检索结果-南通市图书馆

Recent advances and key perspectives of in-situ studies for oxygen evolution reaction in water electrolysis

Green Energy & Environment 2024年第10期9卷 1497-1517页

作者： Yi Wang Zichen Xu Xianhong wu Zhong-Shuai wu State Key Laboratory of Catalysis Dalian Institute of Chemical Physics Chinese Academy of Sciences University of Chinese Academy of Sciences Shijingshan District Dalian National Laboratory for Clean Energy Chinese Academy of Sciences

Electricity-driven water splitting to produce hydrogen is one of the most efficient ways to alleviate energy crisis and environmental pollution problems, in which the anodic oxygen evolution reaction(OER) is the key half-reaction of performance-limiting in water splitting. Given the complicated reaction process and surface reconstruction of the involved catalysts under actual working conditions, unraveling the real active sites, probing multiple reaction intermediates and clarifying catalytic pathways through in-situ characterization techniques and theoretical calculations are essential. In this review, we summarize the recent advancements in understanding the catalytic process, unlocking the water oxidation active phase and elucidating catalytic mechanism of water oxidation by various in-situ characterization techniques. Firstly, we introduce conventionally proposed traditional catalytic mechanisms and novel evolutionary mechanisms of OER, and highlight the significance of optimal catalytic pathways and intrinsic stability. Next, we provide a comprehensive overview of the fundamental working principles,different detection modes, applicable scenarios, and limitations associated with the in-situ characterization techniques. Further, we exemplified the in-situ studies and discussed phase transition detection, visualization of speciation evolution, electronic structure tracking, observation of reaction active intermediates, and monitoring of catalytic products, as well as establishing catalytic structure–activity relationships and catalytic mechanism. Finally, the key challenges and future perspectives for demystifying the water oxidation process are briefly proposed.

关键词： In-situ studies Water splitting Oxygen evolution reaction Catalytic mechanism

来源：

同方期刊数据库评论

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

激波/湍流边界层干扰中的自适应控制技术

引用

国防科技大学学报 2024年第2期46卷 49-61页

作者：黄伟吴瀚钟翔宇杜兆波柳军国防科技大学高超声速技术重点实验室湖南长沙410073

从激波/湍流边界层干扰机理以及流动控制的迫切需求入手,从自适应涡流发生器、自适应鼓包、自适应微射流以及自适应次流循环四个方面对激波/湍流边界层干扰中的自适应控制技术研究进展进行了总结。分析认为,结合AI技术发展自适应流动控... 详细信息

从激波/湍流边界层干扰机理以及流动控制的迫切需求入手,从自适应涡流发生器、自适应鼓包、自适应微射流以及自适应次流循环四个方面对激波/湍流边界层干扰中的自适应控制技术研究进展进行了总结。分析认为,结合AI技术发展自适应流动控制技术,加速控制方式智能化,可作为新一代高超声速飞行器宽速域飞行的重要技术手段。具体来说,就是通过调节外加激励对高超声速飞行器不同区域实现局部流动加/减速、气动热防护、气动控制等功能,根据流场参数建立控制反馈回路,自适应调整局部流场结构,以满足工程实际需求。

关键词：自适应流动控制激波/湍流边界层干扰高超声速飞行器自主决策分离热流峰值

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Enhancing performance of low-temperature processed CsPbI2Br all-inorganic perovskite solar cells using polyethylene oxide-modified TiO_(2)

引用

International Journal of Minerals,Metallurgy and Materials 2024年第4期31卷 786-794页

作者： Xu Zhao Naitao Gao Shengcheng wu Shaozhen Li Sujuan wu School of Electrical and Electronic Engineering Wuhan Polytechnic UniversityWuhan 430023China Institute for Advanced Materials and Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials South China Academy of Advanced OptoelectronicsSouth China Normal UniversityGuangzhou 510006China

CsPbX_(3)-based(X=I,Br,Cl)inorganic perovskite solar cells(PSCs)prepared by low-temperature process have attracted much attention because of their low cost and excellent thermal ***,the high trap state density and serious charge recombination between low-temperature processed TiO_(2)film and inorganic perovskite layer interface seriously restrict the performance of all-inorganic *** a thin polyethylene oxide(PEO)layer is employed to modify TiO_(2)film to passivate traps and promote carrier *** impacts of PEO layer on microstructure and photoelectric characteristics of TiO_(2)film and related devices are systematically *** results suggest that PEO modification can reduce the surface roughness of TiO_(2)film,decrease its average surface potential,and passivate trap *** optimal conditions,the champion efficiency of CsPbI_(2)Br PSCs with PEO-modified TiO_(2)(PEO-PSCs)has been improved to 11.24%from 9.03%of reference ***,the hysteresis behavior and charge recombination have been suppressed in PEO-PSCs.

关键词： polyethylene oxide-modified TiO_(2) film low-temperature process CsPbI_(2)Br-based all-inorganic perovskite solar cells photo-voltaic performance

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

A GNSS Anti-Spoofing Technique Based on the Spatial Distribution Characteristic of the Residual Vectors

引用

Tsinghua Science and Technology 2024年第2期29卷 457-468页

作者： Qi'an wu Xiaowei Cui Mingquan Lu Pengxiang Yang Peng wu Department of Electronic Enginnering Tsinghua UniversityBeijing 100084China Xi’an Modern Control Technology Research Institute Xi’an 710065China

Anti-spoofing is becoming a crucial technique for applications with high navigation accuracy and reliability ***-spoofing technique based on Receiver Autonomous Integrity Monitoring(RAIM)is a good choice for most Global Navigation Satellite System(GNSS)receivers because it does not require any change to the hardware of the ***,the conventional RAIM method can only detect and mitigate a single spoofing *** improved RAIM methods can deal with more spoofing signals,but the computational complexity increases dramatically when the number of satellites in view increase or need additional *** paper proposes a new RAIM method,called the SRV-RAIM method,which has a very low computation complexity regardless of the number of satellites in view and can deal with any number of spoofing *** key to the new method is the spatial distribution characteristic of the Satellites'Residual Vectors(SRV).In replay or generative spoofing scenarios,the pseudorange measurements of spoofing signals are consistent,the residual vectors of real satellites and those of spoofing satellites have good separation characteristics in spatial *** on this characteristic,the SRV-RAIM method is proposed,and the simulation results show that the method can separate the real signals and the spoofing signals with an average probability of 86.55%in the case of 12 visible satellites,regardless of the number of spoofing *** to the conventional traversal-RAIM method,the performance is only reduced by 3.59%,but the computational cost is reduced by 98.3%,so most of the GNSS receivers can run the SRV-RAIM algorithm in time.

关键词： Global Navigation Satellite System(GNSS) anti-spoofing Receiver Autonomous Integrity Monitoring(RAIM) Satellites'Residual Vectors(SRV)

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Effective Identity Authentication Based on Multiattribute Centers for Secure Government Data Sharing

引用

Tsinghua Science and Technology 2024年第3期29卷 736-752页

作者： Meiquan Wang Junhua wu Tongdui Zhang Junhao wu Guangshun Li School of Computer Science Qufu Normal UniversityRizhao 276800China Science and Technology Innovation Service Institution of Rizhao Rizhao 276800China

As one of the essential steps to secure government data sharing,Identity Authentication(IA)plays a vital role in the processing of large ***,the centralized IA scheme based on a trusted third party presents problems of information leakage and single point of failure,and those related to key ***,herein,an effective IA model based on multiattribute centers is ***,a private key of each attribute of a data requester is generated by the attribute authorization *** obtaining the private key of attribute,the data requester generates a personal private ***,a dynamic key generation algorithm is proposed,which combines blockchain and smart contracts to periodically update the key of a data requester to prevent theft by external attackers,ensure the traceability of IA,and reduce the risk of privacy ***,the combination of blockchain and interplanetary file systems is used to store attribute field information of the data requester to further reduce the cost of blockchain information storage and improve the effectiveness of information *** results show that the proposed model ensures the privacy and security of identity information and outperforms similar authentication models in terms of computational and communication costs.

关键词： blockchain identity authentication distribution dynamic key generation

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Design and Implementation of Nonlinear Precoding for MIMO-SDMA Toward 6G Wireless

引用

China Communications 2024年第1期21卷 69-87页

作者： Chaowu wu Yue Xiao Shu Fang Gang wu National Key Laboratory of Wireless Communications University of Electronic Science and Technology of ChinaChengdu 611731China

In this paper,we present a novel and robust nonlinear precoding(NLP)design and detection structure specifically tailored for multiple-input multipleoutput space division multiple access(MIMO-SDMA)systems toward 6G *** approach aims to effectively mitigate the impact of imperfect channel estimation by leveraging the channel fluctuation mean square error(MSE)for reconstructing a highly accurate precoding matrix at the ***,we introduce a simplified receiver structure that eliminates the need for equalization,resulting in reduced interference and notable enhancements in overall system *** conduct both computer simulations and experimental tests to validate the efficacy of our proposed *** results reveals that the proposed NLP scheme offers significant performance improvements,making it particularly well-suited for the forthcoming 6G wireless.

关键词： MIMO-SDMA nonlinear precoding Tomlinson-Harashima precoding(THP) vector perturbation(VP)

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Optically levitated micro gyroscopes with an MHz rotational vaterite rotor

引用

Microsystems & Nanoengineering 2024年第3期10卷 219-227页

作者： Kai Zeng Xiangming Xu Yulie wu Xuezhong wu Dingbang Xiao College of Intelligence Science and Technology National University of Defense TechnologyChangsha 410073China College of Information and Communication National University of Defense TechnologyWuhan 430000China Key Laboratory of Satellite Navigation Technology National University of Defense TechnologyChangsha 410073China

The field of levitated optomechanics has experienced significant advancements in manipulating the translational and rotational dynamics of optically levitated particles and exploring their sensing *** concept of using optically levitated particles as gyroscopes to measure angular motion has long been explored but has not yet been proven either theoretically or *** this study,we present the first rotor gyroscope based on optically levitated high-speed rotating *** gyroscope is composed of a micrometer-size ellipsoidal vaterite particle that is driven to rotate at MHz frequencies in a vacuum *** an external angular velocity is input,the optical axis deviates from its initial position,resulting in changes in the frequency and amplitude of the rotational *** analyzing these changes,the angular velocity of the input can be accurately detected,making it the smallest rotor gyroscope in the *** angular rate bias instability of the gyroscope is measured to be 0.08°/s and can be further improved to as low as 10^(−9)°/h theoretically by cooling the motion and increasing the angular moment of the levitated *** work opens a new application paradigm for levitated optomechanical systems and may pave the way for the development of quantum rotor gyroscopes.

关键词： particles rotational angular

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Integrated Clustering and Routing Design and Triangle Path Optimization for UAV-Assisted Wireless Sensor Networks

引用

China Communications 2024年第4期21卷 178-192页

作者： Shao Liwei Qian Liping wu Mengru wu Yuan College of Information Engineering Zhejiang University of TechnologyHangzhou 310014China State Key Laboratory of Internet of Things for Smart City University of MacaoMacaoChina Department of Computer and Information Science University of MacaoMacaoChina

With the development of the Internet of Things(IoT),it requires better performance from wireless sensor networks(WSNs),such as larger coverage,longer lifetime,and lower ***,a large amount of data generated from monitoring and long-distance transmission places a heavy burden on sensor nodes with the limited battery *** this,we investigate an unmanned aerial vehicles assisted mobile wireless sensor network(UAV-assisted WSN)to prolong the network lifetime in this ***,we use UAVs to assist the WSN in collecting *** the current UAV-assisted WSN,the clustering and routing schemes are determined ***,such a separate consideration might not maximize the lifetime of the whole WSN due to the mutual coupling of clustering and *** efficiently prolong the lifetime of the WSN,we propose an integrated clustering and routing scheme that jointly optimizes the clustering and routing *** the whole network space,it is intractable to efficiently obtain the optimal integrated clustering and routing ***,we propose the Monte-Las search strategy based on Monte Carlo and Las Vegas ideas,which can generate the chain matrix to guide the algorithm to find the solution *** point-to-point collection leads to long collection paths,so a triangle optimization strategy is then proposed that finds a compromise path to shorten the collection path based on the geometric distribution and energy of sensor *** avoid the coverage hole caused by the death of sensor nodes,the deployment of mobile sensor nodes and the preventive mechanism design are *** emergency data transmission mechanism is further proposed to reduce the latency of collecting the latency-sensitive data due to the absence of *** with the existing schemes,the proposed scheme can prolong the lifetime of the UAVassisted WSN at least by 360%,and shorten the collection path of UAVs by 56.24%.

关键词： Monte-Las search strategy triangle path optimization unmanned aerial vehicles wireless sensor networks

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Terminal-selective C（sp3）–H borylation of unbranched alkanes enabled by intermolecular radical sampling and LMCT photocatalysis

引用

National Science Review 2024年第5期11卷 96-98页

作者： Zhexuan Lei Jie wu Department of Chemistry National University of Singapore

The selective functionalization of C（sp3）–H bonds with subtle differences in alkanes is highly sought after due to its atom-and step-efficiency. The activation of C（sp3）–H bonds through hydrogen atom transfer （HAT） has been extensively exploited to produce a valueadded product from unfunctionalized material [1,2].

关键词：

来源：

同方期刊数据库评论

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

BSIN: A Behavior Schema of Information Networks Based on Approximate Bisimulation

引用

Tsinghua Science and Technology 2024年第4期29卷 1092-1104页

作者： wujie Hu Jinzhao wu School of Electrical Engineering Guangxi UniversityNanning 530004China

Information networks are becoming increasingly important in practice. However, their escalating complexity is gradually impeding the efficiency of data mining. A novel network schema called the Behavior Schema of Information Networks (BSIN) is proposed to address this issue. This work defines the behavior of nodes as connected paths in BSIN, proposes a novel function distinguish behavior differences, and introduces approximate bisimulation into the acquisition of quotient sets for node types. The major highlight of BSIN is its ability to directly obtain a high-efficiency network on the basis of approximate bisimulation, rather than reducing the existing information network. It provides an effective representation of information networks, and the resulting novel network has a simple structure that more efficiently expresses semantic information than current network representations. The theoretical analysis of the connected paths between the original and the obtained networks demonstrates that errors are controllable;and semantic information is approximately retained. Case studies show that BSIN yields a simple network and is highly cost-effective.

关键词： data mining information network approximate bisimulation controllable error

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

欢迎您,

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案：

请选择收藏分类：

通借通还

欢迎您,

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：