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Chinese Optics Letters 2024年第6期22卷 177-181页

作者： Kailu Wang Haicheng Mei Jingsong Gao liang Xu Hongbing jiang Yi Liu Shanghai Key Laboratory of Modern Optical System University of Shanghai for Science and TechnologyShanghai 200093China State Key Laboratory for Mesoscopic Physics School of PhysicsPeking UniversityBeijing 100871China CAS Center for Excellence in Ultra-intense Laser Science Shanghai 201800China

Coherent optical emission of free induction decay (FID) excited by the multiple-photon resonance has been recently observed in nitrogen ions produced by intense femtosecond laser *** we report that orbit angular momentum (OAM) of the pump laser pulses can be transferred to the much longer pulsed free induction decay emission with the OAM *** was found that when the pump laser frequency approaches the fraction of the 391.4 nm emission (ν_(0)/5),an FID emission is emitted whereas its topological charge was identified to be 5 times of the pump *** to the reduced laser intensity with a vortex pump compared to the conventional Gaussian beam,the resonant pump laser wavelength presents a redshift,and the FID signal is significantly weaker.

关键词： air lasing orbital angular momentum free induction decay femtosecond pulses photoionization

Refractive index sensing based on a twisted nano-kirigami metasurface

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Photonics Research 2024年第2期12卷 218-225页

作者： SHUQI QIAO XIAOCHEN ZHANG QINGHUA liang YANG WANG CHANG-YIN JI XIAOWEI LI LAN jiang SHUAI FENG HONGLIAN GUO JIAFANG LI School of Science Minzu University of ChinaBeijing 100081China Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement(Ministry of Education) Beijing Key Laboratory of Nanophotonics&Ultrafine Optoelectronic Systemsand School of PhysicsBeijing Institute of TechnologyBeijing 100081China Laser Micro/Nano Fabrication Laboratory School of Mechanical EngineeringBeijing Institute of TechnologyBeijing 100081China

Plasmonic sensing technology has attracted considerable attention for high sensitivity due to the ability to effectively localize and manipulate *** this study,we demonstrate a refractive index(RI)sensing scheme based on open-loop twisted meta-molecule arrays using the versatile nano-kirigami *** sensing has the features of a small footprint,flexible control,and simple *** engineering the morphology of meta-molecules or the RI of the ambient medium,the chiral surface lattice resonances can be significantly enhanced,and the wavelength,intensity,and sign of circular dichroism(CD)can be flexibly *** the relation between the wavelength of the CD peak and the RI of the superstrate,the RI sensor achieves a sensitivity of 1133 nm/***,we analyze these chiroptical responses by performing electromagnetic multipolar decomposition and electric field *** study may serve as an ideal platform for applications of RI measurement and provide new insights into the manipulation of chiral light–matter interactions.

关键词： twisted chiral index

O_(2) adsorption on Fe_(3)O_(4) (110) surface and effect of gangue element Al doping: combined study of binding experiment and ab initio molecular dynamics

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Journal of Iron and Steel Research International 2024年第4期31卷 810-827页

作者： Zheng-jian Liu Hui-qing jiang Yao-zu Wang Jian-liang Zhang Hong-mei Qiao An-yang Zheng Fang-yu Guo School of Metallurgical and Ecological Engineering University of Science and Technology BeijingBeijing 100083China School of Intelligence Science and Technology University of Science and Technology BeijingBeijing 100083China Beijing Shougang Co. Ltd.Qian'an 064404HebeiChina Department of Physics National University of Defense TechnologyChangsha 410128HunanChina

At high temperature,the chemical reaction mechanism at the interface of magnetite and the influence mechanism of gangue element Al on the oxidation performance of magnetite are not *** addition,due to the limitation of existing experimental equipment,it is difficult to clarify the interface reaction mechanism in the oxidation process and the influence mechanism of Al on the surface oxidation reaction of Fe_(3)O_(4) at an atomic scale at high *** surface oxidation reaction mechanism of magnetite and the influence mechanism of Al on the oxidation of magnetite were studied by experiments and AIMD(ab initio molecular dynamics).The experimental results show that the existence of Al_(2)O_(3) will reduce the initial oxidation temperature and comprehensive oxidation performance of *** AIMD results show that aluminum can accelerate the interface reaction rate of Fe_(3)O_(4) in the high-temperature oxidation atmosphere,but the strong Al-O binding ability is not conducive to the transfer of O atoms in the oxidation process.

关键词： Ironmaking Magnetite oxidation Interface reaction Adsorption-Gangue aluminum AIMD

SDGSAT-1: Capabilities for Monitoring and Evaluating SDG Indicators

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空间科学学报 2024年第4期44卷 677-686页

作者： GUO Huadong DOU Changyong liang Dong jiang Nijun TANG Yunwei MA Wenyong International Research Center for Big Data for Sustainable Development Beijing 100094 Key Laboratory of Digital Earth Science Aerospace Information Research InstituteChinese Academy of SciencesBeijing 100094 University of Chinese Academy of Sciences Beijing 100049

SDGSAT-1,the world's first science satellite dedicated to assisting the United Nations 2030 Sustainable Development Agenda,has been operational for over two and a half *** provides valuable data to aid in implementing the Sustainable Development Goals *** its Open Science Program,the satellite has maintained consistent operations and delivered free data to scientific and technological users from 88 *** program has produced a wealth of scientific output,with 72 papers,including 28 on data processing methods and 44 on applications for monitoring progress toward SDGs related to sustainable cities,clean energy,life underwater,climate action,and clean water and ***-1 is equipped with three key instruments:a multispectral imager,a thermal infrared spectrometer,and a glimmer imager,which have enabled ground-breaking research in a variety of domains such as water quality analysis,identification of industrial heat sources,assessment of environmental disaster impacts,and detection of forest *** precise measurements and ongoing monitoring made possible by this invaluable data significantly advance our understanding of various environmental *** are essential for making well-informed decisions on a local and global *** its application to academic research,SDGSAT-1 promotes global cooperation and strengthens developing countries'capacity to accomplish their sustainable development *** the satellite continues to gather and distribute data,it plays a pivotal role in developing strategies for environmental protection,disaster management and relief,and resource *** initiatives highlight the satellite's vital role in fostering international collaboration and technical innovation to advance scientific knowledge and promote a sustainable future.

关键词： SDGSAT-1 Earth observation Remote sensing SDGs

Structural Geology and Chronology of Shear Zones along the Shangdan Suture in Qinling Orogenic Belt,China:Implications for Late Mesozoic Intra-Continental Deformation of East Asia

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Journal of Earth Science 2024年第2期35卷 376-393页

作者： Falak Sheir Wei Li Le Zhang Basil Alabowsh Liuqing jiang Li liang Sainan Gao Shair Baz Umar Ashraf State Key Laboratory of Continental Dynamics Department of GeologyNorthwest UniversityXi’an710069China Institute of Geology University of PunjabLahore45590Pakistan

The Shangdan suture zone(SDZ)in the Qinling orogenic belt(QOB)is a key to understanding the East Asia tectonic *** SDZ gives information about convergent processes between the North China Block(NCB)and South China Block(SCB).In the Late Mesozoic,several shear zones evolved along the SDZ boundary that helps us comprehend the collisional deformation between the NCB and SCB,which was neglected in previous *** shear zones play an essential role in the tectonic evolution of the East Asia *** study focuses on the deformation and geochronology of two shear zones distributed along the SDZ,identified in the Shaliangzi and Maanqiao *** shear sense indicators and kinematic vorticity numbers(0.54–0.90)suggest these shear zones have sinistral shear and sub-simple shear deformation *** quartz’s dynamic recrystallization and c-axis fabric analysis in the Maanqiao shear zone(MSZ)revealed that the MSZ experienced deformation under green-schist facies conditions at∼400–500℃.The Shaliangzi shear zone deformed under amphibolite facies at∼500–700℃.The^(40)Ar/^(39)Ar(muscovite-biotite)dating of samples provided a plateau age of 121–123 *** with previously published data,our results concluded that QOB was dominated by compressional tectonics during the Late Early ***,we suggested that the Siberian Block moved back to the south and Lhasa-Qiantang-Indochina Block to the north,which promoted intra-continental compressional tectonics.

关键词： Qinling orogenic belt Shangdan suture zone shear zone Late Mesozoic intra-continental deformation East Asia tectonics

Enabling superior electrochemical performance of NCA cathode in Li_(5.5)PS_(4.5)Cl_(1.5)-based solid-state batteries with a dual-electrolyte layer

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Chinese Chemical Letters 2024年第4期35卷 231-236页

作者： Ziling jiang Shaoqing Chen Chaochao Wei Ziqi Zhang Zhongkai Wu Qiyue Luo liang Ming Long Zhang Chuang Yu School of Chemistry and Chemical Engineering Huazhong University of Science and TechnologyWuhan 430074China State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China Innovation Center for Chemical Sciences College of ChemistryChemical Engineering and Materials ScienceSoochow UniversitySuzhou 215123China College of Physics and Energy Fujian Normal UniversityFuzhou 350117 China

LiNi_(0.8)Co_(0.15)Al_(0.05)O_(2)(NCA) is a promising cathode for sulfide-based solid-state lithium batteries(ASSLBs)profiting from its high specific capacity and voltage plateau, which yielding high energy density. However, the inferior interfacial stability between the bare NCA and sulfides limits its electrochemical performance. Hereien, the dual-electrolyte layer is proposed to mitigate this effect and enhance the battery performances of NCA-based ASSLIBs. The Li_(3)InCl_6 wih high conductivity and excellent electrochemcial stability act both as an ion additives to promote Li-ion diffusion across the interface in the cathode and as a buffer layer between the cathode layer and the solid electrolyte layer to avoid side reactions and improve the interface stability. The corresponding battery exhibits high discharge capacities and superior cyclabilities at both room and elevated temperatures. It exhibits discharge performance of 237.04 and216.07 m Ah/g at 0.1 and 0.5 C, respectively, when cycled at 60 ℃, and sustains 95.9% of the capacity after100 cycles at 0.5 C. The work demonstrates a simple strategy to ensure the superior performances of NCA in sulfide-based ASSLBs.

关键词： LiNi_(0.8)Co_(0.15)Al_(0.05)O_(2) Li_(5.5)PS_(4.5)Cl_(1.5) Double solid electrolyte layer configuration Operating temperatures Electrochemical performances

Revealing the size effect of Fe S2on solid-state battery performances at different operating temperatures

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Chinese Chemical Letters 2024年第6期35卷 189-194页

作者： Chaochao Wei Ru Wang Zhongkai Wu Qiyue Luo Ziling jiang liang Ming Jie Yang Liping Wang Chuang Yu School of Chemistry and Chemical Engineering Huazhong University of Science and TechnologyWuhan 430074China State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China School of Materials and Energy University of Electronic Science and Technology of ChinaChengdu 611731China

FeS_(2) shows significant potential as cathode material for all-solid-state lithium batteries(ASSLBs)due to its high theoretical specific capacity,low cost,and environmental ***,the poor ion/electron conductivity and large volume variation effect of FeS_(2) inhibit its practical ***,the influence of particle size of FeS_(2) on the corresponding sulfide-based solid-state batteries is carefully investigated by tuning FeS_(2) ***,low operating temperature is chosen to mitigate the large volume changes during cycling in the battery.S-FeS_(2) with smaller particle sizes delivers superior electrochemical performances than that of the larger L-FeS_(2) in Li_(5.5)PS_(4.5)Cl_(1.5)-based ASSLBs under different operating temperatures.S-FeS_(2) shows stable discharge capacities during 50 cycles with a current density of 0.1 m A/cm^(2)under -20℃.When the current density rises to 1.0 m A/cm^(2),it delivers an initial discharge capacity of 146.9 m Ah/g and maintains 63% of the capacity after 100 *** work contributes to constructing ASSLBs enables excellent electrochemical performances under extreme operating temperatures.

关键词： FeS_(2) Size effect Li_(5.5)PS_(4.5)Cl_(1.5) electrolytes Operating temperatures Electrochemical performances

Efficient guiding and focusing of intense laser pulse using periodic thin slits

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Matter and Radiation at Extremes 2024年第4期9卷 29-39页

作者： L.Xu T.W.Huang K.jiang C.N.Wu H.Peng P.C.hen R.Li H.B.zhuo C.T.Zhou Shenzhen Key Laboratory of Ultraintense Laser and Advanced Material Technology Center for Intense Laser ApplicationTechnologyand College of Engineering PhysicsShenzhen Technology UniversityShenzhen 518118People’s Republic of China

Slits have been widely used in laser-plasma interactions as plasma optical components for generating high-harmonic light and controlling laser-driven particle ***,we propose and demonstrate that periodic thin slits can be regarded as a new breed of optical elements for efficient focusing and guiding of intense laser *** fundamental physics of intense laser interaction with thin slits is studied,and it is revealed that relativistic effects can lead to enhanced laser focusing far beyond the pure diffractive focusing *** addition,the interaction of an intense laser pulse with periodic thin slits makes it feasible to achieve multifold enhancement in both laser intensity and energy transfer efficiency compared with conventional *** results provide a novel method for manipulating ultra-intense laser pulses and should be of interest for many laser-based applications.

关键词： laser pulse intense

Multiscale engineering of molecular electrocatalysts for the rapid hydrogen evolution reaction

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Nano Research 2024年第7期17卷 6026-6031页

作者： Huan Li Zhan jiang Yubo Yuan Yirong Tang Jie Zao Wentao Zhang Peiyi Han Xun Zhang Bulin Chen Yongye liang Department of Materials Science and Engineering Southern University of Science and TechnologyShenzhen 518055China South China Institute of Environmental Sciences Guangzhou 510655China

Molecular electrocatalysts have demonstrated potential for the hydrogen evolution reaction(HER)due to their well-defined structures and high intrinsic *** rapid production of hydrogen requires molecular electrocatalysts to operate at high current densities,which still presents a *** this work,we demonstrate that molecularly dispersed electrocatalysts of cobalt phthalocyanine anchored on carbon nanotubes(CoPc MDEs)are superior candidates due to the efficient charge transport between the substrate and the active *** intrinsic activity can be enhanced by introducing functional groups on *** facilitate mass transport,di(ethylene glycol)substituted CoPc molecules are further anchored on a threedimensional self-supported electrode(CoPc-DEG MDE@CC),enabling continuous operation for 25 h at−1000 mA/cm^(2)in 1.0 M *** study demonstrates the potential of molecular electrocatalysts for HER and emphasizes the importance of adjusting intrinsic activity,and charge and mass transport capacity for practical molecular electrocatalysts.

关键词： hydrogen evolution reaction cobalt phthalocyanine intrinsic activity mass transport

Tourmaline guiding the electric field and dechlorination pathway of 2,3-dichlorophenol by Desulfitobacterium hafniense

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Journal of Environmental Sciences 2024年第1期135卷 262-273页

作者： Yue Lu Fangyi liang Fanzhi Qin Linrui Zhong Jianhong jiang Qi Liu Shoujuan Zhang Ming Yan Changzheng Fan Haoran Dong College of Environmental Science and Engineering Hunan UniversityChangsha 410082China Shenzhen Research Institute Hunan UniverisyShenzhen 510082China Key Laboratory of Environment Biology and Pollution Control Hunan UniversityMinistry of EducationChangsha 410082China China Machinery International Engineering Design&Research Institute Co. Ltd.Changsha 410007China Hunan Engineering Research Center for Water Treatment Process&Equipment Changsha 410007China

The dehalogenation of organohalides has been a research hotspot in bioremediation field;however,the influence of tourmaline,a natural ore that can generate spontaneous electric field,on organohalide-respiring bacteria(OHRB)and their dechlorination process is not well *** this study,the effect and mechanism of tourmaline on the reductive dechlorination of 2,3-dichlorophenol(2,3-DCP)by Desulfitobacterium hafniense DCB-2Twere *** characterization results confirmed that tourmaline had good stability and the optimal dosage of tourmaline was 2.5 g/L,which shortened the total time required for dechlorination reaction to 72 ***,tourmaline amendment also increased the proportion of 2-chlorophenol(2-CP)from 18%to 30%of end products,while that of 3-CP decreased *** theoretical calculations showed that the bond charge of the orthosubstituted chlorine declined from-0.179 to-0.067,and that of meta-substituted chlorine increased from-0.111 to-0.129,which indicated that the spontaneous electric field of tourmaline affected the charge distribution of 2,3-DCP and was more conducive to the generation of ***,tourmaline with the spontaneous electric field affected the reductive dechlorination pathway of Desulfitobacterium,and the tourmaline-OHRB combining system might serve as a novel strategy for the bioremediation of environments polluted with chlorinated phenols.

关键词： Reductive dechlorination Desulfitobacterium hafniense Tourmaline Electric field 2 3-dichlorophenol