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Mechanistic investigation on the Hg^(0)elimination ability of MnO_(x)-CeO_(x)nanorod adsorbents:effects of Mn/Ce molar ratio

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Waste Disposal and Sustainable Energy 2024年第2期6卷 185-196页

作者： Shujie Gao Xiaoxiang Wang Yaolin Wang kai zhu Changxing Hu Dong Ye College of Quality and Safety Engineering China Jiliang UniversityHangzhou 310018China Key Laboratory of Biomass Chemical Engineering of Ministry of Education Institute of Industrial Ecology and EnvironmentCollege of Chemical and Biological EngineeringZhejiang UniversityHangzhou 310027China Department of Electrical Engineering and Electronics University of LiverpoolLiverpool L693GJUK Ningbo Tech University No.1 Qianhu South RoadNingbo 315100China

Mercury pollution is created by coal combustion processes in multi-component *** injection was identified as a potential strategy for capturing Hg^(0)from waste gases,with adsorbents serving as the primary *** hydro-thermal approach was used to synthesize a series of MnO_(x)-CeO_(x)nanorod adsorbents with varying Mn/Ce molar ratios to maximize the Hg^(0)capture *** CeO,had weak Hg elimination activity;<8%Hg^(0)removal efficiency was obtained from 150℃to 250℃.With the addition of MnOr,the amount of surface acid sites and the relative concentration of Mn4+*** ensured the sufficient adsorption and oxidation of Hg while overcoming the limitations of restricted adsorbate-adsorbent interactions caused by the lower surface area,endowing MnO_(x)-CeO_(x)with increased Hg^(0)removal *** the molar ratio of Mn/Ce reached 6/4,the adsorbent's Hg^(0)removal efficiency remained over 92%at 150℃and 200℃.As the molar ratio of Mn/Ce grew,the adsorbent's Hg^(0)elimination capacity declined due to decreased surface area,weakened acidity,and decreased activity of Mn^(4+);<75%Hg^(0)removal efficiency was reached between 150℃and 250℃for virgin *** the overall Hg'elimination reactions,Mn4+and *** in charge of oxidizing Hg^(0)to Hg^(0),with Ce^(4+)acting as a promoter to aid in the regeneration of Mn^(4+),Because of its limited adaptability to flue gas components,further optimization of the MnO_(x)-CeO_(x)nanorod adsorbent is required.

关键词： Hg^(0)capture MnO_(x)-CeO_(x)nanorods Mn/Ce molar ratio Acid properties Redox behaviors

Pillar effect induced by ultrahigh phosphorous/nitrogen doping enables graphene/MXene film with excellent cycling stability for alkali metal ion storage

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Journal of Energy Chemistry 2024年第6期93卷 146-156,I0004页

作者： Meng Qin Yiwei Yao Junjie Mao Chi Chen kai zhu Guiling Wang Dianxue Cao Jun Yan Key Laboratory of Superlight Materials and Surface Technology Ministry of EducationCollege of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin 150001HeilongjiangChina Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials and Xiamen Institute of Rare Earth MaterialsHaixi InstituteChinese Academy of SciencesXiamen 361021FujianChina

Graphene's large theoretical surface area and high conductivity make it an attractive anode material for potassium-ion batteries(PIBs).However,its practical application is hindered by small interlayer distance and long ion transfer ***,this paper aims to address the issue by introducing MXene through a simple and scalable method for assembling graphene and realizing ultrahigh P doping *** findings reveal that MXene and P-C bonds have a "pillar effect" on the structure of graphene,and the P-C bond plays a primary *** addition,N/P co-doping introduces abundant defects,providing more active sites for K^(+) storage and facilitating K^(+) *** expected,the developed ultrahigh phosphorous/nitrogen co-doped flexible reduced graphene oxide/MXene(NPrGM) electrode exhibits remarkable reversible discharge capacity(554 mA hg^(-1) at 0.05 A g^(-1)),impressive rate capability(178 mA h g^(-1) at 2 A g^(-1)),and robust cyclic stability(0.0005% decay per cycle after 10,000 cycles at 2 A g^(-1)).Furthermore,the assembled activated carbon‖NPrGM potassium-ion hybrid capacitor(PIHC) can deliver an impressive energy density of 131 W h kg^(-1) and stable cycling performance with 98.1% capacitance retention after5000 cycles at 1 A g^(-1).Such a new strategy will effectively promote the practical application of graphene materials in PIBs/PIHCs and open new avenues for the scalable development of flexible films based on two-dimensional materials for potential applications in energy storage,thermal interface,and electromagnetic shielding.

关键词： Graphene MXene Phosphorous doping Pillar effect Potassium-ion batteries

Petroleum pitch derived hard carbon via NaCl-template as anode materials with high rate performance for sodium ion battery

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Frontiers of Chemical Science and Engineering 2024年第7期18卷 1-10页

作者： Baoyu Wu Hao Sun Xiaoxue Li Yinyi Gao Tianzeng Bao Hongbin Wu kai zhu Dianxue Cao Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education College of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin 150001China Hunan Hongshan New Energy Technology Co. LtdYiyang 413000China

Sodium-ion batteries(SIBs)have garnered significant interest in energy storage due to their similar working mechanism to lithium ion batteries and abundant reserves of sodium *** facile synthesis of a carbon-based anode materials with capable electrochemical performance is key to promoting the practical application of *** this work,a combination of petroleum pitch and recyclable sodium chloride is selected as the carbon source and template to obtain hard carbon(HC)anode for *** times and temperatures are optimized by assessing the sodium ion storage behavior of different HC *** optimized HC exhibits a remarkable capacity of over 430 mAh·g^(-1) after undergoing full activation through 500 cycles at a density of current of 0.1 A·g^(-1).Furthermore,it demonstrates an initial discharge capacity of 276 mAh·g^(-1) at a density of current of 0.5 A·g^(-1).Meanwhile,the optimized HC shows a good capacity retention(170 mAh·g^(-1) after 750 cycles)and a remarkable rate ability(166 mAh·g^(-1) at 2 A·g^(-1)).The enhanced capacity is attributed to the suitable degree of graphitization and surface area,which improve the sodium ion transport and storage.

关键词： petroleum pitch hard carbon sodium-ion batteries high rate recyclable template

Depositional process of hyperpycnal flow deposits:A case study on Lower Cretaceous Sangyuan outcrop in the Luanping Basin,Northeast China

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China Geology 2024年第3期7卷 505-516页

作者： De-zhi Yan Ru-kai zhu Hao Shou Zhao-hui Xu Wei-hong Liu Si-cheng zhu Zhi-cheng Lei Jing-ya Zhang Chang Liu Yi Cai Huai-min Xu Research Institute of Petroleum Exploration and Development PetroChinaBeijing 100083China National Energy Tight Oil and Gas R&D Center Beijing 100083China PetroChina Key Laboratory of Oil and Gas Reservoir Beijing 100083China State Key Laboratory of Petroleum Resources and Prospecting China University of Petroleum(Beijing)Beijing 102249China College of Geosciences China University of Petroleum(Beijing)Beijing 102249China Jiangxi Engineering Laboratory on Radioactive Geoscience and Big Data Technology Department of Information and EngineeringEast China University of TechnologyNanchang 330013China

Sedimentary process research is of great significance for understanding the distribution and characteristics of *** the detailed observation and measurement of the Sangyuan outcrop in Luanping Basin,this paper studies the depositional process of the hyperpycnal flow deposits,and divides their depositional process into three phases,namely,acceleration,erosion and *** the acceleration phase,hyperpycnal flow begins to enter the basin nearby,and then speeds up *** developed in the acceleration phase are *** addition,the original deposits become unstable and are taken away by hyperpycnal flows under the eroding *** a result,there are a lot of mixture of red mud pebbles outside the basin and gray mud pebbles within the *** the erosion phase,the reverse deposits are eroded and become thinner or even ***,no reverse grading characteristic is found in the proximal major channel that is closer to the source,but it is still preserved in the middle branch channel that is far from the *** entering the deceleration phase,normally grading deposits appear and cover previous *** final deposits in the basin are *** are reverse,and others are *** are superimposed with each other under the action of hyperpycnal *** analysis of the Sangyuan outcrop demonstrates the sedimentary process and distribution of hyperpycnites,and reasonably explain the sedimentary characteristics of *** is helpful to the prediction of oil and gas exploration targets in gravity flow deposits.

关键词： Hyperpycnal flow Sedimentary characteristics Depositional process Gravity flow deposit Hyperpycnite Red mud pebble Gray mud pebble Oil and gas exploration engineering Luanping Basin

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判定有限自动机可重置的二次多项式下界

华中科技大学学报（自然科学版） 2024年第2期52卷 42-48页

作者：朱凯毛宜军梁早清华南农业大学数学与信息学院广东广州510642 广东省食品质量安全重点实验室广东广州510642

对有限自动机重置判定问题和道路着色问题的时间复杂性下界进行研究,证明了这两个问题的条件下界分别是关于自动机状态数和有向图顶点数的二次多项式.这说明当指数时间猜想(ETH)成立时,两个问题现有的二次算法很大可能就是理论上最好的... 详细信息

对有限自动机重置判定问题和道路着色问题的时间复杂性下界进行研究,证明了这两个问题的条件下界分别是关于自动机状态数和有向图顶点数的二次多项式.这说明当指数时间猜想(ETH)成立时,两个问题现有的二次算法很大可能就是理论上最好的.对于有限自动机重置判定问题,建立从两个有限自动机交问题到它的细粒度归约,利用细粒度归约的传递性,得到其下界是关于状态数的二次多项式;对于道路着色问题,由于求解问题至少与验证问题的解一样难,可将判定某个有限自动机是否可重置看成验证道路着色问题的解,从而得出其下界是关于顶点数的二次多项式.

关键词：自动机重置判定问题道路着色问题细粒度复杂性指数时间猜想两个自动机交

二硫化钼薄膜增强超高强度不锈钢摩擦学及疲劳性能研究

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表面技术 2024年第15期53卷 45-56页

作者：杜娟孙涛朱凯樊小强朱旻昊成都飞机工业(集团)有限责任公司成都610073 西南交通大学材料科学与工程学院成都610031

目的通过表面处理技术提高USS122G不锈钢摩擦学性能及力学性能。方法采用闭合场非平衡磁控溅射技术在USS122G不锈钢表面沉积MoS_(2)薄膜,分别测试了镀MoS_(2)薄膜的USS122G不锈钢力学性能、抗腐蚀性能、弯曲性能、低周疲劳性能及滚动接... 详细信息

目的通过表面处理技术提高USS122G不锈钢摩擦学性能及力学性能。方法采用闭合场非平衡磁控溅射技术在USS122G不锈钢表面沉积MoS_(2)薄膜,分别测试了镀MoS_(2)薄膜的USS122G不锈钢力学性能、抗腐蚀性能、弯曲性能、低周疲劳性能及滚动接触疲劳性能,探索了在干摩擦与石墨烯润滑脂条件下的摩擦学性能,并通过扫描电镜与XRD对MoS_(2)薄膜进行形貌与成分分析。结果成功在USS122G不锈钢表面沉积了MoS_(2)薄膜,镀MoS_(2)薄膜的USS122G不锈钢的纳米硬度为6.8GPa。镀膜后的USS122G不锈钢的阻抗模量为1.06×10^(5)Ω·cm^(2),腐蚀电流密度为1.91×10^(‒6)A/cm^(2)。镀MoS_(2)薄膜的USS122G镀层脱落的最大弯曲力约为3695N。在滚动接触疲劳测试中,镀MoS_(2)试样较未镀膜的USS122G钢的磨痕深度更浅、宽度更窄。MoS_(2)薄膜能有效提升USS122G不锈钢基底的减摩与耐磨性,在干摩擦条件下,与未镀膜的USS122G不锈钢相比,镀MoS_(2)薄膜的USS122G不锈钢的摩擦因数从0.8降低至0.06~0.07,磨损率从1.68×10^(‒5)mm^(3)/(N·m)减少到9.41×10^(‒8) mm^(3)/(N·m)。在脂润滑条件下,USS122G不锈钢的摩擦因数在0.12左右,镀MoS_(2)薄膜后摩擦因数一直稳定在0.103左右。结论镀MoS_(2)薄膜的USS122G较未镀膜的USS122G不仅提升了疲劳性能,还显著改善了摩擦学性能,提高了基底的使用寿命。

关键词：二硫化钼薄膜 USS122G不锈钢润滑脂摩擦学性能

水位波动和植被恢复对三峡水库消落带土壤原核微生物群落结构的交互影响

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环境科学 2024年第5期45卷 2715-2726页

作者：梅渝黄平王鹏朱凯重庆交通大学河海学院重庆400074 中国科学院重庆绿色智能技术研究院重庆400714 中国科学院+大学重庆学院重庆400714

水库消落带是典型的生态脆弱敏感区.水位波动是影响消落带土壤环境的主要因素,植被恢复是消落带土壤保育的重要手段.然而,在水库消落带中,水位波动和植被恢复对土壤微生物群落结构的交互影响尚不清楚.为此,选取三峡水库消落带中不同水... 详细信息

水库消落带是典型的生态脆弱敏感区.水位波动是影响消落带土壤环境的主要因素,植被恢复是消落带土壤保育的重要手段.然而,在水库消落带中,水位波动和植被恢复对土壤微生物群落结构的交互影响尚不清楚.为此,选取三峡水库消落带中不同水位高程的撂荒草地和人工林地为研究对象,利用16S rRNA高通量测序技术探究土壤原核微生物群落组成和多样性,并探讨驱动土壤原核微生物群落结构的主要环境因子.结果表明,消落带的低水位高程中土壤原核微生物α多样性最高,其中163 m高程的Pielou_e指数、Shannon指数和Simpson指数显著高于168 m高程,Chao1指数和Shannon指数显著高于173 m高程.但撂荒草地和人工林地的土壤菌群α多样性并无显著差异.同时,水位波动和植被恢复均对土壤原核微生物的群落组成产生显著影响,不同样地中生物标志物类别具有明显差异.值得注意的是,植被恢复模式差异对土壤原核微生物群落结构的影响强于水位波动.此外,层次分割结果显示土壤pH是三峡水库消落带土壤原核微生物群落结构变化的主要驱动因子.以上结果可深化对水库消落带土壤微生物群落结构的认识,并为水库消落带生态系统的恢复重建提供科学参考.

关键词：水库消落带水位波动植被恢复土壤原核微生物群落结构

RuCo alloy nanoparticles embedded within N-doped porous two-dimensional carbon nanosheets:a high-performance hydrogen evolution reaction catalyst

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Tungsten 2024年第1期6卷 114-123页

作者： Jin-Hui Wang Shao-Wei Yang Fu-Bin Ma Yi-Ke Zhao Shi-Nuo Zhao Zheng-Yu Xiong Dong Cai Hai-Dong Shen kai zhu Qiu-Yu Zhang Yue-Ling Cao Tian-Shuai Wang He-Peng Zhang Research and Development Institute of Northwestern Polytechnical University in Shenzhen Shenzhen 518057China Xi’an Key Laboratory of Functional Organic Porous Materials School of Chemistry and Chemical EngineeringNorthwestern Polytechnical UniversityXi’an 710129China School of Power and Energy Northwestern Polytechnical UniversityXi’an 710129China Chongqing Science and Technology Innovation Center of Northwestern Polytechnical University Chongqing 401135China

Developing cost-effective electrocatalysts with high activity and stability especially at high current density is of great significance for the large-scale commercial application of electrochemical water splitting to hydrogen production but still remains ***,we report an effective confinement pyrolysis strategy to fabricate embedded ruthenium-cobalt nanoclusters supported on N-doped porous two-dimensional carbon nanosheets(RuCo@CN).Markedly,the embedded structure can effectively prevent the migration,agglomeration,and leaching of nanoparticles,thus endowing the RuCo@CN catalyst with high *** be exact,high stability with up to 650 h can be achieved at high current density(-500 and-1000 mA·cm^(-2)).Besides,the RuCo@CN catalysts also exhibit highly reactive with low overpotentials of only 11mV at-10 mA·cm^(-2).Density functional theory calculations reveal that the introduction of cobalt reduces the decomposition barrier of H_(2)O for RuCo@CN alloy,thus promoting hydrogen evolution reaction.

关键词： Hydrogen evolution reaction Confinement pyrolysis strategy Mosaic structure Stability

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基于开源物联网技术的温室环境监测系统设计

农机化研究 2024年第12期46卷 204-207,212页

作者：朱凯李鹏北京开放大学北京100081 北京智芯微电子科技有限公司北京100083

物联网是对传统互联网的拓展与延伸,可将不同信息传感设备与互联网结合,实现“人”、“机”和“环境”之间的信息交互。近年来,物联网在农业生产领域得到了广泛的应用与发展。在农业生产中使用传感器、嵌入式系统和执行器实现对农业环... 详细信息

物联网是对传统互联网的拓展与延伸,可将不同信息传感设备与互联网结合,实现“人”、“机”和“环境”之间的信息交互。近年来,物联网在农业生产领域得到了广泛的应用与发展。在农业生产中使用传感器、嵌入式系统和执行器实现对农业环境信息的采集与通信。数据传输与集合是农业物联网技术的核心,如何实现数据高性能传输与存储是当前农业物联网系统亟待解决的关键问题。为此,提出了一种基于无线传感器网络和物联网开源网关的环境监测系统,允许在AWS上实现可扩展的物联网解决方案,且使用低成本的硬件和基于Linux系统的开源网关平台形成完整的新型物联网系统。通过搭建测试环境对系统运行功能和性能进行测试与分析,结果表明:提出的方案具有良好的功能体验与性能表现。研究结果对于解决农业物联网的发展与数据通信具有一定的推动作用。

关键词：温室环境信息监测物联网嵌入式系统

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