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nitrogen addition promotes soil carbon accumulation globally

Science China Life Sciences 2025年第1期 284-293页

作者： Xuemei Yang Suhui Ma Erhan Huang Danhua Zhang Guoping Chen jiangling zhu Chengjun ji Biao zhu Lingli Liu jingyun Fang Institute of Ecology College of Urban and Environmental Sciencesand Key Laboratory for Earth Surface Processes of the Ministry of EducationPeking University Ministry of Education Key Laboratory for Transboundary Ecosecurity of Southwest China School of Ecology and Environmental ScienceYunnan University State Key Laboratory of Vegetation and Environmental Change Institute of BotanyChinese Academy of Sciences

Soil is the largest carbon(C) reservoir in terrestrial ecosystems and plays a crucial role in regulating the global C cycle and climate *** nitrogen(n) deposition has been widely considered as a critical factor affecting soil organic carbon(SOC) storage, but its effect on SOC components with different stability remains unclear. Here, we analyzed extensive empirical data from 304 sites worldwide to investigate how SOC and its components respond to n addition. Our analysis showed that n addition led to a significant increase in bulk SOC(6.7%), with greater increases in croplands(10.6%) and forests(6.0%) compared to grasslands(2.1%). Regarding SOC components, n addition promoted the accumulation of plant-derived C(9.7%–28.5%) over microbial-derived C(0.2%), as well as labile(5.7%) over recalcitrant components(–1.2%), resulting in a shift towards increased accumulation of plant-derived labile C. Consistently, n addition led to a greater increase in particulate organic C(11.9%) than mineral-associated organic C(3.6%), suggesting that n addition promotes C accumulation across all pools, with more increase in unstable than stable pools. The responses of SOC and its components were best predicted by the n addition rate and net primary productivity. Overall, our findings suggest that n enrichment could promote the accumulation of plant-derived and non-mineral associated C and a subsequent decrease in the overall stability of soil C pool, which underscores the importance of considering the effects of n enrichment on SOC components for a better understanding of C dynamics in soils.

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Defect Engineering with Rational Dopants Modulation for High-Temperature Energy Harvesting in Lead-Free Piezoceramics

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nAnO-MICRO LETTERS 2025年第1期17卷 1-15页

作者： Xi, Kaibiao Guo, jianzhe Zheng, Mupeng zhu, Mankang Hou, Yudong Beijing Univ Technol Coll Mat Sci & Engn Key Lab Adv Funct Mat Minist Educ Beijing 100124 Peoples R China

High temperature piezoelectric energy harvester (HT-PEH) is an important solution to replace chemical battery to achieve independent power supply of HT wireless sensors. However, simultaneously excellent performances, including high figure of merit (FOM), insulation resistivity (rho) and depolarization temperature (T-d) are indispensable but hard to achieve in lead-free piezoceramics, especially operating at 250 degrees C has not been reported before. Herein, well-balanced performances are achieved in BiFeO3-BaTiO3 ceramics via innovative defect engineering with respect to delicate manganese doping. Due to the synergistic effect of enhancing electrostrictive coefficient by polarization configuration optimization, regulating iron ion oxidation state by high valence manganese ion and stabilizing domain orientation by defect dipole, comprehensive excellent electrical performances (T-d = 340 degrees C, rho(250) (degrees C) > 10(7) Omega cm and FOM2(50 degrees C) = 4905 x 10(-15 )m(2) n-1) are realized at the solid solubility limit of manganese ions. The HT-PEHs assembled using the rationally designed piezoceramic can allow for fast charging of commercial electrolytic capacitor at 250 degrees C with high energy conversion efficiency (eta = 11.43%). These characteristics demonstrate that defect engineering tailored BF-BT can satisfy high-end HT-PEHs requirements, paving a new way in developing self-powered wireless sensors working in HT environments.

关键词： Lead-free piezoceramic Defect engineering Dopants modulation High-temperature Piezoelectric energy harvester

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Constructing Donor–Acceptor‑Linked COFs Electrolytes to Regulate Electron Density and Accelerate the Li^(+)Migration in Quasi‑Solid‑State Battery

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nano-Micro Letters 2025年第1期17卷 456-471页

作者： Genfu Zhao Hang Ma Conghui Zhang Yongxin Yang Shuyuan Yu Haiye zhu Yongjiang Sun Hong Guo School of Materials and Energy International Joint Research Center for Advanced Energy Materials of Yunnan ProvinceYunnan UniversityKunming 650091People’s Republic of China Yunnan Yuntianhua Co. LtdR&D CenterKunming 650228People’s Republic of China Southwest United Graduate School Kunming 650091People’s Republic of China

Regulation the electronic density of solid-state electrolyte by donor–acceptor(D–A)system can achieve highly-selective Li^(+)transportation and conduction in solid-state Li metal *** study reports a high-performance solid-state electrolyte thorough D–A-linked covalent organic frameworks(COFs)based on intramolecular charge transfer *** other reported COFbased solid-state electrolyte,the developed concept with D–A-linked COFs not only achieves electronic modulation to promote highly-selective Li^(+)migration and inhibit Li dendrite,but also offers a crucial opportunity to understand the role of electronic density in solid-state Li metal *** introduced strong electronegativity F-based ligand in COF electrolyte results in highlyselective Li^(+)(transference number 0.83),high ionic conductivity(6.7×10^(-4)S cm^(−1)),excellent cyclic ability(1000 h)in Li metal symmetric cell and high-capacity retention in Li/LiFePO_(4)cell(90.8%for 300 cycles at 5C)than substituted C-and n-based *** is ascribed to outstanding D–A interaction between donor porphyrin and acceptor F atoms,which effectively expedites electron transferring from porphyrin to F-based ligand and enhances Li^(+)***,we anticipate that this work creates insight into the strategy for accelerating Li^(+)conduction in high-performance solid-state Li metal batteries through D–A system.

关键词： Electronic modulation engineering Donor-acceptor-linked covalent organic frameworks Quasi-solid-state Li metal battery

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Reduced mesencephalic astrocyte-derived neurotrophic factor expression by mutant androgen receptor contributes to neurodegeneration in a model of spinal and bulbar muscular atrophy pathology

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neural Regeneration Research 2025年第9期20卷 2655-2666页

作者： Yiyang Qin Wenzhen zhu Tingting Guo Yiran Zhang Tingting Xing Peng Yin Shihua Li Xiao-jiang Li Su Yang Guangdong Key Laboratory of non-human Primate Research Key Laboratory of CNS Regeneration(Ministry of Education)Guangdong–HongKong–Macao Institute of CNS RegenerationJinan UniversityGuangzhouGuangdong ProvinceChina

Spinal and bulbar muscular atrophy is a neurodegenerative disease caused by extended CAG trinucleotide repeats in the androgen receptor gene,which encodes a ligand-dependent transcription facto *** mutant androgen receptor protein,characterized by polyglutamine expansion,is prone to misfolding and forms aggregates in both the nucleus and cytoplasm in the brain in spinal and bulbar muscular atrophy *** aggregates alter protein-protein interactions and compromise transcriptional *** this study,we reported that in both cultured n2a cells and mouse brain,mutant androgen receptor with polyglutamine expansion causes reduced expression of mesencephalic astrocyte-de rived neurotrophic *** n of mesencephalic astrocyte-derived neurotrophic factor amelio rated the neurotoxicity of mutant androgen receptor through the inhibition of mutant androgen receptor *** down endogenous mesencephalic astrocyte-derived neurotrophic factor in the mouse brain exacerbated neuronal damage and mutant androgen receptor *** findings suggest that inhibition of mesencephalic astrocyte-derived neurotrophic factor expression by mutant androgen receptor is a potential mechanism underlying neurodegeneration in spinal and bulbar muscular atrophy.

关键词： androgen receptor mesencephalic astrocyte-derived neurotrophic factor mouse model neurodegeneration neuronal loss neurotrophic factor polyglutamine disease protein misfolding spinal and bulbar muscular atrophy transcription factor

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Fabrication of carbon-supported Al2O3 nanoparticles via spontaneous cross-linking to enhance selective hydrogenation of furfural

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journal of Energy Chemistry 2025年第1期100卷 612-620页

作者： Weiwei Yu Xinbao Zhang Hongyu Chen Yanan Wang Shaoguo Li Fucun Chen Zhenni Liu Xiujie Li Xiangxue zhu State Key Laboratory of Catalysis Dalian Institute of Chemical Physics Chinese Academy of Sciences

Selective hydrogenation of furfural to furfuryl alcohol is a great challenge in the hydrogenation field due to thermodynamic preference for hydrogenation of C=C over C=***,a novel Al2O3/C-u hybrid catalyst,composed of n-modified dendritic carbon networks supporting Al2O3nanoparticles,was successfully prepared via carbonizing the freeze-dried gel from spontaneous cross-linking of alginate,Al3+and *** obtained carbon-supported Al2O3hybrid catalyst has a high ratio （31%） of Al species in pentahedral-coordinated *** introduction of urea enhances the surface n content,the ratio of pyrrolic n,and specific surface area of catalyst,leading to improved adsorption capacity of C=O and the accessibility of active *** the furfural hydrogenation reaction with isopropyl alcohol as hydrogen donor,Al2O3/C-u catalyst achieved a 90%conversion of furfural with 98.0% selectivity to furfuryl alcohol,outperforming that of commercial γ-***,Al2O3/C-u demonstrates excellent catalytic stability in the recycling tests attributed to the synergistic effect of abundant weak Lewis acid sites and the anchoring effect of the carbon network on *** work provides an innovative and facile strategy for fabrication of carbon-supported Al2O3hybrid catalysts with rich AlVspecies,serving as a high selective hydrogenation catalyst through MPV reaction route.

关键词： Selective hydrogenation Furfural Furfuryl alcohol Cross-linking MPV route

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Synthesis and Antitumor Activity of 2-[1-(2-Formylamido-3-phenylpropionyloxy)alkyl]-1,4dihydroxy-9,10-anthraquinone Derivatives

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Chemical Research in Chinese Universities 2012年第6期28卷 971-975页

作者： j1n Li-li jIn Guang-zhu College of Pharmacy Yanbian University Yanji 133002 P. R. China

A series of 2-[1-（2-formylamido-3-phenylpropionyloxy）alkyl]-1,4-dihydroxy-9,10-anthraquinone（2FPADHAQ） derivatives was designed and *** antitumor activities were tested against L1210 tumor cells and P388 mouse leukemic tumor cells in vitro and in ICR mice bearing sarcoma 180 cells in ***,the introduction of 2-formylamido-3-phenyl-propanoic acid（2-FPPA） into the C-2-alkyl side chain C＇-1 hydroxy group in 2-（1-hydroxyalkyl）-1,4-dihydroxy-9,10-anthraquinones（2-HDHAQ） enhanced the antitumor activity compared with the starting materials.2-FPADHAQ with alkyl chains longer than the pentyl group had negligible activity,whereas compounds 2b,2c,2d and 2e possessing shorter chains demonstrated moderate cytotoxic activity[50% effective dose（ED 50） of L1210 and P388 are 2.61―4.75 and 5.84―8.74 μg/mL],whereas compound 2l with an aromatic system showed strong cytotoxic activity.T/C（%） values[（average survival days in the test group）/（average survival days in the control group）×100%] also show that the introduction of 2-FPPA into the side chain of 2-HDHAQ enhanced antitumor *** data suggest that the introduction of an amino acid into the starting material may increase its affinity for DnA or its selectivity for proliferating cancer cells.

关键词： Anthraquinone Antitumor Cytotoxicity Phenylalanine

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Buried interface bridging for inverted cesium-formamidinium triiodide perovskite solar cells with long operational stability

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Science China Chemistry 2025年第01期 163-173页

作者： Chenhui Zhang Chunjun Liang Fulin Sun Ting zhu Xinghai Huang Yuzhu Guo Xinyu Guo Kunyang Ge Dan Li Fangtian You Zhiqun He Key Laboratory of Luminescence and Optical Information Ministry of Education Institute of Optoelectronic TechnologyBeijing Jiaotong University Department of Physics School of Physical Science and Engineering Beijing Jiaotong University

In the field of perovskite solar cells(PSCs), the research on defects in the buried interface has been relatively limited due to its non-exposure; however, this interface significantly impacts the performance enhancement of inverted PSCs. This study employs phenylethylammonium chloride(PEACl) molecules as a buffer layer to modify the buried interface of p-i-n structured PSCs,aiming to enhance the uniformity of self-assembled monolayers(Sams) and facilitate the uniform nucleation and growth of perovskite films on the substrate. Furthermore, the introduction of the PEACl buffer layer effectively passivates defects at the bottom of the perovskite layer and notably enhances the crystal quality of the perovskite film by mitigating residual stress,thereby reducing nonradiative recombination loss. Following these optimizations, the MA-free PSCs treated with PEACl achieve a power conversion efficiency(PCE) of 24.11%, with significant improvements in storage, thermal stability, and operational stability. Particularly noteworthy is the device's performance in an unencapsulated state, whereas after 1,500 hours of continuous light operation stability testing, it retains 97% of its original efficiency. This study not only enriches the systematic understanding of the characteristics of the buried interface in PSCs but also contributes significantly to advancing the commercial production of perovskite photovoltaic technology.

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Coercivity Enhancement of nd-Fe-B Thin Film Magnets through Dy Surface Diffusion Process

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journal of Materials Science & Technology 2011年第9期27卷 826-830页

作者： C.Y. You j. zhu n. Tian Z.X. Lu State Key Laboratory for Advanced Metals and Materials University of Science and Technology Beijing Beijing 100083 China School of Materials Science and Engineering Xi＇an University of Technology Xi＇an 710048 China

The Dy capping layer was deposited at different temperatures on the nd-Fe-B thin films to investigate the mechanism of the coercivity enhancement through the Dy surface diffusion. The highest coercivity of 2005 kA/m （25.2 kOe） was obtained at the Dy deposition temperature of 460℃, which was significantly higher than the value of 1297 kA/m （16.3 kOe） without Dy capping layer. By performing the transmission electron microscopy （TEM） analysis, it was found that some of the grain boundaries were enriched with nd element, which could be partly ascribed to the promotion by the Dy surface diffusion. In comparison to the evolution of the spin reorientation temperature of nd2Fe14B phase after the deposition of the Dy capping layer, it is concluded that structural modification plays a significant role in the coercivity enhancement due to the Dy surface diffusion.

关键词： nd-Fe-B thin film Coercivity enhancement Dy layer Microstructure

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Deep learning-based key-block classification framework for discontinuous rock slopes

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journal of Rock Mechanics and Geotechnical Engineering 2022年第4期14卷 1131-1139页

作者： Honghu zhu Mohammad Azarafza Haluk Akgün School of Earth Sciences and Engineering Nanjing UniversityNanjing210023China Department of Civil Engineering Tabriz UniversityTabriz***Iran Department of Geological Engineering Middle East Technical UniversityAnkara06800Turkey

The key-blocks are the main reason accounting for structural failure in discontinuous rock slopes, and automated identification of these block types is critical for evaluating the stability conditions. This paper presents a classification framework to categorize rock blocks based on the principles of block theory. The deep convolutional neural network(Cnn) procedure was utilized to analyze a total of 1240 highresolution images from 130 slope masses at the South Pars Special Zone, Assalouyeh, Southwest *** on Goodman’s theory, a recognition system has been implemented to classify three types of rock blocks, namely, key blocks, trapped blocks, and stable blocks. The proposed prediction model has been validated with the loss function, root mean square error(RMSE), and mean square error(MSE). As a justification of the model, the support vector machine(SVM), random forest(RF), Gaussian naïve Bayes(GnB), multilayer perceptron(MLP), Bernoulli naïve Bayes(BnB), and decision tree(DT) classifiers have been used to evaluate the accuracy, precision, recall, F1-score, and confusion matrix. Accuracy and precision of the proposed model are 0.95 and 0.93, respectively, in comparison with SVM(accuracy = 0.85, precision = 0.85), RF(accuracy = 0.71, precision = 0.71), GnB(accuracy = 0.75,precision = 0.65), MLP(accuracy = 0.88, precision = 0.9), BnB(accuracy = 0.75, precision = 0.69), and DT(accuracy = 0.85, precision = 0.76). In addition, the proposed model reduced the loss function to less than 0.3 and the RMSE and MSE to less than 0.2, which demonstrated a low error rate during processing.

关键词： Block theory Discontinuous rock slope Deep learning Convolutional neural network Image-based classification

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Flow imbalance in MHD flows in splitting ducts with locally different electric conductivities of the walls

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journal of Hydrodynamics 2018年第5期30卷 920-927页

作者： Yang Luo Mengqi zhu C.n.Kim Department of Mechanical Engineering Graduate School Kyung Hee University Department of Mechanical Engineering College of Engineering Kyung Hee University

In this study, three-dimensional liquid-metal magnetohydrodynamic splitting flows in a duct with one inflow channel and two outflow channels with locally different wall electric conductivities（different conductance ratios） are computationally examined. The numerical calculation is achieved with the use of CFX code, with a structured grid system chosen after a series of mesh independence tests. The detailed features of the MHD flows are depicted in a case where the electric conductivities of the two outflow ducts are quite different. Also, the interdependency among the current, fluid velocity, pressure and electric potential is elucidated in order to describe the electromagnetic characteristics of the liquid-metal flows. The result shows that the imbalance of the mass flow rate in the two outflow channels strongly depends on the wall conductivity（i.e., conductance ratio） of each outflow channel.

关键词： Liquid metal flow splitting duct flow imbalance numerical examination conductance ratio

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