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克尔凯郭尔与卢卡奇马克思主义哲学观的流变

武汉大学学报（哲学社会科学版） 2025年第1期78卷 77-85页

作者：温权武汉大学马克思主义学院湖北武汉430072

克尔凯郭尔并非卢卡奇偶然提及的学术注脚,而是其理解马克思的背景支援。卢卡奇在不同时期都对克尔凯郭尔作了选择性评述,并将其接受或重构马克思主义哲学的曲折心路历程逐一呈现:通过质疑克尔凯郭尔在人与世界相统一问题上遭遇的“审... 详细信息

克尔凯郭尔并非卢卡奇偶然提及的学术注脚,而是其理解马克思的背景支援。卢卡奇在不同时期都对克尔凯郭尔作了选择性评述,并将其接受或重构马克思主义哲学的曲折心路历程逐一呈现:通过质疑克尔凯郭尔在人与世界相统一问题上遭遇的“审美—伦理”悖论,青年卢卡奇从心灵掘进到阶级意识,将“主体—总体”辩证图式看作马克思的认识论地平,由此创作出《历史与阶级意识》;之后,为回应该书引起的争议,盛年的卢卡奇以批判克尔凯郭尔的非理性主义为契机,尝试清除“主体—总体”辩证图式中残余的主体形而上学痕迹,开始在方法论维度正视生产实践与经济规律间的有机联系;及至晚年,当卢卡奇立足社会存在,抨击克尔凯郭尔有关主体优先性的宗教幻象时,他又把社会性的“自在—自为”运动内嵌于人性的“主体—总体”辩证图式,并根据超然的悟性,默认马克思主义哲学是将经济规律置于从属地位的劳动本体论,再度退回《历史与阶级意识》的主体形而上学谋划。不难看出,在卢卡奇臧否克尔凯郭尔与马克思的“主体—总体”辩证桥段中,当事人对“人之实然性和应然性的现实统一”问题所秉持的龃龉心态暴露无遗。这也恰好说明,卢卡奇一生都徘徊于正统的马克思主义与人道的马克思主义之间。

关键词： “主体—总体”辩证图式克尔凯郭尔卢卡奇《历史与阶级意识》

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无机麦秸碎料板制备及性能

功能材料 2015年第1期46卷 1112-1116页

作者：符彬李新功潘亚鸽郑霞吴义强钟文泉中南林业科技大学长沙410004 连云港保丽森实业有限公司江苏连云港222000

以麦秸碎料和无机胶粘剂为主要原料,通过冷压成型工艺制备无机麦秸碎料板,研究了胶草比及板材密度对板材性能的影响,并通过X射线衍射仪、热重分析仪及扫描电镜等仪器分析了胶草比及板材密度对无机麦秸碎料板性能影响机制。结果表明,胶... 详细信息

以麦秸碎料和无机胶粘剂为主要原料,通过冷压成型工艺制备无机麦秸碎料板,研究了胶草比及板材密度对板材性能的影响,并通过X射线衍射仪、热重分析仪及扫描电镜等仪器分析了胶草比及板材密度对无机麦秸碎料板性能影响机制。结果表明,胶草比增加,麦秸碎料对无机成分水化反应的"隔阻"效应减弱,水化反应速度加快,反应更完全,结晶更完整,胶凝材料生成量增加,板材IB增大,TS减小,MOR和MOE先增大后减小。胶草比增大,麦秸碎料在板材中的分布均匀性增加,界面接合性能变好,界面摩擦阻力增大,板材力学性能变好,热稳定性增加。板材密度增加可以促进并加速无机成分水化反应,胶凝材料生成量增加,板材MOR、MOE及IB增大,而TS减小。密度增大板材密实度增加,无机胶粘剂各晶相颗粒间的相互作用增强,界面摩擦阻力及热运动阻力增大,板材力学性能变好,热稳定性增加。

关键词：无机麦秸碎料板胶草比密度物理力学性能

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Metal-organic frameworks with dinuclear metal centers for synergistically boosting CO2 photoreduction

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Science China Chemistry 2025年第01期 201-208页

作者： Hui-Feng Wang wen-Jie Shi Yu-Xin Yang Bao-Xia Dong Tong-Bu Lu Di-Chang zhong School of Chemistry and Chemical Engineering Yangzhou University Institute for New Energy Materials and Low Carbon Technologies School of Materials Science and Engineering Tianjin University of Technology

Dinuclear metal synergistic catalysis （DMSC） has been proved powerful in boosting CO2reduction,while this has not been achieved in heterogeneous catalysts with long-range order *** this study,we,by introduction of metal catalytic centers into an indium-based metal-organic framework （MOF）,obtained a series of isostructural In-MOFs,including three MOFs with mononuclear metal catalytic center （M-In）,three MOFs with dinuclear homometallic catalytic centers （MM-In）,and three MOFs with dinuclear heterometallic catalytic centers (MM’-In,M/M’=Co（II）,Ni（II）,Zn（II）).It was found that all these MOFs can serve as catalysts for photochemical CO2reduction to *** with M-In,the catalytic activities of MM-In were obviously enhanced,and that of MM’-In was further significantly *** example,the CO yield of Co Zn-In reaches a record value of 12,700μmol g-1h-1,which is 4.0,8.1,9.4,and 18.6-fold higher than that of Co Co-In,Zn Zn-In,Co-In,and Zn-In,***,the catalytic activities of Co Ni-In and Ni Zn-In also show different fold increase than those of corresponding dinuclear homometallic and mononuclear metallic *** results of control experiments and theoretical calculation reveal that the higher catalytic activities of MM-In over M-In can be ascribed to the DMSC effect,and the higher catalytic activity of MM’-In over MM-In can be ascribed to the strengthened DMSC *** work reveals the relationship between DMSC effect and bimetal centers in CO2reduction,which provides new insights into the DMSC and paves a new way to design highly active catalysts for photochemical CO2reduction.

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Stepwise assembly to construct stable copper(I) cluster-based circularly polarized luminescent MOFs

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Science China Chemistry 2025年

作者： Jing-wen Xie Meng-Ting Wang Yan Jin Si Li Jian-Hua Qin Shuang-quan Zang Tomas C.W.Mak College of Chemistry Henan Key Laboratory of Crystalline Molecular Functional Materials Zhengzhou University College of Chemistry and Chemical Engineering Luoyang Normal University Department of Chemistry The Chinese University of Hong Kong

Circularly polarized luminescence （CPL） materials have been extensively studied in recent years owing to their widespread applications in 3D display,optical storage,optical anti-counterfeiting,and biological imaging,***（I） clusters have emerged as a promising candidate for CPL materials,driven by their cost-effectiveness,superior luminescent properties,precise structure,and low ***,the poor environmental stability of copper（I） clusters renders their synthesis and preservation challenging,thereby significantly impeding their ***,we have designed and synthesised a chiral double-coordinated ligand in order to construct copper（I） cluster nodes that can be further *** anticipated,by utilizing stepwise assembly strategy,a Cu4cluster node co-modified by chiral alkynyl ligands and triphenylphosphine was further assembled with Cd2+ions to obtain 2D layers structure,L/*** L/D-Cu4-Cd exhibits excellent stability and optical properties,including bright yellow emission,solvent-responsive luminescence,and CPL activity with a maximum glumup to 2.0×10-3,which shows potential applications in the WLED and *** interestingly,the material also exhibits deflection ability towards different wavelengths of linearly polarized light,showing certain potential in the preparation of circular polarizer.

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挤压系统参数对大豆粕蛋白NSI的影响研究

山东理工大学学报（自然科学版） 2008年第3期22卷 10-13页

作者：钟文泉申德超解铁民山东理工大学轻工与农业工程学院山东淄博255049 东北农业大学食品学院黑龙江哈尔滨150030

用二次正交组合试验设计法研究了挤压机模孔长度、阻流环直径、喂入量、套筒温度等挤压系统参数对大豆粕蛋白NSI的影响规律并得到了大豆粕蛋白NSI值高于50%的最佳挤压系统参数.

关键词：大豆氮溶解指数(NSI) 挤压膨化

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A versatile synthetic strategy towards rare earth based metal-organic frameworks

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Science China Chemistry 2025年

作者： quan Shi Yun-Hao Xu Ming-Hui Chen Peng Zhao wen-Bo Deng Ji Xiong Kai Guo Ya-Qing Feng Bao Zhang School of Chemical Engineering and Technology Tianjin University Tianjin Collaborative Innovation Center of Chemical Science and Engineering Guangdong Laboratory Chemistry & Fine Chemical Industry Jieyang Center

Rare earth metal-organic frameworks (RE-MOFs) have drawn wide attention owing to diverse network structures and various application ***,due to the unpredictable formation of the nodes,it is still challenging to design novel RE-MOFs.A novel versatile strategy was developed employing a RE-acetate complex (RE2(CH3COO)6·4H2O) as a precursor to construct RE-MOFs.2D RE-MOFs (RE-DBP) and 3D RE-MOFs (RE-TCPP) could be obtained by using dicarboxylic porphyrin ligands H2DBP and tetracarboxylic porphyrin ligands H2TCPP,*** RE-MOFs were further synthesized to verify the universality of the *** crystalline RE-MOFs could also be prepared at room temperature via the developed strategy,which could significantly promote large-scale preparation and practical application of *** proof of the concept,the performance of porphyrin-based RE-MOFs was investigated in the photocatalytic cycloaddition of CO2with *** the RE-DBP(Co) MOFs,Tb-DBP(Co) exhibited the best photocatalytic performance,which was also greater than that of the corresponding 3D MOF Tb-TCPP(Co) due to the optimal 2D structure and thus the accelerated photogenerated charge separation and transfer *** work not only provides a novel versatile strategy to design and develop RE-MOFs,but also proposes a promising approach for the potential bulk production of RE-MOFs at room temperature.

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Polarization-encoded neural networks with simplified grating patch

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Science China Technological Sciences 2025年

作者： Chengyan zhong Xiang WANG Lingfei LI Yuanchi CUI Lei XIAO Dawei SONG Junxiong GUO wen HUANG Yufeng GUO Yu LIU College of Integrated Circuit Science and Engineering Nanjing University of Posts and Telecommunications National and Local Joint Engineering Laboratory of RF Integration and Micro-Assembly Technology College of Integrated Circuits Hangzhou Global Scientific and Technological Innovation Centre Zhejiang University Nanjing Mumusili Technology Co. LTD School of Integrated Circuits Tsinghua University Institute of Advanced Study School of Electronic Information and Electrical Engineering Chengdu University State Key Laboratory of Electronic Thin Films and Integrated Devices School of Integrated Circuit Science and EngineeringUniversity of Electronic Science and Technology of China

Optical neural networks (ONNs) offer a promising solution for high-performance, energy-efficient artificial intelligence hardware by leveraging the parallelism and speed of light. However, the large-scale implementation of ONNs remains challenging due to the bulky footprint and complex control of optical synapses. In this work, we propose and simulate a plasmonic polarized synaptic architecture that overcomes the diffraction limit and enables ultra-compact ONNs. By tuning the polarization state of incident light, the optical transmittance through each plasmonic unit can be dynamically adjusted to represent a synaptic weight. Our plasmonic structures, with features as small as 40 nm, operate well below this limit in the visible spectrum (400–750 nm). Compared with diffraction and interference-based circuit designs, our proposed method achieves a substantial reduction in synaptic density by factors of 150000-fold and 1500-fold, respectively. Furthermore, we successfully demonstrate a proof-of-concept plasmonic ONN applied to the Canadian Institute for Advanced Research—10classes (CIFAR-10) dataset using a Visual Geometry Group network with 16 layers (VGG16) model. After training for 80epochs, the network achieves an accuracy of 93%. The polarization-tunable plasmonics paves the way towards scalable ONNs for next-generation artificial intelligence (AI) accelerators and smart sensors.

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Cobalamin-dependent radical S-adenosyl-L-methionine protein functions with a partner to successively methylate tricyclic indole alkaloid for chuangxinmycin maturation and derivatization

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Science China Chemistry 2025年第1期 308-316页

作者： Sili Wang Jiancheng Huang Yanan Du Wei Huang Yufeng Xue Xiaokun Xu Guannan zhong Yuanyuan Shi Bin Hong Xiaoying Bian wen Liu State Key Laboratory of Chemical Biology Shanghai Institute of Organic Chemistry University of Chinese Academy of SciencesChinese Academy of Sciences State Key Laboratory of Microbial Technology Shandong University National Health Commission (NHC) Key Laboratory of Biotechnology for Microbial Drugs Institute of Medicinal BiotechnologyChinese Academy of Medical Science & Peking Union Medical College

Cobalamin(Cbl)-dependent radical S-adenosyl-L-methionine(SAM) proteins constitute the largest collection of the radical SAM superfamily that has hundreds of thousands of individual members. Many of these proteins are involved in the biosynthesis of pharmaceutically important natural products to catalyze chemically demanding reactions. In the biosynthetic pathway of chuangxinmycin(CXM), a unique indole alkaloid antibiotic with potent anti-infective activity, functionalization of the characteristic thiopyrano[4,3,2-cd]indole scaffold by regio-and stereoselective C3-methylation is believed to rely on a Cbl-dependent radical process, which, however, remained to be reconstituted biochemically. We here report the dissection of this enzymatic process, which requires the incorporation of Cxm8, a Cbl-dependent radical SAM protein, with Cxm9, a DUF5825family protein that shares no homology to any proteins of known functions. Cxm8 and Cxm9 function together by forming an unexpected heterodimeric complex that selectively catalyzes C3-methylation of the tricyclic indole-S-hetero ring system in a successive manner, achieving CXM and a recently identified, C3-dimethylated congener. Detailed biochemical characterization,isotope labeling, structural simulation and bioinformatics analysis rationalized the catalysis of the Cxm8/Cxm9 complex and particularly the necessity of the DUF5825 protein for C3-methylase activity. This is the first example that a Cbl-dependent protein acts with a partner to exhibit radical SAM activity.

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Giant Monopole Resonance with Boltzmann-Nordheim-Vlasov Model

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Chinese Physics Letters 1996年第10期13卷 724-726页

作者： wen Wan-xin zhong Ji-quan JIN Gen-ming Institute of Modern Physics Chinese Academy of SciencesLanzhou 730000 CCAST(World Laboratory) P.O.Box 8730Beijing 100080

The Boltzmann-Nordheim-Vlasov (BNV) model was employed to investigate the giant monopole resonance (GMR) built on very excited residula nuclei formed in heavy-ion collisions. Roughly speaking the GMR energy of BNV model is very similar to the value given by the empirical formual EGMR = 31.2A^(-l/3) + 20.6A^(-l/6) and hardly changes with impact parameter and bombarding energy.

关键词： energy. excited Boltzmann