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Deep Insight of Design,Mechanism,and Cancer Theranostic Strategy of Nanozymes

Nano-Micro Letters 2024年第2期16卷 165-217页

作者： Lu Yang Shuming Dong Shili Gai Dan Yang He Ding Lili Feng Guixin Yang ziaur.rehman Piaoping Yang Key Laboratory of Superlight Materials and Surface Technology Ministry of EducationCollege of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin 150001People’s Republic of China Yantai Research Institute Harbin Engineering UniversityYantai 264000People’s Republic of China Key Laboratory of Green Chemical Engineering and Technology of Heilongjiang Province College of Material Science and Chemical EngineeringHarbin University of Science and TechnologyHarbin 150040People’s Republic of China Department of Chemistry Quaid-i-Azam UniversityIslamabad 45320Pakistan

Since the discovery of enzyme-like activity of Fe3O4 nanoparticles in 2007,nanozymes are becoming the promising substitutes for natural enzymes due to their advantages of high catalytic activity,low cost,mild reaction conditions,good stability,and suitable for large-scale ***,with the cross fusion of nanomedicine and nanocatalysis,nanozyme-based theranostic strategies attract great attention,since the enzymatic reactions can be triggered in the tumor microenvironment to achieve good curative effect with substrate specificity and low side ***,various nanozymes have been developed and used for tumor *** this review,more than 270 research articles are discussed systematically to present progress in the past five ***,the discovery and development of nanozymes are ***,classification and catalytic mechanism of nanozymes are ***,activity prediction and rational design of nanozymes are focused by highlighting the methods of density functional theory,machine learning,biomimetic and chemical ***,synergistic theranostic strategy of nanozymes are ***,current challenges and future prospects of nanozymes used for tumor theranostic are outlined,including selectivity,biosafety,repeatability and stability,in-depth catalytic mechanism,predicting and evaluating activities.

关键词： Nanozymes Classification Prediction and design Catalytic mechanism Tumor theranostics

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Absorbed dose estimations of ^(131)I for critical organs using the GEANT4 Monte Carlo simulation code

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Chinese Physics C 2012年第11期36卷 1150-1156页

作者： ziaur Rahman Shakeel ur rehman Waheed Arshed Nasir M Mirza Abdul Rashid Jahan Zeb Health Physics Division Pakistan Institute of Nuclear Science & TechnologyNiloreIslamabad 45650Pakistan Department of Physics & Applied Mathematics Pakistan Institute of Engineering & Applied SciencesNiloreIslamabad 45650Pakistan

The aim of this study is to compare the absorbed doses of critical organs of 131I using the MIRD （Medical Internal Radiation Dose） with the corresponding predictions made by GEANT4 simulations. S- values （mean absorbed dose rate per unit activity） and energy deposition per decay for critical organs of 131I for various ages, using standard cylindrical phantom comprising water and ICRP soft-tissue material, have also been estimated. In this study the effect of volume reduction of thyroid, during radiation therapy, on the calculation of absorbed dose is also being estimated using GEANT4. Photon specific energy deposition in the other organs of the neck, due to 131I decay in the thyroid organ, has also been estimated. The maximum relative difference of MIRD with the GEANT4 simulated results is 5.64% for an adult＇s critical organs of 131I. Excellent agreement was found between the results of water and ICRP soft tissue using the cylindrical model. S-values are tabulated for critical organs of 131I, using 1, 5, 10, 15 and 18 years （adults） individuals. S-values for a cylindrical thyroid of different sizes, having 3.07% relative differences of GEANT4 with Siegel ＆ Stabin results. Comparison of the experimentally measured values at 0.5 and 1 m away from neck of the ionization chamber with GEANT4 based Monte Carlo simulations results show good agreement. This study shows that GEANT4 code is an important tool for the internal dosimetry calculations.

关键词： mean absorbed dose rate GEANT4 Monte Carlo simulation and 131I critical organs

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局域结构优化Li-Ni-Te-O正极的电化学可逆性（英文）

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中国科学技术大学学报 2019年第4期49卷 259-267页

作者：齐家新王星博苏晓智解晖 rehman ziaur 陶石储旺盛中国科学技术大学国家同步辐射实验室安徽合肥230026 中国科学院上海应用物理研究所上海光源上海201204 常熟理工学院物理与电子工程学院江苏常熟215500

利用固相法合成了一系列化合物Li1+xNi3/4-5/4xTe1/4+1/4xO2(x=0,0.14,0.33,0.46,0.50和0.60).在x=0.33时,发现C2/m晶体结构中存在一种新奇的围绕Ni离子的短程有序P1-like区域,此区域表现出一种松散结合的局域结构以及更快的Li+迁移率,... 详细信息

利用固相法合成了一系列化合物Li1+xNi3/4-5/4xTe1/4+1/4xO2(x=0,0.14,0.33,0.46,0.50和0.60).在x=0.33时,发现C2/m晶体结构中存在一种新奇的围绕Ni离子的短程有序P1-like区域,此区域表现出一种松散结合的局域结构以及更快的Li+迁移率,进而保证了优越的结构和电化学可逆性.通过非原位X射线吸收谱(XAS)、X射线衍射(XRD)、X射线光电子能谱(XPS)和电化学表征研究了材料的性能.证明了这种性能与稳定的短程-长程有序结构以及Ni氧化还原电子对有关.该研究提供了发展高性能富锂正极材料的新思路.

关键词：锂离子电池正极材料局域结构

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