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Two-dimensional vanadium nanosheets as a remarkably effective catalyst for hydrogen storage in MgH_(2)

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Rare Metals 2021年第11期40卷 3195-3204页

作者： zhi-yu lu Hai-Jie yu Xiong lu Meng-Chen Song Fu-Ying Wu Jia-Guang Zheng zhi-Fei yuan Liu-Ting Zhang School of Energy and Power Jiangsu University of Science and TechnologyZhenjiang 212003China Analysis and Testing Center Jiangsu University of Science and TechnologyZhenjiang 212003China

Magnesium hydride(MgH_(2)),which possesses high hydrogen density of 7.6 wt%,abundant resource and non-toxicity,has captured intense attention as one of the potential hydrogen storage ***,the practical application of Mg/MgH_(2) system is suffering from high thermal stability,sluggish absorption and desorption ***,two-dimensional(2D) vanadium nanosheets(V_(NS)) were successfully prepared via a facile wet chemical ball milling method and proved to be highly effective on improving the hydrogen storage performance of MgH_(2).For instance,the MgH_(2)+7 wt% V_(NS) composite began to release hydrogen at 187.2℃,152 ℃ lower than that of additive-free MgH_(2).At 300℃,6.3 wt% hydrogen was released from the MgH_(2)+7 wt% V_(NS) composite within 10 *** addition,the fully dehydrogenated sample could absorb hydrogen even at room temperature under hydrogen pressure of 3.2 MPa.X-ray diffractometer(XRD) and transmission electron microscopy(TEM)results confirmed metallic vanadium served as catalytic unit for facilitating the de/rehydrogenation reaction of MgH_(2).This finding presents an example of facile synthesis of two-dimensional(2D) vanadium with excellent catalysis,which may shed light on future design and preparation of highly effective layered catalysts for hydrogen storage and other energy-related areas.

关键词： Hydrogen storage Magnesium hydride Two-dimensional vanadium nanosheets Catalytic effect

SIMULATION OF LAGRANGIAN DISPERSION USING A LAGRANGIAN STOCHASTIC MODEL AND DNS IN A TURBULENT CHANNEL FLOW

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Journal of Hydrodynamics 2009年第6期21卷 767-773页

作者： luO Jian-ping lu zhi-ming LIU yu-lu School of Mechanical and Automation Engineering Shanghai Institute of Technology Shanghai 200235 China Shanghai Institute of Applied Mathematics and Mechanics Shanghai University Shanghai 200072 China

The mean square displacements of fluid particles in a turbulent channel flow at Reτ = 100 are investigated using a modified Langevin equation, and are compared with DNS results. Both the Lagrangian integral time scales directly obtained from DNS and the predicted values using an empirical relation between the Eulerian and the Lagrangian integral time scales are used in the modified Langevin equation to test the effects of integral time scales on the dispersion of particles. The results show that the slight variation of the Lagrangian integral time scale has little influence on the dispersion. The agreement between results of the model equation and those of DNS is satisfactory except the streamwise dispersion for intermediate times （ 20 〈 t^＋〈 300 ）, where the results of the model equation are slightly overestimated compared to those of DNS. The cause of such discrepancy is discussed.

关键词： turbulent channel flow Lagrangian dispersion Lagrangian stochastic model

TURBULENT MIXING AND EVOluTION IN A STABLY STRATIFIED FLOW WITH A TEMPERATURE STEP

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Journal of Hydrodynamics 2009年第1期21卷 84-92页

作者： QIU Xiang ZHANG Dao-xiang lu zhi-ming LIU yu-lu Shanghai Institute of Applied Mathematics and Mechanics Shanghai University Shanghai 200072 China Department of Mathematics Shanghai University Shanghai 200444 China

Large-Eddy Simulation （LES） is applied to examine the turbulent mixing and evolution in a stably stratified flow with a thermally sharp interface. Turbulent velocity intensities and turbulent kinetic energy are analyzed by considering the mean shear and stratification effects. The evolution of turbulent mixing layer and turbulent structures are mainly investigated. The results show that the streamwise intensities are much larger than the vertical intensities, and vertical fluctuations decay more rapidly at the presence of stratification. The qualitatively computational results suggest that the mixing layer, defined by the mean temperature, inclines to the side with small inlet velocity. The evolution of the half-width of the mixing layer shows two different slopes. The turbulent structure with high vorticity is restricted in the mixing layer especially in strong stratified cases.

关键词： stratified turbulence turbulent mixing turbulent structure Large-Eddy Simulation (LES)

NUMERICAL SIMULATION OF THE DISPERSION IN OSCILLATING FLOWS WITH REVERSIBLE AND IRREVERSIBLE WALL REACTIONS

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Journal of Hydrodynamics 2009年第4期21卷 482-490页

作者： ZHANG Dao-xiang lu zhi-ming LIU yu-lu NG Chiu-On Shanghai Institute of Applied Mathematics and Mechanics Shanghai University Shanghai 200072 China College of Mathematics and Computer Science Anhui Normal University Wuhu 241000 China Department of Mechanical Engineering The University of Hong Kong Hong Kong China

This is a study on the mass transport of a solute or contaminant in oscillating flows through a circular tube with a reactive wall layer. The reaction consists of a reversible component due to phase exchange between the flowing fluid and the wall layer, and an irreversible component due to absorption into the wall. The short-time dispersion characteristics are numerically investigated, incorporating the coupling effects between the flow oscillation, sorption kinetics, and retardation due to phase partitioning. The effects of various dimensionless parameters e.g., Da （the Damkoehler number）, α （phase partitioning number）, F （dimensionless absorption number）, and δ （dimensionless Stokes boundary layer number） on dispersion are discussed. In particular, it is found that there exist trinal peaks of the breakthrough curves in some cases.

关键词： dispersion flow oscillation wall reactions

Spatio-temporal patterns and climatic drivers of spring phenology in eight forest communities across the north-south transitional zone of China

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Journal of Geographical Sciences 2025年第1期35卷 17-38页

作者： ZHU Wenbin lu yu Institute of Geographic Sciences and Natural Resources Research CAS School of Geographical Science Nanjing University of Information Science & Technology

The Qinba Mountains are climatically and ecologically recognized as the northsouth transitional zone of *** of its phenology is critical for comprehending the response of vegetation to climatic *** retrieved the start of spring phenology （SOS）of eight forest communities from the MODIS products and adopted it as an indicator for spring *** analysis,partial correlation analysis,and Geo Detector were employed to reveal the spatio-temporal patterns and climatic drivers of *** results indicated that the SOS presented an advance trend from 2001 to 2020,with a mean rate of–0.473 d yr–*** SOS of most forests correlated negatively with air temperature （TEMP） and positively with precipitation （PRE）,suggesting that rising TEMP and increasing PRE in spring would forward and delay SOS,*** dominant factors influencing the sensitivity of SOS to climatic variables were altitude,forest type,and latitude,while the effects of slope and aspect were relatively *** response of SOS to climatic factors varied significantly in space and among forest communities,partly due to the influence of altitude,slope,and aspect.

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Catalytic Performance of Carbon Smoke over Ag-LSCF Composite Catalysts

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Journal of Wuhan University of Technology(Materials Science) 2025年第1期40卷 30-34页

作者： GUO Guanlun HAN Ming lu Shaomin yu Jing JU Hongling 无 Hubei Key Laboratory of Advanced Technology for Automotive Components&Hubei Collaborative Innovation Center for Automotive Components Technology Wuhan University of TechnologyWuhan 430070China College of Mechanical and Transportation Southwest Forestry UniversityKunming 650000China

To improve the catalytic performance of La_(0.6)Sr_(0.4)Co_(0.2)Fe_(0.8)O_(3)(LSCF)towards carbon soot,we utilized the impregnation method to incorporate Ag into the prepared LSCF *** conducted a series of characterization tests and evaluated the soot catalytic activity of the composite catalyst by comparing it with the LaCoO_(3) group,LaFeO_(3) group,and catalyst-free *** results indicate that the Ag-LSCF composite catalyst exhibits the highest soot catalytic activity,with the characteristic temperature values of 376.3,431.1,and 473.9℃at 10%,50%,and 90%carbon soot conversion,*** values are 24.8,20.2,and 23.1℃lower than those of the LSCF *** also shows that LSCF can improve the catalytic activity of soot after compounding with Ag,and reflects the necessity of using catalysts in soot combustion *** characterization and BET test show that Ag-LSCF has more abundant surface-adsorbed oxygen species,larger specific surface area and pore volume than LSCF,which also proves that Ag-LSCF has higher soot catalytic activity.

关键词： metallic composites carbon smoke oxidation perovskite catalyst soot

GFRF R-CNN:Object Detection Algorithm for Transmission Lines

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Computers, Materials & Continua 2025年第1期82卷 1439-1458页

作者： Xunguang Yan Wenrui Wang Fanglin lu Hongyong Fan Bo Wu Jianfeng yu Shanghai Advanced Research Institute Chinese Academy of SciencesShanghai201210China University of Chinese Academy of Sciences Beijing100049China Jingwei Textile Machinery Co. Ltd.Beijing100176China

To maintain the reliability of power systems,routine inspections using drones equipped with advanced object detection algorithms are essential for preempting power-related *** increasing resolution of drone-captured images has posed a challenge for traditional target detection methods,especially in identifying small objects in high-resolution *** study presents an enhanced object detection algorithm based on the Faster Regionbased Convolutional Neural Network(Faster R-CNN)framework,specifically tailored for detecting small-scale electrical components like insulators,shock hammers,and screws in transmission *** algorithm features an improved backbone network for Faster R-CNN,which significantly boosts the feature extraction network’s ability to detect fine *** Region Proposal Network is optimized using a method of guided feature refinement(GFR),which achieves a balance between accuracy and *** incorporation of Generalized Intersection over Union(GIOU)and Region of Interest(ROI)Align further refines themodel’s *** results demonstrate a notable improvement in mean Average Precision,reaching 89.3%,an 11.1%increase compared to the standard Faster *** highlights the effectiveness of the proposed algorithm in identifying electrical components in high-resolution aerial images.

关键词： Faster R-CNN transmission line object detection GIOU GFR

Metal-organic frameworks with dinuclear metal centers for synergistically boosting CO2 photoreduction

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Science China Chemistry 2025年第1期68卷 201-208页

作者： Hui-Feng Wang Wen-Jie Shi yu-Xin Yang Bao-Xia Dong Tong-Bu lu Di-Chang Zhong School of Chemistry and Chemical Engineering Yangzhou University Institute for New Energy Materials and Low Carbon Technologies School of Materials Science and Engineering Tianjin University of Technology

Dinuclear metal synergistic catalysis （DMSC） has been proved powerful in boosting CO2reduction,while this has not been achieved in heterogeneous catalysts with long-range order *** this study,we,by introduction of metal catalytic centers into an indium-based metal-organic framework （MOF）,obtained a series of isostructural In-MOFs,including three MOFs with mononuclear metal catalytic center （M-In）,three MOFs with dinuclear homometallic catalytic centers （MM-In）,and three MOFs with dinuclear heterometallic catalytic centers (MM’-In,M/M’=Co（II）,Ni（II）,Zn（II）).It was found that all these MOFs can serve as catalysts for photochemical CO2reduction to *** with M-In,the catalytic activities of MM-In were obviously enhanced,and that of MM’-In was further significantly *** example,the CO yield of Co Zn-In reaches a record value of 12,700μmol g-1h-1,which is 4.0,8.1,9.4,and 18.6-fold higher than that of Co Co-In,Zn Zn-In,Co-In,and Zn-In,***,the catalytic activities of Co Ni-In and Ni Zn-In also show different fold increase than those of corresponding dinuclear homometallic and mononuclear metallic *** results of control experiments and theoretical calculation reveal that the higher catalytic activities of MM-In over M-In can be ascribed to the DMSC effect,and the higher catalytic activity of MM’-In over MM-In can be ascribed to the strengthened DMSC *** work reveals the relationship between DMSC effect and bimetal centers in CO2reduction,which provides new insights into the DMSC and paves a new way to design highly active catalysts for photochemical CO2reduction.

关键词： metal-organic frameworks dinuclear metal centers synergistic catalysis CO2 reduction photocatalysis

Advances in the Development of Gradient Scaffolds Made of Nano‑Micromaterials for Musculoskeletal Tissue Regeneration

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Nano-Micro Letters 2025年第3期17卷 455-500页

作者： Lei Fang Xiaoqi Lin Ruian Xu lu Liu yu Zhang Feng Tian Jiao Jiao Li Jiajia Xue Beijing Laboratory of Biomedical Materials Beijing University of Chemical TechnologyBeijing 100029People’s Republic of China State Key Laboratory of Organic‑Inorganic Composites Beijing University of Chemical TechnologyBeijing 100029People’s Republic of China School of Biomedical Engineering Faculty of Engineering and ITUniversity of Technology SydneySydneyNSW 2007Australia

The intricate hierarchical structure of musculoskeletal tissues,including bone and interface tissues,necessitates the use of complex scaffold designs and material structures to serve as tissue-engineered *** has led to growing interest in the development of gradient bone scaffolds with hierarchical structures mimicking the extracellular matrix of native tissues to achieve improved therapeutic *** on the anatomical characteristics of bone and interfacial tissues,this review provides a summary of current strategies used to design and fabricate biomimetic gradient scaffolds for repairing musculoskeletal tissues,specifically focusing on methods used to construct compositional and structural gradients within the *** latest applications of gradient scaffolds for the regeneration of bone,osteochondral,and tendon-to-bone interfaces are ***,the current progress of testing gradient scaffolds in physiologically relevant animal models of skeletal repair is discussed,as well as the challenges and prospects of moving these scaffolds into clinical application for treating musculoskeletal injuries.

关键词： Gradient scaffolds Musculoskeletal tissues Advanced manufacturing Biomaterials Tissue regeneration