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Synergistic effect of bonding heterogeneity and phonon localization in introducing excellent thermoelectric properties in layered heteroanionic NdZnSbO material

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Journal of Energy Chemistry 2025年第1期100卷 259-272页

作者： Da wan.Shuwei Tang Shulin Bai Xiaodong Li Peng Ai wan.ong Guo Tuo zheng College of Materials Science and Engineering Liaoning Technical University Faculty of Chemistry Northeast Normal University

Layered rare-earth metal oxides, harnessing the dual properties of oxides and two-dimensional layered materials, exhibit remarkable thermal stability and quantum confinement effects. Therefore, this work adopts the first-principles calculation combined with the Boltzmann transport theory to predict the thermoelectric properties of NdZnSbO compound. The coexistence of weak interlayer van der Waals interactions, robust intralayer ionic bonding, and partial covalent bonding leads to remarkable bonding heterogeneity, which engenders pronounced phonon scattering and imposes constraints on thermal transport along the out-of-plane direction. The weakened chemical bonds induced by the antibonding states, together with the rattling-like behavior of the Zn atom, culminate in the profound anharmonicity in the layered NdZnSbO compound. The weakening bond and heavy element contribute to the softness of phonon modes, which significantly diminishes the phonon group velocity. The redistribution-dominated four-phonon scattering process spans a large optical gap, which effectively reduces the lattice thermal conductivity. The NdZnSbO compound exhibits direct semiconductor characteristic with a bandgap of 0.73 e V by adopting the Heyd-Scuseria-Ernzerhof(HSE06) functional in combination with spin–orbit coupling(SOC) effect. The multi-valley feature of NdZnSbO compound augur favorably for band degeneracy, thus amplifying the power factor. Consequently, an optimal figure-of-merit(ZT) of 3.40 at 900 K is achieved for the n-type NdZnSbO compound. The present study delves deeply insights into the origins for the low thermal conductivity of NdZnSbO compound and proposes an optimization scheme to enhance overall thermoelectric performance.

关键词： Bond strength (chemical)

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Numerical simulation of local and global mixing/segregation characteristics in a gas–solid fluidized bed

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Chinese Journal of Chemical Engineering 2022年第4期35卷 72-86页

作者： zhen wan.Youjun Lu State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049China

Researches on solids mixing and segregation are of great significance for the operation and design of fluidized bed *** this paper,the local and global mixing and segregation characteristics of binary mixtures were investigated in a gas–solid fluidized bed by computational fluid dynamics-discrete element method(CFD-DEM)coupled approach.A methodology based on solids mixing entropy was developed to quantitatively calculate the mixing degree and time of the *** mixing curves of global mixing entropy were acquired,and the distribution maps of local mixing entropy and mixing time were also *** comparing different operating conditions,the effects of superficial gas velocity,particle density ratio and size ratio on mixing/segregation behavior were *** showed that for the partial mixing state,the fluidized bed can be divided into three parts along the bed height:complete segregation area,transition area and stable mixing *** areas showed different mixing/segregation *** gas velocity promoted the local and global mixing of binary *** increase in particle density ratio and size ratio enlarged the complete segregation area,reduced the mixing degree and increased the mixing time in the stable mixing area.

关键词： Discrete element method Solids mixing Binary mixtures Fluidized bed

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Cholesterol metabolism: physiological versus pathological aspects in intracerebral hemorrhage

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Neural Regeneration Research 2025年第4期20卷 1015-1030页

作者： Ruoyu Huang Qiuyu Pang Lexin zheng Jiaxi Lin Hanxi Li Lingbo wan.Tao wan. Department of Forensic Science School of Basic Medicine and Biological SciencesSuzhou Medicine College of Soochow UniversitySuzhouJiangsu ProvinceChina

Cholesterol is an important component of plasma membranes and participates in many basic life functions,such as the maintenance of cell membrane stability,the synthesis of steroid hormones,and *** plays a key role in the establishment and maintenance of the central nervous *** brain contains 20%of the whole body’s cholesterol,80%of which is located within myelin.A huge number of processes(e.g.,the sterol regulatory element-binding protein pathway and liver X receptor pathway)participate in the regulation of cholesterol metabolism in the brain via mechanisms that include cholesterol biosynthesis,intracellular transport,and *** brain injuries or diseases involving crosstalk among the processes above can affect normal cholesterol metabolism to induce detrimental ***,we hypothesized that cholesterol-related molecules and pathways can serve as therapeutic targets for central nervous system *** hemorrhage is the most severe hemorrhagic stroke subtype,with high mortality and *** cholesterol levels are associated with the risk of intracerebral ***,secondary pathological changes after intracerebral hemorrhage are associated with cholesterol metabolism dysregulation,such as neuroinflammation,demyelination,and multiple types of programmed cell *** cholesterol accumulation in the brain has been found after intracerebral *** this paper,we review normal cholesterol metabolism in the central nervous system,the mechanisms known to participate in the disturbance of cholesterol metabolism after intracerebral hemorrhage,and the links between cholesterol metabolism and cell *** also review several possible and constructive therapeutic targets identified based on cholesterol metabolism to provide cholesterol-based perspectives and a reference for those interested in the treatment of intracerebral hemorrhage.

关键词： cell death cholesterol metabolism intracerebral hemorrhage myelination therapeutic target

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Quantum public-key crypto via EPR pairs

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Science China(Physics,Mechanics & Astronomy) 2025年第1期Mechanics & Astronomy) .卷 58-63页

作者： Xiang-Qun Fu hong-Wei Li Jian-hong Shi Tan Li wan.Su Bao Henan Key Laboratory of Quantum Information and Cryptography Information Engineering University Synergetic Innovation Center of Quantum Information and Quantum Physics University of Science and Technology of China

With the development of quantum computing technology, quantum public-key cryptography is gradually becoming an alternative to the existing classical public-key cryptography. This paper designs a quantum trapdoor one-way function via EPR pairs and quantum measurements. Based on this, a new quantum public-key cryptosystem is presented, which offers forward security,and can resist the chosen-plaintext attack and chosen-ciphertext attack. Compared with the existing quantum public-key cryptos,eavesdropping can be automatically detected in this new quantum public-key cryptosystem under a necessary condition, which is also detailed in the paper.

关键词： quantum public-key crypto trapdoor one-way function EPR pairs

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Instantaneous mixing characteristics of binary mixtures differing in density in a gas-solid fluidised bed

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Particuology 2020年第6期18卷 63-71页

作者： zhen wan.Youjun Lu Hao wan. State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong UniversityXi'an 710049ShaanxiChina

Characterisations of instantaneous mixing behaviours in fluidised beds with binary mixtures has many *** studied the instantaneous mixing characteristics of binary mixtures in a 2-D quasi gas-solid fluidised bed using a capacitance probe *** method enabled the quantitative assessment of instantaneous mixing behaviours,including mixing index,rate,and *** kinds of binary mixtures of similar size but different density were used for the transient and steady fluidisation experiments in a bubbling fluidised *** mixing curves of initially segregated binary mixtures were acquired,and the instantaneous characteristics for the entire process were *** equation was proposed to describe the mixing process and predict the mixing degree over *** comparing experiments with different working conditions,the effects of superficial gas velocity and density ratio on the mixing in the centre and at the wall of the fluidised bed were *** the stable fluidisation stage,the axial concentration profiles of the mixtures were obtained,and the mechanisms of mixing were *** showed that the mixing level increased logarithmically with time and eventually reached a relatively stable *** the superficial gas velocity and reducing the density ratio promoted mixing and reduced mixing *** superficial gas velocities tended to mix the mixtures well and quickly,regardless of the density ratio of the two components.

关键词： Binary mixtures Fluidised bed Mixing Instantaneous characteristics

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Particle convective heat transfer near the wall in a supercritical water fluidized bed by single particle model coupled with CFD-DEM

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Particuology 2023年第2期73卷 47-58页

作者： Tianning Zhang zhen wan.Youjun Lu State Key Laboratory of Multiphase Flow in Power Engineering(SKLMFPE) Xi'an Jiaotong UniversityXi'an710049ShaanxiChina Xi'an Electronic Engineering Research Institute Xi'an710100ShaanxiChina

Supercritical water fluidized bed(SCWFB)is a promising reactor to gasify biomass or *** optimization design is closely related to wall-to-bed heat transfer,where particle convective heat transfer plays an important *** paper evaluates the particle convective heat transfer coefficient(h_(pc))at the wall in SCWFB using the single particle *** critical parameters in the single particle model which is difficult to get experimentally are obtained by the computational fluid dynamics-discrete element method(CFD-DEM).The contact statistics related to particle-to-wall heat transfer,such as contact number and contact distance,are also *** results show that particle residence time(τ),as the key parameter to evaluate h_(pc),is found to decrease with rising velocity,while increase with larger thermal boundary layer thickness.τfollows a gamma function initially adopted in the gas-solid fluidized bed,making it possible to evaluate h_(pc) in SCWFB by a simplified single particle *** theoretical predicted h_(pc) tends to increase with rising thermal gradient thickness at a lower velocity(1.5 U_(mf)),while first decreases and then increases at higher velocity(1.75 and 2 U_(mf)).h_(pc) occupies 30%-57%of the overall wall-to-bed heat transfer coefficient for a particle diameter of 0.25 *** results are helpful to predict the overall wall-to-bed heat transfer coefficient in SCWFB combined with a reasonable fluid convective heat transfer model from a theoretical perspective.

关键词： Supercritical water Fluidized bed Particle residence time Discrete element method Single particle model

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An advanced higher-order theory for laminated composite plates with general lamination angles

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Acta Mechanica Sinica 2011年第5期27卷 720-729页

作者： zhen Wu hong Zhu wan.Ji Chen Key Laboratory of Liaoning Province forComposite Structural Analysis of Aerocraft and Simulation Shenyang Aerospace University 110136 Shenyang China

This paper proposes a higher-order shear deformation theory to predict the bending response of the laminated composite and sandwich plates with general lamination *** proposed theory a priori satisfies the continuity conditions of transverse shear stresses at ***,the number of unknown variables is independent of the number of *** first derivatives of transverse displacements have been taken out from the inplane displacement fields,so that the C 0 shape functions are only required during its finite element *** to C 0 continuity requirements,the proposed model can be conveniently extended for implementation in commercial finite element *** verify the proposed theory,the fournode C 0 quadrilateral element is employed for the interpolation of all the displacement parameters defined at each nodal point on the composite *** results show that following the proposed theory,simple C 0 finite elements could accurately predict the interlaminar stresses of laminated composite and sandwich plates directly from a constitutive equation,which has caused difficulty for the other global higher order theories.

关键词： Laminated and sandwich composites Higherorder theory C 0 continuity requirement Transverse shear stress

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Multiple model predictive control of perching maneuver based on guardian maps

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Chinese Journal of Aeronautics 2022年第5期35卷 347-360页

作者： Rui CAO Huiwen wan.zhen HE Yuping LU College of Automated Engineering Nanjing University of Aeronautics and AstronauticsNanjing 210016China

Considering the strong nonlinearity of Unmanned Aerial Vehicles(UAVs)resulting from high Angle of Attack(AOA)and fast maneuvering,we present a multi-model predictive control strategy for UAV maneuvering,which has a small amount of online ***,we divide the maneuver envelope of UAV into several sub-regions on the basis of the gap metric theory.A novel algorithm is then developed to determine the ploytopic model for each *** to this,a Robust Model Predictive Control based on the Idea of Comprehensive optimization(ICE-RMPC)is *** control law is designed offline and optimized online to reduce the computational ***,the ICE-RMPC method is applied to design the controllers of *** addition,to guarantee the stability of whole closed-loop system,a multi-model switching control strategy based on guardian maps is put ***,the tracking performance of proposed control strategy is demonstrated by an illustrative example.

关键词： Guardian maps Model predictive control Multi-Model switching rule Online comprehensive design Perching maneuver

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The breaking of spin symmetry in the single-particle resonances in deformed nuclei

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Nuclear Science and Techniques 2024年第3期35卷 237-245页

作者： zhen-Yu zheng Shou-wan.Chen Quan Liu School of Physics and Optoelectronic Engineering Anhui UniversityHefei 230601China

The exploration of spin symmetry (SS) in nuclear physics has been instrumental in identifying atomic nucleus *** this study,we solve the Dirac equation from the relativistic mean field (RMF) in complex momentum *** investigated SS and its breaking in single-particle resonant states within deformed nuclei,with a focus on the illustrative *** was the initial discovery of a resonant spin doublet in a deformed nucleus,with the expectation of the SS approaching the continuum *** increasing single-particle energy,the splitting of the resonant spin doublets widened *** escalating splitting implies diminishing adherence to the SS,indicating a departure from the expected behavior as the energy levels *** also analyzed the width of the resonant states,showing that lower orbital angular momentum resonances possess shorter decay times and that SS is preserved within broad resonant doublets,as opposed to narrow resonant *** the radial density of the upper components for the bound-state and resonant-state doublets,it becomes evident that while SS is well-preserved in the bound states,it deteriorates in the resonant *** impact of nuclear deformation (β_(2)) on SS was examined,demonstrating that an increase in β_(2) resulted in higher energy and width splitting in the resonant spin doublets,which is attributed to increased component ***,the sensitivity of spin doublets to various potential parameters such as surface diffuseness (a),radius (R),and depth (Σ0) is discussed,emphasizing the role of these parameters in *** study provides valuable insights into the behavior of spin doublets in deformed nuclei and their interplay with the nuclear structure,thereby advancing our understanding of SS in the resonance state.

关键词： Spin symmetry Resonant states Deformed nuclei Complex-momentum representation

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Mutual regulation of microglia and astrocytes after Gas6 inhibits spinal cord injury

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Neural Regeneration Research 2025年第2期20卷 557-573页

作者： Jiewen Chen Xiaolin Zeng Le wan. Wenwu Zhang Gang Li Xing Cheng Peiqiang Su Yong wan.Xiang Li Department of Spine Surgery The First Affiliated HospitalSun Yat-sen UniversityGuangzhouGuangdong ProvinceChina Guangdong Province Key Laboratory of Orthopedics and Traumatology GuangzhouGuangdong ProvinceChina

Invasive inflammation and excessive scar formation are the main reasons for the difficulty in repairing nervous tissue after spinal cord *** and astrocytes play key roles in the spinal cord injury micro-environment and share a close ***,the mechanisms involved remain *** this study,we found that after spinal cord injury,resting microglia(M0)were polarized into pro-inflammatory phenotypes(MG1 and MG3),while resting astrocytes were polarized into reactive and scar-forming *** expression of growth arrest-specific 6(Gas6)and its receptor Axl were significantly down-regulated in microglia and astrocytes after spinal cord *** vitro experiments showed that Gas6 had negative effects on the polarization of reactive astrocytes and pro-inflammatory microglia,and even inhibited the cross-regulation between *** further demonstrated that Gas6 can inhibit the polarization of reactive astrocytes by suppressing the activation of the Yes-associated protein signaling ***,in turn,inhibited the polarization of pro-inflammatory microglia by suppressing the activation of the nuclear factor-κB/p65 and Janus kinase/signal transducer and activator of transcription signaling *** vivo experiments showed that Gas6 inhibited the polarization of pro-inflammatory microglia and reactive astrocytes in the injured spinal cord,thereby promoting tissue repair and motor function ***,Gas6 may play a role in the treatment of spinal cord *** can inhibit the inflammatory pathway of microglia and polarization of astrocytes,attenuate the interaction between microglia and astrocytes in the inflammatory microenvironment,and thereby alleviate local inflammation and reduce scar formation in the spinal cord.

关键词： astrocytes Axl cell polarization Gas6 Hippo signal inflammatory micro-environment intercellular interaction microglia single-cell sequencing spinal cord injury

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