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Unsaturated bi-heterometal clusters in metal-vacancy sites of 2D MoS2 for efficient hydrogen evolution

Carbon Energy 2024年第3期6卷 264-275页

作者： Gonglei Shao jie Xu Shasha Gao zhang zhang Song Liu Xu zhang zhen Zhou Interdisciplinary Research Center for Sustainable Energy Science and Engineering(IRC4SE2) School of Chemical EngineeringZhengzhou UniversityZhengzhouHenanChina College of Chemistry and Materials Engineering Wenzhou UniversityWenzhouZhejiangChina Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education) College of ChemistryNankai UniversityTianjinChina State Key Laboratory of Chemo/Biosensing and Chemometrics Institute of Chemical Biology and Nanomedicine(ICBN)College of Chemistry and Chemical EngineeringHunan UniversityChangshaHunanChina Institute of New Energy Material Chemistry School of Materials Science and EngineeringNankai UniversityTianjinChina

The valence states and coordination structures of doped heterometal atoms in two-dimensional(2D)nanomaterials lack predictable regulation ***,a robust method is proposed to form unsaturated heteroatom clusters via the metal-vacancy restraint mechanism,which can precisely regulate the bonding and valence state of heterometal atoms doped in 2D molybdenum *** unsaturated valence state of heterometal Pt and Ru cluster atoms form a spatial coordination structure with Pt–S and Ru–O–S as catalytically active *** them,the strong binding energy of negatively charged suspended S and O sites for H+,as well as the weak adsorption of positively charged unsaturated heterometal atoms for H*,reduces the energy barrier of the hydrogen evolution reaction proved by theoretical ***,the electrocatalytic hydrogen evolution performance is markedly improved by the ensemble effect of unsaturated heterometal atoms and highlighted with an overpotential of 84 mV and Tafel slope of 68.5 mV dec^(−1).In brief,this metal vacancy-induced valence state regulation of heterometal can manipulate the coordination structure and catalytic activity of heterometal atoms doped in the 2D atomic lattice but not limited to 2D nanomaterials.

关键词： clusters hydrogen evolution reaction metal vacancy MoS2 unsaturated heterometal

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Murine model of acute myocarditis and cerebral cortical neuron edema induced by coxsackievirus B4

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Zoological Research 2018年第1期39卷 52-57页

作者： zhao-peng dong qian wang zhen-jie zhang michael j.carr dong li wei-feng shi key laboratory of etiology and epidemiology of emerging infectious diseases in universities of shandong taishan medical universityTaian Shandong 271000China shanghai jinshan center for disease control and prevention Shanghai 201599China school of public health taishan medical universityTaian Shandong 271016China global station for zoonosis control global institution for collaborative research and education(gi-core)hokkaido universitySapporo 060-8589Japan national virus reference laboratory school of medicineuniversity college dublinDublin 4Ireland

Globally, coxsackievirus B4 （CV-B4） has been continuously isolated and evidence suggests an association with the development of pancreatitis and type I diabetes. In addition, CV-B4 is also associated with myocarditis and severe central nervous system （CNS） complications, which remain poorly studied and understood. In the present study, we established an institute for Cancer Research （ICR） mouse model of CV-B4 infection and examined whether CV-B4 infection resulted in a predisposition to myocarditis and CNS infection. We found high survival in both the treatment and control group, with no significant differences in clinical outcomes observed. However, pathological lesions were evident in both brain and heart tissue of the CV-B4-infected mice. in addition, high viral loads were found in the neural and cardiac tissues as early as 2 days post infection. Expressions of IFN-y and IL-6 in sera were significantly higher in CV-B4-infected mice compared to uninfected negative controls, suggesting the involvement of these cytokines in the development of histopathological lesions. Our murine model successfully reproduced the acute myocarditis and cerebral cortical neuron edema induced by CV-B4, and may be useful for the evaluation of vaccine candidates and potential antivirals against CV-B4 infection.

关键词： Coxsackievirus B4 Myocarditis CNS Edema Neurons

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Precise immobilization of metal single atoms into a porphyrinic metal-organic framework for an efficient alkene hydrosilylation

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Nano Research 2024年第7期17卷 5914-5921页

作者： Chun-Ying Chen Qi-jie Mo Fu-zhen Li Hai-Li Song Li zhang MOE Laboratory of Bioinorganic and Synthetic Chemistry Lehn Institute of Functional MaterialsSchool of ChemistrySun Yat-Sen UniversityGuangzhou 510006China

Alkene hydrosilylation is one of the most concise and atom-economical methods to synthesize organosilicon ***,we reported the precise immobilization of metal single atoms(M-SAs;M=Ru,Rh,Ir,Pd,Pt,and Au)into a porphyrinic metalorganic framework(MOF)of PCN-222(PCN=porous coordination network),and then applied the resultant MOF composites of M-SAs@PCN-222 to alkene *** solvent-free conditions,Pt-SAs@PCN-222 displayed an especially high catalytic efficiency with the turnover frequency up to 119 s−1 and the maximum turnover number of 906,250 at room *** and theoretical studies revealed that there existed strong interactions between Pt-SAs@PCN-222 and the substrates,which helped to condense the substrates in the cavities of the porous *** density functional theory calculations and molecular dynamics simulations disclosed that PCN-222 could transfer electrons to Pt-SAs to enhance the silane oxidative addition and drive the reaction to proceed smoothly via Chalk–Harrod pathway.

关键词： alkene hydrosilylation single atom catalysts metal-organic frameworks precision chemistry synergistic catalysis

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Design Research of a Novel Aftercool-Humidifier Concept for Humid Air Turbine Cycle

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Journal of Thermal Science 2024年第3期33卷 951-969页

作者： zhang Junzheng XU zhen School of Energy and Power Engineering Shandong UniversityJi’nan250061China Shandong Engineering Laboratory for High-efficiency Energy Conservation and Energy Storage Technology&Equipment Shandong UniversityJi’nan250061China

Humid air turbine cycle(HAT)has potential of electrical efficiencies comparable to combined cycle,with lower investment cost and NO_(x) *** typical heat exchanger network of HAT consists of intercooler(if there is),aftercooler,recuperator,economizer and humidifier,which brings higher efficiency but makes the system more *** simplify HAT layout,a novel humidifier concept is proposed by integrating the aftercooler into traditional counter-current *** on this concept,a one-dimensional model including pressure drop and exergy calculation is established to distinguish the thermodynamic and hydrodynamic characteristics,and then the structural parameters,such as the number of rows and columns,tube diameter,pitch and type for a micro HAT are *** results show that the aftercool-humidifier plays the same role as original aftercooler and humidifier,and can match the in-tube air,out-tube air and water stream well with lower *** the case of micro HAT cycle,the volume of heat and mass transfer area can be reduced by 47%compared with traditional *** major thermal resistance occurred in the convection heat transfer process inside the tube;however,using enhanced tube cannot effectively improve the compactness of device.

关键词： humid air turbine cycle humidifier thermodynamic analysis one-dimensional model

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An interlaminar damage shell model for typical composite structures

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Chinese Journal of Aeronautics 2024年第1期37卷 118-137页

作者： jie ZHOU zhen WU zhengliang LIU Xiaohui REN School of Aeronautics Northwestern Polytechnical UniversityXi’an 710072China National Key Laboratory of Strength and Structural Integrity Xi’an 710065China School of Mechanical Engineering Xi’an Aeronautical UniversityXi’an 710065China

Using the plate/shell elements in commercial software,accurate analysis of interlaminar initial damage in typical composite structures is still a challenging *** propose an accurate and efficient model for analysis of interlaminar initial damage,the following work is carried out:(A)A higher-order theory is firstly proposed by introducing the local Legendre polynomials,and then a novel shell element containing initial damage prediction is developed,which can directly predict transverse shear stresses without any postprocessing *** variables at each node are independent of number of layers,so the proposed model is more efficient than the 3D-FEM.(B)Compression experiment is carried out to verify the capability of the proposed *** results obtained from the proposed model are in good agreement with experimental data.(C)Several examples have been analyzed to further assess the capability of the proposed model by comparing to the 3D-FEM ***,accuracy and efficiency have been evaluated in different damage criterion by comparing with the selected *** numerical results show that the proposed model can well predict the initial interlaminar damage as well as other ***,the model is implemented with UEL subroutine,so that the present approach can be readily utilized to analyze the initial damage in typical composite structures.

关键词： Compression experiment Finite element method Initial damage Interlaminar stress Plate/shell element

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Carrimycin in the treatment of acute promyelocytic leukemia combined with pulmonary tuberculosis: A case report

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World Journal of Clinical Cases 2024年第3期12卷 623-629页

作者： Fu-Yu Yang Lei Shao jie Su zhen-Meng zhang Department of Infectious Diseases The Affiliated Central Hospital of Shandong First Medical UniversityJinan 250013Shandong ProvinceChina

BACKGROUND Pulmonary tuberculosis(PTB)is prevalent in immunocompromised populations,including patients with hematologic malignancies,human immunodeficiency virus infections,and chronic *** treatment for acute promyelocytic leukemia(APL)combined with PTB is *** patients show an extremely poor ***,studies should establish efficient treatment options to improve patient survival and *** SUMMARY A 60-year-old male with pain in the right side of his chest and a fever for 4 d visited the outpatient department of our *** blood smear revealed 54%*** bone marrow examinations,variant APL with TNRC18-RARA fusion gene was *** computed tomography scan showed bilateral pneumonitis with bilateral pleural effusions,partial atelectasis in the lower lobes of both lungs,and the bronchoalveolar lavage fluid gene X-Pert test was positive,indicative of ***,ethambutol(EMB),and isoniazid(INH)were administered since he could not receive chemotherapy as the WBC count decreased *** one week of treatment with carrimycin,the patient recovered from fever and received *** was very effective and his white blood cells counts got back to *** being given five months with rifampin,EMB and INH and chemotherapy,the patient showed complete remission from pneumonia and *** We report a case of PTB treated successfully with carrimycin with APL that requires chemotherapy.

关键词： Carrimycin Hematologic disease Acute myeloid leukemia Acute promyelocytic leukemia Pulmonary tuberculosis Case report

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Nuclear charge radius predictions by kernel ridge regression with odd-even effects

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Nuclear Science and Techniques 2024年第2期35卷 94-102页

作者： Lu Tang zhen-Hua zhang Mathematics and Physics Department North China Electric Power UniversityBeijing 102206China Hebei Key Laboratory of Physics and Energy Technology North China Electric Power UniversityBaoding 071000China

The extended kernel ridge regression(EKRR)method with odd-even effects was adopted to improve the description of the nuclear charge radius using five commonly used nuclear *** are:(i)the isospin-dependent A^(1∕3) formula,(ii)relativistic continuum Hartree-Bogoliubov(RCHB)theory,(iii)Hartree-Fock-Bogoliubov(HFB)model HFB25,(iv)the Weizsacker-Skyrme(WS)model WS*,and(v)HFB25**** the last two models,the charge radii were calculated using a five-parameter formula with the nuclear shell corrections and deformations obtained from the WS and HFB25 models,*** each model,the resultant root-mean-square deviation for the 1014 nuclei with proton number Z≥8 can be significantly reduced to 0.009-0.013 fm after considering the modification with the EKRR *** best among them was the RCHB model,with a root-mean-square deviation of 0.0092 *** extrapolation abilities of the KRR and EKRR methods for the neutron-rich region were examined,and it was found that after considering the odd-even effects,the extrapolation power was improved compared with that of the original KRR *** strong odd-even staggering of nuclear charge radii of Ca and Cu isotopes and the abrupt kinks across the neutron N=126 and 82 shell closures were also calculated and could be reproduced quite well by calculations using the EKRR method.

关键词： Nuclear charge radius Machine learning Kernel ridge regression method

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Finer discrimination of brain activation with local multivariate distance

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Progress in Natural Science:Materials International 2007年第12期17卷 1508-1514页

作者： zhen Zonglei, Tian jie and zhang Hui(Medical Image Processing Group, Key Laboratory of Complex Systems and Intelligence Science, Institute of Automation, Chinese Academy of Sciences, Beijing 100080, China) Medical Image Processing Group Key Laboratory of Complex Systems and Intelligence Science Institute of Automation Chinese Academy of Sciences Beijing 100080 China

The organization of human brain function is diverse on different spatial scales. Various cognitive states are always represented as distinct activity patterns across the specific brain region on fine scales. Conventional univariate analysis of functional MRI data seeks to determine how a particular cognitive state is encoded in brain activity by analyzing each voxel separately without considering the fine-scale patterns information contained in the local brain regions. In this paper, a local multivariate distance mapping (LMDM) technique is proposed to detect the brain activation and to map the fine-scale brain activity patterns. LMDM directly represents the local brain activity with the patterns across multiple voxels rather than individual voxels, and it employs the multivariate distance between different patterns to discriminate the brain state on fine scales. Experiments with simulated and real fMRI data demonstrate that LMDM technique can dramatically increase the sensitivity of the detection for the fine-scale brain activity patterns which contain the subtle information of the experimental conditions.

关键词： functional magnetic resonance imaging (fMRI) statistical analysis multivariate distance local pattern pattern classification.

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SG-NeRF:Sparse-Input Generalized Neural Radiance Fields for Novel View Synthesis

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Journal of Computer Science & Technology 2024年第4期39卷 785-797页

作者： Kuo Xu jie Li zhen-Qiang Li Yang-jie Cao School of Cyber Science and Engineering Zhengzhou UniversityZhengzhou 450002China Intelligent Big Data System(iBDSys)Lab Shanghai Jiao Tong UniversityShanghai 200240China School of Computer and Artificial Intelligence Zhengzhou UniversityZhengzhou 450001China

Traditional neural radiance fields for rendering novel views require intensive input images and pre-scene optimization,which limits their practical *** propose a generalization method to infer scenes from input images and perform high-quality rendering without pre-scene optimization named SG-NeRF(Sparse-Input Generalized Neural Radiance Fields).Firstly,we construct an improved multi-view stereo structure based on the convolutional attention and multi-level fusion mechanism to obtain the geometric features and appearance features of the scene from the sparse input images,and then these features are aggregated by multi-head attention as the input of the neural radiance *** strategy of utilizing neural radiance fields to decode scene features instead of mapping positions and orientations enables our method to perform cross-scene training as well as inference,thus enabling neural radiance fields to generalize for novel view synthesis on unseen *** tested the generalization ability on DTU dataset,and our PSNR(peak signal-to-noise ratio)improved by 3.14 compared with the baseline method under the same input *** addition,if the scene has dense input views available,the average PSNR can be improved by 1.04 through further refinement training in a short time,and a higher quality rendering effect can be obtained.

关键词： Neural Radiance Fields(NeRF) multi-view stereo(MVS) new view synthesis(NVS)

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Sum-Rate Maximization in Active RIS-Assisted Multi-Antenna WPCN

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China Communications 2024年第6期21卷 23-39页

作者： Jiang jie Lyu Bin Chen Pengcheng Yang zhen School of Communications and Information Engineering Nanjing University of Posts and TelecommunicationsNanjing 210003China Jiangsu Provincial Key Laboratory of Photonic and Electronic Materials Sciences and Technology Nanjing UniversityNanjing 210003China

In this paper,we propose an active reconfigurable intelligent surface(RIS)enabled hybrid relaying scheme for a multi-antenna wireless powered communication network(WPCN),where the active RIS is employed to assist both wireless energy transfer(WET)from the power station(PS)to energyconstrained users and wireless information transmission(WIT)from users to the receiving station(RS).For further performance enhancement,we propose to employ both transmit beamforming at the PS and receive beamforming at the *** formulate a sumrate maximization problem by jointly optimizing the RIS phase shifts and amplitude reflection coefficients for both the WET and the WIT,transmit and receive beamforming vectors,and network resource *** solve this non-convex problem,we propose an efficient alternating optimization algorithm with the linear minimum mean squared error criterion,semidefinite relaxation(SDR)and successive convex approximation ***,the tightness of applying the SDR is *** results demonstrate that our proposed scheme with 10 reflecting elements(REs)and 4 antennas can achieve 17.78%and 415.48%performance gains compared to the single-antenna scheme with 10 REs and passive RIS scheme with 100 REs,respectively.

关键词： active reconfigurable intelligent surface beamforming sum-rate maximization wireless powered communication network

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