the X-ray absorption fine structure analysis and first-principles calculations,Pt SA was bonded with Ni sites of amorphous Ni(OH)_(2),rather than conventional O sites,resulting in negatively charged Pt^(δ-).In situ Raman spectroscopy revealed that the changed configuration and electronic states greatly enhanced absorbability for activated hydrogen atoms,which were the essential intermediate for alkaline hydrogen evolution *** hydrogen spillover process was revealed from amorphous Ni(OH)_(2)that effectively cleave the H-O-H bond of H_(2)O and produce H atom to the Pt SA sites,leading to a low overpotential of 48 mV in alkaline electrolyte at-1000 mA cm^(-2)mg^(-1)_(Pt),evidently better than commercial Pt/C *** work provided new strategy for the control-lable modulation of the local structure of SA catalysts and the systematic regulation of the electronic states.

关键词： Hydrogen evolution reaction Amorphous Pt single atoms Hydrogen spillover