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甲烷在钠基蒙脱土吸附的第一性原理研究

原子与分子物理学报 2025年第2期42卷 8-14页

作者：方志杰李博宋昌辉刘美玲何秋芝刘翔莫曼广西科技大学电子工程学院柳州545006 广西科技大学土木建筑工程学院柳州545006 广西科技大学医学部柳州545006

随着经济的发展,能源需求日益增加,为了弥补国内少油缺气短板,页岩气的开发成为近期新能源的热点,探索页岩气储存规律是页岩气能源开发的关键所在.本文采用密度泛函理论的第一性原理方法,计算甲烷(CH_(4))在钠基蒙脱土表面和层间的吸附... 详细信息

随着经济的发展,能源需求日益增加,为了弥补国内少油缺气短板,页岩气的开发成为近期新能源的热点,探索页岩气储存规律是页岩气能源开发的关键所在.本文采用密度泛函理论的第一性原理方法,计算甲烷(CH_(4))在钠基蒙脱土表面和层间的吸附能,对比吸附前后的态密度和物理结构以及差分电荷密度.结果表明:钠基蒙脱土表面吸附中,甲烷最佳选择是桥位,吸附能为-0.08eV,被吸附后甲烷的键长和键角变化率均小于0.96%.层间吸附中,伴随着甲烷吸附量增加,纳基蒙脱土体积向c轴方向线性增加,a、b轴方向则变化不大.总态密度随着吸附量的增加,总能级数量也增加,甲烷分子的分波态密度峰向低能级移动.本文的研究成果,从原子角度分析了甲烷在蒙脱石表面以及层间的吸附能力,为解释页岩气在页岩储存规律提供理论依据.

关键词：钠基蒙脱土第一性原理甲烷吸附态密度

Efficacy and safety of vitrectomy with internal limiting membrane peeling for diabetic macular edema: a Meta-analysis

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International Journal of Ophthalmology(English edition) 2018年第11期11卷 1848-1855页

作者： Xin-Ying Hu Huan liu Li-na Wang Yu-zhi Ding Jie Luan Department of Ophthalmology Zhongda Hospital Southeast University Department of Epidemiology & Biostatistics School of Public Health Southeast University

AIM： To evaluate the efficacy and safety of vitrectomy with internal limiting membrane（ILM） peeling for diabetic macular edema（DME）. METHODS： The PubMed, Embase, Web of Science, Cochrane, SionMed, ***, CNKI databases and Wanfang databases, published until Oct. 2017, were searched to identify studies comparing the clinical outcomes following vitrectomy with and without ILM peeling, for treating DME. Pooled results were expressed as odds ratios（ORs） with corresponding 95% confidence intervals（CI） for vitrectomy with and without ILM peeling with regard to best corrected visual acuity（BCVA）, central macular thickness（CMT）, and complication incidents. RESULTS： A total of 14 studies involving 857 eyes were included of which three studies were Chinese and the rests were English literatures. Meta-analysis indicated that compared with vitrectomy alone, vitrectomy with ILM peeling could improve BCVA more obviously（OR=1.66, 95%CI： 1.12-2.46, P=0.01） and had higher rate of CMT reduction（OR=3.89, 95%CI： 1.37-11.11, P=0.01）. There were significant statistical differences between the two surgical methods for both BCVA and CMT（P〈0.05）. For the incidence of intraoperative and postoperative complications, the incidence of epiretinal membrane（ERM） was slightly lower in the ILM peeling group than the group without ILM peeling（OR=0.38, 95%CI： 0.07-2.00, P=0.25）, although insignificant statistically. Other incidences of overall complications, iatrogenic peripheral retinal break and increased intraocular pressure indicated no significant difference between two groups（OR=1.19, 95%CI： 0.82-1.73, P=0.36; OR=1.21, 95%CI： 0.66-2.21, P=0.53; OR=1.34, 95%CI： 0.75-2.40, P=0.32）. CONCLUSION： Vitrectomy is effective for DME and the effect can be improved by additional ILM peeling, especially for anatomical efficacy, without increasing the incidence of intraoperative and postoperative complications. However, it is imperative to gain more evaluation in the future due to the paucity of

关键词： internal limiting membrane vitrectomy diabetic macular edema Meta-analysis

Fuzzy adaptive tracking control within the full envelope for an unmanned aerial vehicle

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Chinese Journal of Aeronautics 2014年第5期27卷 1273-1287页

作者： liu zhi Wang Yong Department of Automation Science and Electrical Engineering Beihang University

Motivated by the autopilot of an unmanned aerial vehicle（UAV） with a wide flight envelope span experiencing large parametric variations in the presence of uncertainties, a fuzzy adaptive tracking controller（FATC） is proposed. The controller consists of a fuzzy baseline controller and an adaptive increment, and the main highlight is that the fuzzy baseline controller and adaptation laws are both based on the fuzzy multiple Lyapunov function approach, which helps to reduce the conservatism for the large envelope and guarantees satisfactory tracking performances with strong robustness simultaneously within the whole envelope. The constraint condition of the fuzzy baseline controller is provided in the form of linear matrix inequality（LMI）, and it specifies the satisfactory tracking performances in the absence of uncertainties. The adaptive increment ensures the uniformly ultimately bounded（UUB） predication errors to recover satisfactory responses in the presence of uncertainties. Simulation results show that the proposed controller helps to achieve high-accuracy tracking of airspeed and altitude desirable commands with strong robustness to uncertainties throughout the entire flight envelope.

关键词： Flight control systems Full flight envelope Fuzzy adaptive tracking control Fuzzy multiple Lyapunov function Fuzzy T–S model Single hidden layer neural network

YME1L overexpression exerts pro-tumorigenic activity in glioma by promoting Gai1 expression and Akt activation

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Protein & Cell 2023年第3期14卷 223-229页

作者： Fang liu Gang Chen Li-na Zhou Yin Wang zhi-qing Zhang Xihu Qin Cong Cao Department of Neurosurgery The Affiliated Changzhou No.2 People's Hospital of Nanjing Medical UniversityChangzhou 213004China Department of Neurosurgery TheFirst Affliated Hospital of SoochowUniversitySuzhou 215006China Department of Radiotherapy and Oncology Affliated Kunshan Hospital of Jiangsu UniversitySuzhou 215300China Department of Neurology and Clinical Research Center of Neurological Disease The Second Affiliated Hospital of Soochow UniversitySuzhou 215004China Jiangsu Key Laboratory of Neuropsychiatric Diseases and Institute of Neuroscience Soochow UniversitySuzhou 215031China Department of General surgery The Affiliated Changzhou No.2 People's Hospital of Nanjing Medical UniversityChangzhou 213004China

DearEditor,Identifying novel glioma-driven signaling molecules and exploring the corresponding molecularly targeted therapies are essential for better and effcient glioma ***1L(YME1 Like 1 ATPase),a primary member of the AAA family of ATPase,is located at the inner mitochondrial membrane(Anand et al.,2014;MacVicar et al.,2019;Ohba et al.,2020).YME1L is essential for maintaining mitochondrial morphology,function,and plasticity(Anand et al.,2014;MacVicar et al.,2019;Ohba et al.,2020).YME1L assembles into a homo-oligomeric complex within the inner mitochondrial membrane(Anand et al.,2014;MacVicar et al.,2019;Ohba et al.,2020).Moreover,YME1L can degrade mitochondrial proteins,including lipid-transferring proteins,IM translocation proteins.

关键词： glioma activation

Efficient multiuser detector based on box-constrained deregularization and its FPGA design

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Journal of Systems Engineering and Electronics 2012年第2期23卷 179-187页

作者： zhi Quan Jie liu Department of Electrical Engineering Federal University of Juiz de ForaJuiz de Fora 36036900Brazil School of Information Engineering Department of Electronic Information EngineeringZhengzhou UniversityZhengzhou 450001P.R.China RF Engines Limited Newport PO305WBUK

Multiuser detection can be described as a quadratic optimization problem with binary constraint. Many techniques are available to find approximate solution to this problem. These tech- niques can be characterized in terms of complexity and detection performance. The ＂efficient frontier＂ of known techniques include the decision-feedback, branch-and-bound and probabilistic data association detectors. The presented iterative multiuser detection technique is based on joint deregularized and box-constrained so- lution to quadratic optimization with iterations similar to that used in the nonstationary Tikhonov iterated algorithm. The deregulari- zation maximizes the energy of the solution, this is opposite to the Tikhonov regularization where the energy is minimized. However, combined with box-constraints, the deregularization forces the solution to be close to the binary set. We further exploit the box- constrained dichotomous coordinate descent （DCD） algorithm and adapt it to the nonstationary iterative Tikhonov regularization to present an efficient detector. As a result, the worst-case and aver- age complexity are reduced down to K28 and K2~ floating point operation per second, respectively. The development improves the ＂efficient frontier＂ in multiuser detection, which is illustrated by simulation results. Finally, a field programmable gate array （FPGA） design of the detector is presented. The detection performance obtained from the fixed-point FPGA implementation shows a good match to the floating-point implementation.

关键词： multiuser detection dichotomous coordinate descent (DCD) box-constrained DCD deregularization Tikhonov regular- ization low complexity field-programmable gate array (FPGA).

Distributed state estimation and data fusion in wireless sensor networks using multi-level quantized innovation

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Science China(Information Sciences) 2016年第2期59卷 217-231页

作者： zhi ZHANG Jianxun LI liu liu Department of Automation Shanghai Jiao Tong University Key Laboratory of System Control and Information Processing Ministry of Education of China College of Telecommunications & Information Engineering Nanjing University of Posts and Telecommunications

Low energy consumption and limited power supply are significant factors for wireless sensor networks(WSNs); thus, distributed state estimation and data fusion with quantized innovation are explored. The universal features of practical WSNs are investigated, and a dynamic transmission strategy is introduced. Furthermore,quantization state estimation based on Bayesian theory is derived. Unlike previous algorithms suitable for processing scalar measurement, the proposed distributed data fusion algorithm is applicable to general vector measurement. Furthermore, the efficiency of the proposed dynamic transmission strategy is analyzed. It is concluded that the proposed algorithm is more efficient than previous methods, and its estimation accuracy comparable to that of the standard Kalman filtering, which is based on analog-amplitude vector measurement.

关键词： data fusion distributed state estimation target tracking Kalman filtering quantization wireless sensor networks

In situ formed three-dimensional (3D) lithium-boron(Li-B) alloy as a potential anode for next-generation lithium batteries

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Rare Metals 2021年第12期40卷 3494-3500页

作者： Hai-Feng Huang Yi-na Gui Fu Sun zhi-Jian liu Hui-Long Ning Chen Wu Li-Bao Chen State Key Laboratory of Powder Metallurgy Central South UniversityChangsha 410083China Institute of Bioenergy and Bioprocess Technology Chinese Academy of SciencesQingdao 266101China

The practical application of the lithium anode in lithium metal batteries(LMBs) has been hindered by the uncontrollable growth of lithium dendrite and the high volumetric change during cycling. Herein, the in situ formed three-dimensional(3D) lithium-boron(Li-B) alloy is suggested as an excellent alternative to the Li metal, in which the 3D Li B skeleton can mitigate the growth of Li dendrites and volumetric change. In this study, the Li-B alloy anodes with different B contents were manufactured by high-temperature melting. It was found that the boron content had a significant effect on the electrochemical performance of the Li-B alloy. The Li-B alloy with the least B content(10 wt%, 10LiB) demonstrated the lowest overpotential of 0.0852 V after 300 h and the lowest interface resistance. However, the full cell with 15LiB as the anode displayed the best cycling performance of 115 m Ah·g^(-1) after 100 cycles with a columbic efficiency greater than 97%. The obtained results suggest that the in situ formed three-dimensional Li-B alloy anode can be an excellent alternative to the Li anode via tuning B contents for next-generation high energy density LMBs.

关键词： Li-B alloy 3D skeleton Solid electrolyte interface(SEI) Anode Lithium metal battery

甲烷/乙烷混合工质纳米液膜蒸发传质特性的研究

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原子与分子物理学报 2025年第5期42卷 72-80页

作者：林小晨丁鑫李雅宁兰志向刘纳张林阳郭健翔青岛理工大学环境与市政工程学院青岛266520 青岛娄山河水务资源有限公司青岛266000

采用分子动力学模拟方法研究了五种不同配比甲烷/乙烷混合工质纳米液膜的汽化过程,从蒸发现象、能量变化、涨落耗散规律及相对分子汽化量四个方面分析了混合工质的蒸发传质特性.结果表明:混合工质纳米液膜中甲烷配比越大,汽化起始时间越... 详细信息

采用分子动力学模拟方法研究了五种不同配比甲烷/乙烷混合工质纳米液膜的汽化过程,从蒸发现象、能量变化、涨落耗散规律及相对分子汽化量四个方面分析了混合工质的蒸发传质特性.结果表明:混合工质纳米液膜中甲烷配比越大,汽化起始时间越早,汽化过程越剧烈,汽化的持续时间越短,固定吸附层越薄,模拟体系动能和势能的增量越小,乙烷的存在会抑制甲烷的汽化;由涨落耗散分析可得,甲烷配比越大,对乙烷汽化的促进作用越强,汽化弛豫时间越短,整体汽化速率越快,传质效果越好.

关键词：混合工质纳米液膜传热传质涨落耗散分子动力学模拟

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On the surface brightness radial profile of the extendedγ-ray sources

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Science China(Physics,Mechanics & Astronomy) 2022年第1期65卷 84-91页

作者： Rui-zhi Yang Bing liu Department of Astronomy School of Physical SciencesUniversity of Science and Technology of ChinaHefei 230026China CAS Key Labrotory for Research in Galaxies and Cosmology University of Science and Technology of ChinaHefei 230026China School of Astronomy and Space Science University of Science and Technology of ChinaHefei 230026China Key Laboratory of Modern Astronomy and Astrophysics(nanjing University) Ministry of EducationNanjing 210093China

The morphology of the extendedγ-ray source is governed by the propagation process of parent relativistic *** this paper,we investigate the surface brightness radial profile of extendedγ-ray sources illuminated by cosmic ray protons and electrons,considering the radiation mechanisms,projection effects,and the response of *** find that the parent particle species and the propagation process can cause considerable differences in the observed radial ***,the surface brightness profile can be used as a unique tool to identify the radiation mechanism and the propagation process of the parent *** addition,we also discuss the possible implications regarding the latest discoveries from very/ultra-high energyγ-ray instruments like LHAASO and HAWC.

关键词： cosmic rays γ-ray sources diffuse emission