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Catalytic oxidation of toluene by manganese oxides:Effect of K^(+)doping on oxygen vacancy

Journal of Environmental Sciences 2024年第8期142卷 43-56页

作者： zhenzhen huang Haiyang Li Xuejun Zhang Yanli Mao Yinghan Wu Wei Liu Hongrun Gao Mengru Zhang Zhongxian Song Faculty of Environmental and Municipal Engineering Henan Key Laboratory of Water Pollution Control and Rehabilitation TechnologyHenan University of Urban ConstructionPingdingshan 467036China College of Environmental and Safety Engineering Shenyang University of Chemical TechnologyShenyang 110142China

Alkali metal potassium was beneficial to the electronic regulation and structural stability of transition metal oxides.Herein,K ions were introduced into manganese oxides by different methods to improve the degradation efficiency of toluene.The results of activity experiments indicated that KMnO_(4)-HT(HT:Hydrothermal method)exhibited outstanding low-temperature catalytic activity,and 90%conversion of toluene can be achieved at 243℃,which was 41℃and 43℃lower than that of KNO_(3)-HT and Mn-HT,respectively.The largest specific surface area was observed on KMnO_(4)-HT,facilitating the adsorption of toluene.The formation of cryptomelane structure over KMnO_(4)-HT could contribute to higher content of Mn^(3+)and lattice oxygen(Olatt),excellent low-temperature reducibility,and high oxygen mobility,which could increase the catalytic performance.Furthermore,two distinct degradation pathways were inferred.PathwayⅠ(KMnO_(4)-HT):toluene→benzyl→benzoic acid→carbonate→CO_(2)and H2O;PathwayⅡ(Mn-HT):toluene→benzyl alcohol→benzoic acid→phenol→maleic anhydride→CO_(2)and H2O.Fewer intermediates were detected on KMnO_(4)-HT,indicating its stronger oxidation capacity of toluene,which was originated from the doping of K^(+)and the interaction between K-O-Mn.More intermediates were observed on Mn-HT,which can be attributed to the weaker oxidation ability of pure Mn.The results indicated that the doping of K^(+)can improve the catalytic oxidation capacity of toluene,resulting in promoted degradation of intermediates during the oxidation of toluene.

关键词： Catalytic oxidation Preparation method Cryptomelane Mn^(3+)and lattice oxygen

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Spatiotemporal Evolution of Ecosystem Service Value in Caohai National Nature Reserve

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Meteorological and Environmental Research 2024年第2期15卷 14-21页

作者： Denghong huang zhenzhen ZHANG Jintong REN Guizhou University of Engineering Science/Guizhou Province Key Laboratory of Ecological Protection and Restoration of Typical Plateau Wetlands Bijie 551799China School of Karst Science Guizhou Normal UniversityGuiyang 550025China

Wetland ecosystems are important regulators of global climate change.Studying the spatiotemporal changes and driving mechanisms of their ecosystem service values(ESV)is beneficial for the sustainable development of wetlands.This paper uses the equivalent factor method,based on land use changes,to reveal the spatiotemporal evolution of the ecosystem service value in the Caohai National Nature Reserve(CNNR).The results show the following:①from 2000 to 2020,there was a significant decrease in the core zone s arable land area,with an increase in forest and water areas.Construction land mainly increased in the experimental area,and the grassland area showed a fluctuating change of first increasing and then decreasing;②in 2000,2010,and 2020,the ecosystem service value of the study area was 302 million,296 million,and 325 million yuan,respectively,showing a trend of fluctuating growth,with the value of wetland ecosystems playing a dominant role;③regulatory services are the main contributors to the ecosystem service value in the study area,with a contribution rate of 60%.Hydrological regulation is the ecosystem function with the highest value in wetland ecosystem services,contributing more than 35%to the ESV in all three periods;④in terms of spatial distribution,the core zone s ecosystem service value is dominant.Looking at the total ecosystem service value of the region,the core zone>the experimental area>the buffer zone.In terms of ESV per unit area,the core zone(89000 yuan/hm^(2))is significantly higher than the buffer zone(39100 yuan/hm^(2))and the experimental area(15800 yuan/hm^(2)).The study can provide a basis for research and spatial management of ecosystem services in wetland ecosystems and nature reserves.

关键词： Ecosystem service value(ESV) Equivalent factor method Land use change Wetland ecosystem CNNR

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Spatiotemporal Evolution of Ecological Quality in Typical Karst Ecologically Fragile Areas Based on Remote Sensing Ecological Indexes

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Meteorological and Environmental Research 2024年第2期15卷 22-28页

作者： Denghong huang Zhiying ZHANG zhenzhen ZHANG School of Karst Science/School of Geography&Environmental Science Guizhou Normal UniversityGuiyang 550025China State Engineering Technology Institute for Karst Desertification Control Guiyang 550025China

Fast and effective remote sensing monitoring is an important means for analyzing the spatio-temporal changes in ecological quality in fragile karst regions.This study focuses on Guanling Autonomous County,a national-level demonstration county for comprehensive desertification control.Based on Landsat TM/OLI remote sensing image data from 2005,2010,2015,and 2020,remote sensing ecological indices were used to analyze the spatio-temporal changes in ecological quality in Guanling Autonomous County from 2005 to 2020.The results show that:①the variance contribution rates of the first principal component for the four periods were 66.31%,71.59%,63.18%,and 75.24%,indicating that PC1 integrated most of the characteristics of the four indices,making the RSEI suitable for evaluating ecological quality in karst mountain areas;②the remote sensing ecological index grades have been increasing year by year,with an overall trend of improving ecological quality.The area of higher-grade ecological quality has increased spatially,while fragmented patches have gradually decreased,becoming more concentrated in the low-altitude areas in the northwest and east,and there is a trend of expansion towards higher-altitude areas;③the ecological environment quality in most areas has improved,with the improvement in RSEI spatio-temporal variation becoming more noticeable with increasing slope.Areas of higher-grade quality appeared in 2010,and the range of higher-grade quality expanded with increasing slope.

关键词： Ecological quality Remote sensing ecological index Karst mountainous area Ecological fragility Guanling Autonomous County

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Spatiotemporal Evolution of Ecological Quality in Alpine Freshwater Lake Nature Reserves in the Past 20 Years

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Meteorological and Environmental Research 2024年第2期15卷 29-36页

作者： Denghong huang Chenli LIAO zhenzhen ZHANG Jintong REN Guizhou University of Engineering Science/Guizhou Province Key Laboratory of Ecological Protection and Restoration of Typical Plateau Wetlands Bijie 551799China School of Karst Science Guizhou Normal UniversityGuiyang 550025China School of Geography&Environmental Science Guizhou Normal UniversityGuiyang 550025China

The Caohai Nature Reserve is one of the three major plateau freshwater lakes in China.Since the 1950s,human activities such as land reclamation and population relocation have greatly damaged Caohai.A rapid evaluation of the spatiotemporal evolution trend of the ecological quality of the Caohai Nature Reserve is significant for the maintenance and construction of the ecosystem in this area.The research is based on the Google Earth Engine(GEE)remote sensing cloud computing platform.Landsat TM/OLI images from May to October in five time periods:2000-2002,2004-2006,2009-2011,2014-2016,and 2019-2021 were obtained to reconstruct the optimal cloud image set by averaging the images in each time period.By constructing four ecological indicators:Greenness(NDVI),Wetness(Wet),Hotness(LST),and Dryness(NDBSI),and using Principal Component Analysis(PCA)method to obtain the Remote Sensing Ecological Index(RSEI)for the corresponding years,the spatiotemporal variation of ecological quality in the Caohai Nature Reserve over 20 years was analyzed.The results indicate:①the mean value of RSEI increased from 0.460 in 2000-2002 to 0.772 in 2019-2021,a 67.83%increase,indicating a significant improvement in the ecological quality of the reserve over the 20 years;②from the perspective of functional zoning of the Caohai Nature Reserve,the ecological quality of the core area showed a degrading trend,while the ecological quality of the buffer zone and experimental zone significantly improved;③with the implementation of ecological restoration projects,the ecological quality of the reserve gradually recovered and improved from 2014 to 2021.The trend of RSEI value changes is well correlated with human interventions,indicating that the PCA-based RSEI model can be effectively used for ecological quality assessment in lake areas.

关键词： Ecological restoration Ecological quality Remote sensing ecological index Google Earth Engine Caohai Nature Reserve

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Lymphangiogenesis contributes to exercise-induced physiological cardiac growth

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Journal of Sport and Health Science 2022年第4期11卷 466-478页

作者： Yihua Bei zhenzhen huang Xing Feng Lin Li Meng Wei Yujiao Zhu Shuqin Liu Chen Chen Mingming Yin Huimin Jiang Junjie Xiao Cardiac Regeneration and Ageing Lab Institute of Geriatrics(Shanghai University)Affiliated Nantong Hospital of Shanghai University(The Sixth People’s Hospital of Nantong)School of MedicineShanghai UniversityNantong 226011China Shanghai Engineering Research Center of Organ Repair School of Life ScienceShanghai UniversityShanghai 200444China Clinical Laboratory Center Beijing Hospital of Traditional Chinese MedicineBeijing 100010China

Background:Promoting cardiac lymphangiogenesis exerts beneficial effects for the heart.Exercise can induce physiological cardiac growth with cardiomyocyte hypertrophy and increased proliferation markers in cardiomyocytes.However,it remains unclear whether and how lymphangiogenesis contributes to exercise-induced physiological cardiac growth.We aimed to investigate the role and mechanism of lymphangiogenesis in exercise-induced physiological cardiac growth.Methods:Adult C57 BL6/J mice were subjected to 3 weeks of swimming exercise to induce physiological cardiac growth.Oral treatment with vascular endothelial growth factor receptor 3(VEGFR3) inhibitor SAR1 3 1 675 was used to investigate whether cardiac lymphangiogenesis was required for exercise-induced physiological cardiac growth by VEGFR3 activation.Furthermore,human dermal lymphatic endothelial cell(LEC)-conditioned medium was collected to culture isolated neonatal rat cardiomyocytes to determine whether and how LECs could influence cardiomyocyte proliferation and hypertrophy.Results:Swimming exercise induced physiological cardiac growth accompanied by a remarkable increase of cardiac lymphangiogenesis as evidenced by increased density of lymphatic vessel endothelial hyaluronic acid receptor 1-positive lymphatic vessels in the heart and upregulated LYVE-1 and Podoplanin expressions levels.VEGFR3 was upregulated in the exercised heart,while VEGFR3 inhibitor SAR131675 attenuated exercise-induced physiological cardiac growth as evidenced by blunted myocardial hypertrophy and reduced proliferation marker Ki67 in cardiomyocytes,which was correlated with reduced lymphatic vessel density and downregulated LYVE-1 and Podoplanin in the heart upon exercise.Furthermore,LEC-conditioned medium promoted both hypertrophy and proliferation of cardiomyocytes and contained higher levels of insulinlike growth factor-1 and the extracellular protein Reelin,while LEC-conditioned medium from LECs treated with SAR131675 blocked these effects.Functional rescue assays further demonstr

关键词： Cardiac lymphatics Exercise Physiological cardiac hypertrophy Proliferation VEGFR3

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Aptamer-Based Cell-Surface Profiling with Single-Cell Resolution Enables Precise Cancer Characterization

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CCS Chemistry 2024年第1期6卷 196-207页

作者： Liujun Xu Yawei Feng Tong Wang Shenhuan Li Kangli Xu Yue Sun Yi Luo Yishan Ye Yan Miao Yun Dong zhenzhen Guo Qing Zhang Benshang Li He huang Xue-Qiang Wang Liping Qiu Weihong Tan Molecular Science and Biomedicine Laboratory State Key Laboratory of Chemo/Biosensing and ChemometricsCollege of Chemistry and Chemical EngineeringCollege of BiologyAptamer Engineering Center of Hunan ProvinceHunan UniversityChangshaHunan 410082 The Key Laboratory of Zhejiang Province for Aptamers and Theranostics Zhejiang Cancer HospitalHangzhou Institute of MedicineChinese Academy of SciencesHangzhouZhejiang 310022 Institute of Molecular Medicine Renji HospitalShanghai Jiao Tong University School of MedicineCollege of Chemistry and Chemical EngineeringShanghai Jiao Tong UniversityShanghai 200240 Bone Marrow Transplantation Center The First Affiliated HospitalSchool of MedicineZhejiang UniversityHangzhou 310003 Institute of Hematology Zhejiang UniversityHangzhou 310003 Department of Hematology and Oncology Shanghai Children’s Medical CenterShanghai Jiao Tong University School of MedicineShanghai Jiao Tong UniversityShanghai 200127

Molecular profiling of cell-surface proteins is a powerful strategy for precise cancer diagnosis.While mass cytometry(MC)enables synchronous detection of over 40 cellular parameters,its full potential in disease classification is challenged by the limited types of recognition probes currently available.In this work,we synthesize a panel of heavy isotopeconjugated aptamers to profile cancer-associated signatures on the surface of hematological malignancy(HM)cells.Based on 15 molecular signatures,we performed cell-surface profiling that allowed the precise classification of 8 HM cell lines.Combined with machine-learning technology,this aptamer-based MC platform also achieved multiclass identification of HM subtypes in clinical sampleswith 100%accuracy in the training cohort and 80%accuracy in the test cohort.Therefore,we report an effective and practical strategy for precise cancer classification at the singlecell level,paving the way for its clinical use in the near future.

关键词： molecular profiling cancer diagnosis mass cytometry aptamers machine learning

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溶质引起的自由液面Marangoni铺展研究综述

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力学学报 2024年第6期56卷 1511-1528页

作者：黄彦如黄睿雯马雪李真珍滕宏辉北京理工大学宇航学院北京100081 巴黎西岱大学复杂物质与系统实验室法国巴黎75013

Marangoni流动是一种由表面张力梯度驱动的界面铺展和液体内部的对流.其中,表面张力梯度可以通过温度或溶质的不均匀分布来调控.由溶质引起的Marangoni铺展在呼吸道药物输送等生物医学领域、复杂结构颗粒制备和镀膜等先进制造领域有着... 详细信息

Marangoni流动是一种由表面张力梯度驱动的界面铺展和液体内部的对流.其中,表面张力梯度可以通过温度或溶质的不均匀分布来调控.由溶质引起的Marangoni铺展在呼吸道药物输送等生物医学领域、复杂结构颗粒制备和镀膜等先进制造领域有着重要应用.溶质分子的诸多物理化学过程都会对Marangoni铺展的动力学产生影响,例如分子在界面上的输运、液滴与基底之间的物质交换、挥发性溶质在自由液面的蒸发,都会对表面张力梯度起到动态的调控作用.同时,在铺展液体特殊的本构性质和Marangoni铺展提供的强剪切率的共同作用下,流体会呈现一系列复杂而有趣的现象.文章着重介绍近年来领域内开展的由溶质引起的Marangoni铺展,包括表面活性分子参与的Marangoni铺展,互混液体界面、复杂流体自由液面的Marangoni铺展,以及组分差异性蒸发引起的Marangoni铺展,并阐述它们的演化机制.最后将列举Marangoni铺展在新兴工业领域中的应用,为开发借助溶质的本构性质等物理化学性质实现液体驱动的低能耗器件和生产工艺提供参考.

关键词： Marangoni流表面活性分子接触线不稳定性差异性蒸发

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不同温度条件下水泥混凝土撞击后力学性能数值模拟研究

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混凝土 2024年第5期 43-47页

作者：马臻臻黄波河南职业技术学院河南郑州450046 信阳职业技术学院河南信阳464000

对不同温度条件下的混凝土撞击后的力学性能模拟进行了研究,结果表明:对于单轴冲击压缩试验,冲击速度相同,如果混凝土材料的温度处于405℃以内的条件下,受到温度升高的影响抗压强度虽然会随之增大,但幅度较小;如果混凝土材料的温度已经... 详细信息

对不同温度条件下的混凝土撞击后的力学性能模拟进行了研究,结果表明:对于单轴冲击压缩试验,冲击速度相同,如果混凝土材料的温度处于405℃以内的条件下,受到温度升高的影响抗压强度虽然会随之增大,但幅度较小;如果混凝土材料的温度已经高于405℃,在温度升高的影响下抗压强度则有较大幅度的改变,呈现出快速下降的趋势。当温度从25℃增加到805℃时,在冲击速度为7.5 m/s时,混凝土峰值应力降低65.56%;冲击速度为13.5 m/s时,混凝土峰值应力降低63.87%;冲击速度为17.5 m/s时,混凝土峰值应力降低44.25%。这说明随着温度损伤效应增强,材料强度增幅有所降低。不同温度的混凝土试件冲击速度变化规律表明,材料的峰值应力随冲击速度提高先增加后减小,最终趋于稳定。

关键词：温度条件力学性能撞击数值模拟

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Carbon nanotube-based photothermal membrane for efficient cold air heating and removal of particulate matter and airborne bacteria

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Green Carbon 2024年第1期2卷 101-108页

作者： Weichao Dong Lina huang Xiangju Song Yan Zhang Mengke Liu zhenzhen Ren Long Pang Hui Peng Heqing Jiang Key Laboratory of Biobased Materials Qingdao Institute of Bioenergy and Bioprocess TechnologyChinese Academy of SciencesQingdao 266101China School of Material Science and Engineering Henan Polytechnic UniversityJiaozuo 454003China Shandong Energy Institute Qingdao 266101China Qingdao New Energy Shandong Laboratory Qingdao 266101China University of Chinese Academy of Sciences Beijing 101408China College of Chemistry and Pharmaceutical Engineering HuangHuai UniversityZhumadian 463000China

Indoor heating results in high energy consumption and severe atmospheric pollution.Although the development of solar air heaters provides a sustainable route for indoor thermal comfort,such heaters still face challenges in terms of adequate heat exchange and filtering of atmospheric pollutants.Inspired by solar-driven interfacial evaporation,we propose a multifunctional carbon nanotube-based photothermal membrane for efficient cold air heating and purification via ventilation.Carbon nanotubes endow the membrane with high light absorption and thermal conversion capabilities,thereby sufficiently heating the approaching cold air.With the hierarchical structure formed by phase inversion,the thin upper skin of the composite membrane intercepts micropollutants via the size-sieving effect,whereas the finger-like pores and interpenetrating macrovoids inside the membrane ensure that the heated clear air passes through quickly.A proof-of-principle experiment indicated a cold airflow of 1 L/min across the membrane,yielding a temperature increase of ca.37℃ as well as a PM 2.5 rejection always higher than 93%.Further antibacterial experiments demonstrated that the membrane effectively removed airborne bacteria.This multifunctional carbon nanotube-based photothermal membrane with specific microstructures not only improves the indoor living quality but also provides a sustainable development scheme to coordinate the relationship among energy utilization,building heating,and air purification.

关键词： Indoor heating Carbon nanotubes Multifunctional photothermal membrane Hierarchical structure Particulate matter

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自相似嵌套金属多胞管耐撞性研究

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机械强度 2024年第3期46卷 568-578页

作者：黄翠萍邓小林蔡珍珍梧州学院电子与信息工程学院梧州543003

层级多胞结构具有良好的吸能特性,可以广泛应用于汽车、飞机等交通工具的能量吸收装置中。创新性地设计了两种类型的自相似嵌套金属多胞管,通过数值仿真对其轴向冲击下的耐撞性能开展了系统的研究。结果表明,无论是相同质量还是相同壁厚... 详细信息

层级多胞结构具有良好的吸能特性,可以广泛应用于汽车、飞机等交通工具的能量吸收装置中。创新性地设计了两种类型的自相似嵌套金属多胞管,通过数值仿真对其轴向冲击下的耐撞性能开展了系统的研究。结果表明,无论是相同质量还是相同壁厚,高阶多胞管相比低阶多胞管都具有更好的能量吸收能力。相同质量情况下,高阶多胞管的比能量吸收最高提升了36.45%,冲击力效率最高提升了35.42%;相同壁厚情况下,高阶多胞管的比能量吸收和冲击力效率最大分别增加了80.40%、59.64%。研究表明,所提出的自相似嵌套金属多胞管相比传统多胞管的耐撞性能具有明显改善。最后,系统地开展了阶数、壁厚等结构参数对自相似嵌套金属多胞管耐撞性能的参数化研究。

关键词：自相似结构多胞管轴向冲击数值仿真耐撞性

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