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Chinese Physics B 2021年第7期30卷 253-260页

作者： zhi-yuan wang Zi-Jing Zhang yuan Zhao Department of Physics Harbin Institute of TechnologyHarbin 150001China

The precision measurement of Doppler frequency shifts is of great significance for improving the precision of speed *** paper proposes a precision measurement scheme of tiny Doppler shifts by a parametric amplification process and squeezed vacuum *** scheme takes a parametric amplification process and squeezed vacuum state into a detection system,so that the measurement precision of tiny Doppler shifts can exceed the Cram′er–Rao bound of coherent ***,a simulation study is carried out on the theoretical basis,and the following results are obtained:for the signal light of Gaussian mode,when the amplification factor g=1 and the squeezed factor r=0.5,the measurement error of Doppler frequency shifts is 14.4%of the Cramer–Rao bound of the coherent light in our *** the same time,when the local light mode and squeezed vacuum state mode are optimized,the measurement precision of this scheme can be further improved by√(2n+1)/(n+1)times,where n is the mode-order of the signal light.

关键词： squeezed vacuum state quantum metrology

Effects of creep characteristics of natural gas hydrate-bearing sediments on wellbore stability

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Petroleum Science 2022年第1期19卷 220-233页

作者： Yang Li yuan-Fang Cheng Chuan-Liang Yan zhi-yuan wang Li-Fang Song School of Petroleum Engineering China University of Petroleum(East China)66 West Changjiang RoadHuangdao DistrictQingdao 266000China

Natural gas hydrate(NGH)reservoirs consist of the types of sediments with weak cementation,low strength,high plasticity,and high *** on the kinetics and thermodynamic characteristics of NGH decomposition,herein a heat-fluid-solid coupling model was established for studying the wellbore stability in an NGH-bearing formation to analyze the effects of the creep characteristics of NGH-bearing sediments during long-term *** results demonstrated that the creep characteristics of sediments resulted in larger plastic yield range,thus aggravating the plastic strain accumulation around the ***,the creep characteristics of NGH-bearing sediments could enhance the effects induced by the difference in horizontal in situ stress,as a result,the plastic strain in the formation around the wellbore increased nonlinearly with increasing difference in in situ *** lower the pore pressure,the greater the stress concentration effects and the higher the plastic strain at the ***,the lower the initial NGH saturation,the greater the initial plastic strain and yield range and the higher the equivalent creep *** plastic strain at the wellbore increased nonlinearly with decreasing initial saturation.

关键词： Natural gas hydrates Wellbore stability Creep Plastic yield

Ultrafine nano-scale Cu_(2)Sb alloy confined in three-dimensional porous carbon as an anode for sodium-ion and potassium-ion batteries

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International Journal of Minerals,Metallurgy and Materials 2021年第10期28卷 1666-1674页

作者： Dan wang Qun Ma Kang-hui Tian Chan-Qin Duan zhi-yuan wang Yan-guo Liu School of Materials Science and Engineering Northeastern UniversityShenyang 110819China School of Resources and Materials Northeastern University at QinhuangdaoQinhuangdao 066004China Key Laboratory of Dielectric and Electrolyte Functional Material Hebei Province Qinhuangdao 066004China

Ultrafine nano-scale Cu2Sb alloy confined in a three-dimensional porous carbon was synthesized using NaCl template-assisted vacuum freeze-drying followed by high-temperature sintering and was evaluated as an anode for sodium-ion batteries(SIBs)and potassium-ion batteries(PIBs).The alloy exerts excellent cycling durability(the capacity can be maintained at 328.3 mA·h·g^(-1) after 100 cycles for SIBs and 260 mA·h·g^(-1) for PIBs)and rate capability(199 mA·h·g^(-1) at 5 A·g^(-1) for SIBs and 148 mA·h·g^(-1) at 5 A·g^(-1) for PIBs)because of the smooth electron transport path,fast Na/K ion diffusion rate,and restricted volume changes from the synergistic effect of three-dimensional porous carbon networks and the ultrafine bimetallic *** study provides an ingenious design route and a simple preparation method toward exploring a high-property electrode for K-ion and Na-ion batteries,and it also introduces broad application prospects for other electrochemical applications.

关键词： copper-antimony alloy anode porous carbon potassium-ion batteries sodium-ion batteries

In situ synthesis of Co_(3)O_(4)nanoparticles confined in 3D nitrogendoped porous carbon as an efficient bifunctional oxygen electrocatalyst

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Rare Metals 2020年第12期39卷 1383-1394页

作者： zhi-yuan wang Shun-Da Jiang Chan-Qin Duan Dan wang Shao-Hua Luo Yan-Guo Liu School of Materials Science and Engineering Northeastern UniversityShenyang 110819China Key Laboratory of Dielectric and Electrolyte Functional Material-Hebei Province Qinhuangdao 066004China

The rational exploitation of non-precious metal catalyst with high activity,strong durability and low cost for the oxygen reduction reaction(ORR)and oxygen evolution reaction(OER)is of vital importance for metalair ***,a composite of Co_(3)O_(4)nanoparticles confined in three-dimensional(3 D)N-doped porous carbon(Co-NpCs)was prepared by a simple freeze-drying and in situ pyrolysis *** effect of different dosages of Co(NO_(3))_(2)on the catalytic performance was *** Co-NpC-12%exhibits the best catalytic performance(E_(1/2)=0.78 V,better stability than 20%Pt/C)in ORR and in OER among all the as-synthesized ***,it also exhibits the best bifunctional activity(ΔE=0.849 V).The excellent properties of Co-NpCs are mainly due to the synergy between Co_(3)O_(4)and ***,a high Co_(3)O_(4)loading amount can boost the defect level of the N-doped hierarchical porous carbon and expose more active ***,the unique in situ pyrolysis guarantees a largearea contact between Co_(3)O_(4)and carbon as well as a strong C-O-Co bonding,which promotes charge transfer,avoids the peeling of Co_(3)O_(4)nanoparticles and effectively improves the stability of the *** work is expected to offer a feasible strategy to produce metal oxide/carbon nanocomposite and push forward the development of bifunctional electrocatalyst with high activity and stability.

关键词： Bifunctional electrocatalyst Co_(3)O_(4) Nitrogendoped porous carbon In situ synthesis

The Influence of Different Single Radiation Dose on Delayed Growth of Transplanted Tumor in Athymic Mouse

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Clinical oncology and cancer researeh 2010年第5期7卷 303-309页

作者： zhi-zhen wang zhi-yong yuan Ping wang Key Laboratory of Cancer Prevention and Therapy and Department of Radiation Therapy Tianjin Medical University Tianjin Cancer Institute & Hospital Tianjin 300060 China.

OBJECTIVE To reveal the biological effects and effective dosage in radiotherapy model which applies high single-dose irradiation by animal experiment. METHODS We inoculated subcutaneouly human pancreatic carcinoma cell line （MIA PaCa-2） in the lateral of the right lower extremity of the athymic mouse to grow transplantation tumor. While the median diameter of transplantation tumor reached 10 mm approximately, the animals were randomly divided into 7 groups （6 animals per group） and irradiation by different dose in one fixed with consciousness for fraction （0, 2, 5, 10, 17, 25, 35 Gy）. All were kept on to be bred for observation of the change in gross tumor volume, calculation of delayed growth time and delayed growth curve. RESULTS With increased dose per fraction, cutaneous reaction on the neoplasma surface of the animal, which was mainly moist yellow effusion was more and more severe. When dosage is less than 10 Gy, all animals showed similar effects, that＇s the delayed tumor growth was not obvious. Tumors receiving more than 10 Gy in one fraction showed very good biological effect and the delayed tumor growth was obviously related to dosage. The difference in delayed tumor growth between the 2 groups was statistically significant. The delayed tumor growth time in 10, 17, 25 Gy group was respectively 3 weeks, 6 weeks and more. CONCLUSION The biological effect of the model which applies high single-dose irradiation （more than 10 Gy in one fraction） was very good. The effect of delayed tumor growth was obviously related to the dosage after transplantation tumor was radiated. Because of its higher dose per fraction and biological effects, the model of high single-dose irradiation can get better clinical effects.

关键词： hypofactionation radiotherapy delayed growth curve MIA PaCa-2 oncosis transplanted tumor.

Effect of 1,8-Diiodooctane Content on the Performance of P_(3)HT:PC_(61)BM Bulk Heterojunction Photodetectors

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Chinese Journal of Polymer Science 2021年第7期39卷 831-837页

作者： Xin wang Shi-Jia Gao Jin-Feng Han Yu-Lin Zhang Sai Zhang Wen-Qiang Qiao zhi-yuan wang StateKey Laboratory of Fine Chemicals Department of Polymer Science&MaterialsSchool of Chemical EngineeringDalian University of TechnologyDalian 116024China Department of Materials Science and Engineering and Department of Chemistry Johns Hopkins UniversityBaltimoreMD 21218USA Department of Chemistry Carleton UniversityOntario K1S 5B6Canada

A series of polymer photodetectors with device configuration of ITO/PEDOT:PSS/P_(3)HT:PC_(61)BM/C_(60)/AI were prepared by using P3HT as the donor material and PC61BM as the acceptor *** regulating the content of 1,8-diiodooctane(DIO)(V/V:1%,3%,5%)as a processing additive,the morphology of the active layer can be greatly improved With Ceo as the hole blocking layer,the dark current density of the device can be reduced by about an order of *** employing 3%DIO(V/V)in the active layer processing,the photodetetcors present the best performance,and the detectivity of the device is 1.52×10^(12)Jones at 540 nm under a bias of-0.1 ***,it also has a wider linear dynamic range of 60 dB as well as faster response speed(T1/T2=0.53/0.71μs)than those of devices with other content of DIO additives.

关键词： Polymer photodeteaor Configuration 1,8-Diiodooctane Morphology

Soil organic carbon contents, aggregate stability,and humic acid composition in different alpine grasslands in Qinghai-Tibet Plateau

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Journal of Mountain Science 2016年第11期13卷 2015-2027页

作者： CAO zhi-yuan wang Yong LI Jie ZHANG Jin-jing HE Nian-peng Key Laboratory of Ecosystem Network Observation and Modeling Institute of Geographic Sciences and Natural Resources Research Chinese Academy of Sciences Beijing 100101 China

Alpine grassland soils on Qinghai-Tibet Plateau store approximately 33.5 Pg of organic carbon(C) at 0–0.75 m depth and play an important role in the global carbon *** investigated soil organic C(SOC),water-soluble organic C(WSOC),easily oxidizable organic C(EOC),humic C fractions,aggregate-associated C,aggregate stability,and humic acid(HA) composition along an east-west transect across Qinghai-Tibet Plateau,and explored their spatial patterns and controlling *** contents of SOC,WSOC,EOC,humic C fractions and aggregate-associated C,the proportions of macroaggregates(2-0.25) and micro-aggregates(0.25-0.053 mm),and the aggregate stability indices all increased in the order alpine desert < alpine steppe < alpine *** alkyl C,O-alkyl C,and aliphatic C/aromatic C ratio of HA increased as alpine desert < alpine meadow < alpine steppe,and the trends were reverse for the aromatic C and HB/HI *** annual precipitation and aboveground biomass weresignificantly correlated with the contents of SOC and its fractions,the proportions of macro- and microaggregates,and the aggregate stability indices along this *** all these C fractions,SOC content and aggregate stability were more closely associated with humic C and silt and clay sized C in comparison with WSOC,EOC,and macro- and microaggregate *** results suggested that alpine meadow soils containing higher SOC exhibited high soil aggregation and aggregate *** annual precipitation should be the main climate factor controlling the spatial patterns of SOC,soil aggregation,and aggregate stability in this *** resistant and stable C fractions rather than labile C fractions are the major determinant of SOC stocks and aggregate stability.

关键词： Soil organic carbon Aggregate stability Humic acid Carbon-13 nuclear magnetic resonance Latitudinal transect Qinghai-Tibet Plateau

Double-confined nanoheterostructure Sb/Sb_(2)S_(3)@Ti_(3)C_(2)T_(x)@C toward ultra-stable Li-/Na-ion batteries

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Rare Metals 2024年第5期43卷 2067-2079页

作者： Dan wang Qun Ma Huan He zhi-yuan wang Run-Guo Zheng Hong-Yu Sun Yan-Guo Liu Chun-Li Liu School of Materials Science and Engineering Northeastern UniversityShenyang110819China School of Resources and Materials Northeastern University at QinhuangdaoQinhuangdao 066004China Key Laboratory of Dielectric and Electrolyte Functional Material Hebei Province Qinhuangdao 066004China Department of Physics and Oxide Research Center Hankuk University of Foreign StudiesYongin 17035Korea

Antimony-based materials with high capacities and moderate potentials are promising anodes for lithium-/-sodium-ion ***,their tremendous volume expansion and inferior conductivity lead to poor structural stability and sluggish reaction ***,a doubleconfined nanoheterostructure Sb/Sb_(2)S_(3)@Ti_(3)C_(2)T_(x)@C has been fabricated through a solvothermal method followed by low-temperature heat *** dual protection of“MXene”and“carbon”can better accommodate the volume expansion of Sb/Sb_(2)S_(3).The strong covalent bond(Ti-S,Ti-O-Sb,C-O-Sb)can firmly integrate Sb-based material with Ti_(3)C_(2)T_(x)and carbon,which significantly improves the structure *** addition,the carbon layer can restrain the oxidation of MXenes,and the nano-Sb/Sb_(2)S_(3)can facilitate electron/ion transport and suppress the restacking of *** heterogeneous interface between Sb and Sb_(2)S_(3)can further promote interfacial charge *** MXene-Sb/Sb_(2)S_(3)@C-1 with the optimal Sb content shows high specific capacities,comparable rate properties and ultra-stable cycling performances(250 m Ah·g^(-1)after 2500 cycles at 1 A·g^(-1)for sodium-ion batteries).Ex situ X-ray diffractometer(XRD)test reveals the storage mechanism including the conversion and alloying process of MXene-Sb/Sb_(2)S_(3)@*** voltammetry(CV)test results demonstrate that the pseudocapacitance behavior is dominant in MXene-Sb/Sb_(2)S_(3)@C-1,especially at large *** design paves the way for exploring high-performance alloy-based/conversion-type anode for energy storage devices.

关键词： Sb/Sb_(2)S_(3) MXene Carbon Anode Lithium-ion batteries Sodium-ion batteries

Initial Approach to the Cellular Irradiation Injury of Human Pancreatic Carcinoma Cell Line MIA PaCa-2 by High Dose per Fraction

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Clinical oncology and cancer researeh 2010年第6期7卷 352-358页

作者： zhi-zhen wang Hai-li YU zhi-yong yuan Ping wang Department of Radiation Therapy Tianjin Medical University Cancer Institute and Hospital Tianjin Key Laboratory of Cancer Prevention and Therapy Tianjin 300060 China.

OBJECTIVE To investigate an initial approach of radiotherapy, which produces cellular radiation injury by high dose in one fraction. METHODS Human pancreatic carcinoma cell line MIA PaCa-2, was cultivated and divided into 5 groups： 0, 2, 5, 10, 17 Gy. Cultivated cells were irradiated by 6MV-X ray in one fraction. Analysis were done as follows： comet assay, which assessed the level of DNA damage in the treated cells right after the cell was irradiated, flow cytometry, which was performed at 0, 6, 12, 24, 36 h after the cell line treated to ladder, which quantitatively asses changes of its cell cycle, DNA assessed the degree of DNA injury after 6 and 12 h, and histological examination, which analyzed cellular morphology after 24 h. RESULTS （1） After X-ray irradiated, the morphological change of human pancreatic carcinoma cell line （MIA PaCa-2） was mainly swelling. （2） When the dose of radiation was lower than 10 Gy, increasing the dose could greatly improve cell necrosis, apoptosis and blockage of cell cycle in GJM phase, which was consistent with the theory of radiation biology. （3） When radiation dose was more than the 10 Gy, the peak of apoptotic necrosis appeared strong and early. （4） The degree of DNA injury was also related to the dose of radiation therapy and most obvious in the 10 Gy group and not so obvious in the 17 Gy group. （5） When dose was less than 10 Gy, DNA ladder was a single electrophoretic band; in the 10 Gy group, the electrophoresis showed a multiple ladder band; when dose was more than 10 Gy, a vague and irregular band appeared on the electrophoresis. CONCLUSION Oncotic necrosis may be the main cell death style when dose per fraction is high, which differs from conventional dose fraction radiation therapy.

关键词： dose-response relationship drug necrosis irradiation injury.

Sulfur-doped 3D hierarchical porous carbon network toward excellent potassium-ion storage performance

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Rare Metals 2021年第9期40卷 2464-2473页

作者： Dan wang Kang-Hui Tian Jie wang zhi-yuan wang Shao-Hua Luo Yan-Guo Liu Qing wang Ya-Hui Zhang Ai-Min Hao Ting-Feng Yi School of Materials Science and Engineering Northeastern UniversityShenyang 110819China Key Laboratory of Dielectric Electrolyte Functional Materia-Hebei ProvinceQinhuangdao 066004China School of Resources and Materials Northeastern UniversityQinhuangdao 066004China

Carbonaceous materials are promising anode candidates for potassium-ion batteries, but currently the unsatisfactory cycling and rate performances due to the sluggish diffusion kinetic and serious structure damage during K+ insertion/extraction limit their practical application. Herein, a series of sulfur-doped porous carbons(SPCs) were prepared via a template-assisted freeze-drying followed by the carbonization and sulfuration processes at different temperatures. Among the three as-synthesized samples, SPC-600 exhibits the highest specific capacity(407 mAh·g^(-1) at 0.10 A·g^(-1)), the best rate(242 mAh·g^(-1) at 2.00 A·g^(-1)) and cycling performance(286 m Ah·g^(-1) after 800 cycles at 0.50 A·g^(-1)). All the SPCs display higher capacities than the undoped carbon materials. The excellent electrochemical performance of SPC can be ascribed to the abundant three-dimensional porous structure together with S-doping in the disordered carbon, which is favor of providing adequate reaction active sites as well as fast ion/electron transport paths. The density functional theory(DFT) calculations further demonstrate that the sulfurdoping can promote K-ion adsorption and storage. Meanwhile, the kinetic analyses reveal that surface-induced capacitive mechanism dominates the K-ion storage process in SPCs, which contributes to ultrafast charge storage. This work provides an effective strategy for fabricating highperformance potassium-ion storage electrode materials.

关键词： Potassium-ion batteries Porous carbon Sulfur-doping Density functional theory(DFT)calculations