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Enhancing multifunctional photocatalysis with acetate-assisted cesium doping and unlocking the potential of Z-scheme solar water splitting

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Carbon Energy 2024年第3期6卷 178-195页

作者： Mengmeng Ma Jingzhen Li Xiaogang Zhu Kong Liu Kaige Huang Guodong Yuan Shizhong Yue zhijie wang Shengchun Qu Key Laboratory of Semiconductor Materials Science Beijing Key Laboratory of Low Dimensional Semiconductor Materials and DevicesInstitute of SemiconductorsChinese Academy of SciencesBeijingChina Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijingChina Department of Physics College of Physical Science and TechnologyXiamen UniversityXiamenChina State Key Laboratory for Superlattices and Microstructures Institute of SemiconductorsChinese Academy of SciencesBeijingChina

Graphitic carbon nitride(g-C_(3)N_(4))has been extensively doped with alkali metals to enlarge photocatalytic output,in which cesium(Cs)doping is predicted to be the most efficient.Nevertheless,the sluggish diffusion and doping kinetics of precursors with high melting points,along with imprecise regulation,have raised the debate on whether Cs doping could make sense.For this matter,we attempt to confirm the positive effects of Cs doping on multifunctional photocatalysis by first using cesium acetate with the character of easy manipulation.The optimized Csdoped g-C_(3)N_(4)(CCN)shows a 41.6-fold increase in visible-light-driven hydrogen evolution reaction(HER)compared to pure g-C_(3)N_(4) and impressive degradation capability,especially with 77%refractory tetracycline and almost 100%rhodamine B degradedwithin an hour.The penetration ofCs+is demonstrated to be a mode of interlayer doping,and Cs–N bonds(especially with sp^(2) pyridine N in C═N–C),along with robust chemical interaction and electron exchange,are fabricated.This atomic configuration triggers the broadened spectral response,the improved charge migration,and the activated photocatalytic capacity.Furthermore,we evaluate the CCN/cadmium sulfide hybrid as a Z-scheme configuration,promoting the visible HER yield to 9.02 mmol g^(−1) h^(−1),which is the highest ever reported among all CCN systems.This work adds to the rapidly expanding field of manipulation strategies and supports further development of mediating served for photocatalysis.

关键词： acetate-assisted cesium doping multifunctional photocatalysis Z-scheme

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Amplified internal electric field of Cs_(2)CuBr_(4)@WO_(3-x)S-scheme heterojunction for efficient CO_(2)photoreduction

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Journal of Energy Chemistry 2024年第5期92卷 521-533页

作者： zhijie Zhang Xuesheng wang Junyi Qian Jiayue Xu School of Materials Science and Engineering Shanghai Institute of TechnologyShanghai 201418China

Heterojunction construction,especially S-scheme heterojunction,represents an efficient universal strategy to achieve high-performance photocatalytic materials.For further performance stimulation of these well-designed heterojunctions,modulating the interfacial internal electric field(IEF)to steer dynamic charge transfer represents a promising approach.Herein,we realized the precise regulation of Fermi level(E_(F))of the oxidation semiconductor(mesoporous WO_(3-x))by tailoring the concentration of oxygen vacancies(V_(O)),maximizing the IEF intensity in Cs_(2)CuBr_(4)@WO_(3-x)(CCB@WO_(3-x))S-scheme heterojunction.The augmented IEF affords a robust driving force for directional electron delivery,leading to boosted charge separation.Hence,the developed CCB@WO_(3-x)S-scheme heterojunction demonstrated outstanding photocatalytic CO_(2)reduction performance,with the electron consumption rate(Relectron)up to 390.34μmol g^(-1)h^(-1),which is 3.28 folds higher than that of pure CCB.An in-depth analysis of the S-scheme electron transfer mode was presented via theoretical investigations,electron spin resonance(ESR),photo-irradiated Kelvin probe force microscopy(KPFM),and in-situ X-ray photoelectron spectroscopy(XPS).Finally,the CO_(2)photoconversion route was explored in detail using in-situ diffuse reflectance infrared Fourier transform spectroscopy(DRIFTS)and DFT theoretical calculations.

关键词： Cs_(2)CuBr_(4) WO_(3-x) Oxygen vacancy S-scheme heterojunction Internal electricfield

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Research on Flexible Job Shop Scheduling Based on Improved Two-Layer Optimization Algorithm

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Computers, Materials & Continua 2024年第1期78卷 811-843页

作者： Qinhui Liu Laizheng Zhu zhijie Gao Jilong wang Jiang Li College of Mechanical and Electrical Engineering Harbin Engineering UniversityHarbin150001China

To improve the productivity,the resource utilization and reduce the production cost of flexible job shops,this paper designs an improved two-layer optimization algorithm for the dual-resource scheduling optimization problem of flexible job shop considering workpiece batching.Firstly,a mathematical model is established to minimize the maximum completion time.Secondly,an improved two-layer optimization algorithm is designed:the outer layer algorithm uses an improved PSO(Particle Swarm Optimization)to solve the workpiece batching problem,and the inner layer algorithm uses an improved GA(Genetic Algorithm)to solve the dual-resource scheduling problem.Then,a rescheduling method is designed to solve the task disturbance problem,represented by machine failures,occurring in the workshop production process.Finally,the superiority and effectiveness of the improved two-layer optimization algorithm are verified by two typical cases.The case results show that the improved two-layer optimization algorithm increases the average productivity by 7.44% compared to the ordinary two-layer optimization algorithm.By setting the different numbers of AGVs(Automated Guided Vehicles)and analyzing the impact on the production cycle of the whole order,this paper uses two indicators,the maximum completion time decreasing rate and the average AGV load time,to obtain the optimal number of AGVs,which saves the cost of production while ensuring the production efficiency.This research combines the solved problem with the real production process,which improves the productivity and reduces the production cost of the flexible job shop,and provides new ideas for the subsequent research.

关键词： Dual resource scheduling workpiece batching rescheduling particle swarm optimization genetic algorithm

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Defect spinel oxides for electrocatalytic reduction reactions

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Nano Research 2024年第5期17卷 3547-3570页

作者： Zhijuan Liu Jinyu Guo Lu-yu Liu Fen wang zhijie Kong Yanyong wang Henan Key Laboratory of Crystalline Molecular Functional Materials Henan International Joint Laboratory of Tumor Theranostical Cluster MaterialsKey Laboratory of Special Environmental Functional Materials(Zhengzhou University)Ministry of EducationGreen Catalysis Centerand College of ChemistryZhengzhou UniversityZhengzhou 450001China State Key Laboratory of Chem/Bio-sensing and Chemometrics College of Chemistry and Chemical EngineeringHunan UniversityChangsha 410082China

Electrocatalytic reduction reactions play a crucial role in electrochemical energy conversion and storage technology,which are emerging technologies to ameliorate environmental problems.Spinel oxides are widely explored in electrocatalytic oxidation reactions but have a poor intrinsic ability to reduction reactions,making their electrocatalytic ability less effective.To improve this,defect engineering is a valuable method for regulating the electronic structure and coordination environment.Herein,this manuscript discusses the use of defect spinel oxides in electrocatalytic reduction reactions,including the different types of defects,construction methods,and characterization techniques.It also outlines the various applications of defect spinel oxides in different electrocatalytic reduction reactions.Finally,it goes over the challenges and future outlooks for defect spinels.This review aims to thoroughly explain how defect spinels work in electrocatalytic reduction reactions and serve as a helpful guide for creating effective electrocatalysts.

关键词： defect spinel oxides electrochemical reduction reactions electrocatalytic mechanism dynamic evolution

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Characterizing the behavior of surge-type glaciers in the Puruogangri Ice Field, Tibetan Plateau

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Journal of Geographical Sciences 2024年第6期34卷 1174-1194页

作者： ZHOU Sugang wang Ninglian LI zhijie YAO Xiaojun ZHANG Yuje QIN Gexia Shaanxi Key Laboratory of Earth Surface System and Environmental Carrying Capacity College of Urban and Environmental SciencesNorthwest UniversityXi'an 710127China Institute of Earth Surface System and Hazards College of Urban and Environmental SciencesNorthwest UniversityXi'an 710127China College of Geography and Environmental Science Northwest Normal UniversityLanzhou 730070China

The Puruogangri Ice Field(PIF), classified as an ultra-continental glacier, is considered extremely stable. However, several glaciers in this area have recently experienced surge events with significant instability and information on surge-type glaciers(STGs) in this region remains scarce. In this study, we identified six STGs and reported the observed characteristics of their surging behavior in the region by mapping glacier boundaries, surface flow velocity information, and glacier surface elevation changes using recent Landsat satellite imagery and shuttle radar topography mission(SRTM), TanDEM, and ASTER digital elevation model(AST14DEM) data. These data provide valuable insights into recent glacial processes, flow instability, and rapid glacial movement. During the active phase of the glaciers,all exhibited frontal advances and changes in surface elevation. Owing to limitations in the satellite imagery, flow velocity profiles were only available for glaciers N1(G089071E33998N),NE1(G089128E33943N), and SE3(G089278E33913N) during the active phase. However,these results effectively reflect the velocity variations in both glaciers before, during, and after the surge. Based on the characteristics of the STG, scientific expeditions, and meteorological data, we believe that the surge in PIF was largely influenced by glacier meltwater and changes in subglacial drainage systems.

关键词： glacier surge glacier surface elevation changes glacier surface velocity Puruogangri Ice Field

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Dissociation of singlet excitons dominates photocurrent improvement in high-efficiency non-fullerene organic solar cells

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Nano Research Energy 2024年第1期3卷 30-37页

作者： Qicong Li Shizhong Yue Zhitao Huang Chao Li Jiaqian Sun Keqian Dong zhijie wang Kong Liu Shengchun Qu Yong Lei Key Laboratory of Semiconductor Materials Science Beijing Key Laboratory of Low Dimensional Semiconductor Materials and DevicesInstitute of SemiconductorsChinese Academy of SciencesBeijing 100083China China Electronics Standardization Institution Beijing 100007China Fachgebiet Angewandte Nanophysik Institut für Physik&IMN MacroNanoTechnische Universität IlmenauIlmenau 98693Germany

In organic solar cells,the singlet and triplet excitons dissociate into free charge carriers with different mechanisms due to their opposite spin state.Therefore,the ratio of the singlet and triplet excitons directly affects the photocurrent.Many methods were used to optimize the performance of the low-efficiency solar cell by improving the ratio of triplet excitons,which shows a long diffusion length.Here we observed that in high-efficiency systems,the proportion of singlet excitons under linearly polarized light excitation is higher than that of circularly polarized light.Since the singlet charge transfer state has lower binding energy than the triplet state,it makes a significant contribution to the charge carrier generation and enhancement of the photocurrent.Further,the positive magnetic field effect reflects that singlet excitons dissociation plays a major role in the photocurrent,which is opposite to the case of low-efficiency devices where triplet excitons dominate the photocurrent.

关键词： polarized light organic solar cell high efficiency singlet/triplet exciton

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Identification, pathogenicity, and fungicide sensitivity of Eutiarosporella dactylidis associated with leaf blight on maize in China

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Journal of Integrative Agriculture 2024年第3期23卷 888-900页

作者： Cheng Guo Xiaojie Zhang Baobao wang Zhihuan Yang Jiping Li Shengjun Xu Chunming wang zhijie Guo Tianwang Zhou Liu Hong Xiaoming wang Canxing Duan Institute of Plant Protection Gansu Academy of Agricultural SciencesLanzhou 730070China Pratacultural College Gansu Agricultural UniversityLanzhou 730070China Shijiazhuang Academy of Agriculture and Forestry Sciences Shijiazhuang 050050China Institute of Crop Sciences Chinese Academy of Agricultural SciencesBejing 100081China

Maize(Zea mays L.) is an economically vital grain crop that is cultivated worldwide. In 2011, a maize foliar disease was detected in Lingtai and Lintao counties in Gansu Province, China. The characteristic signs and symptoms of this disease include irregular chlorotic lesions on the tips and edges of infected leaves and black punctate fruiting bodies in dead leaf tissues. Given favourable environmental conditions, this disease spread to areas surrounding Gansu. In this study, infected leaves were collected from Gansu and Ningxia Hui Autonomous Region between 2018and 2020 to identify the disease-causing pathogen. Based on morphological features, pathogenicity tests, and multilocus phylogenetic analysis involving internal transcribed spacer(ITS), 18S small subunit rDNA(SSU), 28S large subunit rDNA(LSU), translation elongation factor 1-alpha(TEF), and β-tubulin(TUB) sequences, Eutiarosporella dactylidis was identified as the causative pathogen of this newly discovered leaf blight. Furthermore, an in vitro bioassay was conducted on representative strains using six fungicides, and both fludioxonil and carbendazim were found to significantly inhibit the mycelial growth of E. dactylidis. The results of this study provide a reference for the detection and management of Eutiarosporella leaf blight.

关键词： maize leaf blight morphology molecular phylogeny Eutiarosporella dactylidis fungicide sensitivity

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Stability of Rotation Relations of Three Unitaries with the Flip Action in C^(*)-Algebras

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Chinese Annals of Mathematics,Series B 2023年第4期44卷 577-598页

作者： zhijie wang Junyun HU Jiajie HUA College of Data Science Jiaxing UniversityJiaxing 314001ZhejiangChina

The authors show that ifΘ=(θ_(jk))is a 3×3 totally irrational real skewsymmetric matrix,whereθ_(jk)∈[0,1)for j,k=1,2,3,then for anyε>0,there existsδ>0 satisfying the following:For any unital C^(*)-algebra A with the cancellation property,strict comparison and nonempty tracial state space,any four unitaries u1,u2,u3,w∈A such that(1)■,wujw-1=uj-1,w2=1A for j,k=1,2,3;(2)τ(aw)=0 and■for all n∈N,all a∈C^(*)(u1,u2,u3),j,k=1,2,3 and all tracial statesτon A,where C^(*)(u1,u2,u3)is the C^(*)-subalgebra generated by u1,u2 and u3,there exists a 4-tuple of unitaries■in A such that■and■for j,k=1,2,3.The above conclusion is also called that the rotation relations of three unitaries with the flip action is stable under the above conditions.

关键词： C*-Algebras Stability Rotation relation Unitary Flip action

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Stress and Strain in Perovskite/Silicon Tandem Solar Cells

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Nano-Micro Letters 2023年第4期15卷 272-276页

作者： Kong Liu zhijie wang Shengchun Qu Liming Ding Key Laboratory of Semiconductor Materials Science(CAS) Beijing Key Laboratory of Low Dimensional Semiconductor Materials and DevicesInstitute of SemiconductorsChinese Academy of SciencesBeijing 100083People’s Republic of China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049People’s Republic of China Center for Excellence in Nanoscience(CAS) Key Laboratory of Nanosystem and Hierarchical Fabrication(CAS)National Center for Nanoscience and TechnologyBeijing 100190People’s Republic of China

Tandem solar cells based on metal halide perovskites are advancing rapidly during last few years[1–17].The certified power conversion efficiency(PCE)for monolithic perovskite/silicon tandem solar cell reaches 32.5%[18].Since tandem solar cells contain more layers than single-junction solar cells,stress/strain control is an issue during fabrication and further practical operation.The stress can not only affect the stability of the perovskite layer but also change the optoelectronic properties of the films[19–23].

关键词： perovskite halide stability

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Flag Varieties of Type B/C and Twisted Yangian

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Algebra Colloquium 2024年第1期31卷 129-148页

作者： zhijie Dong Haitao Ma Institute for Advanced Study in Mathematics of HIT Harbin Institute of Technology Harbin 150001China College of Mathematical Science Harbin Engineering University Harbin 150001China

We study the convolution algebra H_(*)^(G×C^(*))(Z)of G×C^(*)-equivariant homology group on the Steinberg variety of type B/C and define an algebra Y that maps to H_(*)^(G×C^(*))(Z).We also study the G-equivariant ... 详细信息

关键词： Yangian fag variety convolution algebra

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