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Nitrogen-doped titanium dioxide/schwertmannite nanocomposites as heterogeneous photo-Fenton catalysts with enhanced efficiency for the degradation of bisphenol A

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Journal of Environmental Sciences 2024年第9期143卷 1-11页

作者： Xing-Xing Qiao Yu-Hang Xu Xiang-Ji Liu Sai-Le Chen zhou zhong Ya-Feng Li Jian Lü Fujian Provincial Key Laboratory of Soil Environmental Health and Regulation College of Resources and EnvironmentFujian Agriculture and Forestry UniversityFuzhou 350002China State Key Laboratory of Photocatalysis on Energy and Environment Fuzhou UniversityFuzhou 350116China

Potential health risks related to environmental endocrine disruptors(EEDs)have aroused research hotspots at the forefront of water treatment technologies.Herein,nitrogen-doped titanium dioxide/schwertmannite nanocomposites(N-TiO_(2)/SCH)have been successfully developed as heterogeneous catalysts for the degradation of typical EEDs via photo-Fenton processes.Due to the sustainable Fe(Ⅲ)/Fe(Ⅱ)conversion induced by photoelectrons,as-prepared N-TiO_(2)/SCH nanocomposites exhibit much enhanced efficiency for the degradation of bisphenol A(BPA;ca.100% within 60 min under visible irradiation)in a wide pH range of 3.0-7.8,which is significantly higher than that of the pristine schwertmannite(ca.74.5%)or N-TiO_(2)(ca.10.8%).In this photo-Fenton system,the efficient degradation of BPA is mainly attributed to the oxidation by hydroxyl radical(·OH)and singlet oxygen(^(1)O_(2)).Moreover,the possible catalytic mechanisms and reaction pathway of BPA degradation are systematically investigated based on analytical and photoelectrochemical analyses.This work not only provides a feasible means for the development of novel heterogeneous photo-Fenton catalysts,but also lays a theoretical foundation for the potential application of mineral-based materials in wastewater treatment.

关键词： Titanium dioxide Schwertmannite Fenton reaction Environmental endocrine disruptors Photocatalysis

Reliable calculations of nuclear binding energies by the Gaussian process of machine learning

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Nuclear Science and Techniques 2024年第6期35卷 130-144页

作者： Zi-Yi Yuan Dong Bai Zhen Wang zhong-zhou Ren School of Physics Science and Engineering Tongji UniversityShanghai 200092China College of Science Hohai UniversityNanjing 211100China Key Laboratory of Advanced Micro-Structure Materials Ministry of EducationShanghai 200092China

Reliable calculations of nuclear binding energies are crucial for advancing the research of nuclear physics.Machine learning provides an innovative approach to exploring complex physical problems.In this study,the nuclear binding energies are modeled directly using a machine-learning method called the Gaussian process.First,the binding energies for 2238 nuclei with Z>20 and N>20 are calculated using the Gaussian process in a physically motivated feature space,yielding an average deviation of 0.046 MeV and a standard deviation of 0.066 MeV.The results show the good learning ability of the Gaussian process in the studies of binding energies.Then,the predictive power of the Gaussian process is studied by calculating the binding energies for 108 nuclei newly included in AME2020.The theoretical results are in good agreement with the experimental data,reflecting the good predictive power of the Gaussian process.Moreover,the-decay energies for 1169 nuclei with 50≤Z≤110 are derived from the theoretical binding energies calculated using the Gaussian process.The average deviation and the standard deviation are,respectively,0.047 MeV and 0.070 MeV.Noticeably,the calculated-decay energies for the two new isotopes 204 Ac(Huang et al.Phys Lett B 834,137484(2022))and 207 Th(Yang et al.Phys Rev C 105,L051302(2022))agree well with the latest experimental data.These results demonstrate that the Gaussian pro-cess is reliable for the calculations of nuclear binding energies.Finally,the-decay properties of some unknown actinide nuclei are predicted using the Gaussian process.The predicted results can be useful guides for future research on binding energies and-decay properties.

关键词： Nuclear binding energies decay Machine learning Gaussian process

Multi-soliton solutions, breather-like and bound-state solitons for complex modified Korteweg–de Vries equation in optical fibers

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Chinese Physics B 2024年第6期33卷 119-123页

作者：兰中周 School of Computer Information Management Inner Mongolia University of Finance and EconomicsHohhot 010070China

Under investigation in this paper is a complex modified Korteweg–de Vries(KdV) equation, which describes the propagation of short pulses in optical fibers. Bilinear forms and multi-soliton solutions are obtained through the Hirota method and symbolic computation. Breather-like and bound-state solitons are constructed in which the signs of the imaginary parts of the complex wave numbers and the initial separations of the two parallel solitons are important factors for the interaction patterns. The periodic structures and position-induced phase shift of some solutions are introduced.

关键词： complex modified KdV equation multi-soliton solutions breather-like bound-state

Application of neoadjuvant chemoradiotherapy and neoadjuvant chemotherapy in curative surgery for esophageal cancer:A metaanalysis

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World Journal of Gastrointestinal Oncology 2024年第1期16卷 214-233页

作者： Mao-Xiu Yuan Qi-Gui Cai Zhen-Yang Zhang Jian-zhong zhou Cai-Yun Lan Jiang-Bo Lin The Graduate School Fujian Medical UniversityFuzhou 350000Fujian ProvinceChina Department of Thoracic Surgery Affiliated Hospital of Jinggangshan UniversityJi’an 343000Jiangxi ProvinceChina Department of Thoracic Surgery Fujian Medical University Union HospitalFuzhou 350000Fujian ProvinceChina

BACKGROUND The effectiveness of neoadjuvant therapy in esophageal cancer(EC)treatment is still a subject of debate.AIM To compare the clinical efficacy and toxic side effects between neoadjuvant chemoradiotherapy(nCRT)and neoadjuvant chemotherapy(nCT)for locally advanced EC(LAEC).METHODS A comprehensive search was conducted using multiple databases,including PubMed,EMBASE,MEDLINE,Science Direct,The Cochrane Library,China National Knowledge Infrastructure,Wanfang Database,Chinese Science and Technology Journal Database,and Chinese Biomedical Literature Database Article.Studies up to December 2022 comparing nCRT and nCT in patients with EC were selected.RESULTS The analysis revealed significant differences between nCRT and nCT in terms of disease-free survival.The results indicated that nCRT provided better outcomes in terms of the 3-year overall survival rate(OSR)[odds ratio(OR)=0.95],complete response rate(OR=3.15),and R0 clearance rate(CR)(OR=2.25).However,nCT demonstrated a better 5-year OSR(OR=1.02)than nCRT.Moreover,when compared to nCRT,nCT showed reduced risks of cardiac complications(OR=1.15)and pulmonary complications(OR=1.30).CONCLUSION Overall,both nCRT and nCT were effective in terms of survival outcomes for LAEC.However,nCT exhibited better performance in terms of postoperative complications.

关键词： Esophageal cancer Neoadjuvant chemoradiotherapy Radical resection for esophageal cancer Neoadjuvant chemotherapy Meta-analysis

Three cancers in the renal pelvis,bladder,and colon:A case report

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World Journal of Clinical Cases 2024年第2期12卷 392-398页

作者： Jing Chen Hua-Yan Huang Hui-Chun zhou Lin-Xiao Liu Chuang-Fan Kong Quan zhou Jian-Ming Fei Yuan-Ming Zhu Hu Liu Ye-Chen Tang Cheng-zhong zhou Department of General Surgery The Second Affiliated Hospital of Jiaxing UniversityJiaxing 314000Zhejiang ProvinceChina Department of Pathology The Second Affiliated Hospital of Jiaxing UniversityJiaxing 314000Zhejiang ProvinceChina Department of Medical Imaging The Second Affiliated Hospital of Jiaxing UniversityJiaxing 314000Zhejiang ProvinceChina Department of Urology The Second Affiliated Hospital of Jiaxing UniversityJiaxing 31400Zhejiang ProvinceChina

BACKGROUND Multiple primary cancers are rare occurrences that can involve either metachronous or synchronous development.It is particularly rare for an individual to have more than two primary cancers.In this report,we present a case study of an elderly man who was diagnosed with three heterochronous cancers in the renal pelvis,bladder,and colon.CASE SUMMARY On December 30,2014,a 51-year-old Chinese man was admitted to our hospital with complaints of intermittent painless gross hematuria for the preceding week.A computed tomography(CT)scan revealed wall thickening in the left ureter’s upper segment,while a CT urography revealed a left renal pelvis tumor.A successful laparoscopic radical resection of the left renal pelvis tumor was subsequently performed at Shanghai zhongshan Hospital in January 2015.The pathological findings after the surgery revealed a low-grade papillary urothelial carcinoma of the renal pelvis.The final pathological tumor stage was pT1N0M0.After surgery,this patient received 6 cycles of intravenous chemotherapy with gemcitabine and carboplatin,as well as bladder infusion therapy with gemcitabine.On December 18,2017,the patient was admitted once again to our hospital with a one-day history of painless gross hematuria.A CT scan showed the presence of a space-occupying lesion on the posterior wall of bladder.Cystoscopic examination revealed multiple tumors in the bladder and right cutaneous ureterostomy was performed under general anesthesia on December 29,2017.The postoperative pathological findings disclosed multifocal papillary urothelial carcinoma of the bladder(maximum size 3.7 cm×2.6 cm).The bladder cancer was considered a metastasis of the renal pelvis cancer after surgery.The pathological tumor stage was pT1N0M1.The patient refused chemotherapy after surgery.After another six years,the patient returned on February 28,2023,complaining of periumbilical pain that had lasted six days.This time,a CT scan of the abdomen showed a tumor in the ascending colon,but a subsequent colonoscopy examinat

关键词： Metachronous primary carcinoma Renal pelvis carcinoma Bladder carcinoma Colon carcinoma Case report

Constructing oxygen deficiency-rich V_(2)O_(3)@PEDOT cathode for high-performance aqueous zinc-ion batteries

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Rare Metals 2024年第2期43卷 635-646页

作者： Dong-Fei Sun Zi-Juan Wang Tian Tian Xin Yu Dan-Dan Yu Xiao-zhong zhou Guo-Fu Ma Zi-Qiang Lei Key Laboratory of Eco-functional Polymer Materials of the Ministry of Education Key Laboratory of Eco-environmental Polymer Materials of Gansu ProvinceSchool of College of Chemistry and Chemical EngineeringNorthwest Normal UniversityLanzhou730070China

Aqueous zinc-ion batteries(AZIBs)have attracted widespread attention due to the advantages of high safety and environmental friendliness.Although V_(2)O_(3) is a promising cathode,the strong electrostatic interaction between Zn^(2+) and V_(2)O_(3) crystal,and the sluggish reaction kinetics still limit their application in AZIBs.Herein,the oxygen defects rich V_(2)O_(3) with conducive poly(3,4-ethylenedioxythiophene)(PEDOT)shell(V_(2)O_(3)-Od@PEDOT)was fabricated for AZIBs by combining the sulfur-assisted thermal reduction and in-situ polymerization method.The introduced oxygen vacancies of V_(2)O_(3)–Od@PEDOT weaken the electrostatic interaction between Zn^(2+) and the host material,improving the interfacial electron transport,while the PEDOT coating enhances the structural stability and conductivity of V_(2)O_(3),thus accelerating the reaction kinetics.Based on the advantages,V_(2)O_(3)–Od@PEDOT electrode delivers a reversible capacity of 495 mAh·g^(−1) at 0.1 A·g^(−1),good rate capability(189 mAh·g^(−1)at 8.0 A·g^(−1)),and an impressive cycling stability with 90.1%capacity retention over 1000 cycles at 8.0 A·g^(−1).The strategy may provide a path for exploiting the other materials for high performance AZIBs.

关键词： Oxygen defects V_(2)O_(3) PEDOT Electrochemical self-optimization Aqueous zinc-ion batteries

Pattern-reconfigurable antenna-assisted secret key generation from multipath fading channels

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Frontiers of Information Technology & Electronic Engineering 2023年第12期24卷 1803-1814页

作者： Zheng WAN Mengyao YAN Kaizhi HUANG zhou zhong Xiaoming XU Yajun CHEN Fan WU PLA Strategic Support Force Information Engineering University Zhengzhou450001China Purple Mountain Laboratories for Network and Communication Security Nanjing210096China

Physical layer key generation(PKG)technology leverages reciprocal channel randomness to generate shared secret keys.However,multipath fading at the receiver may degrade the correlation between legitimate uplink and downlink channels,resulting in a low key generation rate(KGR).In this paper,we propose a PKG scheme based on the pattern-reconfigurable antenna(PRA)to boost the secret key capacity.First,we propose a reconfigurable intelligent surface(RIS)based PRA architecture with the capability of flexible and reconfigurable antenna patterns.Then,we present the PRA-based PKG protocol to improve the KGR via mitigation of the effects of multipath fading.Specifically,a novel algorithm for estimation of the multipath channel parameters is proposed based on atomic norm minimization.Thereafter,a novel optimization method for the matching reception of multipath signals is formulated based on the improved binary particle swarm optimization(BPSO)algorithm.Finally,simulation results show that the proposed scheme can resist multipath fading and achieve a high KGR compared to existing schemes.Moreover,our findings indicate that the increased degree of freedom of the antenna patterns can significantly increase the secret key capacity.

关键词： Physical layer security Secret key generation Reconfigurable intelligent surface Multipath fading Pattern-reconfigurable antenna

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数字消费补贴与公平竞争政策

广东社会科学 2024年第1期 27-36页

作者：钟洲蔡跃洲中国社会科学院数量经济与技术经济研究所北京100732

借助数字平台的覆盖范围和数据技术优势发放数字消费补贴,已成为各级政府创新财政政策实施方式、提高补贴发放效率的重要创新举措,也是中国数字平台特有的创新活动。然而,2020年以来各省及各主要城市的实践表明,依托数字平台发放数字消... 详细信息

借助数字平台的覆盖范围和数据技术优势发放数字消费补贴,已成为各级政府创新财政政策实施方式、提高补贴发放效率的重要创新举措,也是中国数字平台特有的创新活动。然而,2020年以来各省及各主要城市的实践表明,依托数字平台发放数字消费补贴很容易产生“对适用商品、商户进行不合理限制”“对发放、核销数字平台进行不合理限制”两类行政性垄断风险,不利于我国统一大市场建设,有必要采取针对性治理措施。应以竞争中性原则指导数字消费补贴政策的出台过程,明确相关适用商品、商户与发放、核销平台的遴选标准,优化公平竞争审查的实施。

关键词：财政补贴消费券公平竞争审查行政性垄断

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论反垄断监测预警制度的建构

经济与管理评论 2024年第3期40卷 59-71页

作者：钟洲李军林中国社会科学院数量经济与技术经济研究所北京100732 中国社会科学院经济大数据与政策评估实验室北京100732 中国人民大学应用经济学院北京100872

党的二十大提出要加强反垄断和反不正当竞争,破除地方保护和行政性垄断,依法规范和引导资本健康发展。为了更好地推进相关工作,对垄断风险进行提前预判、精准防范,有必要在探索中国式现代化的过程中,构建反垄断监测预警制度。我国反垄... 详细信息

党的二十大提出要加强反垄断和反不正当竞争,破除地方保护和行政性垄断,依法规范和引导资本健康发展。为了更好地推进相关工作,对垄断风险进行提前预判、精准防范,有必要在探索中国式现代化的过程中,构建反垄断监测预警制度。我国反垄断监测预警制度应定位为“发现线索、提前预防”,并确定结构性异动监测预警与行为性异动监测预警两个主要方向。在此基础上,探讨了监测预警制度与重点行业竞争状况评估、反垄断执法与行业监管的协同,并选取了若干经济指标,对监测预警模型的构建进行了探索,就互联网等行业进行的实证研究初步验证了监测预警模型的有效性。

关键词：反垄断监测预警制度预警模型平台经济