检索结果-南通市图书馆

Science China Chemistry 2024年第9期67卷 3153-3161页

作者： Yuehua Man An Li Haowei Tang Jianlu Sun Yating Fei Yichen Du Xiaosi zhou School of Chemistry and Materials Science Nanjing Normal UniversityNanjing 210023China

VS_(4) has a unique layered atomic chain structure and has the potential to become a high-performance cathode material of magnesium-ion batteries with a high capacity and long cycle ***,low conductivity and sluggish Mg^(2+)diffusivity during cycling limit its practical application in large-scale energy ***,a cooperative assembly-directed strategy is adopted to synthesize VS_(4) nanorods grown in situ on carbon nanotubes(CNTs/VS_(4)).VS_(4) nanorods are tightly anchored to CNTs through V-O-C interface covalent bonds,and CNTs can enhance the electronic conductivity of the *** addition,the ion insertion reaction using Mg^(2+)and Mg Cl^(+)as carriers reduces the polar barrier for divalent Mg^(2+)ion *** rationally designed architecture promotes ion diffusion and electron transfer,thus facilitating reaction *** cooperative assembly-oriented strategy can endow CNTs/VS_(4) with excellent magnesium storage properties,including a high reversible capacity of 223.2 m Ah g^(-1)at a current density of 50 m A g^(-1),a remarkable discha.ge capacity of 91.8 m Ah g^(-1)even at 2,000 m A g^(-1),and an impressive capacity retention of 85.2% after 1,000 cycles at 500 m A g^(-1).Moreover,this strategy can serve as a general synthetic method for the complexation of VS_(4) with other carbon nanostructures.

关键词： transition metal sulfides carbon nanostructure interfacial covalent bond magnesium-ion batteries cathode

Insight of enriched basalts into the nature and evolution of mantle lithosphere beneath craton margins

在线全文

学校读者我要写书评

暂无评论

Science China Earth Sciences 2024年第10期67卷 3128-3142页

作者： Hong-Kun DAI Jianping ZHENg Qing XIONg Linlin HU Xiang zhou State Key Laboratory of geological Processes and Mineral Resources School of Earth Sciences China University of Geosciences

Refractory lithospheric deep roots are the cornerstone for the prolonged stability of cratons and mantle xenoliths are normally the key targets for study on the evolution of such deep roots. In regions with few mantle xenoliths, the basalts enriched in radiogenic isotopic compositions due to marked lithospheric mantle contribution are crucial to unmask the lithospheric mantle evolution based on a comprehensive study involving petrology, geochemistry and thermodynamic modelling. Here, the Early Cretaceous basalts from the northwest North China Craton with few mantle xenoliths are taken as an example to show the significance of enriched basalts on the study of lithospheric mantle. These basalts are characterized by high silica and alkali contents（SiO2=45.8–59.8 wt.%, K2O+Na2O=4.81–9.88 wt.%）, arc-type trace-element patterns and enriched radiogenic isotope compositions(e.g., εNd=-2.64–-12.88,87Sr/86Sr=0.7063–0.7093). The TiO2and FeO（total） contents are higher than those of natural and experimental melts from refractory mantle peridotite but comparable to those of partial melts of fertile mantle *** high contents of fluid-loving elements（e.g., Rb and Ba） suggest source metasomatism by aqueous fluids. Combined with thermodynamic modelling and regional tectonic history, these enriched basalts likely record simultaneous decompression melting of asthenosphere and low-extent melting of thin and fertile lithospheric mantle fluxed by aqueous fluids from the subducted Paleo-Asian oceanic slab. The newly unmasked lithospheric mantle under the western NCC contrasts with the coeval thick and refractory one supporting the eastern NCC, and highlights that the craton destruction, especially the loss of its ancient refractory mantle root, should take place in a diachronous manner related to the craton-girded subduction episodes. Our study illustrates the potential of enriched basalts to recover the nature and evolution of mantle lithosphere beneath craton margins and associated

关键词： Enriched basalts Lithospheric mantle Northwest North China Craton Tectonic histories Early Cretaceous

同方期刊数据库

Suitability of SDN and MEC to facilitate digital twin communication over LTE-A

在线全文

学校读者我要写书评

暂无评论

Digital Communications and Networks 2024年第2期10卷 347-354页

作者： Hikmat Adhami Mohammad Alja’afreh Mohamed Hoda Jiaqi Zhao Yong zhou Abdulmotaleb El Saddik Mohamed bin Zayed University of Artificial Intelligence Masdar CityAbu DhabiUnited Arab Emirates School of Computer Science and Technology China University of Mining and TechnologyXuzhou221116China School of Electrical Engineering and Computer Science University of OttawaOttawaONK1N 6N5Canada

Haptic is the modality that complements traditional multimedia,i.e.,audiovisual,to evolve the next wave of innovation at which the Internet data stream can be excha.ged to enable remote skills and control *** will require ultra-low latency and ultra-high reliability to evolve the mobile experience into the era of Digital Twin and Tactile *** the 5th generation of mobile networks is not yet widely deployed,Long-Term Evolution(LTE-A)latency remains much higher than the 1 ms requirement for the Tactile Internet and therefore the Digital *** work investigates an interesting solution based on the incorporation of Software-defined networking(SDN)and Multi-access Mobile Edge Computing(MEC)technologies in an LTE-A network,to deliver future multimedia applications over the Tactile Internet while overcoming the QoS *** network scenarios were designed and simulated using Riverbed modeler and the performance was evaluated using several time-related Key Performance Indicators(KPIs)such as throughput,End-2-End(E2E)delay,and *** best scenario possible is clearly the one integrating MEC and SDN approaches,where the overall delay,jitter,and throughput for haptics-attained 2 ms,0.01 ms,and 1000 packets per *** results obtained give clear evidence that the integration of,both SDN and MEC,in LTE-A indicates performance improvement,and fulfills the standard requirements in terms of the above KPIs,for realizing a Digital Twin/Tactile Internet-based system.

关键词： LTE-A 5g Digital twin Tactile Internet KPIs SDN MEC NFV Haptic

Sulphur-template method for facile manufacturing porous silicon electrodes with enhanced electrochemical performance

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Chinese Chemical Letters 2024年第8期35卷 433-436页

作者： Peng zhou Ziang Jiang Yang Li Peng Xiao Feixiang Wu Powder Metallurgy Research Institute School of Metallurgy and EnvironmentCentral South UniversityChangsha 410083China

Sulphur(S)-template method based on conventional slurry-casting method has been developed to pro-duce porous silicon(Si)*** facile fabrication technology is suitable for current production line and expected to be widely applied to various electrode materials under large volume cha.ge during ***,S particles as template agent are mixed with active material Si,carbon conductor and binder forming uniform *** casting and drying,the electrodes are immersed in carbon disul-fide solution to remove S particles rapidly,generating pores in-situ at the original position of S *** analysis shows that the pores inside electrodes are able to shorten lithium ion diffusion paths,reduce normal expansion rate and decrease formation of cracks in the Si electrode(2 mg_(Si)/cm^(2)),demonstrating a reversible capacity of 951 mAh/g at 0.5 A/g after 100 cycles(with a capacity retention of 99.5%)and a capacity of-826 mAh/g at 2 A/g.

关键词： Sulphur-template Porous electrodes Silicon anodes Low volume expansion Lithium-ion batteries

An intermittent lithium deposition model based on CuMnbimetallic MOF derivatives for composite lithium anode with ultrahigh areal capacity and current densities

在线全文

学校读者我要写书评

暂无评论

Nano Research 2024年第4期17卷 2763-2769页

作者： Tao Wei Yanyan zhou Cheng Sun Xingtong guo Shoudong Xu Daifen Chen Yongfu Tang School of Energy and Power Jiangsu University of Science and TechnologyZhenjiang 212003China State Key Laboratory of Metastable Materials Science and Technology(MMST) Hebei Key Laboratory of Applied ChemistryYanshan UniversityQinhuangdao 066004China College of Materials Science and Engineering Taiyuan University of TechnologyTaiyuan 030024China

Recently,three-dimensional(3D)conductive frameworks have been chosen as the host for composite lithium(Li)metal anode because of their exceptional electrical conductivity and remarkable thermal and electrochemical ***,Li tends to accumulate on the top of the 3D frameworks with homogenous lithiophilicity and Li dendrite still *** work firstly designed a bimetallic metal-organic framework(MOF)(CuMn-MOF)derived Cu_(2)O and Mn_(3)O_(4) nanoparticles decorated carbon cloth(CC)substrates(CC@Cu_(2)O/Mn_(3)O_(4))to fabricate a composite Li *** to the synergistic effects of lithiophilic Cu_(2)O and Mn_(3)O_(4),the CC@Cu_(2)O/Mn_(3)O_(4)@Li symmetrical cell can afford a prolonged cycling lifespan(1400 h)under an ultrahigh current density and areal capacity(6 mA·cm^(-2)/6 mAh·cm^(-2)).When coupled with the LiFePO_(4)(LFP)cathode,the LFP||CC@Cu_(2)O/Mn_(3)O_(4)@Li full cell demonstrated a superior performance of 89.7 mAh·g^(-1) even at an extremely high current density(10 C).Furthermore,it can also be matched well with LiNi_(0.5)Co^(0).2Mn_(0.3)O_(2)(NCM523)***,to explain the excellent performances of the CC@Cu_(2)O/Mn_(3)O_(4)@Li composite anode,an intermittent model was also *** study offers a novel model that can enhance our comprehension of the Li deposition behavior and pave the way to attain stable and safe Li metal anodes by employing bimetallic MOF-derived materials to construct 3D frameworks.

关键词： lithium metal anode(LMA) three-dimensional(3D)frameworks intermittent lithiophilic model high areal capacity bimetallic metal-organic frameworks(MOFs)

Targeting the adenosine A2A receptor for neuroprotection and cognitive improvement in traumatic brain injury and Parkinson's disease

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Chinese Journal of Traumatology 2024年第3期27卷 125-133页

作者： Yan Zhao Yuan-guo zhou Jiang-Fan Chen Department of Army Occupational Disease State Key Laboratory of TraumaBurns and Combined InjuryResearch Institute of SurgeryDaping HospitalArmy Medical University.Chongqing400042China The Molecular Neuropharmacology Laboratory and the Eye-Brain Research Center The State Key Laboratory of OphthalmologyOptometry and Vision ScienceWenzhou Medical UniversityWenzhou325035Zhejiang ProvinceChina Oujiang Laboratory(Zhejiang Lab for Regenerative Medicine Vision and Brain Health)Wenzhou325035Zhejiang ProvinceChina

Adenosine exerts its dual functions of homeostasis and neuromodulation in the brain by acting at mainly 2 g-protein coupled receptors,called A1 and A2A *** adenosine A2A receptor(A2AR)antagonists have been clinically pursued for the last 2 decades,leading to final approval of the istradefylline,an A2AR antagonist,for the treatment of OFF-Parkinson's disease(PD)*** approval paves the way to develop novel therapeutic methods for A2AR antagonists to address 2 major unmet medical needs in PD and traumatic brain injury(TBI),namely neuroprotection or improving *** this review,we first consider the evidence for aberrantly increased adenosine signaling in PD and TBI and the sufficiency of the increased A2AR signaling to trigger neurotoxicity and cognitive *** further discuss the increasing preclinical data on the reversal of cognitive deficits in PD and TBI by A2AR antagonists through control of degenerative proteins and synaptotoxicity,and on protection against TBI and PD pathologies by A2AR antagonists through control of ***,we provide the supporting evidence from multiple human prospective epidemiological studies which revealed an inverse relation between the consumption of caffeine and the risk of developing PD and cognitive decline in aging population and Alzheimer's disease ***,the convergence of clinical,epidemiological and experimental evidence supports the validity of A2AR as a new therapeutic target and facilitates the design of A2AR antagonists in clinical trials for disease-modifying and cognitive benefit in PD and TBI patients.

关键词： Receptor,Adenosine A2A Adenosine A2 receptor antagonists Parkinson's disease Brain injuries,traumatic

VSAN:A new visualization method for super-large-scale academic networks

在线全文

学校读者我要写书评

暂无评论

Frontiers of Computer Science 2024年第1期18卷 119-137页

作者： Qi LI Xingli WANg Luoyi FU Xinde CAO Xinbing WANg Jing ZHANg Chenghu zhou Department of Electronic Engineering Shanghai Jiao Tong UniversityShanghai 200240China Department of Computer Science and Engineering Shanghai Jiao Tong UniversityShanghai 200240China School of Environmental Science and Engineering Shanghai Jiao Tong UniversityShanghai 200240China School of Oceanography Shanghai Jiao Tong UniversityShanghai 200240China Institute of geographic Sciences and Natural Resources Research Chinese Academy of SciencesBeijing 100101China

As a carrier of knowledge,papers have been a popular choice since ancient times for documenting everything from major historical events to breakthroughs in science and *** the booming development of science and technology,the number of papers has been growing *** like the fact that Internet of Things(IoT)allows the world to be connected in a flatter way,how will the network formed by massive academic papers look like?Most existing visualization methods can only handle up to hundreds of thousands of node size,which is much smaller than that of academic networks which are usually composed of millions or even more *** this paper,we are thus motivated to break this scale limit and design a new visualization method particularly for super-large-scale academic networks(VSAN).Nodes can represent papers or authors while the edges means the relation(e.g.,citation,coauthorship)between *** order to comprehensively improve the visualization effect,three levels of optimization are taken into account in the whole design of VSAN in a progressive manner,i.e.,bearing scale,loading speed,and effect of layout *** main contributions are two folded:(1)We design an equivalent segmentation layout method that goes beyond the limit encountered by state-of-the-arts,thus ensuring the possibility of visually revealing the correlations of larger-scale academic entities.(2)We further propose a hierarchical slice loading approach that enables users to observe the visualized graphs of the academic network at both macroscopic and microscopic levels,with the ability to quickly zoom between different *** addition,we propose a“jumping between nebula graphs”method that connects the static pages of many academic graphs and helps users to form a more systematic and comprehensive understanding of various academic *** our methods to three academic paper citation datasets in the AceMap database confirms the visualization scalability of VSAN in t

关键词： academic networks large graph visualization graph layout graph loading

Roles of nanoparticles in arsenic mobility and microbial community composition in arsenic-enriched soils

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Journal of Environmental Sciences 2024年第4期138卷 301-311页

作者： Ting Luo Qining Zheng Jie Yu Weihao Liang Yan Sun guixiang Quan Feng zhou School of Environmental Science and Engineering Yancheng Institute of TechnologyYancheng 224051China Jiangsu Provincial Key Laboratory of Coastal Ecology and Pollution Control Yancheng 224051China School ofEnvironment and Civil Engineering Jiangnan UniversityWuxi 214122China

Environmental effects of nano remediation engineering of arsenic(As)pollution need to be *** this study,the roles of Fe_(2)O_(3)and TiO_(2)nanoparticles(NPs)on the microbial mediated As mobilization from As contaminated soil were *** addition of Fe_(2)O_(3)and TiO_(2)NPs restrained As(V)release,and stimulated As(Ⅲ)***(V)concentration decreased by 94% and 93% after Fe_(2)O_(3)addition,and decreased by 89% and 45% after Ti O_(2)addition compared to the Biotic and Biotic+Acetate(amended with sodium acetate)controls,*** maximum values of As(Ⅲ)were 20.5 and 27.1μg/L at 48 d after Fe_(2)O_(3)and TiO_(2)NPs addition,respectively,and were higher than that in Biotic+Acetate control(12.9μg/L).The released As co-precipitated with Fe in soils in the presence of Fe_(2)O_(3)NPs,but adsorbed on TiO_(2)NPs in the presence of TiO_(2)***,the addition of NPs amended with sodium acetate as the electron donor clearly promoted As(V)reduction induced by *** NPs addition cha.ged the relative abundance of soil bacterial community,while Proteobacteria(42.8%-70.4%),Planctomycetes(2.6%-14.3%),and Firmicutes(3.5%-25.4%)were the dominant microorganisms in *** potential As/Fe reducing bacteria were related to Pseudomonas,geobacter,Desulfuromonas,and *** addition of Fe_(2)O_(3)and TiO_(2)NPs induced to the decrease of arr A *** results indicated that the addition of NPs had a negative impact on soil microbial population in a long *** findings offer a relatively comprehensive assessment of Fe_(2)O_(3)and TiO_(2)NPs effects on As mobilization and soil bacterial communities.

关键词： Fe_(2)O_(3)and TiO_(2)nanoparticles Arsenic reduction Mobilization Functional gene Microbial community

Reviewing electrochemical stability of ionic liquids-/deep eutectic solvents-based electrolytes in lithium-ion,lithium-metal and post-lithium-ion batteries for green and safe energy

在线全文

学校读者我要写书评

暂无评论

green Energy & Environment 2024年第6期9卷 966-991页

作者： Yu Chen Shuzi Liu Zixin Bi Zheng Li Fengyi zhou Ruifen Shi Tiancheng Mu Department of Chemistry and Material Science Langfang Normal UniversityNO.100 Aimin West RoadLangfangHebei065000China Department of Chemistry Renmin University of ChinNO.59 Zhongguancun StreetHaidian DistrictBeijing100872China

Sustainable energy is the key issue for the environment protection,human activity and economic *** liquids(ILs)and deep eutectic solvents(DESs)are dogmatically regarded as green and sustainable electrolytes in lithium-ion,lithium-metal(e.g.,lithium-sulphur,lithium-oxygen)and post-lithium-ion(e.g.,sodium-ion,magnesium-ion,and aluminum-ion)*** electrochemical stability of ILs/DESs is one of the prerequisites for green,sustainable and safe energy;while easy electrochemical decomposition of ILs/DESs would be contradictory to the concept of green chemistry by adding the cost,releasing volatile/hazardous by-products and hindering the ***,(1)are ILs/DESs-based electrolytes really electrochemically stable when they are not used in batteries?(2)are ILs/DESs-based electrolytes really electrochemically stable in real batteries?(3)how to design ILs/DESs-based electrolytes with high electrochemical stability for batteries to achieve sustainability and green development?Up to now,there is no summary on this topic,to the best of our ***,we review the effect of chemical structure and non-structural factors on the electrochemical stability of ILs/DESs in simulated *** importantly,electrochemical stability of ILs/DESs in real lithium-ion,lithium-metal and post-lithium-ion batteries is concluded and ***,the strategies to improve the electrochemical stability of ILs/DESs in lithium-ion,lithium-metal and post-lithium-ion batteries are *** review would provide a guide to design ILs/DESs with high electrochemical stability for lithium-ion,lithium-metal and postlithium-ion batteries to achieve sustainable and green energy.

关键词： green solvents Decomposition Sustainable chemistry Lithium-oxygen batteries Lithium-sulphur batteries Sodium-ion batteries

Simultaneous removal of Cd(Ⅱ)and As(Ⅴ)by ferrihydrite-biochar composite:Enhanced effects of As(Ⅴ)on Cd(Ⅱ)adsorption

在线全文

学校读者我要写书评

暂无评论

Journal of Environmental Sciences 2024年第5期139卷 267-280页

作者： Wenjun Zeng Yang Lu Jingyan zhou Jie Zhang Yuanxiao Duan cha.gxun Dong Wencheng Wu College of Sciences Nanjing Agricultural UniversityNanjing 210095China South China Institute of Environmental Sciences Ministry of Ecology and EnvironmentGuangzhou 510655China guangdong Engineering&Technology Research Center for System Control of Livestock and Poultry breeding Pollution Guangzhou 510655China

The coexistence of cadmium(Cd(Ⅱ))and arsenate(As(Ⅴ))pollution has long been an environmental ***,a porous carbonaceous material with tunable functionality,has been used for the remediation of contaminated ***,it is still challenging for the dynamic quantification and mechanistic understanding of the simultaneous sequestration of multi-metals in biochar-engineered environment,especially in the presence of *** this study,ferrihydrite was coprecipitated with biochar to investigate how ferrihydritebiochar composite affects the fate of heavy metals,especially in the coexistence of Cd(Ⅱ)and As(Ⅴ).In the solution system containing both Cd(Ⅱ)and As(Ⅴ),the maximum adsorption capacities of ferrihydrite-biochar composite for Cd(Ⅱ)and As(Ⅴ)reached 82.03μmol/g and 531.53μmol/g,respectively,much higher than those of the pure biochar(26.90μmol/g for Cd(Ⅱ),and 40.24μmol/g for As(Ⅴ))and ferrihydrite(42.26μmol/g for Cd(Ⅱ),and 248.25μmol/g for As(Ⅴ)).Cd(Ⅱ)adsorption increased in the presence of As(Ⅴ),possibly due to the cha.ges in composite surface cha.ge in the presence of As(Ⅴ),and the increased dispersion of ferrihydrite by *** microscopic and mechanistic results showed that Cd(Ⅱ)complexed with both biochar and ferrihydrite,while As(Ⅴ)was mainly complexed by ferrihydrite in the Cd(Ⅱ)and As(Ⅴ)coexistence *** posed vital importance for the co-adsorption of Cd(Ⅱ)and As(Ⅴ).The different distribution patterns revealed by this study help to a deeper understanding of the behaviors of cations and anions in the natural environment.

关键词： Ferrihydrite Biochar Cadmium Arsenate Simultaneous sequestration Binding mechanisms